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Tc solution from 
Mo to be obtained by (
) reaction; A Preliminary study using inactive Re instead of TcTanase, Masakazu*; Fujisaki, Saburo*; Ota, Akio*; Shiina, Takayuki*; Yamabayashi, Hisamichi*; Takeuchi, Nobuhiro*; Tsuchiya, Kunihiko; Kimura, Akihiro; Suzuki, Yoshitaka; Ishida, Takuya; et al.
Radioisotopes, 65(5), p.237 - 245, 2016/05
no abstracts in English
Tc-radiopharmaceuticals obtained from Mo produced by 
Mo(n,2n)Mo and fission of 
UHashimoto, Kazuyuki; Nagai, Yasuki; Kawabata, Masako; Sato, Nozomi*; Hatsukawa, Yuichi; Saeki, Hideya; Motoishi, Shoji*; Ota, Masayuki; Konno, Chikara; Ochiai, Kentaro; et al.
Journal of the Physical Society of Japan, 84(4), p.043202_1 - 043202_4, 2015/04
Times Cited Count：8 Percentile：53(Physics, Multidisciplinary)Tc production from (n,
)Mo based on solvent extractionKimura, Akihiro; Awaludin, R.*; Shiina, Takayuki*; Tanase, Masakazu*; Kawauchi, Yukimasa*; Gunawan, A. H.*; Lubis, H.*; Sriyono*; Ota, Akio*; Genka, Tsuguo; et al.
Proceedings of 3rd Asian Symposium on Material Testing Reactors (ASMTR 2013), p.109 - 115, 2013/11
JP, 2011-173260 
Patent publication (In Japanese)
Tc is generated by decay of Mo. Production of Mo is carried out by (n,f) method with high enriched uranium targets, and the production are currently producing to meet about 95% of global supply. Recently, it is difficult to carry out a stable supply for some problems such as aging of reactors etc. Furthermore, the production has difficulties in nuclear proliferation resistance etc. Thus, (n,) method has lately attracted considerable attention. The (n,) method has several advantages, but the extremely low specific activity makes its uses less convenient than (n,f) method. We proposed a method based on the solvent extraction, followed by adsorption of Tc with alumina column. In this paper, a practical production of Tc was tried by the method with 1Ci of Mo produced in MPR-30. The recovery yields were approximately 70%. Impurity of Mo was less than 4.0
10
% and the radiochemical purity was over 99.2%.
Mo-Tc production process by (n,) reaction with irradiated high-density MoO
pelletsTsuchiya, Kunihiko; Nishikata, Kaori; Tanase, Masakazu*; Shiina, Takayuki*; Ota, Akio*; Kobayashi, Masaaki*; Yamamoto, Asaki*; Morikawa, Yasumasa*; Takeuchi, Nobuhiro*; Kaminaga, Masanori; et al.
Proceedings of 6th International Symposium on Material Testing Reactors (ISMTR-6) (Internet), 9 Pages, 2013/10
no abstracts in English
Tc production from (n,)Mo based on solvent extraction and column chromatographyKimura, Akihiro; Awaludin, R.*; Shiina, Takayuki*; Tanase, Masakazu*; Kawauchi, Yukimasa*; Gunawan, A. H.*; Lubis, H.*; Sriyono*; Ota, Akio*; Genka, Tsuguo; et al.
Proceedings of 6th International Symposium on Material Testing Reactors (ISMTR-6) (Internet), 7 Pages, 2013/10
JP, 2011-173260Patent publication (In Japanese)
This research is development of Tc production. Tc is generated by decay of Mo. The supply of Mo in Japan depends entirely on the import from foreign countries. Thus, it is needed to supply Mo stably by the domestic manufacturing. A practical production of Tc was tried by the method with 1 Ci of Mo produced in MPR-30. The results showed that the recovery yields were approximately 70%. The concentration of the product obtained was estimated to be corresponding to about 30 GBq (800 mCi)/ml when 150g of MoO was irradiated for 5 days in MPR-30. Impurity of Mo was less than 4.410%, which was lower than that of Japanese tentative regulation criteria. The radiochemical purity was higher than 99.8% that cleared the tentative regulation (95%) of Japan.
Nagai, Yasuki; Hashimoto, Kazuyuki; Hatsukawa, Yuichi; Saeki, Hideya; Motoishi, Shoji; Sonoda, Nozomi; Kawabata, Masako; Harada, Hideo; Kin, Tadahiro*; Tsukada, Kazuaki; et al.
