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Takahashi, Yoshio*; Yamaguchi, Akiko; Yomogida, Takumi
Treatise on Geochemistry, 3rd edition, Vol.6, 46 Pages, 2025/00
With the recent development of measurement techniques, new approaches to the environmental geochemistry of radionuclides have been applied for various research targets. In this review article, several topics within the last 10-15 years in the field of environmental geochemistry of radionuclides have been discussed. In particular, this article mainly focused on two topics, (i) studies on the migration of radionuclides emitted by the Fukushima Dai-ichi Nuclear Power Plant (FDNPP) accident in 2011 and (ii) the development of X-ray absorption fine structure (XAFS) spectroscopy and its application to the geochemical processes of radionuclides.
Yomogida, Takumi; Hashimoto, Tadashi; Okumura, Takuma*; Yamada, Shinya*; Tatsuno, Hideyuki*; Noda, Hirofumi*; Hayakawa, Ryota*; Okada, Shinji*; Takatori, Sayuri*; Isobe, Tadaaki*; et al.
Analyst, 149(10), p.2932 - 2941, 2024/03
Times Cited Count:1 Percentile:63.46(Chemistry, Analytical)In this study, we successfully applied a transition-edge sensor (TES) spectrometer as a detector for microbeam X-ray measurements from a synchrotron X-ray light source to determine uranium (U) distribution at the micro-scale and its chemical species in biotite obtained from the U mine. It is difficult to separate the fluorescent X-ray of the U L line at 13.615 keV from that of the Rb K
line at 13.395 keV in the X-ray fluorescence spectrum with an energy resolution of approximately 220 eV of the conventional silicon drift detector (SDD). Meanwhile, the fluorescent X-rays of U L
and Rb K
were fully separated by TES with 50 eV energy resolution at the energy of around 13 keV. The successful peak separation by TES led to an accurate mapping analysis of trace U in micro-X-ray fluorescence measurements and a decrease in the signal-to-background ratio in micro-X-ray absorption near edge structure spectroscopy.
Miyagawa, Akihisa*; Takahashi, Takumi*; Kuzure, Yoshiaki*; Iwamoto, Hibiki*; Arai, Tsuyoshi*; Nagatomo, Shigenori*; Watanabe, So; Sano, Yuichi; Nakatani, Kiyoharu*
Analytical Sciences, 39(11), p.1929 - 1936, 2023/11
Times Cited Count:1 Percentile:17.17(Chemistry, Analytical)In this study, we revealed the Eu(III) distribution in a single diglycolamide-derivative extractant (TODGA)-impregnated polymer-coated silica particle. The reaction of Eu(III) with two TODGA molecules in the polymer layer was the rate-limiting process, as evidenced by the absence of any correlation between the rate constants (k and k
) and concentrations of Eu(III) and HNO
.
Miyagawa, Akihisa*; Hayashi, Naoki*; Kuzure, Yoshiaki*; Takahashi, Takumi*; Iwamoto, Hibiki*; Arai, Tsuyoshi*; Nagatomo, Shigenori*; Miyazaki, Yasunori; Hasegawa, Kenta; Sano, Yuichi; et al.
Bulletin of the Chemical Society of Japan, 96(7), p.671 - 676, 2023/07
Times Cited Count:5 Percentile:61.67(Chemistry, Multidisciplinary)We investigated the distribution mechanism of Eu(III) in a single polymer-coated silica particle including nitrilotriacetamide (NTA) extractants known as HONTA and TOD2EHNTA. The present study provides a valuable approach for the evaluation and enhancement of the functionality of "single extractant-impregnated polymer-coated silica particle".
Li, W.*; Yamada, Shinya*; Hashimoto, Tadashi; Okumura, Takuma*; Hayakawa, Ryota*; Nitta, Kiyofumi*; Sekizawa, Oki*; Suga, Hiroki*; Uruga, Tomoya*; Ichinohe, Yuto*; et al.
