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Journal Articles

Validation study on SFR core bowing codes using Joyo ex-core experiment data; Single duct bowing benchmark

Ohgama, Kazuya; Doda, Norihiro; Uwaba, Tomoyuki; Futagami, Satoshi; Tanaka, Masaaki; Yamano, Hidemasa; Ota, Hirokazu*; Ogata, Takanari*; Wozniak, N.*; Shemon, E.*; et al.

Proceedings of International Conference on Nuclear Fuel Cycle (GLOBAL2024) (Internet), 4 Pages, 2024/10

To enhance the accuracy of the safety evaluations in sodium-cooled fast reactors, it is necessary to develop a method to realistically evaluate the reactivity caused by core deformation. In this regard, Japan and the United States jointly conducted a benchmark analysis of thermal bowing experiments of a single duct of Joyo-type fuel assembly. The aim was to confirm the validity of the core bowing analysis codes. Comparisons of analysis and test results revealed that the core bowing analysis codes used by both countries were able to reasonably predict the axial distribution of horizontal duct displacement of a single duct due to thermal bowing and the contact load on the duct pad.

Journal Articles

Validation study on SFR core bowing codes using Joyo ex-core experiment data; Multiple duct bowing benchmark

Wozniak, N.*; Shemon, E.*; Feng, B.*; Ohgama, Kazuya; Doda, Norihiro; Uwaba, Tomoyuki; Futagami, Satoshi; Tanaka, Masaaki; Yamano, Hidemasa; Ota, Hirokazu*; et al.

Proceedings of International Conference on Nuclear Fuel Cycle (GLOBAL2024) (Internet), 4 Pages, 2024/10

To enhance the accuracy of the safety evaluations in sodium-cooled fast reactors, it is necessary to develop a method to realistically evaluate the reactivity caused by core deformation. In this regard, Japan and the United States jointly conducted a benchmark analysis of thermal bowing experiments using multiple ducts of Joyo-type fuel assembly. The aim was to confirm the validity of the core bowing analysis codes. Comparisons of analysis and test results revealed that the core bowing analysis codes used by both countries were able to reasonably predict the thermal bowing of a row of assemblies.

Journal Articles

Extraction of Se(iv) and Se(vi) from aqueous HCl solution by using a diamide-containing tertiary amine

Narita, Hirokazu*; Maeda, Motoki*; Tokoro, Chiharu*; Suzuki, Tomoya*; Tanaka, Mikiya*; Shiwaku, Hideaki; Yaita, Tsuyoshi

RSC Advances (Internet), 13(25), p.17001 - 17007, 2023/06

 Times Cited Count:3 Percentile:34.10(Chemistry, Multidisciplinary)

no abstracts in English

Journal Articles

Environmental effects on layer-dependent dynamics of Dirac fermions in quasicrystalline bilayer graphene

Zhao, Y.*; Suzuki, T.*; Iimori, T.*; Kim, H.-W.*; Ahn, J. R.*; Horio, Masafumi*; Sato, Yusuke*; Fukaya, Yuki; Kanai, T.*; Okazaki, K.*; et al.

Physical Review B, 105(11), p.115304_1 - 115304_8, 2022/03

 Times Cited Count:1 Percentile:7.32(Materials Science, Multidisciplinary)

no abstracts in English

Journal Articles

Thermally altered subsurface material of asteroid (162173) Ryugu

Kitazato, Kohei*; Milliken, R. E.*; Iwata, Takahiro*; Abe, Masanao*; Otake, Makiko*; Matsuura, Shuji*; Takagi, Yasuhiko*; Nakamura, Tomoki*; Hiroi, Takahiro*; Matsuoka, Moe*; et al.

