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Journal Articles

Enhancement of element production by incomplete fusion reaction with weakly bound deuteron

Wang, H.*; Otsu, Hideaki*; Chiga, Nobuyuki*; Kawase, Shoichiro*; Takeuchi, Satoshi*; Sumikama, Toshiyuki*; Koyama, Shumpei*; Sakurai, Hiroyoshi*; Watanabe, Yukinobu*; Nakayama, Shinsuke; et al.

Communications Physics (Internet), 2(1), p.78_1 - 78_6, 2019/07

 Times Cited Count:5 Percentile:62.37(Physics, Multidisciplinary)

Searching for effective pathways for the production of proton- and neutron-rich isotopes through an optimal combination of reaction mechanism and energy is one of the main driving forces behind experimental and theoretical nuclear reaction studies as well as for practical applications in nuclear transmutation of radioactive waste. We report on a study on incomplete fusion induced by deuteron, which contains one proton and one neutron with a weak binding energy and is easily broken up. This reaction study was achieved by measuring directly the cross sections for both proton and deuteron for $$^{107}$$Pd at 50 MeV/u via inverse kinematics technique. The results provide direct experimental evidence for the onset of a cross-section enhancement at high energy, indicating the potential of incomplete fusion induced by loosely-bound nuclei for creating proton-rich isotopes and nuclear transmutation of radioactive waste.

Journal Articles

M$"o$ssbauer and magnetic study of neptunyl(+1) complexes

Nakamoto, Tadahiro*; Nakamura, Akio; Takeda, Masuo*

M$"o$ssbauer Spectroscopy; Applications in Chemistry, Biology, and Nanotechnology, p.95 - 114, 2013/10

Journal Articles

Lanthanides ($$^{151}$$Eu and $$^{155}$$Gd)-M$"o$ssbauer spectroscopic study of defect-fluorite oxides coupled with new defect crystal chemistry model

Nakamura, Akio; Igawa, Naoki; Okamoto, Yoshihiro; Hinatsu, Yukio*; Wang, J.*; Takahashi, Masashi*; Takeda, Masuo*

M$"o$ssbauer Spectroscopy; Applications in Chemistry, Biology, and Nanotechnology, p.71 - 94, 2013/10

Journal Articles

Defect-fluorite oxides; Ln (Eu and Gd) M$"o$ssbauer study coupled with new defect-crystal-chemistry model

Nakamura, Akio; Igawa, Naoki; Okamoto, Yoshihiro; Wang, J.*; Hinatsu, Yukio*; Takahashi, Masashi*; Takeda, Masuo*

Hyperfine Interactions, 217(1-3), p.17 - 26, 2013/04

 Times Cited Count:1 Percentile:54.32

Journal Articles

Molecular magnetism in neptunyl(+1,+2) complexes; $$^{237}$$Np-M$"o$ssbauer and magnetic study

Nakamura, Akio; Nakada, Masami; Nakamoto, Tadahiro*; Kitazawa, Takafumi*; Takeda, Masuo*

Journal of Alloys and Compounds, 444-445, p.621 - 633, 2007/10

 Times Cited Count:3 Percentile:30.36(Chemistry, Physical)

no abstracts in English

Journal Articles

Defect-fluorite oxides M$$_{1-y}$$Ln$$_{y}$$O$$_{2-y/2}$$ (Ln = lanthanide; M = Hf, Zr, Ce, U, Th); Structure, property, and applications

Nakamura, Akio; Masaki, Nobuyuki; Otobe, Haruyoshi; Hinatsu, Yukio*; Wang, J.*; Takeda, Masuo*

Pure and Applied Chemistry, 79(10), p.1691 - 1729, 2007/10

 Times Cited Count:14 Percentile:48.92(Chemistry, Multidisciplinary)

no abstracts in English

Journal Articles

Magnetic property of neptunyl (+2) complex NpO$$_{2}$$(C$$_{6}$$H$$_{7}$$O$$_{2}$$)$$_{2}$$(C$$_{5}$$H$$_{5}$$N)

Nakamura, Akio; Nakada, Masami; Nakamoto, Tadahiro*; Kitazawa, Takafumi*; Takeda, Masuo*

Journal of Magnetism and Magnetic Materials, 310(2, Part2), p.1447 - 1449, 2007/03

