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Journal Articles

Experiences in dismantlement of gloveboxes for wet recovery and other use that are contaminated with nuclear fuel materials

Kitamura, Akihiro; Hirano, Hiroshi*; Yoshida, Masato; Takeuchi, Kentaro

Hoken Butsuri (Internet), 58(2), p.76 - 90, 2023/08

The alpha contaminated gloveboxes have been dismantled for over 20 years in Plutonium Fuel Fabrication Facility. The so called wet recovery equipment gloveboxes, which recover plutonium and uranium from scrap fuel by dissolving and extracting processes, were chosen as the priority gloveboxes to be dismantled. These gloveboxes and other gloveboxes in the same room were size reduced and removed up until 2022. Also, non-radioactive ancillary facility and non-radioactive giant glovebox were removed from 2007 to 2010 for ease of glovebox dismantling activities that follows and for making waste storage spaces. Several incidents were occurred and recidivism prevention measures were implemented on each occasion. In this report, glovebox dismantling activities we conducted in the past 20 years are reviewed and lessons we have learned are summarized.

Journal Articles

First observation of $$^{28}$$O

Kondo, Yosuke*; Achouri, N. L.*; Al Falou, H.*; Atar, L.*; Aumann, T.*; Baba, Hidetada*; Boretzky, K.*; Caesar, C.*; Calvet, D.*; Chae, H.*; et al.

Nature, 620(7976), p.965 - 970, 2023/08

 Times Cited Count:6 Percentile:93.26(Multidisciplinary Sciences)

no abstracts in English

Journal Articles

Intruder configurations in $$^{29}$$Ne at the transition into the island of inversion; Detailed structure study of $$^{28}$$Ne

Wang, H.*; Yasuda, Masahiro*; Kondo, Yosuke*; Nakamura, Takashi*; Tostevin, J. A.*; Ogata, Kazuyuki*; Otsuka, Takaharu*; Poves, A.*; Shimizu, Noritaka*; Yoshida, Kazuki; et al.

Physics Letters B, 843, p.138038_1 - 138038_9, 2023/08

 Times Cited Count:2 Percentile:83.53(Astronomy & Astrophysics)

Detailed $$gamma$$-ray spectroscopy of the exotic neon isotope $$^{28}$$Ne has been performed using the one-neutron removal reaction from $$^{29}$$Ne. Based on an analysis of parallel momentum distributions, a level scheme with spin-parity assignments has been constructed for $$^{28}$$Ne and the negative-parity states are identified for the first time. The measured partial cross sections and momentum distributions reveal a significant intruder p-wave strength providing evidence of the breakdown of the N = 20 and N = 28 shell gaps. Only a weak, possible f-wave strength was observed to bound final states. Large-scale shell-model calculations with different effective interactions do not reproduce the large p-wave and small f-wave strength observed experimentally, indicating an ongoing challenge for a complete theoretical description of the transition into the island of inversion along the Ne isotopic chain.

Journal Articles

Sodium-cooled Fast Reactors

Ohshima, Hiroyuki; Morishita, Masaki*; Aizawa, Kosuke; Ando, Masanori; Ashida, Takashi; Chikazawa, Yoshitaka; Doda, Norihiro; Enuma, Yasuhiro; Ezure, Toshiki; Fukano, Yoshitaka; et al.

Sodium-cooled Fast Reactors; JSME Series in Thermal and Nuclear Power Generation, Vol.3, 631 Pages, 2022/07

This book is a collection of the past experience of design, construction, and operation of two reactors, the latest knowledge and technology for SFR designs, and the future prospects of SFR development in Japan. It is intended to provide the perspective and the relevant knowledge to enable readers to become more familiar with SFR technology.

Journal Articles

Identification of advanced spin-driven thermoelectric materials via interpretable machine learning

Iwasaki, Yuma*; Sawada, Ryoto*; Stanev, V.*; Ishida, Masahiko*; Kirihara, Akihiro*; Omori, Yasutomo*; Someya, Hiroko*; Takeuchi, Ichiro*; Saito, Eiji; Yorozu, Shinichi*

npj Computational Materials (Internet), 5, p.103_1 - 103_6, 2019/10

 Times Cited Count:47 Percentile:87.54(Chemistry, Physical)

Journal Articles

Enhancement of element production by incomplete fusion reaction with weakly bound deuteron

Wang, H.*; Otsu, Hideaki*; Chiga, Nobuyuki*; Kawase, Shoichiro*; Takeuchi, Satoshi*; Sumikama, Toshiyuki*; Koyama, Shumpei*; Sakurai, Hiroyoshi*; Watanabe, Yukinobu*; Nakayama, Shinsuke; et al.