Journal of the Physical Society of Japan, 82(6), p.064201_1 - 064201_7, 2013/06
Times Cited Count：43 Percentile：85.02(Physics, Multidisciplinary)Tc production from (n, ) MoTanase, Masakazu*; Shiina, Takayuki*; Kimura, Akihiro; Nishikata, Kaori; Fujisaki, Saburo*; Ota, Akio*; Kobayashi, Masaaki*; Yamamoto, Asaki*; Kawauchi, Yukimasa*; Tsuchiya, Kunihiko; et al.
Proceedings of 5th International Symposium on Material Testing Reactors (ISMTR-5) (Internet), 9 Pages, 2012/10
Tc is used as a radiopharmaceutical and manufactured from the parent nuclide of Mo. Extraction method of Tc from (n, ) Mo have been developed, as a part of the industrial use expansion after JMTR will re-start. In this research, the method proposed would be applicable to a practical production of Tc obtained from (n, ) Mo in large quantities. The method proposed would be applicable to a practical production of Tc obtained from (n, ) Mo in large quantities.
Mo-Tc domestic production with high-density MoO pellets by (n,) reactionTsuchiya, Kunihiko; Tanase, Masakazu*; Takeuchi, Nobuhiro*; Kobayashi, Masaaki*; Hasegawa, Yoshio*; Yoshinaga, Hideo*; Kaminaga, Masanori; Ishihara, Masahiro; Kawamura, Hiroshi
Proceedings of 5th International Symposium on Material Testing Reactors (ISMTR-5) (Internet), 10 Pages, 2012/10
As one of effective uses of the JMTR, JAEA has a plan to produce Mo by (n, ) method, a parent nuclide of Tc. In case of Japan, the supplying of Mo depends only on imports from foreign countries. The R&D on production method of Mo -Tc has been performed with Japanese industrial users under the cooperation programs. The main R&D items for the production are (1) Fabrication of irradiation target such as the sintered MoO pellets, (2) Separation and concentration of Tc by the solvent extraction from Mo solution, (3) Examination of Tc solution for a medicine, and (4) Mo recycling from Mo generator and solution. In this paper, the status of the R&D is introduced for the production of Mo -Tc.
-ray and neutron area monitoring system for the IFMIF/EVEDA accelerator buildingTakahashi, Hiroki; Maebara, Sunao; Kojima, Toshiyuki; Kubo, Takashi; Sakaki, Hironao; Takeuchi, Hiroshi; Shidara, Hiroyuki; Hirabayashi, Keiichi*; Hidaka, Kosuke*; Shigyo, Nobuhiro*; et al.
Fusion Engineering and Design, 86(9-11), p.2795 - 2798, 2011/10
Times Cited Count：2 Percentile：18.29(Nuclear Science & Technology)In the IFMIF/EVEDA accelerator, the engineering validation up to 9 MeV by employing the deuteron beam of 125 mA are planning at the BA site in Rokkasho, Aomori, Japan, the personnel protection system (PPS) is indispensable. The PPS inhibit the beam by receiving the interlock signal from the -ray and neutron monitoring system. The -ray and neutron detection level which is planned to be adopted are "80 keV to 1.5 MeV (-ray)" and "0.025 eV to 15 MeV (neutron)". For the present shielding design, it is absolutely imperative for the safety review to validate the shielding ability which makes detection level lower than these -ray and neutron detector. For this purpose, the energy reduction of neutron and photon for water and concrete is evaluated by PHITS code. From the calculating results, it is found that the photon energy range extended to 10 MeV by water and concrete shielding material only, an additional shielding to decrease the photon energy of less than 1.5 MeV is indispensable.
Tc-MDP using Tc separated from Mo produced by Mo(
,2)MoNagai, Yasuki; Hatsukawa, Yuichi; Kin, Tadahiro; Hashimoto, Kazuyuki; Motoishi, Shoji; Konno, Chikara; Ochiai, Kentaro; Takakura, Kosuke; Sato, Yuichi*; Kawauchi, Yukimasa*; et al.
Journal of the Physical Society of Japan, 80(8), p.083201_1 - 083201_4, 2011/08
Times Cited Count：15 Percentile：65.33(Physics, Multidisciplinary)We have for the first time succeeded to separate Tc from a Mo oxide sample irradiated by accelerator neutrons, and to formulate Tc-methylene diphosphonate (Tc-MDP). Mo, the mother nuclide of Tc, was produced by the Mo(,2)Mo reaction using about 14 MeV neutrons provided at the Fusion Neutronics Source of Japan Atomic Energy Agency. The Tc was separated from Mo by the sublimation method, and its radionuclide purity was confirmed to be higher than 99.99%. The labeling efficiency of Tc-MDP was shown to be higher than 99%. These values exceed the United States Pharmacopeia requirements for a fission product, Mo. Consequently, a Tc radiopharmaceutical preparation formed by using the mentioned Mo can be a promising substitute for the fission product Mo. A longstanding problem to ensure a reliable and constant supply of Mo in Japan can be partially mitigated.
