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Yoshimura, Kazuo; Doda, Norihiro; Igawa, Kenichi*; Tanaka, Masaaki; Yamano, Hidemasa
Journal of Nuclear Engineering and Radiation Science, 9(2), p.021601_1 - 021601_9, 2023/04
Feedback reactivity automatically caused by radial expansion of the core is known as one of the inherent safety features in a sodium-cooled fast reactor (SFR). In order to validate the evaluation models of the reactivity feedback equipped in the in-house plant dynamics analysis code named Super-COPD, the benchmark analyses for the unprotected loss of heat sink (ULOHS) tests of BOP-302R and BOP-301 in an experimental SFR, EBR-II were conducted and the applicability of the evaluation method for the reactivity feedback was indicated during the ULOHS even, by comparing the numerical results and the experimental data.
Doda, Norihiro; Uwaba, Tomoyuki; Ohgama, Kazuya; Yoshimura, Kazuo; Nemoto, Toshiyuki*; Tanaka, Masaaki; Yamano, Hidemasa
Nihon Kikai Gakkai Kanto Shibu Dai-29-Ki Sokai, Koenkai Koen Rombunshu (Internet), 5 Pages, 2023/03
An evaluation method for reactivity feedback due to core deformation during reactor power increase in sodium-cooled fast reactors is being developed for realistic core design evaluation. In this evaluation method, fuel assembly bowing was modeled with a beam element of the finite element method, and the assembly's pad contact between adjacent assemblies was modeled with a dedicated element which could consider the wrapper tube cross-sectional distortion and the pad stiffness depending on pad contact conditions. This fuel assembly bowing analysis model was verified for thermal bowing of a single assembly and assembly pad contact between adjacent assemblies in a core as past benchmark problems. The calculation results by this model showed good agreement with those of reference solutions of theoretical solutions or results by participating institutions in the benchmark. This study confirmed that the analysis model was able to calculate thermal assembly bowing appropriately.
Doda, Norihiro; Yoshimura, Kazuo; Hamase, Erina; Yokoyama, Kenji; Uwaba, Tomoyuki; Tanaka, Masaaki
Proceedings of Technical Meeting on State-of-the-art Thermal Hydraulics of Fast Reactors (Internet), 3 Pages, 2022/09
ARKADIA-Design is being developed to support the optimization of sodium-cooled fast reactors in the conceptual design stage. Design optimization requires various types of numerical analysis: 1-D plant dynamics analysis for efficient evaluation of various design options and multi-dimensional analysis for a detailed evaluation of local phenomena, including multi-physics. For those analyses, ARKADIA-Design performs whole plant analyses based on the multi-level simulation (MLS) technique in which the analysis codes are coupled to simulate the phenomena in an intended degree of resolution. This paper describes an outline of the coupling analysis methods in the MLS of the ARKADIA-Design and the numerical simulations of the experimental fast breeder reactor EBR-II tests by the coupled analysis.
Yoshimura, Kazuo; Doda, Norihiro; Fujisaki, Tatsuya*; Igawa, Kenichi*; Tanaka, Masaaki; Yamano, Hidemasa
Proceedings of 29th International Conference on Nuclear Engineering (ICONE 29) (Internet), 10 Pages, 2022/08
To confirm the applicability of the reactivity model, the authors have been conducting the benchmark exercises of the unprotected loss of heat sink event tests in a pool-type experimental fast reactor EBR-II. In the blind phase in the benchmark analyses using the plant dynamics analysis (1D) code in which the cold pool was modeled by means of the perfect mixing volume, it was found the increase of the core inlet temperature was evaluated lower than that of the measured data and the feedback reactivity was underestimated, because the thermal stratification in the cold pool was ignored. Then, the detailed model of the cold pool for the computational fluid dynamics (CFD) code was introduced and the 1D-CFD codes coupling method was applied to the benchmark analyses. It was confirmed that both the thermal stratification in the cold pool and the increase of the core inlet temperature were successfully reproduced.