Communications Physics (Internet), 2(1), p.78_1 - 78_6, 2019/07

 Times Cited Count:8 Percentile:55.71(Physics, Multidisciplinary)

Searching for effective pathways for the production of proton- and neutron-rich isotopes through an optimal combination of reaction mechanism and energy is one of the main driving forces behind experimental and theoretical nuclear reaction studies as well as for practical applications in nuclear transmutation of radioactive waste. We report on a study on incomplete fusion induced by deuteron, which contains one proton and one neutron with a weak binding energy and is easily broken up. This reaction study was achieved by measuring directly the cross sections for both proton and deuteron for $$^{107}$$Pd at 50 MeV/u via inverse kinematics technique. The results provide direct experimental evidence for the onset of a cross-section enhancement at high energy, indicating the potential of incomplete fusion induced by loosely-bound nuclei for creating proton-rich isotopes and nuclear transmutation of radioactive waste.

Journal Articles

Machine-learning guided discovery of a new thermoelectric material

Iwasaki, Yuma*; Takeuchi, Ichiro*; Stanev, V.*; Gilad Kusne, A.*; Ishida, Masahiko*; Kirihara, Akihiro*; Ihara, Kazuki*; Sawada, Ryoto*; Terashima, Koichi*; Someya, Hiroko*; et al.

Scientific Reports (Internet), 9, p.2751_1 - 2751_7, 2019/02

 Times Cited Count:61 Percentile:93.15(Multidisciplinary Sciences)

Journal Articles

Lessons learned from the risk communication with the public after the Fukushima Daiichi Nuclear Power Plant accident

Kono, Takahiko; Tanaka, Masato*; Sakoda, Akihiro; Tanaka, Hitomi*; Takeuchi, Masato*; Kataoka, Noriaki*

Proceedings of World Engineers Convention Australia 2019 (WEC 2019) (Internet), p.486 - 496, 2019/00

Journal Articles

Technical estimation for mass production of highly-concentrated $$^{rm 99m}$$Tc solution from $$^{99}$$Mo to be obtained by ($$n,gamma$$) reaction; A Preliminary study using inactive Re instead of $$^{rm 99m}$$Tc

Tanase, Masakazu*; Fujisaki, Saburo*; Ota, Akio*; Shiina, Takayuki*; Yamabayashi, Hisamichi*; Takeuchi, Nobuhiro*; Tsuchiya, Kunihiko; Kimura, Akihiro; Suzuki, Yoshitaka; Ishida, Takuya; et al.

Radioisotopes, 65(5), p.237 - 245, 2016/05

no abstracts in English

Journal Articles

Effects of irradiation induced Cu clustering on vickers hardness and electrical resistivity of Fe-Cu model alloys

Tobita, Toru; Nakagawa, Sho*; Takeuchi, Tomoaki; Suzuki, Masahide; Ishikawa, Norito; Chimi, Yasuhiro; Saito, Yuichi; Soneda, Naoki*; Nishida, Kenji*; Ishino, Shiori*; et al.

Journal of Nuclear Materials, 452(1-3), p.241 - 247, 2014/09

 Times Cited Count:17 Percentile:78.17(Materials Science, Multidisciplinary)

Three kinds of Fe-based model alloys, Fe-0.018 atomic percent (at.%) Cu, Fe-0.53at.%Cu, and Fe-1.06at.%Cu were irradiated with 2 MeV electrons up to the dose of 2$$times$$10$$^{-5}$$ dpa at 250$$^{circ}$$C. After the irradiation, the increase in Vickers hardness and the decrease in electrical resistivity were observed. The increase in hardness by electron irradiation is proportional to the product of the Cu contents and the square root of the electron dose. The decrease in electrical resistivity is proportional to the product of the square of Cu contents and the electron dose. Cu clustering in the materials with electron irradiation and thermal aging was observed by means of the three dimensional atom probes (3D-AP). The change in Vickers hardness and electrical resistivity is well correlated with the volume fraction of Cu clusters.

