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Journal Articles

Intercalative and non-intercalative photo-recharge using all-solid-state cells for solar energy conversion and storage

Yoshimoto, Masataka*; Tamura, Kazuhisa; Watanabe, Kenta*; Shimizu, Keisuke*; Horisawa, Yuhei*; Kobayashi, Takeshi*; Tsurita, Hanae*; Suzuki, Kota*; Kanno, Ryoji*; Hirayama, Masaaki*

Sustainable Energy & Fuels (Internet), 8(6), p.1236 - 1244, 2024/03

Photo-rechargeable systems, which can efficiently convert and store solar energy into chemical energy within single devices, are essential to harness sunlight effectively. Photo-(de)intercalation plays a pivotal role in the functionality of photorechargeable systems. Nevertheless, the photo-(de)intercalation process has not been conclusively confirmed owing to potential interference from side reactions, such as the decomposition of liquid electrolytes and the elution of electrode materials. In this study, we successfully demonstrated photo-responsive Li$$^{+}$$-deintercalation using an all-solid-state thin-film battery comprised of epitaxially-grown anatase TiO$$_{2}$$ doped with Nb (a-TiO$$_{2}$$:Nb) as the cathode. Under light irradiation, Li$$^{+}$$-deintercalation occurred and was subsequently reversibly intercalated into a-TiO$$_{2}$$:Nb during discharge.

Journal Articles

Arrangements for telephone consultation on radiation health effects in a nuclear emergency in Japan; Lessons learned from the nuclear accident in Fukushima, Japan, 2011

Okuno, Hiroshi; Kawakami, Takeshi; Watanabe, Fumitaka; Horikoshi, Hidehiko*

Journal of Disaster Research, 18(8), p.911 - 917, 2023/12

In response to residents' concerns about the radiation health effects following the nuclear accidents at the Fukushima Daiichi Nuclear Power Station of the Tokyo Electric Power Company in March 2011, the Japan Atomic Energy Agency (JAEA) established a telephone consultation system. Eight toll-free telephone lines were prepared, and employees with knowledge of radiation health effects were assigned for consultation. Approximately 35,000 consultations were conducted from March 17, 2011, to September 18, 2012. The results of the text mining analysis revealed that the greatest source of anxiety was the impact on children's health from radiation. The JAEA's system for telephone consultation was improved following this telephone consultation experience. The description of telephone hotlines in the International Atomic Energy Agency (IAEA) guide, GSG-14, was discussed for further improvements of the JAEA's telephone consultation system.

Journal Articles

Decontamination and solidification treatment on spent liquid scintillation cocktail

Watanabe, So; Takahatake, Yoko; Ogi, Hiromichi*; Osugi, Takeshi; Taniguchi, Takumi; Sato, Junya; Arai, Tsuyoshi*; Kajinami, Akihiko*

Journal of Nuclear Materials, 585, p.154610_1 - 154610_6, 2023/11

 Times Cited Count:0 Percentile:0.01

Journal Articles

Development of nondestructive elemental analysis system for Hayabusa2 samples using muonic X-rays

Osawa, Takahito; Nagasawa, Shunsaku*; Ninomiya, Kazuhiko*; Takahashi, Tadayuki*; Nakamura, Tomoki*; Wada, Taiga*; Taniguchi, Akihiro*; Umegaki, Izumi*; Kubo, Kenya*; Terada, Kentaro*; et al.