Kabumoto, Hiroshi; Takeuchi, Suehiro; Ishizaki, Nobuhiro; Yoshida, Takahiro*; Ishiguro, Takayuki*; Yamaguchi, Kazushi*
Proceedings of 6th Annual Meeting of Particle Accelerator Society of Japan (CD-ROM), p.1120 - 1122, 2010/03
The JAEA-Tokai tandem accelerator was built for basic science researches with heavy ions. Its superconducting booster was completed in 1994 for increasing the acceleration energy of ions. The booster consists of 40 superconducting acceleration resonators and 10 cryostats. Every resonator is a coaxial quarter wave resonator (QWR) of which frequency is 129.8MHz, and optimum beam velocity is 10% of the light velocity. When it was built, the acceleration field gradients of superconducting resonators were 5.0MV/m at RF power input of 4W on their average. The performance decrease little by little, and it become 4.0MV/m now. Some of the resonators generate X-rays from a low electric field. A field emission will be occurred from small contaminations accumulated on the surfaces of niobium. We examined the high pressure water jet rinsing (HPWR) to re-recondition the superconducting booster. The HPWR is the technology of removing small contaminations on resonator surfaces, and very effective for the improvement of acceleration field gradients. The acceleration field gradients of 20 on-line resonators were improved from 4.4MV to 5.7MV on their average.
Kabumoto, Hiroshi; Takeuchi, Suehiro; Ishizaki, Nobuhiro; Yoshida, Takahiro*; Ishiguro, Takayuki*; Yamaguchi, Kazushi*
Dai-22-Kai Tandemu Kasokuki Oyobi Sono Shuhen Gijutsu No Kenkyukai Hokokushu, p.129 - 132, 2010/01
The JAEA-Tokai tandem accelerator was built for basic science researches with heavy ions. Its superconducting booster was completed in 1994 for increasing the acceleration energy of ions. The booster consists of 40 superconducting acceleration resonators and 10 cryostats. Every resonator is a coaxial quarter wave resonator (QWR) of which frequency is 129.8 MHz, and optimum beam velocity is 10% of the light velocity. When it was built, the acceleration field gradients of superconducting resonators were 5.0 MV/m at RF power input of 4 W on their average. The performance decrease little by little, and it become 4.0 MV/m now. Some of the resonators generate X-rays from a low electric field. A field emission will be occurred from small contaminations accumulated on the surfaces of niobium. We examined the high pressure water jet rinsing (HPWR) to re-recondition the superconducting booster. The HPWR is the technology of removing small contaminations on resonator surfaces, and very effective for the improvement of acceleration field gradients. The acceleration field gradients of 20 on-line resonators were improved from 4.4 MV to 5.7 MV on their average.
Kabumoto, Hiroshi; Takeuchi, Suehiro; Matsuda, Makoto; Ishizaki, Nobuhiro; Otokawa, Yoshinori
Nuclear Instruments and Methods in Physics Research A, 612(2), p.221 - 224, 2010/01
Times Cited Count：1 Percentile：13.85(Instruments & Instrumentation)We have designed and fabricated a superconducting twin-quarter-wave resonator (Twin-QWR) made of niobium and copper for the acceleration of low velocity heavy ions. The resonator has two inner conductors and three acceleration gaps which give a resonant frequency of 129.8 MHz and an optimum beam velocity of 6% of the light velocity. Each inner conductor resonates like in a coaxial quarter-wave line resonator. The resonator was designed to have a separable structure so that we could treat the inner conductor's part fully made of high purity niobium apart from the outer conductor made of niobium and copper. We obtained an acceleration field gradient of 5.8 MV/m at an RF power input of 4 W.