Journal Articles

Development of a model to predict a radionuclide distribution based on soil migration after Fukushima Dai-ichi Nuclear Power Plant accident

Yamaguchi, Masaaki; Maekawa, Keisuke; Takeuchi, Shinji*; Kitamura, Akihiro; Onishi, Yasuo*

Genshiryoku Bakkuendo Kenkyu (CD-ROM), 20(2), p.53 - 69, 2013/12

We developed a simple novel and fast simulation model to predict a long-term distribution of $$^{137}$$Cs deposited on the land surface of Fukushima due to the Fukushima Dai-ichi Nuclear Power Plant accident triggered by a magnitude 9.0 earthquake and resulting tsunami on 11 March 2011. The model utilizes the Geographical Information System (GIS) to integrate online open data provided by individual institutes, and simulate mechanisms of soil erosion, transport and sedimentation. A preliminary calculation shows the significant deposition of sediments in lakes and reservoirs and eroded silt and clay tend to be transported downstream to river mouths than eroded sand. These results were found to be qualitatively consistent with existing data.

Journal Articles

Development of $$^{99m}$$Tc production from (n,$$gamma$$)$$^{99}$$Mo based on solvent extraction

Kimura, Akihiro; Awaludin, R.*; Shiina, Takayuki*; Tanase, Masakazu*; Kawauchi, Yukimasa*; Gunawan, A. H.*; Lubis, H.*; Sriyono*; Ota, Akio*; Genka, Tsuguo; et al.

Proceedings of 3rd Asian Symposium on Material Testing Reactors (ASMTR 2013), p.109 - 115, 2013/11

JP, 2011-173260   Patent publication (In Japanese)

$$^{99m}$$Tc is generated by decay of $$^{99}$$Mo. Production of $$^{99}$$Mo is carried out by (n,f) method with high enriched uranium targets, and the production are currently producing to meet about 95% of global supply. Recently, it is difficult to carry out a stable supply for some problems such as aging of reactors etc. Furthermore, the production has difficulties in nuclear proliferation resistance etc. Thus, (n,$$gamma$$) method has lately attracted considerable attention. The (n,$$gamma$$) method has several advantages, but the extremely low specific activity makes its uses less convenient than (n,f) method. We proposed a method based on the solvent extraction, followed by adsorption of $$^{99m}$$Tc with alumina column. In this paper, a practical production of $$^{99m}$$Tc was tried by the method with 1Ci of $$^{99}$$Mo produced in MPR-30. The recovery yields were approximately 70%. Impurity of $$^{99}$$Mo was less than 4.0$$times$$10$$^{-5}$$% and the radiochemical purity was over 99.2%.

Journal Articles

Development of in-reactor observation system using Cherenkov light, 4

Kimura, Nobuaki; Takeuchi, Tomoaki; Shibata, Akira; Takemoto, Noriyuki; Kimura, Akihiro; Naka, Michihiro; Nishikata, Kaori; Tanimoto, Masataka; Tsuchiya, Kunihiko; Sano, Tadafumi*; et al.

KURRI Progress Report 2012, P. 209, 2013/10

In research reactors, CCD cameras are used to observe reactor core for reactor operation management, e.g. to prevent debris from falling. In order to measure the reactor power and fuel burnup exactly by means of observation of Cherenkov light, the development of the on-line measurement device started in 2009. In this study, the wavelength and the absolute irradiance of the Cherenkov light were measured by a spectrometer, and the Cherenkov light was observed by the CCD camera. As a result, the measurement value is good agreement with the nominal value. On the other hand, the value by the visible imaging system was obtained the same tendency of nominal transmittance value of ND-filters.

Journal Articles

Development of $$^{99m}$$Tc production from (n,$$gamma$$)$$^{99}$$Mo based on solvent extraction and column chromatography

Kimura, Akihiro; Awaludin, R.*; Shiina, Takayuki*; Tanase, Masakazu*; Kawauchi, Yukimasa*; Gunawan, A. H.*; Lubis, H.*; Sriyono*; Ota, Akio*; Genka, Tsuguo; et al.