ACS Earth and Space Chemistry (Internet), 7(4), p.699 - 711, 2023/04

The concentrations of carbon and other major elements in asteroid samples provide very important information on the birth of life on the Earth and the solar-system evolution. Elemental analysis using muonic X-rays is one of the best analytical methods to determine the elemental composition of solid materials, and notably, is the only method to determine the concentration of light elements in bulk samples in a non-destructive manner. We developed a new analysis system using muonic X-rays to measure the concentrations of carbon and other major elements in precious and expectedly tiny samples recovered from the asteroid Ryugu by spacecraft Hayabusa2. Here we report the development process of the system in 4 stages and their system configurations, The analysis system is composed of a stainless-steel analysis chamber, an acrylic glove box for manipulating asteroid samples in a clean environment, and Ge semiconductor detectors arranged to surround the analysis chamber. The performance of the analysis system, including the background level, which is crucial for the measurement, was greatly improved from the first stage to the later ones. Our feasibility study showed that the latest model of our muonic X-ray analysis system is capable of determining the carbon concentration in Hayabusa2's sample model with an uncertainty of less than 10 percent in a 6-day measurement.

Journal Articles

Nature of the physicochemical process in water photolysis uncovered by a computer simulation

Kai, Takeshi; Toigawa, Tomohiro; Ukai, Masatoshi*; Fujii, Kentaro*; Watanabe, Ritsuko*; Yokoya, Akinari*

Journal of Chemical Physics, 158(16), p.164103_1 - 164103_8, 2023/04

New insight into water radiolysis and photolysis is indispensable in the dramatic progress of sciences and technologies in various research areas. In the radiation field, reactive hydrated electrons are considerably produced along radiation tracks. Although the formation results from a transient dynamic correlation between ejected electrons and water, the individual mechanisms of electron thermalization, delocalization, and polarization are unknown. Using a dynamic Monte Carlo code, we show herein that the ejected electrons are immediately delocalized by molecular excitations in parallel with phonon polarization and gradually thermalized by momentum transfer with an orientation polarization in a simultaneous manner. Our results show that these mechanisms heavily depend on the intermolecular vibration and rotation modes peculiar to water. We expect our approach to be a powerful technique for connecting physical and chemical processes in various solvents.

Journal Articles

Design and actual performance of J-PARC 3 GeV rapid cycling synchrotron for high-intensity operation

Yamamoto, Kazami; Kinsho, Michikazu; Hayashi, Naoki; Saha, P. K.; Tamura, Fumihiko; Yamamoto, Masanobu; Tani, Norio; Takayanagi, Tomohiro; Kamiya, Junichiro; Shobuda, Yoshihiro; et al.

Journal of Nuclear Science and Technology, 59(9), p.1174 - 1205, 2022/09

 Times Cited Count:3 Percentile:80.29(Nuclear Science & Technology)

In the Japan Proton Accelerator Research Complex, the purpose of the 3 GeV rapid cycling synchrotron (RCS) is to accelerate a 1 MW, high-intensity proton beam. To achieve beam operation at a repetition rate of 25 Hz at high intensities, the RCS was elaborately designed. After starting the RCS operation, we carefully verified the validity of its design and made certain improvements to establish a reliable operation at higher power as possible. Consequently, we demonstrated beam operation at a high power, namely, 1 MW. We then summarized the design, actual performance, and improvements of the RCS to achieve a 1 MW beam.

Journal Articles

Measurement of nuclide production cross sections for proton-induced reactions on $$^{rm nat}$$Ni and $$^{rm nat}$$Zr at 0.4, 1.3, 2.2, and 3.0 GeV

Takeshita, Hayato*; Meigo, Shinichiro; Matsuda, Hiroki*; Iwamoto, Hiroki; Nakano, Keita; Watanabe, Yukinobu*; Maekawa, Fujio

Nuclear Instruments and Methods in Physics Research B, 527, p.17 - 27, 2022/09

 Times Cited Count:0 Percentile:56.43(Instruments & Instrumentation)

To improve accuracy of nuclear design of accelerator driven nuclear transmutation systems and so on, nuclide production cross sections on Ni and Zr were measured for GeV energy protons. The measured results were compared with PHITS calculations, JENDL/HE-2007 and so on.