Analytica Chimica Acta, 1240, p.340755_1 - 340755_9, 2023/02
Times Cited Count:10 Percentile:64.21(Chemistry, Analytical)no abstracts in English
Yomogida, Takumi; Akiyama, Daisuke*; Ouchi, Kazuki; Kumagai, Yuta; Higashi, Kotaro*; Kitatsuji, Yoshihiro; Kirishima, Akira*; Kawamura, Naomi*; Takahashi, Yoshio*
Inorganic Chemistry, 61(50), p.20206 - 20210, 2022/12
Times Cited Count:5 Percentile:52.06(Chemistry, Inorganic & Nuclear)FeUO was studied to clarify the electronic structure of U(V) in a metal monouranate compound. We obtained the peak splitting of HERFD-XANES spectra utilizing high-energy-resolution fluorescence detection-X-ray absorption near edge structure (HERFD-XANES) spectroscopy at the U L
-edge, which is a novel technique in the U(V) compounds. Theoretical calculations revealed that the peak splitting was caused by splitting the 6d orbital of U(V). Such distinctive electronic states are of major interest to researchers and engineers working in various fields, from fundamental physics to the nuclear industry and environmental sciences for actinide elements.
Takahashi, Atsushi*; Chiba, Mirei*; Tanahara, Akira*; Aida, Jun*; Shimizu, Yoshinaka*; Suzuki, Toshihiko*; Murakami, Shinobu*; Koarai, Kazuma; Ono, Takumi*; Oka, Toshitaka; et al.
Scientific Reports (Internet), 11(1), p.10355_1 - 10355_11, 2021/05
Times Cited Count:9 Percentile:44.37(Multidisciplinary Sciences)Komatsu, Kazuki*; Iwasaki, Tsugumi*; Murata, Kosuke*; Yamashiro, Hideaki*; Goh, V. S. T.*; Nakayama, Ryo*; Fujishima, Yohei*; Ono, Takumi*; Kino, Yasushi*; Shimizu, Yoshinaka*; et al.
Reproduction in Domestic Animals, 56(3), p.484 - 497, 2021/03
Times Cited Count:12 Percentile:83.82(Agriculture, Dairy & Animal Science)We have established an archive system of livestock and wild animals from the surrounding ex-evacuation zone. Wildlife within the alert zone have been exposed to low-dose-rate (LDR) radiation for a long and continuous time. In this study, we analysed the morphological characteristics of the testes and in vitro fertilization (IVF) capacity of cryopreserved sperm of raccoons from the ex-evacuation zone of the FDNPP accident. This study revealed that the chronic and LDR radiation exposure associated with the FDNPP accident had no adverse effect on the reproductive characteristics and functions of male raccoons.
Kato, Takemi*; Sugawara, Katsuaki*; Ito, Naohiro*; Yamauchi, Kunihiko*; Sato, Takumi*; Oguchi, Tamio*; Takahashi, Takashi*; Shiomi, Yuki*; Saito, Eiji; Sato, Takafumi*
Physical Review Materials (Internet), 4(8), p.084202_1 - 084202_6, 2020/08
Times Cited Count:4 Percentile:16.46(Materials Science, Multidisciplinary)Watanabe, Masao; Nojiri, Hiroyuki*; Ito, Shinichi*; Kawamura, Seiko; Kihara, Takumi*; Masuda, Takatsugu*; Sahara, Takuro*; Soda, Minoru*; Takahashi, Ryuta
JPS Conference Proceedings (Internet), 25, p.011024_1 - 011024_5, 2019/03
Recently, neutron scattering experiments have been rapidly progressed under high magnetic field. In the J-PARC, proto-type compact pulse magnet system with the power supply, the coil and the sample stick has been developed. Basic specifications of the power supply are as follows; maximum charged voltage with capacitor is 2 kV, maximum current is 8 kA, repetition rate is a pulse per several minutes and pulse duration is several msec. Maximum magnetic field in the coil is more than 30 Tesla. The sample stick is designed for Orange-Cryostat. In this presentation, We report the details of the pulsed magnet system and the performance of it on neutron scattering experiments at MLF beam line (HRC).