Yoshimura, Kazuo; Doda, Norihiro; Tanaka, Masaaki; Fujisaki, Tatsuya*; Murakami, Satoshi*; Vilim, R. B.*
Proceedings of 19th International Topical Meeting on Nuclear Reactor Thermal Hydraulics (NURETH-19) (Internet), 16 Pages, 2022/03
In Japan Atomic Energy Agency, the multilevel simulation system which enables consistent evaluation from the whole plant behavior to the local phenomena is being developed to optimize plant design and enhance the safety of sodium-cooled fast reactors. To validate the coupling method in the MLS system, the 1D-CFD coupling method using Super-COPD for 1D plant dynamics analysis and Fluent for multi-dimensional CFD analysis was applied to the analyses of loss of flow tests in EBR-II. It was confirmed that it could predict multi-dimensional thermal-hydraulic phenomena such as thermal stratification in the upper plenum, Z-shaped pipe, and cold pool, holding the whole plant behavior simultaneously. Moreover, the applicability of the 1D-CFD coupling method to the evaluation of the phenomena in natural circulation conditions was confirmed by comparing the results of the 1D-CFD couple analyses and the measured data.
Nishimura, Shoichiro*; Torii, Hiroyuki*; Fukao, Yoshinori*; Ito, Takashi; Iwasaki, Masahiko*; Kanda, Sotaro*; Kawagoe, Kiyotomo*; Kawall, D.*; Kawamura, Naritoshi*; Kurosawa, Noriyuki*; et al.
Physical Review A, 104(2), p.L020801_1 - L020801_6, 2021/08
Times Cited Count:8 Percentile:79.69(Optics)Yoshimura, Kazuo; Doda, Norihiro; Tanaka, Masaaki; Yamano, Hidemasa; Igawa, Kenichi*
Proceedings of 28th International Conference on Nuclear Engineering (ICONE 28) (Internet), 8 Pages, 2021/08
The numerical results of the benchmark analyses for the unprotected loss of heat sink (ULOHS) tests in the pool-type experimental SFR in the United States, EBR-II (BOP-302R and BOP-301) are discussed in order to validate the evaluation method of the reactivity feedback equipped in the in-house plant dynamics analysis code named Super-COPD. By comparing the numerical results and the experimental data, the profiles of the increase of the core inlet temperature and the decrease of the reactor power calculated by Super-COPD were comparable with those of the experimental data and the applicability of the evaluation method for the reactivity feedback was indicated during the ULOHS event.
Kitazato, Kohei*; Milliken, R. E.*; Iwata, Takahiro*; Abe, Masanao*; Otake, Makiko*; Matsuura, Shuji*; Takagi, Yasuhiko*; Nakamura, Tomoki*; Hiroi, Takahiro*; Matsuoka, Moe*; et al.
Nature Astronomy (Internet), 5(3), p.246 - 250, 2021/03
Times Cited Count:27 Percentile:97(Astronomy & Astrophysics)Here we report observations of Ryugu's subsurface material by the Near-Infrared Spectrometer (NIRS3) on the Hayabusa2 spacecraft. Reflectance spectra of excavated material exhibit a hydroxyl (OH) absorption feature that is slightly stronger and peak-shifted compared with that observed for the surface, indicating that space weathering and/or radiative heating have caused subtle spectral changes in the uppermost surface. However, the strength and shape of the OH feature still suggests that the subsurface material experienced heating above 300 C, similar to the surface. In contrast, thermophysical modeling indicates that radiative heating does not increase the temperature above 200
C at the estimated excavation depth of 1 m, even if the semimajor axis is reduced to 0.344 au. This supports the hypothesis that primary thermal alteration occurred due to radiogenic and/or impact heating on Ryugu's parent body.
Kitazato, Kohei*; Milliken, R. E.*; Iwata, Takahiro*; Abe, Masanao*; Otake, Makiko*; Matsuura, Shuji*; Arai, Takehiko*; Nakauchi, Yusuke*; Nakamura, Tomoki*; Matsuoka, Moe*; et al.