Journal Articles

Nuclide production cross section of $$^{nat}$$Lu target irradiated with 0.4-, 1.3-, 2.2-, and 3.0-GeV protons

Takeshita, Hayato; Meigo, Shinichiro; Matsuda, Hiroki; Iwamoto, Hiroki; Nakano, Keita; Watanabe, Yukinobu*; Maekawa, Fujio

JAEA-Conf 2021-001, p.207 - 212, 2022/03

Prediction of nuclide production of spallation products by high-energy proton injection plays a fundamental and important role in shielding design of high-intensity proton accelerator facilities such as accelerator driven nuclear transmutation system (ADS). Since the prediction accuracy of the nuclear reaction models used in the production quantity prediction simulation is insufficient, it is necessary to improve the nuclear reaction models. We have measured nuclide production cross sections for various target materials with the aim of acquiring experimental data and improving nuclear reaction models. In this study, 1.3-, 2.2- and 3.0-GeV proton beams were irradiated to $$^{nat}$$Lu target, and nuclide production cross-section data were acquired by the activation method. The measured data were compared with several nuclear reaction models used in Monte Carlo particle transport calculation codes to grasp the current prediction accuracy and to study how the nuclear reaction model could be improved.

Journal Articles

Measurement of nuclide production cross sections for proton-induced reactions on Mn and Co at 1.3, 2.2, and 3.0 GeV

Takeshita, Hayato*; Meigo, Shinichiro; Matsuda, Hiroki*; Iwamoto, Hiroki; Nakano, Keita; Watanabe, Yukinobu*; Maekawa, Fujio

Nuclear Instruments and Methods in Physics Research B, 511, p.30 - 41, 2022/01

 Times Cited Count:1 Percentile:66.98(Instruments & Instrumentation)

Nuclide production cross sections for proton-induced reactions on Mn and Co at incident energies of 1.3, 2.2, and 3.0 GeV were measured by the activation method at the J-PARC. In total, 143 production cross sections of reaction products were obtained. Among them, the cross sections of $$^{55}$$Mn(p,X)$$^{38}$$S and $$^{55}$$Mn(p,X)$$^{41}$$Ar were measured for the first time. The stable proton beam and well established beam monitoring system contributed to the reduction of the systematic uncertainties to typically less than 5%, which was better than those of the previous data. To examine the prediction capabilities of spallation reaction models and evaluated data library, the measured data were compared with the spallation reaction models in PHITS (INCL4.6/GEM, etc.), INCL++/ABLA07, and the JENDL/HE-2007 library. The comparison of the mean square deviation factors indicated that both INCL4.6/GEM and JENDL/HE-2007 showed better agreement with the measured data than the others.

Journal Articles

PSTEP: Project for solar-terrestrial environment prediction

Kusano, Kanya*; Ichimoto, Kiyoshi*; Ishii, Mamoru*; Miyoshi, Yoshizumi*; Yoden, Shigeo*; Akiyoshi, Hideharu*; Asai, Ayumi*; Ebihara, Yusuke*; Fujiwara, Hitoshi*; Goto, Tadanori*; et al.

Earth, Planets and Space (Internet), 73(1), p.159_1 - 159_29, 2021/12

 Times Cited Count:6 Percentile:52.8(Geosciences, Multidisciplinary)

The PSTEP is a nationwide research collaboration in Japan and was conducted from April 2015 to March 2020, supported by a Grant-in-Aid for Scientific Research on Innovative Areas from the Ministry of Education, Culture, Sports, Science and Technology of Japan. It has made a significant progress in space weather research and operational forecasts, publishing over 500 refereed journal papers and organizing four international symposiums, various workshops and seminars, and summer school for graduate students at Rikubetsu in 2017. This paper is a summary report of the PSTEP and describes the major research achievements it produced.

Journal Articles

Dynamical response of transition-edge sensor microcalorimeters to a pulsed charged-particle beam

Okumura, Takuma*; Azuma, Toshiyuki*; Bennet, D. A.*; Caradonna, P.*; Chiu, I.-H.*; Doriese, W. B.*; Durkin, M. S.*; Fowler, J. W.*; Gard, J. D.*; Hashimoto, Tadashi; et al.

