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Hirota, Noriaki; Takeda, Ryoma; Ide, Hiroshi; Tsuchiya, Kunihiko; Kobayashi, Yoshinao*
Nuclear Materials and Energy (Internet), 45, p.102009_1 - 402009_10, 2025/12
Using SUS304L stainless steel, which is employed in reactor structural components, the effects of grain refinement on stress corrosion cracking occurring under nuclear reactor operating conditions were investigated. As a result, after conducting slow strain rate testing (SSRT) in air and nuclear reactor operating environments, a comparison of the tensile properties of SUS304L with the same grain size revealed that elongation significantly decreased with increasing grain size under nuclear reactor operating conditions. In SSRT conducted in air, the 
-value obtained from the Hall-Petch relationship was lower than the conventional values. Observations showed the absence of cracks on SUS304L with 0.59 and 1.52 
m grains; however, SUS304L with larger grains exhibited rougher fracture surfaces and side cracks. Thin oxide films were formed on SUS304L with 0.59 m and 1.52 m grains, while SUS304L with coarse grains of 28.4 m or larger enabled the formation of oxide films with over 2 m thickness. Cr
O
films were formed on SUS304L with 0.59 m, 1.52 m, and 28.4 m, while CrO and Fe based oxides were formed on SUS304L with 39.5 m and 68.6 m. Crystal orientation analysis revealed linear surface layers without cracks in the 
-phase for SUS304L with 0.59 m and 1.52 m. In materials with Larger grain sizes, surface irregularities and cracks were observed in the -phase. In fine-grained SUS304L, lattice diffusion caused uniform O diffusion in the -phase, resulting in the formation of a thin CrO layer that suppressed cracks. In coarse-grained SUS304L, grain boundary diffusion caused Fe oxide formation at the grain boundaries, weakening them, and supersaturated O led to the formation of thick films comprising CrO and Fe-based oxides, resulting in peeling and cracking.
Dei, Shuntaro; Shibata, Masahito*; Negishi, Kumi*; Sugiura, Yuki; Amano, Yuki; Bateman, K.*; Wilson, J.*; Yokoyama, Tatsunori; Kagami, Saya; Takeda, Masaki; et al.
Results in Earth Sciences (Internet), 3, p.100097_1 - 100097_16, 2025/12
Interactions between cement and host rock in geological repositories for radioactive waste will result in a chemically disturbed zone, which may potentially affect the long-term safety. This paper investigates the chemical evolution at the interface between cement (Ordinary Portland Cement: OPC and Low Alkaline Cement: LAC) and mudstone after 11 years of in situ reactions at the Horonobe Underground Research Laboratory. The study combines various analytical techniques to identify the key reactions at the cement-rock interface, including cement dissolution, precipitation of secondary minerals such as calcite and C-(A-)S-H phases, cation exchange in montmorillonite and reduced porosity in mudstone. The study also highlights the effects of cement-mudstone interactions on radionuclide migration, such as reduction of diffusivity due to reduced porosity and enhancement of sorption due to incorporation into secondary minerals in the altered mudstone.
Nakayama, Masashi; Ishii, Eiichi; Hayano, Akira; Aoyagi, Kazuhei; Murakami, Hiroaki; Ono, Hirokazu; Takeda, Masaki; Mochizuki, Akihito; Ozaki, Yusuke; Kimura, Shun; et al.