Magnetic property of a nitrogen (N)-coordinated neptunyl (+2) (Np(VI)) complex. 1 NpO$$_{2}$$(acac)$$_{2}$$(py) (acac=C$$_{6}$$H$$_{7}$$O$$_{2}$$, py=C$$_{5}$$H$$_{5}$$N) was studied by DC magnetization (M) measurements. While previous $$^{237}$$Np M$"o$ssbauer data of 1 exhibited para magnetic-relaxation spectra similar to other oxo-neptunyls (+1,+2), the DC-$$M$$ data have revealed many strikingly different features of 1 from the latter: first, its reciprocal susceptibility ($$chi$$$$^{-1}$$) vs. $$T$$(K) plots showed a peculiar strongly field ($$H$$)-dependent nonparamagnetic behavior, which suggests the presence of small ferromagnetic component with $$T$$$$_{C}$$$$>$$300 K. In addition, its low-temperature isothermal $$M$$ exhibited anomalous relaxation behavior involving initial over-responsive $$M$$ change and subs equent drift back to its "equilibrium" value ($$M$$$$_{rm eq}$$). Moreover, such $$M$$$$_{rm eq}$$ showed strong perturbation effect from the SQUID-$$M$$ measurement itself. Such novel magnetic features suggest the presence of a largely metastable fluctuating magnetic (spin plus orbital) state in 1 as a collective body of individual Ising-type neptunyl (O=Np=O)$$^{+2}$$ molecular magnets.

Journal Articles

Revaluation of the correlation of isomer shift with Np-O bond length in various neptunyl(V and VI) compounds

Saeki, Masakatsu; Nakada, Masami; Kawasaki, Takeshi*; Nishimura, Tatsuru*; Kitazawa, Takafumi*; Takeda, Masuo*

Journal of Radioanalytical and Nuclear Chemistry, 270(2), p.379 - 384, 2006/11

 Times Cited Count:1 Percentile:10.64(Chemistry, Analytical)

no abstracts in English

Journal Articles

Molecular magnetism of neptunyl (+2) complex NpO$$_{2}$$(C$$_{6}$$H$$_{7}$$O$$_{2}$$)$$_{2}$$(C$$_{5}$$H$$_{5}$$N)

Nakamura, Akio; Nakada, Masami; Nakamoto, Tadahiro*; Kitazawa, Takafumi*; Takeda, Masuo*

Journal of the Physical Society of Japan, 75(Suppl.), p.146 - 148, 2006/08

no abstracts in English

Journal Articles

Correlation of crystal structures with electric field gradients in the fluorite- and pyrochlore-type compounds in the Gd$$_{2}$$O$$_{3}$$-ZrO$$_{2}$$ system

Wang, J.*; Otobe, Haruyoshi; Nakamura, Akio; Takeda, Masuo*

Journal of Solid State Chemistry, 176(1), p.105 - 110, 2003/11

 Times Cited Count:12 Percentile:41.15(Chemistry, Inorganic & Nuclear)

no abstracts in English

Journal Articles

Structural properties of the fluorite- and pyrochlore-type compounds in the Gd$$_{2}$$O$$_{3}$$-ZrO$$_{2}$$ system xGdO$$_{1.5}$$-(1-x)ZrO$$_{2}$$ with 0.18 $$leq$$ x $$leq$$ 0.62

Wang, J.*; Nakamura, Akio; Takeda, Masuo*

Solid State Ionics, 164(3-4), p.185 - 191, 2003/11

 Times Cited Count:32 Percentile:79.26(Chemistry, Physical)

no abstracts in English

Journal Articles

A New type of neptunyl(VI) hydroxide which is topologically similar to $$alpha$$-UO$$_{2}$$(OH)$$_{2}$$

Nakada, Masami; Kitazawa, Takafumi*; Saito, Takashi*; Wang, J.*; Takeda, Masuo*; Yamashita, Toshiyuki; Saeki, Masakatsu

Bulletin of the Chemical Society of Japan, 76(7), p.1375 - 1378, 2003/07

 Times Cited Count:4 Percentile:23.45(Chemistry, Multidisciplinary)

no abstracts in English

Oral presentation

Local-structure of Gd$$_{2}$$Zr$$_{2}$$O$$_{7}$$ and Gd$$_{2}$$Ti$$_{2}$$O$$_{7}$$ probed by EXAFS and $$^{155}$$Gd-Moessbauer methods

Okamoto, Yoshihiro; Fuentes, A.*; Takahashi, Masashi*; Takeda, Masuo*; Nakamura, Akio

no journal, , 

13 (Records 1-13 displayed on this page)
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