IEEE Transactions on Applied Superconductivity, 31(5), p.2101704_1 - 2101704_4, 2021/08

 Times Cited Count:1 Percentile:11.71(Engineering, Electrical & Electronic)

A superconducting transition-edge sensor (TES) microcalorimeter is an ideal X-ray detector for experiments at accelerator facilities because of good energy resolution and high efficiency. To study the performance of the TES detector with a high-intensity pulsed charged-particle beam, we measured X-ray spectra with a pulsed muon beam at the Japan Proton Accelerator Research Complex (J-PARC) in Japan. We found substantial temporal shifts of the X-ray energy correlated with the arrival time of the pulsed muon beam, which was reasonably explained by pulse pileup due to the incidence of energetic particles from the initial pulsed beam.

Journal Articles

Deexcitation dynamics of muonic atoms revealed by high-precision spectroscopy of electronic $$K$$ X rays

Okumura, Takuma*; Azuma, Toshiyuki*; Bennet, D. A.*; Caradonna, P.*; Chiu, I. H.*; Doriese, W. B.*; Durkin, M. S.*; Fowler, J. W.*; Gard, J. D.*; Hashimoto, Tadashi; et al.

Physical Review Letters, 127(5), p.053001_1 - 053001_7, 2021/07

 Times Cited Count:9 Percentile:78.48(Physics, Multidisciplinary)

We observed electronic $$K$$X rays emitted from muonic iron atoms using a superconducting transition-edge-type sensor microcalorimeter. The energy resolution of 5.2 eV in FWHM allowed us to observe the asymmetric broad profile of the electronic characteristic $$K$$$$alpha$$ and $$K$$$$beta$$ X rays together with the hypersatellite $$K$$$$alpha$$ X rays around 6 keV. This signature reflects the time-dependent screening of the nuclear charge by the negative muon and the $$L$$-shell electrons, accompanied by electron side-feeding. Assisted by a simulation, this data clearly reveals the electronic $$K$$- and $$L$$-shell hole production and their temporal evolution during the muon cascade process.

Journal Articles

Upgrade history and present status of the general control system for the Materials and Life Science Experimental Facility at J-PARC

Sakai, Kenji; Oi, Motoki; Haga, Katsuhiro; Kai, Tetsuya; Nakatani, Takeshi; Kobayashi, Yasuo*; Watanabe, Akihiko*

JPS Conference Proceedings (Internet), 33, p.011151_1 - 011151_6, 2021/03

For safely and efficiently operating a spallation neutron source and a muon target, a general control system (GCS) operates within Materials and Life Science Experimental Facility (MLF), GCS administers operation processes and interlocks of many instruments for various operation statuses. It consists of several subsystems such as an integral control system (ICS), interlock systems (ILS), shared servers, network system, and timing distribution system (TDS). Although GCS is an independent system that controls the target stations, it works closely with the control systems of other facilities in J-PARC. Since the first beam injection in 2008, GCS has operated stably without any serious troubles after modification based on commissioning for operation and control. Then, significant improvements in GCS such as upgrade of ICS by changing its framework software and function enhancement of ILS were proceeded until 2015, in considering sustainable long-term operation and maintenance. In recent years, many instruments in GCS have replaced due to end of production and support of them. In this way, many modifications have been proceeded in the entire GCS after start of beam operation. Under these situation, it is important to comprehend upgrade history and present status of GCS in order to decide its upgrade plan for the coming ten years. This report will mention upgrade history, present status and future agenda of GCS.