JAEA-Review 2025-027, 80 Pages, 2025/09
JAEA-Review-2025-027.pdf:6.22MB
The Horonobe Underground Research Laboratory Project is being pursued by the Japan Atomic Energy Agency to enhance the reliability of relevant technologies for geological disposal of high-level radioactive waste through investigating the deep geological environment within the host sedimentary rocks at Horonobe Town in Hokkaido, north Japan. In the fiscal year 2025, we continue R&D on "Study on near-field system performance in geological environment" and "Demonstration of repository design options". These are identified as key R&D challenges to be tackled in the Horonobe underground research plan for the fiscal year 2020 onwards. In the "Study on near-field system performance in geological environment", we continue to obtain data from the full-scale engineered barrier system performance experiment, and work on the specifics of the full-scale engineered barrier system dismantling experiment. As for "Demonstration of repository design options", the investigation, design, and evaluation techniques are to be systemized at various scales, from the tunnel to the pit, by means of an organized set of evaluation methodologies for confinement performance at these respective scales. Preliminary borehole investigations will be conducted within a 500 m gallery, with the objectives of obtaining rock strength and rock permeability data, as well as surveying the extent of the excavation damaged zone surrounding the test tunnel via tomographic analysis. A planning study for the in-situ construction test will be conducted to investigate the construction of backfill material and watertight plugs. The volume of water inflow associated with the excavation of the 500 m gallery will be observed, and its magnitude will be compared with the range of water inflow predicted in the analysis. The test plan to determine the extent of the excavation damaged zone around the pit, which is planned to be constructed in the 500 m gallery, will be studied to determine the in-situ excavation damaged zone. In addition, the investigation and evaluation methods for the amount of water inflow from fractures and the extent of the excavation damaged zone around the pit will be organized. Concerning the construction and maintenance of the subsurface facilities, excavation of the West Access Shaft and the 500 m gallery will continue. It is anticipated that the construction of the facilities will be completed by the end of the fiscal year 2025. In addition, we continue R&D on the following three tasks in the Horonobe International Project; Task A: Solute transport experiment with model testing, Task B: Systematic integration of repository technology options, and Task C: Full-scale engineered barrier system dismantling experiment.
Watanabe, Taku*; Maejima, Yui*; Ueda, Yuki; Motokawa, Ryuhei; Takabatake, Ai*; Takeda, Shinichi*; Fudoji, Hiroshi*; Kishikawa, Keiki*; Koori, Michinari*
Langmuir, 41(34), p.22762 - 22773, 2025/09
Times Cited Count：0 Percentile：0.00The assembled structures of melanin particles, i.e., colloidal particles coated with a melanin-like polydopamine (PDA) layer, create vivid structural colors. While the thickness of the PDA layer influences the particle arrangement and optical properties, the underlying mechanism has remained controversial. We demonstrate that the water swelling characteristics of PDA are crucial factors governing the dispersion and aggregation of these particles in solution. Detailed comparisons between dry and wet conditions revealed that the PDA layer readily absorbs water molecules, which leads to significant swelling in the thicker layers. The swelling of the PDA layers determined whether the particles remained dispersed or partially aggregated in the water, ultimately controlling the particle arrangement in the dry state once the water evaporated. These findings provide insights into the self-assembly of colloidal particles and offer a strategy for tuning the periodic particle order. This feature is pivotal for various applications in optical and sensing technologies.
Chiu, I.-H.; Osawa, Takahito; Sumita, Takehiro*; Ikeda, Mizuha*; Ninomiya, Kazuhiko*; Takeda, Shinichiro*; Minami, Takahiro*; Takahashi, Tadayuki*; Watanabe, Shin*
Applied Radiation and Isotopes, 222, p.111845_1 - 111845_7, 2025/08
Takeda, Takeshi
JAEA-Data/Code 2025-005, 106 Pages, 2025/06
JAEA-Data-Code-2025-005.pdf:2.93MB
JAEA has been creating input data for pressurized water reactor (PWR) analysis with RELAP5/MOD3.3 code, mainly based on design information for the four-loop PWR's Tsuruga Power Station Unit-2 as the reference reactor of the Large Scale Test Facility (LSTF). The cold leg large-break loss-of-coolant accident (LBLOCA) calculation in the flamework of the BEMUSE program is cited as a representative OECD/NEA activity related to the PWR analysis. The new regulatory requirements for PWRs in Japan include the event of loss of recirculation functions from emergency core cooling system (ECCS) in the cold leg LBLOCA. This event should be evaluated the effectiveness of measures against severe core damage. The input data for this study were made preparations to analyze the PWR LBLOCA, which is one of the design basis accidents that should be postulated in the safety design. This report describes the main features of the input data for the PWR LBLOCA analysis. The PWR model comprised a reactor vessel, pressurizer (PZR), hot legs, steam generators (SGs), SG secondary-side system, crossover legs, cold legs, and ECCS. A four-loop PWR was simulated by two loops in the LBLOCA calculation. Specifically, loop-A attached with the PZR corresponded to three loops, and loop-B mounted with the break was equal to one loop. The nodalization schemes of the PWR components were referred to those of the LSTF components. Moreover, interpretations were added to the main input data for the PWR LBLOCA analysis, and further information such as the basis for determining the input data was provided. In addition, transient analysis was performed employing the prepared input data for the loss of ECCS recirculation functions event. The present transient analysis was confirmed to be appropriate generally by comparing with the calculation in the previous study using the RELAP5/MOD3.3 code. Furthermore, sensitivity analyses were executed exploiting the RELAP5/MOD3.3 code to clarify the effects of a discharge coefficient through the break and water injection flow rate of the alternative recirculation on the fuel rod cladding surface temperature. This report explains the results of the sensitivity analyses within the defined ranges, which complement some of the content of the previous study's calculation for the loss of ECCS recirculation functions event.