Science, 364(6437), p.272 - 275, 2019/04
Times Cited Count:214 Percentile:99.75(Multidisciplinary Sciences)The near-Earth asteroid 162173 Ryugu, the target of Hayabusa2 sample return mission, is believed to be a primitive carbonaceous object. The Near Infrared Spectrometer (NIRS3) on Hayabusa2 acquired reflectance spectra of Ryugu's surface to provide direct measurements of the surface composition and geological context for the returned samples. A weak, narrow absorption feature centered at 2.72 micron was detected across the entire observed surface, indicating that hydroxyl (OH)-bearing minerals are ubiquitous there. The intensity of the OH feature and low albedo are similar to thermally- and/or shock-metamorphosed carbonaceous chondrite meteorites. There are few variations in the OH-band position, consistent with Ryugu being a compositionally homogeneous rubble-pile object generated from impact fragments of an undifferentiated aqueously altered parent body.
Strasser, P.*; Abe, Mitsushi*; Aoki, Masaharu*; Choi, S.*; Fukao, Yoshinori*; Higashi, Yoshitaka*; Higuchi, Takashi*; Iinuma, Hiromi*; Ikedo, Yutaka*; Ishida, Katsuhiko*; et al.
EPJ Web of Conferences, 198, p.00003_1 - 00003_8, 2019/01
Times Cited Count:13 Percentile:99.33Kataoka, Ryuho*; Nishiyama, Takanori*; Tanaka, Yoshimasa*; Kadokura, Akira*; Uchida, Herbert Akihito*; Ebihara, Yusuke*; Ejiri, Mitsumu*; Tomikawa, Yoshihiro*; Tsutsumi, Masaki*; Sato, Kaoru*; et al.
Earth, Planets and Space (Internet), 71, p.9_1 - 9_10, 2019/01
Times Cited Count:7 Percentile:42.74(Geosciences, Multidisciplinary)Transient ionization of the mesosphere was detected at around 65 km altitude during the isolated auroral expansion occurred at 2221-2226 UT on June 30, 2017. A general-purpose Monte Carlo particle transport code PHITS suggested that significant ionization is possible in the middle atmosphere due to auroral X-rays from the auroral electrons of 10 keV.
Tashiro, Koji*; Kusaka, Katsuhiro*; Hosoya, Takaaki*; Ohara, Takashi; Hanesaka, Makoto*; Yoshizawa, Yoshinori*; Yamamoto, Hiroko*; Niimura, Nobuo*; Tanaka, Ichiro*; Kurihara, Kazuo*; et al.
Macromolecules, 51(11), p.3911 - 3922, 2018/06
Times Cited Count:4 Percentile:16.38(Polymer Science)Ueno, Yasuhiro*; Aoki, Masaharu*; Fukao, Yoshinori*; Higashi, Yoshitaka*; Higuchi, Takashi*; Iinuma, Hiromi*; Ikedo, Yutaka*; Ishida, Katsuhiko*; Ito, Takashi; Iwasaki, Masahiko*; et al.
Hyperfine Interactions, 238(1), p.14_1 - 14_6, 2017/11
Times Cited Count:3 Percentile:87.03Strasser, P.*; Aoki, Masaharu*; Fukao, Yoshinori*; Higashi, Yoshitaka*; Higuchi, Takashi*; Iinuma, Hiromi*; Ikedo, Yutaka*; Ishida, Katsuhiko*; Ito, Takashi; Iwasaki, Masahiko*; et al.