Takahashi, Naoki; Yoshinaka, Kazuyuki; Harada, Akio; Yamanaka, Atsushi; Ueno, Takashi; Kurihara, Ryoichi; Suzuki, Soju; Takamatsu, Misao; Maeda, Shigetaka; Iseki, Atsushi; et al.
Nihon Genshiryoku Gakkai Homu Peji (Internet), 64 Pages, 2016/00
no abstracts in English
Nagao, Seiya*; Niibori, Yuichi*; Tanaka, Tadao; Sasaki, Takayuki*; Saito, Takumi*; Kirishima, Akira*; Yoshikawa, Hideki; Iijima, Kazuki; Hama, Katsuhiro; Iwatsuki, Teruki; et al.
Genshiryoku Bakkuendo Kenkyu (CD-ROM), 20(1), p.3 - 14, 2013/06
This paper shows a current status of groundwater colloids studies on the performance assessment of geological disposal of radioactive wastes in Japan, and summaries realistic approach of the colloids studies at a substantial research network for Japanese universities and institutes.
Tobita, Kenji; Nishio, Satoshi*; Enoeda, Mikio; Nakamura, Hirofumi; Hayashi, Takumi; Asakura, Nobuyuki; Uto, Hiroyasu; Tanigawa, Hiroyasu; Nishitani, Takeo; Isono, Takaaki; et al.
JAEA-Research 2010-019, 194 Pages, 2010/08
This report describes the results of the conceptual design study of the SlimCS fusion DEMO reactor aiming at demonstrating fusion power production in a plant scale and allowing to assess the economic prospects of a fusion power plant. The design study has focused on a compact and low aspect ratio tokamak reactor concept with a reduced-sized central solenoid, which is novel compared with previous tokamak reactor concept such as SSTR (Steady State Tokamak Reactor). The reactor has the main parameters of a major radius of 5.5 m, aspect ratio of 2.6, elongation of 2.0, normalized beta of 4.3, fusion out put of 2.95 GW and average neutron wall load of 3 MW/m. This report covers various aspects of design study including systemic design, physics design, torus configuration, blanket, superconducting magnet, maintenance and building, which were carried out increase the engineering feasibility of the concept.
Tobita, Kenji; Nishio, Satoshi; Enoeda, Mikio; Kawashima, Hisato; Kurita, Genichi; Tanigawa, Hiroyasu; Nakamura, Hirofumi; Honda, Mitsuru; Saito, Ai*; Sato, Satoshi; et al.
Nuclear Fusion, 49(7), p.075029_1 - 075029_10, 2009/07
Times Cited Count:140 Percentile:97.63(Physics, Fluids & Plasmas)Recent design study on SlimCS focused mainly on the torus configuration including blanket, divertor, materials and maintenance scheme. For vertical stability of elongated plasma and high beta access, a sector-wide conducting shell is arranged in between replaceable and permanent blanket. The reactor adopts pressurized-water-cooled solid breeding blanket. Compared with the previous advanced concept with supercritical water, the design options satisfying tritium self-sufficiency are relatively scarce. Considered divertor technology and materials, an allowable heat load to the divertor plate should be 8 MW/m or lower, which can be a critical constraint for determining a handling power of DEMO (a combination of alpha heating power and external input power for current drive).
Bae, Y. S.*; Na, Y. S.*; Oh, Y. K.*; Kwon, M.*; Bak, J. S.*; Lee, G. S.*; Jeong, J. H.*; Park, S. I.*; Cho, M. H.*; Namkung, W.*; et al.
Fusion Science and Technology, 52(2), p.321 - 333, 2007/08
Times Cited Count:23 Percentile:80.90(Nuclear Science & Technology)An 84-GHz, 500-kW gyrotron system have been installed at KSTAR, and the initial test of the gyrotron has been carried out with 20 sec-pulse and an output RF power of 500 kW. The launcher system having with a highly flexible steering mirror was fabricated and would inject 500-kW rf power into the KSTAR plasma. KSTAR will employ 170-GHz EC current drive (CD) in ITER-relevant experiments such as the suppression of the neoclassical tearing modes and the creation of an electron internal transport barrier. A JAEA 170-GHz, 1-MW gyrotron on loan in accordance with a Korea-Japan fusion collaboration agreement, and it will be used for the 170-GHz, 1-MW ECCD system in 2010. This paper describes the current status of the installation and initial conditioning tests of the 84-GHz gyrotron system as well as the development plan of the 170-GHz ECH and CD system. Also, this paper discusses the CD efficiency and the steering range of the second-harmonic X-mode injection.