Journal Articles

Nuclide production cross sections of Ni and Zr irradiated with 0.4-, 1.3-, 2.2-, and 3.0-GeV protons

Takeshita, Hayato; Meigo, Shinichiro; Matsuda, Hiroki; Iwamoto, Hiroki; Maekawa, Fujio; Watanabe, Yukinobu*

JPS Conference Proceedings (Internet), 33, p.011045_1 - 011045_6, 2021/03

To improve accuracy of nuclear design of accelerator driven nuclear transmutation systems, nuclide production cross sections on Ni and Zr, which were candidate materials to be used in ADS, were measured for GeV energy protons. The measured results were compared with PHITS calculations and JENDL/HE-2007.

Journal Articles

A Geochemical approach for identifying marine incursions; Implications for tsunami geology on the Pacific coast of northeast Japan

Watanabe, Takahiro; Tsuchiya, Noriyoshi*; Yamasaki, Shinichi*; Sawai, Yuki*; Hosoda, Norihiro*; Nara, Fumiko*; Nakamura, Toshio*; Komai, Takeshi*

Applied Geochemistry, 118, p.104644_1 - 104644_11, 2020/07

 Times Cited Count:9 Percentile:65.99(Geochemistry & Geophysics)

Possible tsunami inundation areas can be predicted from the distribution of paleo tsunami deposits, which are mainly composed of marine-derived sands and muds on land. Such exotic sandy and muddy layers have been identified by multiple approaches. However, there still remain uncertainties and other useful proxies need to be investigated for the identification of tsunami deposits. Here we show the geochemical signatures of modern tsunami deposits from the Pacific coast of Northeast Japan (2011 Tohoku tsunami), as well as those paleo tsunami deposits, which were taken from the Tohoku District (Jogan, ca. 1080 calibrated ages before present [cal BP] and Yayoi, ca. 2000 cal BP). A geochemical ternary diagram (Seawater-Rock-(As+Metals)) enables the weathering trend of tsunami deposits over ca. 2000 years in the Sendai Plain in the Tohoku to be shown. In the paleo tsunami layers from the Tohoku, the Na/Ti atomic ratios markedly increased to 23.4, and the average values were 19.3$$pm$$3.0 (Jogan and Yayoi tsunami deposits), which were clearly higher than those of other layers (soil deposits, 10.3$$pm$$3.5 on average). These results show that the Na/Ti ratio is a useful indicator of marine incursions in our case. Our rapid and simple method using the Na/Ti ratio can be easily applied to the Tohoku, and it may contribute to the detection of unrecorded muddy tsunami deposits.

Journal Articles

Impact of the angle of incidence on negative muon-induced SEU cross sections of 65-nm Bulk and FDSOI SRAMs

Liao, W.*; Hashimoto, Masanori*; Manabe, Seiya*; Watanabe, Yukinobu*; Abe, Shinichiro; Tampo, Motonobu*; Takeshita, Soshi*; Miyake, Yasuhiro*

IEEE Transactions on Nuclear Science, 67(7), p.1566 - 1572, 2020/07

 Times Cited Count:0 Percentile:0.01(Engineering, Electrical & Electronic)

Muon-induced single event upset (SEU) is predicted to increase with technology scaling. The angle of incidence of terrestrial muons is not always perpendicular to the chip surface. Consequently, the impact of the angle of incidence of muons on SEUs should be evaluated. This study conducts negative muon irradiation tests on bulk SRAM and FDSOI SRAM at two angles of incidence: 0 degree (vertical) and 45 degree (tilted). The tilted incidence drifts the muon energy peak to a higher energy. Moreover, the SEU characteristics (i.e., such as the voltage dependences of the SEU cross sections and multiple cells upset patterns) between the vertical and tilted incidences are similar.