Kabumoto, Hiroshi; Takeuchi, Suehiro; Matsuda, Makoto; Ishizaki, Nobuhiro; Otokawa, Yoshinori
Proceedings of 14th International Conference on RF Superconductivity (SRF 2009) (Internet), p.849 - 853, 2009/11
The JAEA-Tokai tandem accelerator was built for basic science researches with heavy ions. Its superconducting booster was developed for increasing the acceleration energy of ions. We have designed and fabricated a superconducting twin-quarter-wave resonator (Twin-QWR) made of niobium and copper for the acceleration of low velocity heavy ions from TRIAC facility. The resonator has two inner conductors and three acceleration gaps which give a resonant frequency of 129.8 MHz and an optimum beam velocity of 6% of the light velocity. Each inner conductor resonates like in a coaxial quarter-wave line resonator. The resonator was designed to have a separatable structure so that we could treat the inner conductors part fully made of high purity niobium apart from the outer conductor made of niobium and copper. We obtained an acceleration field gradient of 5.8 MV/m at an RF power input of 4 W.
superconducting twin quarter wave resonatorKabumoto, Hiroshi; Takeuchi, Suehiro; Ishizaki, Nobuhiro; Matsuda, Makoto; Otokawa, Yoshinori
JAEA-Conf 2008-005, p.137 - 140, 2008/03
no abstracts in English
Matsuda, Makoto; Sataka, Masao; Takeuchi, Suehiro; Tsukihashi, Yoshihiro; Hanashima, Susumu; Abe, Shinichi; Osa, Akihiko; Ishizaki, Nobuhiro; Tayama, Hidekazu; Nakanoya, Takamitsu; et al.
JAEA-Conf 2008-005, p.42 - 45, 2008/03
In FY2006, a tandem accelerator was operated for 201days. The maximum voltage was 18 MV and the accelerated ion species was 19 elements (26 nuclides). As the trouble case which occurred previous year, the change of the beam shape occurred often in the injection beam line of the tandem accelerator. The cause was the contact failure of the pole connector of the electrostatics quadrupole lens. Generally, it was difficult to confirm the connection status of the opened pole but we specified a connection abnormal part by the capacitive coupling method. This technique is useful technology which can be applied to the other electrostatics optics elements. Because the charging electric current flowed only about usual about 60% and the terminal voltage became unstable, we opened a tank and checked the charging system. As a result, a problem was confirmed to the damaging of resistance and the installation of the cable. In the seminar, the operation, maintenance and the accelerator development of the tandem accelerator in FY2006 are described.
Matsuda, Makoto; Takeuchi, Suehiro; Tsukihashi, Yoshihiro; Hanashima, Susumu; Abe, Shinichi; Osa, Akihiko; Ishizaki, Nobuhiro; Tayama, Hidekazu; Nakanoya, Takamitsu; Kabumoto, Hiroshi; et al.
Dai-19-Kai Tandemu Kasokuki Oyobi Sono Shuhen Gijutsu No Kenkyukai Hokokushu, p.9 - 12, 2007/01
no abstracts in English
Kabumoto, Hiroshi; Takeuchi, Suehiro; Ishizaki, Nobuhiro; Matsuda, Makoto; Otokawa, Yoshinori
Proceedings of 4th Annual Meeting of Particle Accelerator Society of Japan and 32nd Linear Accelerator Meeting in Japan (CD-ROM), p.469 - 471, 2007/00
JAEA and KEK have started acceleration of radioactive nuclear beam (RNB) and stable ion beam (SNB) from Tokai Radioactive Ion Accelerator Complex (TRIAC) in 2005. RNB and SNB are accelerated by SCRFQ and IH linac up to the energy of 1.1 MeV/u. We were planning to re-accelerate the beams in the future by superconducting booster up to energy of 5-8 MeV/u. In order to inject the beams into superconducting booster, we need a pre-booster which is capable of acceleration from 1.1 MeV/u to 2.0 MeV/u. We have started development of superconducting twin quarter wave resonator (Twin-QWR), and have fabricated a prototype Twin-QWR in FY2005. We have carried out performance test of prototype Twin-QWR in FY2006.
Matsuda, Makoto; Takeuchi, Suehiro; Tsukihashi, Yoshihiro; Hanashima, Susumu; Abe, Shinichi; Osa, Akihiko; Ishizaki, Nobuhiro; Tayama, Hidekazu; Nakanoya, Takamitsu; Kabumoto, Hiroshi; et al.
Proceedings of 3rd Annual Meeting of Particle Accelerator Society of Japan and 31st Linear Accelerator Meeting in Japan, p.275 - 277, 2006/00
no abstracts in English
Matsuda, Makoto; Takeuchi, Suehiro; Tsukihashi, Yoshihiro; Horie, Katsuzo*; Ouchi, Isao*; Hanashima, Susumu; Abe, Shinichi; Ishizaki, Nobuhiro; Tayama, Hidekazu; Nakanoya, Takamitsu; et al.
Dai-18-Kai Tandemu Kasokuki Oyobi Sono Shuhen Gijutsu No Kenkyukai Hokokushu, p.11 - 14, 2005/11
no abstracts in English
