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Journal Articles

Band gap formation in graphene by hybridization with Hex-Au(001) reconstructed surface

Terasawa, Tomoo; Matsunaga, Kazuya*; Hayashi, Naoki*; Ito, Takahiro*; Tanaka, Shinichiro*; Yasuda, Satoshi; Asaoka, Hidehito

Vacuum and Surface Science, 66(9), p.525 - 530, 2023/09

As Au (001) surfaces exhibit a quasi-one-dimensional corrugated structure, Hex-Au(001), its periodicity was predicted to change the electronic structure of graphene when graphene was grown on this surface. Furthermore, the hybridization between graphene and Au is known to introduce bandgap and spin polarization into graphene. Here, we report angle-resolved photoemission spectroscopy and density functional theory calculation of graphene on a Hex-Au(001) surface. A bandgap of 0.2 eV in the graphene Dirac cone was observed at the crossing point of the graphene Dirac cone and Au 6sp bands, indicating that the origin of the bandgap formation was the hybridization between the graphene Dirac cone and Au 6sp band. We discussed the hybridization mechanism and anticipated spin injection into the graphene Dirac cone.

Journal Articles

Application of a first-order method to estimate the failure probability of component subjected to thermal transients for optimization of design parameters

Okajima, Satoshi; Mori, Takero; Kikuchi, Norihiro; Tanaka, Masaaki; Miyazaki, Masashi

Mechanical Engineering Journal (Internet), 10(4), p.23-00042_1 - 23-00042_12, 2023/08

In this paper, we propose the simplified procedure to estimate failure probability of components subjected to thermal transient for the design optimization. Failure probability can be commonly used as an indicator of component integrity for various failure mechanisms. In order to reduce number of analyses required for one estimation, we have adopted the First Order Second Moment (FOSM) method as the estimation method of failure probability on the process of the optimization, and an orthogonal table in experiment design method is utilized to define conditions of the analyses for the evaluation of the input parameters for the FOSM method. The superposition of ramp responses is also utilized to evaluate the time history of thermal transient stress instead of finite element analysis. Through the demonstration study to optimize thickness of cylindrical vessel subjected to thermal transient derived from shutdown, we confirmed that the procedure can evaluate the failure probability depending on the cylinder thickness with practical calculation cost.

Journal Articles

First observation of $$^{28}$$O

Kondo, Yosuke*; Achouri, N. L.*; Al Falou, H.*; Atar, L.*; Aumann, T.*; Baba, Hidetada*; Boretzky, K.*; Caesar, C.*; Calvet, D.*; Chae, H.*; et al.

Nature, 620(7976), p.965 - 970, 2023/08

no abstracts in English

Journal Articles

Development of a statistical evaluation method for core hot spot temperature in sodium-cooled fast reactor under natural circulation conditions

Doda, Norihiro; Igawa, Kenichi*; Iwasaki, Takashi*; Murakami, Satoshi*; Tanaka, Masaaki

Nuclear Engineering and Design, 410, p.112377_1 - 112377_15, 2023/08

 Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)

To enhance the safety of sodium-cooled fast reactors, the decay heat in the core must be removed by natural circulation even if the AC power supply to the forced circulation equipment is lost. Under natural circulation conditions, sodium flow is driven by buoyancy, and flow velocity and temperature distribution influence each other. Thus, it is difficult to evaluate the core hot spot temperature by deterministically considering the uncertainties affecting flow and heat. In this study, a statistical evaluation method is developed for the core hot spot temperature by using Monte Carlo sampling methods. The applicability of the core hotspot evaluation method was confirmed in three representative events during natural circulation decay heat removal operations in loop-type sodium-cooled fast reactors.

Journal Articles

Intruder configurations in $$^{29}$$Ne at the transition into the island of inversion; Detailed structure study of $$^{28}$$Ne

Wang, H.*; Yasuda, Masahiro*; Kondo, Yosuke*; Nakamura, Takashi*; Tostevin, J. A.*; Ogata, Kazuyuki*; Otsuka, Takaharu*; Poves, A.*; Shimizu, Noritaka*; Yoshida, Kazuki; et al.