Hyperfine Interactions, 237(1), p.124_1 - 124_9, 2016/12
Times Cited Count:7 Percentile:92.26Sato, Isamu; Tanaka, Kosuke; Koyama, Shinichi; Matsushima, Kenichi*; Matsunaga, Junji*; Hirai, Mutsumi*; Endo, Hiroshi*; Haga, Kazuo*
Energy Procedia, 82, p.86 - 91, 2015/07
Times Cited Count:2 Percentile:18.84(Nuclear Science & Technology)Experiments simulating overheating conditions of fast reactor severe accidents have been previously carried out with irradiated fuels. For the present study, the chemical forms of the fission products (FPs) included in the irradiated fuels were evaluated by thermochemical equilibrium calculations. At temperatures of 2773 K and 2973 K, the most stable forms of Cs, I, Te, Sb, Pd and Ag are gaseous compounds. Cs and Sb detected in the thermal gradient tube (TGT) in the experiments can take gaseous chemical forms of elemental Cs, CsI, CsMoO
, CsO and elemental Sb, SbO, SbTe, respectively. By comparing experimental results and the estimations, it is seen CsI thermochemically behaves in a manner that traps it in the TGT, while elemental Cs trends to move as fine particles. The moving behavior of the gaseous FPs will obey not only thermochemical principles, but also those of particle dynamics.
Tashiro, Koji*; Hanesaka, Makoto*; Yamamoto, Hiroko*; Wasanasuk, K.*; Jayaratri, P.*; Yoshizawa, Yoshinori*; Tanaka, Ichiro*; Niimura, Nobuo*; Kusaka, Katsuhiro*; Hosoya, Takaaki*; et al.
Kobunshi Rombunshu, 71(11), p.508 - 526, 2014/11
Times Cited Count:6 Percentile:23.96(Polymer Science)The crystal structure analysis of various polymer substances has been reviewed on the basis of wide-angle high-energy X-ray and neutron diffraction data. The progress in structural analytical techniques of polymer crystals have been reviewed at first. The structural models proposed so far were reinvestigated and new models have been proposed for various kinds of polymer crystals including polyethylene, poly(vinyl alcohol), poly(lactic acid) and its stereocomplex etc. The hydrogen atomic positions were also clarified by the quantitative analysis of wide-angle neutron diffraction data, from which the physical properties of polymer crystals have been evaluated theoretically. The bonded electron density distribution has been estimated for a polydiacetylene single crystal on the basis of the so-called X-N method or by the combination of structural information derived from X-ray and neutron diffraction data analysis. Some comments have been added about future developments in the field of structure-property relationship determination.
Kusaka, Katsuhiro*; Hosoya, Takaaki*; Yamada, Taro*; Tomoyori, Katsuaki; Ohara, Takashi; Katagiri, Masaki*; Kurihara, Kazuo; Tanaka, Ichiro*; Niimura, Nobuo*
Journal of Synchrotron Radiation, 20(6), p.994 - 998, 2013/11
Times Cited Count:34 Percentile:85.22(Instruments & Instrumentation)The IBARAKI biological crystal diffractometer, iBIX, is a high-performance time-of-flight neutron single-crystal diffractometer for elucidating mainly the hydrogen, protonation and hydration structures of biological macromolecules in various life processes. Since the end of 2008, iBIX has been available to user's experiments supported by Ibaraki University. Since August 2012, an upgrade of the 14-existing detectors has begun and 16 new detectors have been installed for iBIX. The total measurement efficiency of the present diffractometer has been impoved by one order of magnitude from the previous one with the increasing of accelerator power. In December 2012, commissioning of the new detectors was successful, and collection of the diffraction dataset of ribonucrease A as a standard protein was attempted in order to estimate the performance of the upgraded iBIX in comparison with previous results. The resolution of diffraction data, equivalence among intensities of symmetry-related reflections and reliability of the refined structure have been improved dramatically. iBIX is expected to be one of the highest-performance neutron single-crystal diffractometers for biological macromolecules in the world.