Nature Astronomy (Internet), 5(3), p.246 - 250, 2021/03

 Times Cited Count:58 Percentile:96.23(Astronomy & Astrophysics)

Here we report observations of Ryugu's subsurface material by the Near-Infrared Spectrometer (NIRS3) on the Hayabusa2 spacecraft. Reflectance spectra of excavated material exhibit a hydroxyl (OH) absorption feature that is slightly stronger and peak-shifted compared with that observed for the surface, indicating that space weathering and/or radiative heating have caused subtle spectral changes in the uppermost surface. However, the strength and shape of the OH feature still suggests that the subsurface material experienced heating above 300 $$^{circ}$$C, similar to the surface. In contrast, thermophysical modeling indicates that radiative heating does not increase the temperature above 200 $$^{circ}$$C at the estimated excavation depth of 1 m, even if the semimajor axis is reduced to 0.344 au. This supports the hypothesis that primary thermal alteration occurred due to radiogenic and/or impact heating on Ryugu's parent body.

Journal Articles

Precious metal separations

Narita, Hirokazu*; Kasuya, Ryo*; Suzuki, Tomoya*; Motokawa, Ryuhei; Tanaka, Mikiya*

Encyclopedia of Inorganic and Bioinorganic Chemistry (Internet), 28 Pages, 2020/12

Journal Articles

Unique anion-exchange properties of 3,3'-diaminobenzidine resulting in high selectivity for rhodium(III) over palladium(II) and platinum(IV) in a concentrated hydrochloric acid solution

Suzuki, Tomoya*; Ogata, Takeshi*; Tanaka, Mikiya*; Kobayashi, Toru; Shiwaku, Hideaki; Yaita, Tsuyoshi; Narita, Hirokazu*

Analytical Sciences, 35(12), p.1353 - 1360, 2019/12

 Times Cited Count:5 Percentile:17.86(Chemistry, Analytical)

no abstracts in English

Journal Articles

Proton chelating ligands drive improved chemical separations for rhodium

Narita, Hirokazu*; Nicolson, R. M.*; Motokawa, Ryuhei; Ito, Fumiyuki*; Morisaku, Kazuko*; Goto, Midori*; Tanaka, Mikiya*; Heller, W. T.*; Shiwaku, Hideaki; Yaita, Tsuyoshi; et al.

Inorganic Chemistry, 58(13), p.8720 - 8734, 2019/07

 Times Cited Count:20 Percentile:75.87(Chemistry, Inorganic & Nuclear)

Journal Articles

A New approach for measuring the muon anomalous magnetic moment and electric dipole moment

Abe, Mitsushi*; Bae, S.*; Beer, G.*; Bunce, G.*; Choi, H.*; Choi, S.*; Chung, M.*; da Silva, W.*; Eidelman, S.*; Finger, M.*; et al.

Progress of Theoretical and Experimental Physics (Internet), 2019(5), p.053C02_1 - 053C02_22, 2019/05

 Times Cited Count:156 Percentile:99.31(Physics, Multidisciplinary)

This paper introduces a new approach to measure the muon magnetic moment anomaly $$a_{mu}=(g-2)/2$$ and the muon electric dipole moment (EDM) $$d_{mu}$$ at the J-PARC muon facility. The goal of our experiment is to measure $$a_{mu}$$ and $$d_{mu}$$ using an independent method with a factor of 10 lower muon momentum, and a factor of 20 smaller diameter storage-ring solenoid compared with previous and ongoing muon g-2 experiments with unprecedented quality of the storage magnetic field. Additional significant differences from the present experimental method include a factor of 1000 smaller transverse emittance of the muon beam (reaccelerated thermal muon beam), its efficient vertical injection into the solenoid, and tracking each decay positron from muon decay to obtain its momentum vector. The precision goal for $$a_{mu}$$ is a statistical uncertainty of 450 parts per billion (ppb), similar to the present experimental uncertainty, and a systematic uncertainty less than 70 ppb. The goal for EDM is a sensitivity of $$1.5times10^{-21}$$ e$$cdot$$cm.