Chiu, I.-H.; Osawa, Takahito; Ninomiya, Kazuhiko*; Takeda, Shinichiro*; Takahashi, Tadayuki*; Katsuragawa, Miho*; Watanabe, Shin*; Kubo, Kenya*; Saito, Tsutomu*; Mizumoto, Kazumi*; et al.
npj Heritage Science (Internet), 13, p.154_1 - 154_9, 2025/05
Co gamma irradiation test results with calculated resultsTakeda, Ryoma; Shibata, Hiroshi; Takeuchi, Tomoaki; Nakano, Hiroko; Seki, Misaki; Ide, Hiroshi
JAEA-Testing 2024-007, 33 Pages, 2025/03
JAEA-Testing-2024-007.pdf:1.63MB
Japan Materials Testing Reactor (JMTR) in Oarai Research and Development Institute of the Japan Atomic Energy Agency (JAEA) has been developing various reactor materials, irradiation techniques and instruments for more than 30 years. Among them, the development of self-powered neutron detectors (SPNDs) and gamma detectors (SPGDs) has been carried out, and several research results have been reported. In this report, we compare and verify these test results with the theoretical output results obtained by the calculation code created in the JAEA report (JAEA-Data/Code 2021-018). The comparison was made with the irradiation test results of SPGD, a cobalt-60 gamma irradiation facility. As a result, it was found that the calculation results reproduced the test results well when the emitter diameter was relatively small compared to the range of Compton scattered electrons by the gamma rays. On the other hand, when the emitter diameter is relatively large, the output current in the test results is only about half of the calculated output current. The self-shielding effect of the emitter may be one of the reasons for the difference in the emitter diameter, and a new formulation, such as incorporating the effect of self-shielding caused by a larger emitter diameter or a non-isotropic -ray field as a change in the mean electron range or mean minimum energy in the calculation code, is necessary. The new formulation is necessary.
Kawasaki, Takuro; Fukuda, Tatsuo; Yamanaka, Satoru*; Murayama, Ichiro*; Kato, Takanori*; Baba, Masaaki*; Hashimoto, Hideki*; Harjo, S.; Aizawa, Kazuya; Tanaka, Hirohisa*; et al.
Journal of Applied Physics, 137(9), p.094101_1 - 094101_7, 2025/03
Times Cited Count：0 Percentile：0.00(Physics, Applied)Takeda, Takeshi
Nihon Genshiryoku Gakkai-Shi ATOMO
, 67(7), p.407 - 410, 2025/00
no abstracts in English
Takeda, Takeshi
JAEA-Data/Code 2024-014, 76 Pages, 2024/12
JAEA-Data-Code-2024-014.pdf:4.0MB
An experiment denoted as SB-PV-03 was conducted on November 19, 2002 using the Large Scale Test Facility (LSTF) in the Rig of Safety Assessment-V (ROSA-V) Program. The ROSA/LSTF experiment SB-PV-03 simulated a 0.2% pressure vessel bottom small-break loss-of-coolant accident in a pressurized water reactor (PWR). The test assumptions included total failure of high pressure injection system of emergency core cooling system (ECCS) and noncondensable gas (nitrogen gas) inflow to the primary system from accumulator (ACC) tanks of ECCS. Secondary-side depressurization of both steam generators (SGs) as an accident management (AM) action to achieve the depressurization rate of 55 K/h in the primary system was initiated 10 min after the generation of a safety injection signal, and continued afterwards. Auxiliary feedwater injection into the secondary-side of both SGs was started for 30 min with some delay after the onset of the AM action. The AM action was effective on the primary depressurization until the ACC tanks began to discharge nitrogen gas into the primary system. The core liquid level recovered in oscillative manner because of intermittent coolant injection from the ACC system into both cold legs. Therefore, the core liquid level remained at a small drop. The pressure difference between the primary and SG secondary sides became larger after nitrogen gas ingress. Core uncovery occurred by core boil-off during reflux condensation in the SG U-tubes under nitrogen gas influx. When the maximum cladding surface temperature of simulated fuel rods exceeded the pre-determined value of 908 K, the core power was automatically reduced to protect the LSTF core. After the automatic core power reduction, coolant injection from low pressure injection (LPI) system of ECCS into both cold legs led to the whole core quench. After the continuous core cooling was confirmed through the actuation of the LPI system, the experiment was terminated.