Physics Letters B, 843, p.138038_1 - 138038_9, 2023/08

Detailed $$gamma$$-ray spectroscopy of the exotic neon isotope $$^{28}$$Ne has been performed using the one-neutron removal reaction from $$^{29}$$Ne. Based on an analysis of parallel momentum distributions, a level scheme with spin-parity assignments has been constructed for $$^{28}$$Ne and the negative-parity states are identified for the first time. The measured partial cross sections and momentum distributions reveal a significant intruder p-wave strength providing evidence of the breakdown of the N = 20 and N = 28 shell gaps. Only a weak, possible f-wave strength was observed to bound final states. Large-scale shell-model calculations with different effective interactions do not reproduce the large p-wave and small f-wave strength observed experimentally, indicating an ongoing challenge for a complete theoretical description of the transition into the island of inversion along the Ne isotopic chain.

Journal Articles

Probing strain and doping along a graphene wrinkle using tip-enhanced Raman spectroscopy

Balois-Oguchi, M. V.*; Hayazawa, Norihiko*; Yasuda, Satoshi; Ikeda, Katsuyoshi*; Nguyen, T. Q.*; Esca$~n$o, M. C.*; Tanaka, Takuo*

Journal of Physical Chemistry C, 127(12), p.5982 - 5990, 2023/03

Micrometer-sized wrinkles in graphene are known to affect the electronic properties of graphene due to their shape and the strain variations they create. Here, we analyze the strain distribution and doping of a graphene wrinkle having 1.9 nm width using tip-enhanced Raman spectroscopy (TERS) in ambient conditions. We found a strong correlation between the TERS images of the graphene wrinkle and the electronic Raman scattering (eRS) of the Au(111) substrate. Our work demonstrates that the as-fabricated physical and electronic properties of nanometer-sized features, such as wrinkles, can be probed and studied in detail with TERS which is essential for nanodevice characterization.

Journal Articles

Band gap opening in graphene by hybridization with Au (001) reconstructed surfaces

Terasawa, Tomoo; Matsunaga, Kazuya*; Hayashi, Naoki*; Ito, Takahiro*; Tanaka, Shinichiro*; Yasuda, Satoshi; Asaoka, Hidehito

Physical Review Materials (Internet), 7(1), p.014002_1 - 014002_10, 2023/01

 Times Cited Count:0 Percentile:75.82(Materials Science, Multidisciplinary)

Au(001) surfaces exhibit a complex reconstructed structure [Hex-Au(001)] comprising a hexagonal surface and square bulk lattices, yielding a quasi-one-dimensional corrugated surface. When graphene was grown on this surface, the periodicity of the corrugated surface was predicted to change the electronic structure of graphene, forming bandgaps and new Dirac points. Furthermore, the graphene-Au interface is promising for bandgap generation and spin injection due to band hybridization. Here, we report the angle-resolved photoemission spectroscopy and density functional calculation of graphene on a Hex-Au(001) surface. The crossing point of the original and replica graphene $$pi$$ bands showed no bandgap, suggesting that the one-dimensional potential was too small to modify the electronic structure. A bandgap of 0.2 eV was observed at the crossing point of the graphene $$pi$$ and Au $$6sp$$ bands, indicating that the bandgap is generated using hybridization of the graphene $$pi$$ and Au $$6sp$$ bands. We discussed the hybridization mechanism and concluded that the R30 configuration between graphene and Au and an isolated electronic structure of Au are essential for effective hybridization between graphene and Au. We anticipate that hybridization between graphene $$pi$$ and Au $$6sp$$ would result in spin injection into graphene.

Journal Articles

Application of first-order method to estimate structural integrity in a probabilistic form of component subjected to thermal transient for optimization of design parameter

Okajima, Satoshi; Mori, Takero; Kikuchi, Norihiro; Tanaka, Masaaki; Miyazaki, Masashi

Proceedings of 29th International Conference on Nuclear Engineering (ICONE 29) (Internet), 7 Pages, 2022/08

In this paper, we propose the simplified procedure to estimate failure probability of components subjected to thermal transient for the design optimization. Failure probability can be commonly used as an indicator of component integrity for various failure mechanisms. In order to reduce number of analyses required for one estimation, we have adopted the First Order Second Moment (FOSM) method as the estimation method of failure probability on the process of the optimization, and an orthogonal table in experiment design method is utilized to define conditions of the analyses for the evaluation of the input parameters for the FOSM method. Through the demonstration study to optimize thickness of cylindrical vessel subjected to thermal transient derived from shutdown, we confirmed that the procedure can evaluate the failure probability depending on the cylinder thickness with practical calculation cost.