Proceedings of 6th International Symposium on Material Testing Reactors (ISMTR-6) (Internet), 7 Pages, 2013/10

JP, 2011-173260   Patent publication (In Japanese)

This research is development of $$^{99m}$$Tc production. $$^{99m}$$Tc is generated by decay of $$^{99}$$Mo. The supply of $$^{99}$$Mo in Japan depends entirely on the import from foreign countries. Thus, it is needed to supply $$^{99}$$Mo stably by the domestic manufacturing. A practical production of $$^{99m}$$Tc was tried by the method with 1 Ci of $$^{99}$$Mo produced in MPR-30. The results showed that the recovery yields were approximately 70%. The concentration of the product obtained was estimated to be corresponding to about 30 GBq (800 mCi)/ml when 150g of MoO$$_{3}$$ was irradiated for 5 days in MPR-30. Impurity of $$^{99}$$Mo was less than 4.4$$times$$10$$^{-5}$$%, which was lower than that of Japanese tentative regulation criteria. The radiochemical purity was higher than 99.8% that cleared the tentative regulation (95%) of Japan.

Journal Articles

Development of $$^{rm 99m}$$Tc production from (n, $$gamma$$) $$^{99}$$Mo

Tanase, Masakazu*; Shiina, Takayuki*; Kimura, Akihiro; Nishikata, Kaori; Fujisaki, Saburo*; Ota, Akio*; Kobayashi, Masaaki*; Yamamoto, Asaki*; Kawauchi, Yukimasa*; Tsuchiya, Kunihiko; et al.

Proceedings of 5th International Symposium on Material Testing Reactors (ISMTR-5) (Internet), 9 Pages, 2012/10

$$^{rm 99m}$$Tc is used as a radiopharmaceutical and manufactured from the parent nuclide of $$^{99}$$Mo. Extraction method of $$^{rm 99m}$$Tc from (n, $$gamma$$) $$^{99}$$Mo have been developed, as a part of the industrial use expansion after JMTR will re-start. In this research, the method proposed would be applicable to a practical production of $$^{rm 99m}$$Tc obtained from (n, $$gamma$$) $$^{99}$$Mo in large quantities. The method proposed would be applicable to a practical production of $$^{rm 99m}$$Tc obtained from (n, $$gamma$$) $$^{99}$$Mo in large quantities.

Journal Articles

Stability test of RHQT Nb$$_{3}$$Al cable-in-conduit conductor

Koizumi, Norikiyo; Matsui, Kunihiro; Hemmi, Tsutomu; Nakajima, Hideo; Takeuchi, Takao*; Banno, Nobuya*; Kikuchi, Akihiro*

Teion Kogaku, 46(8), p.495 - 499, 2011/08

JAEA and NIMS has been collaborating in development of high performance Rapid-Heating-Quenching-Transformation (RHQT) Nb$$_{3}$$Al CIC conductor, aiming at the application of this conductor to DEMO plant. The technical issue of the RHQT Nb$$_{3}$$Al strand in the application to a fusion magnet is stabilization against perturbation. NIMS developed technique to attach copper stabilizer by using electroplating and a sub-scale CIC conductor is developed using this conductor. JAEA performed stability test of the developed CIC conductor to demonstrate efficiency of this copper stabilization technique. The measured stability margin is sufficiently high compared to the one of similar NbTi CIC conductor previously tested by the authors. Then, it can be concluded that the copper stabilizer works efficiently from view point of stability, resulting in solving the remained technical issues in the RHQT CIC conductor. Therefore, we can say that the RHQT Nb$$_{3}$$Al CIC conductor is the most promising candidate for application to magnet in DEMO plant.

Journal Articles

Characterization of Nb$$_{3}$$Al strands subjected to an axial-strain for fusion DEMO reactor

Hemmi, Tsutomu; Koizumi, Norikiyo; Nunoya, Yoshihiko; Okui, Yoshio*; Matsui, Kunihiro; Nabara, Yoshihiro; Isono, Takaaki; Takahashi, Yoshikazu; Okuno, Kiyoshi; Banno, Nobuya*; et al.