Journal Articles

Speciation of ruthenium(III) chloro complexes in hydrochloric acid solutions and their extraction characteristics with an amide-containing amine compound

Suzuki, Tomoya*; Ogata, Takeshi*; Tanaka, Mikiya*; Kobayashi, Toru; Shiwaku, Hideaki; Yaita, Tsuyoshi; Narita, Hirokazu*

Metals, 8(7), p.558_1 - 558_10, 2018/07

AA2018-0670.pdf:2.11MB

 Times Cited Count:17 Percentile:59.49(Materials Science, Multidisciplinary)

The refining of platinum group metals is based mainly on solvent extraction methods, whereas Ru is selectively recovered by distillation as RuO$$_4$$. Replacement of distillation byextraction is expected to simplify the purification process. To develop an effective extraction system for Ru, we analyzed the Ru species in HCl with UV-Vis and EXAFS spectroscopies, and we examined the properties of Ru extracted with N-2-ethylhexyl-bis(N-di-2-ethylhexyl-ethylamide) amine (EHBAA). EXAFS and UV-Vis spectra of Ru in HCl solutions revealed that the predominant Ru species in 0.5-10 M HCl solutions changed from [RuCl$$_4$$(H$$_2$$O)$$_2$$]$$^-$$ to [RuCl$$_6$$]$$^3$$$$^-$$ with the HCl concentration. The extraction percentages of Ru in the EHBAA system increased with increasing HCl concentration, reached 80% at [HCl] = 5 M, and decreased athigher HCl concentrations. EXAFS analysis of the extracted complex indicated that the Ru$$^3$$$$^+$$ had 5 Cl$$^-$$ and 1 H$$_2$$O in its inner coordination sphere. The similarity of the dependence on HCl concentrations of the extraction in the EHBAA system and the distribution profile of [RuCl$$_5$$(H$$_2$$O)]$$^2$$$$^-$$ on [RuCl$$_n$$(H$$_2$$O)$$_6$$$$_-$$$$_n$$]$$^3$$$$^-$$$$^n$$ suggested that the EHBAA extracted the pentachlorido species.

Journal Articles

Comparison of the extractabilities of tetrachloro- and tetrabromopalladate(II) ions with a thiodiglycolamide compound

Narita, Hirokazu*; Maeda, Motoki*; Tokoro, Chiharu*; Suzuki, Tomoya*; Tanaka, Mikiya*; Motokawa, Ryuhei; Shiwaku, Hideaki; Yaita, Tsuyoshi

Analytical Sciences, 33(11), p.1305 - 1309, 2017/11

 Times Cited Count:11 Percentile:36.78(Chemistry, Analytical)

Journal Articles

Selective extraction of Pt(IV) over Fe(III) from HCl with an amide-containing tertiary amine compound

Maeda, Motoki*; Narita, Hirokazu*; Tokoro, Chiharu*; Tanaka, Mikiya*; Motokawa, Ryuhei; Shiwaku, Hideaki; Yaita, Tsuyoshi

Separation and Purification Technology, 177, p.176 - 181, 2017/04

 Times Cited Count:22 Percentile:55.45(Engineering, Chemical)

Journal Articles

Dipole tracer migration and diffusion tests in fractured sedimentary rock at Horonobe URL

Tanaka, Shingo*; Yokota, Hideharu; Ono, Hirokazu; Nakayama, Masashi; Fujita, Tomoo; Takiya, Hiroaki*; Watanabe, Naoko*; Kozaki, Tamotsu*

Proceedings of 23rd International Conference on Nuclear Engineering (ICONE-23) (DVD-ROM), 6 Pages, 2015/05

Journal Articles

High-resolution Compton cameras based on Si/CdTe double-sided strip detectors

Odaka, Hirokazu*; Ichinohe, Yuto*; Takeda, Shinichiro*; Fukuyama, Taro*; Hagino, Koichi*; Saito, Shinya*; Sato, Tamotsu*; Sato, Goro*; Watanabe, Shin*; Kokubun, Motohide*; et al.

