Contrast dependence of scattering profiles for poly(ethylene glycol) in water; Investigation by small-angle neutron scattering with He spin filter and small-angle X-ray scattering

Ryoki, Akiyuki*; Watanabe, Fumi*; Okudaira, Takuya*; Takahashi, Shingo*; Oku, Takayuki; Hiroi, Kosuke; Motokawa, Ryuhei; Nakamura, Yo*

Journal of Chemical Physics, 160(11), p.114907_1 - 114907_9, 2024/03

https://doi.org/10.1063/5.0192680

Design and actual performance of J-PARC 3 GeV rapid cycling synchrotron for high-intensity operation

Yamamoto, Kazami; Kinsho, Michikazu; Hayashi, Naoki; Saha, P. K.; Tamura, Fumihiko; Yamamoto, Masanobu; Tani, Norio; Takayanagi, Tomohiro; Kamiya, Junichiro; Shobuda, Yoshihiro; et al.

Journal of Nuclear Science and Technology, 59(9), p.1174 - 1205, 2022/09

https://doi.org/10.1080/00223131.2022.2038301

In the Japan Proton Accelerator Research Complex, the purpose of the 3 GeV rapid cycling synchrotron (RCS) is to accelerate a 1 MW, high-intensity proton beam. To achieve beam operation at a repetition rate of 25 Hz at high intensities, the RCS was elaborately designed. After starting the RCS operation, we carefully verified the validity of its design and made certain improvements to establish a reliable operation at higher power as possible. Consequently, we demonstrated beam operation at a high power, namely, 1 MW. We then summarized the design, actual performance, and improvements of the RCS to achieve a 1 MW beam.

High-spatial-resolution measurement of magnetization distribution using polarized neutron imaging

Sasada, Seiji*; Hiroi, Kosuke; Osanai, Kenta*; Shinohara, Takenao; Watanabe, K.*; Uritani, Akira*

Japanese Journal of Applied Physics, 60(12), p.126003_1 - 126003_6, 2021/12

https://doi.org/10.35848/1347-4065/ac3524

Measurement of double-differential thick-target neutron yields of the C() reaction at 12, 20, and 30 MeV

Patwary, M. K. A*; Kin, Tadahiro*; Aoki, Katsumi*; Yoshinami, Kosuke*; Yamaguchi, Masaya*; Watanabe, Yukinobu*; Tsukada, Kazuaki; Sato, Nozomi*; Asai, Masato; Sato, Tetsuya; et al.

Journal of Nuclear Science and Technology, 58(2), p.252 - 258, 2021/02

https://doi.org/10.1080/00223131.2020.1819908

While designing deuteron accelerator neutron sources for radioisotopes production, nuclear data for light elements such as Li, Be, and C have been systematically measured in the deuteron energy range from a few MeV to around 50 MeV. Currently, the experimental data available on double-differential thick-target neutron yields (DDTTNYs) is insufficient, especially for deuteron energies between 18 and 33 MeV. In this study, we measured the DDTTNYs of () reactions on C target for incident deuteron energies of 12, 20, and 30 MeV using the multiple-foils activation method to improve nuclear data insufficiency. We applied the GRAVEL code for the unfolding process to derive the DDTTNYs. The results were compared with the calculation by DEURACS. The present data were also used to confirm the systematics of the differential neutron yields at 0 and total neutron yield per incident deuteron in the wide range of deuteron energy.

Experimental determination of the photooxidation of aqueous I as a source of atmospheric I

Watanabe, Kosuke*; Matsuda, Shohei; Cuevas, C. A.*; Saiz-Lopez, A.*; Yabushita, Akihiro*; Nakano, Yukio*

ACS Earth and Space Chemistry (Internet), 3(4), p.669 - 679, 2019/04

https://doi.org/10.1021/acsearthspacechem.9b00007

The photooxidation of aqueous iodide ions (I) at sea surface results in the emission of gaseous iodine molecules (I) into the atmosphere. It plays a certain role in the transport of iodine from ocean to the atmosphere in the natural cycle of iodine. In this study, we determined the photooxidation parameters, the molar absorption coefficient (()) and the photooxidative quantum yields (()) of I, in the range of 290-500 nm. Through the investigation of the influence of pH and dissolved oxygen (DO) on (), the subsequent emission rates of I following the photooxidation of I in deionized water solution (pH 5.6, DO 7.8 mg L) and artificial seawater solution (pH 8.0, DO 7.0 mg L) were estimated. A global chemistry-climate model employed herein to assess the I ocean emission on a global scale indicated that the photooxidation of I by solar light can enhance the atmospheric iodine budget by up to 8% over some oceanic regions.

Determination of fusion barrier distributions from quasielastic scattering cross sections towards superheavy nuclei synthesis

Tanaka, Taiki*; Narikiyo, Yoshihiro*; Morita, Kosuke*; Fujita, Kunihiro*; Kaji, Daiya*; Morimoto, Koji*; Yamaki, Sayaka*; Wakabayashi, Yasuo*; Tanaka, Kengo*; Takeyama, Mirei*; et al.