IEEE Transactions on Applied Superconductivity, 19(3), p.1540 - 1543, 2009/06

 Times Cited Count:16 Percentile:62.03(Engineering, Electrical & Electronic)

Nb$$_{3}$$Al cable-in-conduit (CIC) conductors have been developed as one of candidates for the fusion DEMO reactor. The performances of superconducting strands in the CIC conductor are affected by transverse electromagnetic force and thermal strain at reaction heat treatment. In order to accurately design the conductors for the fusion DEMO reactor, the performance evaluation of the Nb$$_{3}$$Al strands, which is processed by a rapid heating, quenching and transformation (RHQT) method, was performed under various temperature, magnetic field and axial-strain conditions. The measured and parameterized results of the Nb$$_{3}$$Al strands are presented.

Journal Articles

Status and perspective of the Nb$$_{3}$$Al development

Takeuchi, Takao*; Kikuchi, Akihiro*; Banno, Nobuya*; Kitaguchi, Hitoshi*; Iijima, Yasuo*; Tagawa, Kohei*; Nakagawa, Kazuhiko*; Tsuchiya, Kiyosumi*; Mitsuda, Shiori*; Koizumi, Norikiyo; et al.

Cryogenics, 48(7-8), p.371 - 380, 2008/07

 Times Cited Count:62 Percentile:87.94(Thermodynamics)

Nb$$_{3}$$Al has advantages of better tolerance to strain/stress and a higher critical magnetic field (30 T at 4.2 K) for stoichiometric composition over Nb$$_{3}$$Sn. The rapid-heating, quenching and transformation annealing (RHQT) process enables to form a stoichiometric Nb$$_{3}$$Al with fine grain structures via metastable bcc supersaturated-solid-solution. As a result a large critical current density of Nb$$_{3}$$Al is achieved over the whole range of magnetic fields without trading off the excellent strain tolerance. A long-length of RHQ processing has been established, and a rectangular but Cu stabilized Nb$$_{3}$$Al strand is about be commercially available for NMR uses. Ag or Cu internal stabilization and Cu ion-plating/electroplating techniques have been also developed to enable the stabilized round wire for accelerator and fusion magnets. Successfully energized test coils that were manufactured with a wind-and-react technique have demonstrated that a long piece of Cu stabilized RHQT Nb$$_{3}$$Al wire is really available for practical applications.

Journal Articles

Internally Cu-stabilized RHQT Nb$$_{3}$$Al superconductors with Ta matrix

Takeuchi, Takao*; Tagawa, Kohei*; Noda, Tetsuji*; Banno, Nobuya*; Iijima, Yasuo*; Kikuchi, Akihiro*; Kitaguchi, Hitoshi*; Kosuge, Michio*; Tsuchiya, Kiyosumi*; Koizumi, Norikiyo; et al.

IEEE Transactions on Applied Superconductivity, 16(2), p.1257 - 1260, 2006/06

 Times Cited Count:6 Percentile:37.27(Engineering, Electrical & Electronic)

Next generation nuclear fusion magnets would require a high-current conductor in fields more than 16 T. A CIC conductor of the rapid RHQT processed Nb$$_{3}$$Al may be a promising candidate. Good deformability of intermediately-formed bcc supersaturated-solid solution indeed allowed fabricating such a CIC conductor, which would be subsequently transformation annealed. Ag has been internally included as a basic constituent of a round strand so far, because Ag is almost non-reactive with Nb matrix during the RHQ. However, both of Ag and Nb are not suitable nuclei from the viewpoint of radioactivity when irradiated with neutrons. Recently, we have succeeded in replacing the Nb matrix with Ta that has the advantage of shorter half-life of radioactivity. In the present study, an attempt has been made to replace the Ag internal stabilizer with Cu, in the aim of further reducing radioactivity, based on anticipation that Ta would be less reactive with Cu than Nb did.

Journal Articles

Generation of nanometer-sized silicon tadpoles irradiated with a high intensity laser pulse

Sagisaka, Akito; Azuma, Hirozumi*; Daido, Hiroyuki; Kamiya, Nobuo*; Ito, Tadashi*; Takeuchi, Akihiro*; Suzuki, Noritomo*; Nishimura, Akihiko; Mori, Michiaki; Orimo, Satoshi; et al.

Proceedings of 4th International Congress on Laser Advanced Materials Processing (LAMP 2006) (Internet), 3 Pages, 2006/00

no abstracts in English

28 (Records 1-20 displayed on this page)