Nuclear Instruments and Methods in Physics Research A, 695, p.179 - 183, 2012/12

 Times Cited Count:24 Percentile:82.23(Instruments & Instrumentation)

We have developed a new Si/CdTe semiconductor double-sided strip detector (DSD) Compton camera. The camera consists of a 500-$$mu$$m-thick Si-DSD and four layers of 750-$$mu$$m-thick CdTe-DSDs all of which have common electrode configuration segmented into 128 strips on each side with pitches of 250$$mu$$m. In order to realize high angular resolution and to reduce size of the detector system, a stack of DSDs with short stack pitches of 4 mm is utilized to make the camera. Taking advantage of the excellent energy and position resolutions of the semiconductor devices, the camera achieves high angular resolutions of 4.5 degrees at 356 keV and 3.5 degrees at 662 keV. To obtain such high resolutions together with an acceptable detection efficiency, we demonstrate data reduction methods including energy calibration using Compton scattering continuum and depth sensing in the CdTe-DSD. We also discuss imaging capability of the camera and show simultaneous multi-energy imaging.

JAEA Reports

Development of grout materials for a geological disposal system for high-level radioactive waste, 2

Kawaguchi, Masanao; Nakanishi, Tatsuro; Kishi, Hirokazu; Nobuto, Jun*; Yamada, Tsutomu*; Fujita, Tomoo; Hatanaka, Koichiro

JAEA-Data/Code 2012-007, 250 Pages, 2012/11

JAEA-Data-Code-2012-007.pdf:20.55MB

Cementitious materials are commonly used for rock support, lining, and grouting, their pH plume are considered to have an adverse effect on long-term safety of a geological disposal system. In addition, during the emplacement of waste package with buffer material, it is required to limit amount of groundwater inflow to a certain level by grouting. Therefore, it is necessary to develop new grout materials with penetrability for smaller fractures. We have developed new grout materials, which have better penetrability and are environmentally more friendly than exinting cementitious grout materials since FY 2007. This sequel report shows the most appropriate composition and the penetration characteristic of new grout materials to be suitable for the ${it in-situ}$ experiment based on the result of indoor test carried out after FY 2008.

Journal Articles

Applications and imaging techniques of a Si/CdTe Compton $$gamma$$-ray camera

Takeda, Shinichiro*; Ichinohe, Yuto*; Hagino, Koichi*; Odaka, Hirokazu*; Yuasa, Takayuki*; Ishikawa, Shinnosuke*; Fukuyama, Taro*; Saito, Shinya*; Sato, Tamotsu*; Sato, Goro*; et al.

Physics Procedia, 37, p.859 - 866, 2012/10

 Times Cited Count:25 Percentile:98.53(Physics, Applied)

By using new Compton camera consisting of silicon double-sided strip detector (Si-DSD) and CdTe-DSD developed for the ASTRO-H mission, an experiment was conducted to study its feasibility for advanced hotspot monitoring. In addition to hotspot imaging already provided by commercial imaging systems, the identification of the variety of radioisotopes is realized thanks to the good energy resolution given by the semiconductor detectors. Three radioisotopes of $$^{133}$$Ba (356 keV), $$^{22}$$Na (511 keV) and $$^{137}$$Cs (662 keV) were individually imaged by applying event selection in the energy window and the $$gamma$$-ray images was correctly overlapped by an optical picture. The detection efficiency of 1.68$$times$$10$$^{-4}$$ (effective area: 1.7$$times$$10$$^{-4}$$ cm$$^2$$) and angular resolution of 3.8$$^{circ}$$ were obtained by stacking five detector modules for 662 keV $$gamma$$-ray. The higher detection efficiency required in a specific use can be achieved by stacking more detector modules.

Journal Articles

Characteristic evaluation of colloidal silica grout material developed for a high level radioactive waste geological repository

Kishi, Hirokazu; Kawaguchi, Masanao; Naito, Morimasa; Hatanaka, Koichiro; Nobuto, Jun*; Sugiyama, Hirokazu*

Genshiryoku Bakkuendo Kenkyu (CD-ROM), 19(1), p.3 - 8, 2012/06

To reduce amount of groundwater inflow into a geological repository, the grouting is expected to play a very important role because the geological environment in Japan is often characterized by many fractures and abundant groundwater. Basically, cementitious materials are used for grouting, however the resulting highly alkaline plume released from the materials could influence the long-term performance of barrier system as a consequence of alteration of both the buffer material and the host rock. To minimize such effects, JAEA has carried out research and development on three types of grout material with low-pH performance that decreases influence in the alteration. This paper focuses on the Colloidal silica grout, and presents its unique characteristics obtained from laboratory tests on pH, viscosity, leaching and so on. The results indicate that the grout has good performances in pH and viscosity. It is concluded that the grout can be greatly used for the repository.