Ninomiya, Hiromasa; Akiba, Masato; Fujii, Tsuneyuki; Fujita, Takaaki; Fujiwara, Masami*; Hamamatsu, Kiyotaka; Hayashi, Nobuhiko; Hosogane, Nobuyuki; Ikeda, Yoshitaka; Inoue, Nobuyuki; et al.
Journal of the Korean Physical Society, 49, p.S428 - S432, 2006/12
To contribute DEMO and ITER, the design to modify the present JT-60U into superconducting coil machine, named National Centralized Tokamak (NCT), is being progressed under nationwide collaborations in Japan. Mission, design and strategy of this NCT program is summarized.
Hoshino, Katsumichi; Yamamoto, Takumi; Tamai, Hiroshi; Oasa, Kazumi; Kawashima, Hisato; Miura, Yukitoshi; Ogawa, Toshihide; Shoji, Teruaki*; Shibata, Takatoshi; Kikuchi, Kazuo; et al.
Fusion Science and Technology, 49(2), p.139 - 167, 2006/02
Times Cited Count:2 Percentile:16.81(Nuclear Science & Technology)The main results obtained by the various heating and current drive systems, external coil system and divertor bias system are reviewed from the viewpoint of the advanced active control of the tokamak plasma. Also, the features of each system are described. The contribution of the JFT-2M in these areas are summarized.
Ichimasa, Michiko*; Awagakubo, Sayuri*; Takahashi, Miho*; Tauchi, Hiroshi*; Hayashi, Takumi; Kobayashi, Kazuhiro; Nishi, Masataka; Ichimasa, Yusuke*
Fusion Science and Technology, 48(1), p.759 - 762, 2005/07
Times Cited Count:7 Percentile:44.26(Nuclear Science & Technology)There exists various kinds of HT oxidizing soil bacteria in the world, and we have conducted the investigation of HT oxidation activity of such bacteria. In the fusion facility where deuterium and tritium will be used as its fuel, the system is necessary to eliminate tritium from atmospheric air. General tritium elimination method is oxidation and dehumidification, and high temperature catalyst is used in the present system for oxidation. Application of the HT oxidation bioreactor, which can oxidize in room temperature, to this oxidation process has possibility to get higher tritium elimination efficiency, so we started to study the bioreactor. In the recent study, we can get high oxidation ratio of 85% in the processing conditions of 200 Bq/cm as tritium concentration in air, 100 cm
/min as flow rate and once-through processing using the Caisson Assembly for Tritium Safety Study (CATS) in JAERI. This result encourages this development study.
Ikeda, Yoshitaka; Kasugai, Atsushi; Moriyama, Shinichi; Kajiwara, Ken*; Seki, Masami; Tsuneoka, Masaki*; Takahashi, Koji; Anno, Katsuto; Hamamatsu, Kiyotaka; Hiranai, Shinichi; et al.
Fusion Science and Technology (JT-60 Special Issue), 42(2-3), p.435 - 451, 2002/09
Times Cited Count:26 Percentile:81.82(Nuclear Science & Technology)no abstracts in English
Ikeda, Yoshitaka; Kasugai, Atsushi; Takahashi, Koji; Kajiwara, Ken; Isayama, Akihiko; Ide, Shunsuke; Terakado, Masayuki; Shinozaki, Shinichi; Yokokura, Kenji; Anno, Katsuto; et al.
Fusion Engineering and Design, 53(1-4), p.351 - 363, 2001/01
Times Cited Count:40 Percentile:91.80(Nuclear Science & Technology)no abstracts in English