Journal Articles

Development of ARKADIA for the innovation of advanced nuclear reactor design process (Overview of optimization process development in design optimization support tool, ARKADIA-Design)

Tanaka, Masaaki; Doda, Norihiro; Yokoyama, Kenji; Mori, Takero; Okajima, Satoshi; Hashidate, Ryuta; Yada, Hiroki; Oki, Shigeo; Miyazaki, Masashi; Takaya, Shigeru

Dai-26-Kai Doryoku, Enerugi Gijutsu Shimpojiumu Koen Rombunshu (Internet), 5 Pages, 2022/07

To assist conceptual studies of various reactor systems conducted by private sectors in nuclear power innovation, development of an innovative design system named ARKADIA (Advanced Reactor Knowledge- and AI-aided Design Integration Approach through the whole plant lifecycle) is undergoing to achieve the design of an advanced nuclear reactor as a safe, economic, and sustainable carbon-free energy source. In this paper, focusing on the ARKADIA-Design as a part of it, the progress in the development of optimization processes on the representative problems in the fields of the core design, the plant structure design, and the maintenance schedule planning are introduced.

Journal Articles

Sodium-cooled Fast Reactors

Ohshima, Hiroyuki; Morishita, Masaki*; Aizawa, Kosuke; Ando, Masanori; Ashida, Takashi; Chikazawa, Yoshitaka; Doda, Norihiro; Enuma, Yasuhiro; Ezure, Toshiki; Fukano, Yoshitaka; et al.

Sodium-cooled Fast Reactors; JSME Series in Thermal and Nuclear Power Generation, Vol.3, 631 Pages, 2022/07

This book is a collection of the past experience of design, construction, and operation of two reactors, the latest knowledge and technology for SFR designs, and the future prospects of SFR development in Japan. It is intended to provide the perspective and the relevant knowledge to enable readers to become more familiar with SFR technology.

Journal Articles

Mesospheric ionization during substorm growth phase

Murase, Kiyoka*; Kataoka, Ryuho*; Nishiyama, Takanori*; Nishimura, Koji*; Hashimoto, Taishi*; Tanaka, Yoshimasa*; Kadokura, Akira*; Tomikawa, Yoshihiro*; Tsutsumi, Masaki*; Ogawa, Yasunobu*; et al.

Journal of Space Weather and Space Climate (Internet), 12, p.18_1 - 18_16, 2022/06

 Times Cited Count:0 Percentile:24.42(Astronomy & Astrophysics)

We identified two energetic electron precipitation (EEP) events during the growth phase of moderate substorms and estimated the mesospheric ionization rate for an EEP event for which the most comprehensive dataset from ground-based and space-born instruments was available. The mesospheric ionization signature reached below 70 km altitude and continued for ~15 min until the substorm onset, as observed by the PANSY radar and imaging riometer at Syowa Station in the Antarctic region. We also used energetic electron flux observed by the Arase and POES 15 satellites as the input for the air-shower simulation code PHITS to quantitatively estimate the mesospheric ionization rate. Combining the cutting-edge observations and simulations, we shed new light on the space weather impact of the EEP events during geomagnetically quiet times, which is important to understand the possible link between the space environment and climate.

Journal Articles

Development of a design optimization framework for sodium-cooled fast reactors; Development of coupled analysis control function

Doda, Norihiro; Nakamine, Yoshiaki*; Igawa, Kenichi*; Iwasaki, Takashi*; Murakami, Satoshi*; Tanaka, Masaaki

Keisan Kogaku Koenkai Rombunshu (CD-ROM), 27, 6 Pages, 2022/06

As a part of the development of the "Advanced Reactor Knowledge- and AI-aided Design Integration Approach through the whole plant lifecycle (ARKADIA)" to automatically optimize the life cycle of innovative nuclear reactors including fast reactors, ARKADIA-design is being developed to support the optimization of fast reactor design in the conceptual stage. ARKADIA-Design consists of three systems (Virtual plant Life System (VLS), Evaluation assistance and Application System (EAS), and Knowledge Management System (KMS)). A design optimization framework controls the cooperation between the three systems through the interfaces in each system. This paper reports on the development status of the "VLS interface," which has a control function of coupling analysis codes in VLS.