Journal Articles

The JAEA grouting test at the Grimsel test site; Numerical simulation of the grout injection process of silica sol in fractured rock mass

Koyama, Tomofumi*; Onishi, Yuzo*; Bruines, P.*; Tanaka, Tatsuya*; Hasui, Akinori*; Katayama, Tatsuo*; Kishi, Hirokazu; Kuzuha, Yuji

Proceedings of 2012 ISRM International Symposium; Rock Engineering and Technology for Sustainable Underground Construction (EUROCK 2012) (USB Flash Drive), 10 Pages, 2012/05

Grouting, which involves injection of grout material, is commonly used to decrease the hydraulic conductivity of the fractured rock masses and control the groundwater inflow. However, the mechanism of grout injection process has not been clarified sufficiently yet due to complicated chemical and physical processes of grout. In this study, to simulate the grout injection process, the three-dimensional numerical model based on equivalent continuum approach was developed.

Journal Articles

The JAEA grouting test at the Grimsel test site; Site characterization of a fractured rockmass and preparation of DFN model and its equivalent continuous porous media model

Bruines, P.*; Tanaka, Tatsuya*; Koyama, Tomofumi*; Kishi, Hirokazu; Nakanishi, Tatsuro; Onishi, Yuzo*

Proceedings of 2012 ISRM International Symposium; Rock Engineering and Technology for Sustainable Underground Construction (EUROCK 2012) (USB Flash Drive), 15 Pages, 2012/05

To better understand the grouting process and the effect of grouting on the performance of a nuclear waste repository, the Japanese Atomic Energy Agency (JAEA) has initiated a grouting test carried out in the fractured granite of the Grimsel Test Site (GTS) located in the Swiss Alps. This paper describes the characterization of the rock mass, how the data obtained has been used to make a discrete fracture network (DFN) model and how an up-scaled equivalent continuous porous media (ECPM) model for the purpose of numerical simulation of the grout injection process is generated. The generated DFN model and the up-scaled ECPM model was able to reproduce the measured fracture characteristics (e.g. orientation, density) as well as the hydraulic behavior observed in the field (e.g. transmissivity distribution, anisotropy, heterogeneity) and has proven to be suitable for modeling grouting behavior.

Journal Articles

Tolerance of anhydrobiotic eggs of the tardigrade ${it Ramazzottius varieornatus}$ to extreme environments

Horikawa, Daiki*; Yamaguchi, Ayami*; Sakashita, Tetsuya; Tanaka, Daisuke*; Hamada, Nobuyuki*; Yukuhiro, Fumiko*; Kuwahara, Hirokazu*; Kunieda, Takekazu*; Watanabe, Masahiko*; Nakahara, Yuichi*; et al.

Astrobiology, 12(4), p.283 - 289, 2012/04

 Times Cited Count:25 Percentile:69.10(Astronomy & Astrophysics)

We examined the hatchability of hydrated and anhydrobiotic eggs of the tardigrade ${it Ramazzottius varieornatus}$ to hatch after ionizing irradiation (helium ions), extremely low and high temperatures, and high vacuum. Anhydrobiotic eggs (50% lethal dose; 1690 Gy) were substantially more radioresistant than hydrated ones (50% lethal dose; 509 Gy). Anhydrobiotic eggs also have a broader temperature resistance compared with hydrated ones. Over 70% of the anhydrobiotic eggs treated at high and low temperatures, but all of the hydrated eggs failed to hatch. After exposure to high vacuum conditions, the hatchability of the anhydrobiotic eggs was comparable to that of untreated control eggs.

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