Journal of the Physical Society of Japan, 87(1), p.014201_1 - 014201_9, 2018/01

https://doi.org/10.7566/JPSJ.87.014201

Excitation functions of quasielastic scattering cross sections for the Ca + Pb, Ti + Pb, and Ca + Cm reactions were successfully measured by using the gas-filled recoil-ion separator GARIS. Fusion barrier distributions were extracted from these data, and compared with the coupled-channels calculations. It was found that the peak energies of the barrier distributions for the Ca + Pb and Ti + Pb systems coincide with those of the 2n evaporation channel cross sections for the systems, while that of the Ca + Cm is located slightly below the 4n evaporation ones. This results provide us helpful information to predict the optimum beam energy to synthesize superheavy nuclei.

Observation of doubly-charged ions of francium isotopes extracted from a gas cell

Schury, P.*; Wada, Michiharu*; Ito, Yuta*; Kaji, Daiya*; Haba, Hiromitsu*; Hirayama, Yoshikazu*; Kimura, Sota*; Koura, Hiroyuki; MacCormick, M.*; Miyatake, Hiroari*; et al.

Nuclear Instruments and Methods in Physics Research B, 407, p.160 - 165, 2017/06

https://doi.org/10.1016/j.nimb.2017.06.014

Various isotopes of Ac, Ra, Fr, and Rn were produced by fusion-evaporation reactions using a Ca beam. The energetic ions were stopped in and extracted from a helium gas cell. The extracted ions were identified using a multi-reflection time-of-fight mass spectrograph. In all cases, it was observed that the predominant charge state for the extracted ions, including the alkali Fr, was 2+.

Evaluation of -ray and neutron energy for area monitoring system in the IFMIF/EVEDA accelerator building

Takahashi, Hiroki; Maebara, Sunao; Sakaki, Hironao; Hirabayashi, Keiichi*; Hidaka, Kosuke*; Shigyo, Nobuhiro*; Watanabe, Yukinobu*; Sagara, Kenshi*

Fusion Engineering and Design, 87(7-8), p.1235 - 1238, 2012/08

https://doi.org/10.1016/j.fusengdes.2012.02.109

The Engineering Validation of the IFMIF/EVEDA prototype accelerator, up to 9 MeV by supplying the deuteron beam of 125 mA, will be performed at the BA site in Rokkasho. A design of this area monitoring system, comprising of Si semiconductors and ionization chambers for covering wide energy spectrum of -rays and He counters for neutrons, is now in progress. To establish an applicability of this monitoring system, photon and neutron energies have to be suppressed to the detector ranges of 1.5 MeV and 15 MeV, respectively. For this purpose, the reduction of neutron and photon energies throughout shield of water in a beam dump and concrete layer is evaluated by PHITS code, using the experimental data of neutron source spectra. In this article, a similar model using the beam dump structure and the position with a degree of leaning for concrete wall in the accelerator vault is used, and their energy reduction including the air is evaluated.

Activation analyses by the beam losses in the IFMIF/EVEDA accelerator

Maebara, Sunao; Takahashi, Hiroki; Sakaki, Hironao; Hirabayashi, Keiichi*; Hidaka, Kosuke*; Shigyo, Nobuhiro*; Watanabe, Yukinobu*; Sagara, Kenshi*

JAEA-Conf 2011-002, p.199 - 204, 2011/09

https://jopss.jaea.go.jp/pdfdata/JAEA-Conf-2011-002.pdf

Study on flow-induced-vibration evaluation of large-diameter pipings in a sodium-cooled fast reactor, 1; Sensitivity analysis of turbulent flow models for unsteady short-elbow pipe flow

Aizawa, Kosuke; Nakanishi, Shigeyuki; Yamano, Hidemasa; Kotake, Shoji; Hayakawa, Satoshi*; Watanabe, Osamu*; Fujimata, Kazuhiro*

Proceedings of 6th Japan-Korea Symposium on Nuclear Thermal Hydraulics and Safety (NTHAS-6) (USB Flash Drive), 7 Pages, 2008/11

To evaluate the flow-induced vibration in the actual-sized pipings of JSFR, computer simulation is necessary. In this study, as the first step, sensitivity analysis of turbulence flow models for unsteady short-elbow pipe flow has been carried out with the STAR-CD thermal-hydraulic simulation code. Through the sensibility analysis, the objective of this study is to propose the best analysis models which can reproduce the unsteady characteristics obtained in the 1/3-scale test results with 9.2 m/s of main flow. In this study, to take into account anisotropic characteristics of turbulence, two turbulent flow models were used: large eddy simulation (LES) and Reynolds stress model (RSM). The both validated simulations have reproduced flow separation region and periodic vortex shedding. The simulation results with both models were compared with power spectrum densities of pressure fluctuations which were used in the pipe vibration evaluation. Only the RSM simulation with the best combination has reproduced the pressure-fluctuation power spectrum densities, which were characterized by a peak frequency of 10 Hz in the 1/3 test with 9.2 m/s.