Ono, Hirokazu; Ishii, Eiichi; Takeda, Masaki
Geoenergy (Internet), 2(1), p.geoenergy2023-047_1 - geoenergy2023-047_10, 2024/12
Hosoda, Masahiro*; Omori, Yasutaka*; Orita, Makiko*; Saito, Kimiaki; Sanada, Tetsuya*; Takeda, Hikaru*; Tani, Kotaro*; Tsujiguchi, Takakiyo*; Hirao, Shigekazu*; Hokama, Tomonori; et al.
Hoken Butsuri (Internet), 59(4), p.206 - 207, 2024/12
no abstracts in English
Cs/
Cs isotope ratioShimada, Asako; Tsukahara, Takehiko*; Nomura, Masao*; Takeda, Seiji
Journal of Radioanalytical and Nuclear Chemistry, 333(12), p.6297 - 6310, 2024/12
Times Cited Count：0 Percentile：0.00(Chemistry, Analytical)Kotegawa, Hisashi*; Nakamura, Akira*; Huyen, V. T. N.*; Arai, Yuki*; To, Hideki*; Sugawara, Hitoshi*; Hayashi, Junichi*; Takeda, Keiki*; Tabata, Chihiro; Kaneko, Koji; et al.
Physical Review B, 110(21), p.214417_1 - 214417_8, 2024/12
Times Cited Count：0 Percentile：19.47(Materials Science, Multidisciplinary)Hirota, Noriaki; Nakano, Hiroko; Takeda, Ryoma; Ide, Hiroshi; Tsuchiya, Kunihiko; Kobayashi, Yoshinao*
Zairyo No Kagaku To Kogaku, 61(6), p.248 - 252, 2024/12
A comparative analysis of the 0.2 % yield stress in SUS304L stainless steel revealed that lower strain rates and higher temperatures significantly reduce yield stress. Grain refinement from 68.6 m to 0.59 m minimally impacted the rate of yield stress reduction at slower strain rates. However, finer grains showed a decrease in yield stress at reactor operating temperature compared to room temperature. In slow strain rate tests under conditions promoting intragranular stress corrosion cracking (SCC), SUS304L with grain sizes of 28.4 m or smaller exhibited similar fracture strains comparable to those at reactor operating temperatures, whereas coarse-grained SUS304L showed reduced fracture strain. Microstructural analysis showed that in smaller grains, over 87 % of the fracture surface was ductile. In particular, SUS304L with 0.59 m grains exhibited a higher presence of {111} / 3 boundaries, which decreased with grain growth. These results indicate that grain refinement will suppress intragranular SCC by slowing corrosion progression through increased {111} / 3 boundaries.