Journal Articles

Sorption properties of aluminum hexacyanoferrate for platinum group elements

Mishima, Ria; Inaba, Yusuke*; Tachioka, Sotaro*; Harigai, Miki*; Watanabe, Shinta*; Onoe, Jun*; Nakase, Masahiko*; Matsumura, Tatsuro; Takeshita, Kenji*

Chemistry Letters, 49(1), p.83 - 86, 2020/01

 Times Cited Count:4 Percentile:21.77(Chemistry, Multidisciplinary)

Separation of platinum group metals (PGMs) from high-level liquid waste generated from the reprocessing of spent nuclear fuels is important to produce good quality vitrified glass for final disposal. A new sorbent, Aluminum hexacyanoferrate (AlHCF), was synthesized and the general sorption behavior of PGMs from concentrated nitric acid was examined. Nitric acid caused substantial elution of AlHCF but the sorption of Pd stabilized the structure. Consequently, Rh was sorbed in the presence of Pd, whereas single Rh sorption caused complete dissolution of AlHCF. Relation between sorbed mount of Pd vs eluted Al and Fe revealed that the elution ratio of Al and Fe was not the same as molar ratio of synthesized AlHCF, indicating the re-sorption of Fe resulted in formation of new structure. The sorption mechanism of PGMs by this new sorbent, AlHCF, not only the simple ion exchange, but also oxidation reduction reaction as well as kinetics play important rule. Understanding the general sorption and dissolution behavior will help improve the sorption performance of PGMs by AlHCF.

Journal Articles

Stable structure of hydrogen atoms trapped in tungsten divacancy

Osawa, Kazuhito*; Toyama, Takeshi*; Hatano, Yuji*; Yamaguchi, Masatake; Watanabe, Hideo*

Journal of Nuclear Materials, 527, p.151825_1 - 151825_7, 2019/12

 Times Cited Count:7 Percentile:67.25(Materials Science, Multidisciplinary)

no abstracts in English

Journal Articles

Enhancement of element production by incomplete fusion reaction with weakly bound deuteron

Wang, H.*; Otsu, Hideaki*; Chiga, Nobuyuki*; Kawase, Shoichiro*; Takeuchi, Satoshi*; Sumikama, Toshiyuki*; Koyama, Shumpei*; Sakurai, Hiroyoshi*; Watanabe, Yukinobu*; Nakayama, Shinsuke; et al.

Communications Physics (Internet), 2(1), p.78_1 - 78_6, 2019/07

 Times Cited Count:7 Percentile:56.64(Physics, Multidisciplinary)

Searching for effective pathways for the production of proton- and neutron-rich isotopes through an optimal combination of reaction mechanism and energy is one of the main driving forces behind experimental and theoretical nuclear reaction studies as well as for practical applications in nuclear transmutation of radioactive waste. We report on a study on incomplete fusion induced by deuteron, which contains one proton and one neutron with a weak binding energy and is easily broken up. This reaction study was achieved by measuring directly the cross sections for both proton and deuteron for $$^{107}$$Pd at 50 MeV/u via inverse kinematics technique. The results provide direct experimental evidence for the onset of a cross-section enhancement at high energy, indicating the potential of incomplete fusion induced by loosely-bound nuclei for creating proton-rich isotopes and nuclear transmutation of radioactive waste.

Journal Articles

Mapping measurement for beam energy position monitor system for RIKEN superconducting acceleration cavity

Watanabe, Tamaki*; Toyama, Takeshi*; Hanamura, Kotoku*; Imao, Hiroshi*; Kamigaito, Osamu*; Kamoshida, Atsushi*; Kawachi, Toshihiko*; Koyama, Ryo*; Sakamoto, Naruhiko*; Fukunishi, Nobuhisa*; et al.

Proceedings of 16th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.1105 - 1108, 2019/07

Upgrades for the RIKEN heavy-ion linac (RILAC) involving a new superconducting linac (SRILAC) are currently underway at the RIKEN radioactive isotope beam factory (RIBF). It is crucially important to develop nondestructive beam measurement diagnostics. We have developed a beam energy position monitor (BEPM) system which can measure not only the beam position but also the beam energy simultaneously by measuring the time of flight of the beam. We fabricated 11 BEPMs and completed the position calibration to obtain the sensitivity and offset for each BEPMs. The position accuracy has been achieved to be less than $$pm$$ 0.1 mm by using the mapping measurement.

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