Journal Articles

Chemical species of iodine during sorption by activated carbon; Effects of original chemical species and fulvic acids

Kato, Tomoaki; Kozai, Naofumi; Tanaka, Kazuya; Kaplan, D. I.*; Utsunomiya, Satoshi*; Onuki, Toshihiko

Journal of Nuclear Science and Technology, 59(5), p.580 - 589, 2022/05

 Times Cited Count:3 Percentile:58.27(Nuclear Science & Technology)

This study reports the effect of fulvic acids, which is a natural organic substance generally contained in groundwater, on the oxidation states of radioactive iodine anions (iodide and iodate). Iodide and iodate are contained in the contaminated water of the Fukushima Daiichi Nuclear Power Plant and supposed to be removed by activated carbon (AC) via adsorption. When fulvic acids does not exist in the experimental system, the adsorption of iodide on AC was less than that of iodate and their oxidation states after the adsorption were not changed. When fulvic acids existed, a fraction of the adsorbed iodate was reduced to iodide. This result indicates that the reduction of the adsorbed iodate progresses during the storage of the spent AC.

Journal Articles

${it Operando}$ structure observation of pyroelectric ceramics during power generation cycle

Kawasaki, Takuro; Fukuda, Tatsuo; Yamanaka, Satoru*; Sakamoto, Tomokazu*; Murayama, Ichiro*; Kato, Takanori*; Baba, Masaaki*; Hashimoto, Hideki*; Harjo, S.; Aizawa, Kazuya; et al.

Journal of Applied Physics, 131(13), p.134103_1 - 134103_7, 2022/04

 Times Cited Count:1 Percentile:18.86(Physics, Applied)

Journal Articles

Development of 1D-CFD coupling method through benchmark analyses of SHRT tests in EBR-II

Yoshimura, Kazuo; Doda, Norihiro; Tanaka, Masaaki; Fujisaki, Tatsuya*; Murakami, Satoshi*; Vilim, R. B.*

Proceedings of 19th International Topical Meeting on Nuclear Reactor Thermal Hydraulics (NURETH-19) (Internet), 16 Pages, 2022/03

In Japan Atomic Energy Agency, the multilevel simulation system which enables consistent evaluation from the whole plant behavior to the local phenomena is being developed to optimize plant design and enhance the safety of sodium-cooled fast reactors. To validate the coupling method in the MLS system, the 1D-CFD coupling method using Super-COPD for 1D plant dynamics analysis and Fluent for multi-dimensional CFD analysis was applied to the analyses of loss of flow tests in EBR-II. It was confirmed that it could predict multi-dimensional thermal-hydraulic phenomena such as thermal stratification in the upper plenum, Z-shaped pipe, and cold pool, holding the whole plant behavior simultaneously. Moreover, the applicability of the 1D-CFD coupling method to the evaluation of the phenomena in natural circulation conditions was confirmed by comparing the results of the 1D-CFD couple analyses and the measured data.

Journal Articles

Development of numerical analysis codes for multi-level and multi-physics approaches in an advanced reactor design study

Tanaka, Masaaki; Doda, Norihiro; Mori, Takero; Yokoyama, Kenji; Uwaba, Tomoyuki; Okajima, Satoshi; Matsushita, Kentaro; Hashidate, Ryuta; Yada, Hiroki

Proceedings of 19th International Topical Meeting on Nuclear Reactor Thermal Hydraulics (NURETH-19) (Internet), 16 Pages, 2022/03

Japan Atomic Energy Agency is developing an innovative design system named ARKADIA to achieve the design of an advanced nuclear reactor as a safe, economic, and sustainable carbon-free energy source. In the first phase of its development, ARKADIA-Design for design study and ARKADIA-Safety for safety assessment will be developed individually. In this paper, focusing on the ARKADIA-Design, the concept of the system is described and numerical analysis codes to be used for the multi-level and multi-physics analyses are introduced. Descriptions of the practical functions composed by the analysis codes and the representative problems in application studies for validation are introduced.

Journal Articles

${it In situ}$ spectrometry of terrestrial gamma rays using portable germanium detectors in area of 80 km radius around the Fukushima Daiichi Nuclear Power Plant

Mikami, Satoshi; Tanaka, Hiroyuki*; Okuda, Naotoshi*; Sakamoto, Ryuichi*; Ochi, Kotaro; Uno, Kiichiro*; Matsuda, Norihiro; Saito, Kimiaki