Shimada, Taro; Kabata, Kazuhiko*; Takai, Shizuka; Takeda, Seiji
Proceedings of Probabilistic Safety Assessment and Management & Asian Symposium on Risk Assessment and Management (PSAM17 & ASRAM2024) (Internet), 10 Pages, 2024/10
Nuclear regulatory inspections during the decommissioning phase of nuclear power plants need to be conducted based on risk information, but a method for quantitatively evaluating this risk has not been developed. Therefore, in this study, an event tree of accident events that may occur in the decommissioning phase has been developed, and a code DecAssess-R has been developed to evaluate the exposure risk, which is expressed as the product of the exposure dose and probability of occurrence according to the accident sequence for each equipment to be dismantled. In particular, we have taken into account that the amount of mobile radioactivity that may accumulate in HEPA filters and be released all at once during an accident varies temporally and spatially with the progress of dismantling work. The event tree was constructed based on the results of the survey of domestic and international trouble information in the decommissioning phase and similar dismantling and replacement operations. The event frequencies are based on information from general industries, and the event progression probabilities are based on the equipment failure probabilities in the operation phase. The safety functions to be reduced with the progress of decommissioning were taken into account according to the dismantling work schedule. As a result of the exposure risk assessment for dismantling operations of BWRs and PWRs in Japan, the exposure risk for fire events was the largest. In particular, the exposure risk was greater for the dismantling of components in the reactor building by airborne cutting than for the dismantling of reactor internals, which has the greatest radioactivity in underwater dismantling.
Takeda, Takeshi; Shibata, Taiju
JAEA-Review 2024-040, 29 Pages, 2024/09
JAEA-Review-2024-040.pdf:1.33MB
An important theme of Japan's 6th strategic energy plan is to indicate the energy policy path towards carbon neutrality by 2050. Policy responses for Japan's nuclear energy research and development (R&D) towards 2030 contain the demonstrations of technologies for small modular reactors (SMRs) through international cooperation by 2030. In light of this energy plan, basic policy initiatives over the next 10 years have been compiled to realize Green Transformation (GX), which simultaneously achieves decarbonization and economic growth. Looking overseas, activities of SMR R&D are active internationally, mainly in the US, Canada, Europe, China, and Russia. These activities are not only by heavy industry manufactures and R&D institutes, but also by venture companies. Under these circumstances, the NEA CSNI has gathered an Expert Group on SMRs (EGSMR) to help estimate the safety effects of SMRs. The EGSMR efforts required the submission of responses to several questionnaires whose main purpose was to collect the latest information on the efforts of SMR deployment and research. The first author of this report responded to this based on information from Hitachi-GE Nuclear Energy, Ltd. and Mitsubishi Heavy Industries, Ltd. as well as JAEA. Most of the responses from Japan to the questionnaires are the information that serves as the basis of CSNI Technical Opinion Paper No. 21 (TOP-21). In this report, the Japan's publicly available responses to the questionnaires arranged and additional information are explained, which complements some of the content of the TOP-21. In this manner, the investigation results of R&D related to SMR in Japan, focusing on the EGSMR activities (2022-2023), are summarized. The target of this report is to provide useful information for future discussions on international cooperation concerning SMR as well as nuclear power field human resources development internationally and domestically.
Arai, Yoichi; Watanabe, So; Watanabe, Masayuki; Arai, Tsuyoshi*; Katsuki, Kenta*; Agou, Tomohiro*; Fujikawa, Hisaharu*; Takeda, Keisuke*; Fukumoto, Hiroki*; Hoshina, Hiroyuki*; et al.
Nuclear Instruments and Methods in Physics Research B, 554, p.165448_1 - 165448_10, 2024/09
Times Cited Count：0 Percentile：0.00(Instruments & Instrumentation)Shimada, Taro; Shimada, Asako; Miwa, Kazuji*; Nabekura, Nobuhide*; Sasaki, Toshihisa*; Takai, Shizuka; Takeda, Seiji
JAEA-Research 2024-004, 115 Pages, 2024/06
JAEA-Research-2024-004.pdf:6.02MB
We have studied the confirmation method for the termination of decommissioning of nuclear facilities based on the site release flow presented at the Nuclear Regulation Authority (NRA) study team meeting in 2017, and organized it as a procedure for the site soil. First, the effects of radionuclides released by the Fukushima Daiichi Nuclear Power Station accident are excluded as background radioactivity, and the distribution of radioactivity concentration of facility origin on the site is evaluated using geostatistical method kriging. Then, considering the downstream transport of sediment by surface runoff generated by rainfall that exceeds the infiltration capacity of the ground surface, a series of evaluation procedures are presented to evaluate the exposure dose reflecting future changes from the evaluated radioactivity concentration distribution, and a comparison method with the assumed 0.01 mSv/y as a dose criterion is proposed. Furthermore, an example of the procedure for evaluating the distribution of contamination in the subsurface was also presented for the case where groundwater is affected.