Yokoyama, Takeshi*; Mizuguchi, Mineyuki*; Nabeshima, Yuko*; Kusaka, Katsuhiro*; Yamada, Taro*; Hosoya, Takaaki*; Ohara, Takashi; Kurihara, Kazuo; Tanaka, Ichiro*; Niimura, Nobuo*
Journal of Synchrotron Radiation, 20(6), p.834 - 837, 2013/11
Times Cited Count:5 Percentile:30.27(Instruments & Instrumentation)Transthyretin (TTR) is a tetrameric protein. TTR misfolding and aggregation are associated with human amyloid diseases. Dissociation of the TTR tetramer is believed to be the rate-limiting step in the amyloid fibril formation cascade. Low pH is known to promote dissociation into monomer and the formation of amyloid fibrils. In order to reveal the molecular mechanisms underlying pH sensitivity and structural stabilities of TTR, neutron diffraction studies were conducted using the IBARAKI Biological Crystal Diffractometer with the time-of-flight method. Crystals for the neutron diffraction experiments were grown up to 2.5 mm for four months. The neutron crystal structure solved at 2.0
revealed the protonation states of His88 and the detailed hydrogen-bond network depending on the protonation states of His88. This hydrogen-bond network is involved in monomer-monomer and dimer-dimer interactions, suggesting that the double protonation of His88 by acidification breaks the hydrogen-bond network and causes the destabilization of the TTR tetramer. Structural comparison with the X-ray crystal structure at acidic pH identified the three amino acid residues responsible for the pH sensitivity of TTR. Our neutron model provides insights into the molecular stability related to amyloidosis.
Yamada, Taro*; Kurihara, Kazuo; Onishi, Yuki*; Tamada, Taro; Tomoyori, Katsuaki; Masumi, Kenji*; Tanaka, Ichiro*; Kuroki, Ryota; Niimura, Nobuo*
Biochimica et Biophysica Acta; Proteins and Proteomics, 1834(8), p.1532 - 1538, 2013/08
Times Cited Count:15 Percentile:45.92(Biochemistry & Molecular Biology)The protonation states and hydration structures of the -thrombin-bivalirubin complex were studied by joint XN refinement of the single crystal X-ray and neutron diffraction data at resolutions of 1.6 and 2.8
, respectively. The atomic distances were estimated by carrying out X-ray crystallographic analysis at 1.25
resolution. The complex represents a model of the enzyme-product (EP) complex of
-thrombin. The neutron scattering length maps around the active site suggest that the side chain of H57/H was deuterated. The joint XN refinement showed that occupancies for D
1 and D
2 of H57/H were 1.0 and 0.7, respectively. However, no significant neutron scattering length density was observed around the hydroxyl oxygen O
of S195/H, which was close to the carboxylic carbon atom of dFPR-COOH. These observations suggest that the O
atom of S195/H is deprotonated and maintains its nucleophilicity in the EP complex. In addition to the active site, the hydration structures of the S1 subsite and the Exosite I, which are involved in the recognition of bivalirudin, are presented.
Onishi, Yuki*; Yamada, Taro*; Kurihara, Kazuo; Tanaka, Ichiro*; Sakiyama, Fumio*; Masaki, Takeharu*; Niimura, Nobuo*
Biochimica et Biophysica Acta; Proteins and Proteomics, 1834(8), p.1642 - 1647, 2013/08
Times Cited Count:7 Percentile:21.99(Biochemistry & Molecular Biology)The structure of the free-form of protease I (API) at pD 8.0 was refined by simultaneous use of single crystal X-ray and neutron diffraction data sets to investigate the protonation states of key catalytic residues of the serine protease. Occupancy refinement of the catalytic triad in the active site of API free-form showed that ca. 30% of the imidazole ring of H57 and ca. 70% of the hydroxyl group of S194 were deuterated. This observation indicates that a major fraction of S194 is protonated in the absence of a substrate. The protonation state of the catalytic triad in API was compared with the bovine
-trypsin-BPTI complex. The comparison led to the hypothesis that close contact of a substrate with S194 could lower the acidity of its hydroxyl group, thereby allowing H57 to extract the hydrogen from the hydroxyl group of S194. H210, which is a residue specific to API, does not form a hydrogen bond with the catalytic triad residue D113. Instead, H210 forms a hydrogen bond network with S176, H177 and a water molecule. The close proximity of the bulky, hydrophobic residue W169 may protect this hydrogen bond network, and this protection may stabilize the function of API over a wide pH range.