Nihon Genshiryoku Gakkai Wabun Rombunshi, 20(4), p.159 - 178, 2021/12

In order to know the background radiation level where the area affected by the Fukushima Daiichi Nuclear Power Plant accident in 2011, terrestrial gamma rays had been measured by using portable germanium detectors repeatedly from 2013 through 2019, at 370 locations within 80 km radius area centered on the Fukushima Daiichi Nuclear Power Plant. Radioactive concentrations of Uranium 238, Thorium 232, Potassium 40 and kerma rates in air due to terrestrial gamma rays were obtained at those locations based on the method of ICRU report 53. Averaged concentrations of $$^{238}$$U, $$^{232}$$Th and $$^{40}$$K were 18.8, 22.7, 428 Bq/kg, respectively, and kerma rate in air over the area was found to be 0.0402 $$mu$$Gy/h. The obtained kerma rates in air were compared to those reported in literatures. It was confirmed that the data were correlated with each other, and were agreed within the range of their uncertainty. This is because the kerma rate in air due to terrestrial gamma rays is depend on geology. The similar trend to previous findings was observed that the kerma rate in air at locations geologically classified as Mesozoic era, Granite and Rhyolite were statistically significantly higher than the others.

Journal Articles

Development of an integrated computer code system for analyzing irradiation behaviors of a fast reactor fuel

Uwaba, Tomoyuki; Nemoto, Junichi*; Ito, Masahiro*; Ishitani, Ikuo*; Doda, Norihiro; Tanaka, Masaaki; Otsuka, Satoshi

Nuclear Technology, 207(8), p.1280 - 1289, 2021/08

 Times Cited Count:3 Percentile:36.29(Nuclear Science & Technology)

Computer codes for irradiation behavior analysis of a fuel pin and a fuel pin bundle and for coolant thermal hydraulics analysis were coupled into an integrated code system. In the system, each code provides data required by other codes and the analyzed results are shared among them. The system allows for the synthesizing of analyses of thermal, chemical and mechanical behaviors in a fuel subassembly under irradiation. A test analysis was made for a fuel subassembly containing a mixed oxide fuel pin bundle irradiated in a fast reactor. The results of the analysis were presented with transverse cross-sectional images of the fuel subassembly and three-dimensional images of a fuel pin and fuel pin bundle models. For detailed evaluation, various irradiation behaviors of all fuel pins in the subassembly were analyzed and correlated with irradiation conditions.

Journal Articles

Thermally altered subsurface material of asteroid (162173) Ryugu

Kitazato, Kohei*; Milliken, R. E.*; Iwata, Takahiro*; Abe, Masanao*; Otake, Makiko*; Matsuura, Shuji*; Takagi, Yasuhiko*; Nakamura, Tomoki*; Hiroi, Takahiro*; Matsuoka, Moe*; et al.

Nature Astronomy (Internet), 5(3), p.246 - 250, 2021/03

 Times Cited Count:30 Percentile:96.87(Astronomy & Astrophysics)

Here we report observations of Ryugu's subsurface material by the Near-Infrared Spectrometer (NIRS3) on the Hayabusa2 spacecraft. Reflectance spectra of excavated material exhibit a hydroxyl (OH) absorption feature that is slightly stronger and peak-shifted compared with that observed for the surface, indicating that space weathering and/or radiative heating have caused subtle spectral changes in the uppermost surface. However, the strength and shape of the OH feature still suggests that the subsurface material experienced heating above 300 $$^{circ}$$C, similar to the surface. In contrast, thermophysical modeling indicates that radiative heating does not increase the temperature above 200 $$^{circ}$$C at the estimated excavation depth of 1 m, even if the semimajor axis is reduced to 0.344 au. This supports the hypothesis that primary thermal alteration occurred due to radiogenic and/or impact heating on Ryugu's parent body.

Journal Articles

Simple pretreatment method for tritium measurement in environmental water samples using a liquid scintillation counter

Nakasone, Shunya*; Yokoyama, Sumi*; Takahashi, Tomoyuki*; Ota, Masakazu; Kakiuchi, Hideki*; Sugihara, Shinji*; Hirao, Shigekazu*; Momoshima, Noriyuki*; Tamari, Toshiya*; Shima, Nagayoshi*; et al.

Plasma and Fusion Research (Internet), 16, p.2405035_1 - 2405035_5, 2021/02

Removal of impurities such as organic and other types of dissolved matters from environmental water samples is required for precise analysis of tritium with a liquid scintillation counting method. In general, a distillation method is a conventional one for tritium analysis in environmental water samples, but is a time-consuming process that takes 24 hours for removal of impurities. We have proposed a rapid pretreatment method for tritium analysis, that uses ion exchange resins. In this study, we performed batch experiments, to evaluate the effectiveness of the ion exchange resins on the tritium measurement. The results obtained demonstrated that removal of impurities in the sample water by ion exchange resins can be achieved during a short period of time (i.e., in 5 min).

409 (Records 1-20 displayed on this page)