Introduce of pin-indentation deformation model into fuel pin bundle deformation analysis code "BAMBOO"

Uwaba, Tomoyuki; Ito, Masahiro*; Ishitani, Ikuo*

JAEA-Technology 2025-002, 25 Pages, 2025/06

JAEA-Technology-2025-002.pdf:2.06MB

In spacer wire-type fast reactor fuel assemblies, when the bundle-duct interaction (BDI) becomes severe, contact loads applied to claddings via wires cause oval-deformation of the cladding cross-sections. The cladding oval-deformation may become significant especially in the pins at the outermost periphery of the bundle because they are subjected to a large load from the duct via their wires. In this case the cladding oval-deformation occurs in such a manner that the wire is partially sinking into the cladding, and as a result the cladding is locally dented. We developed a model to simulate such cladding local deformation and integrated the model into the BDI analysis code "BAMBOO". In the out-of-pile bundle compression tests, the gaps between pins and the duct became smaller than the wire diameter when the bundle was compressed despite the existence of a wires between the bundle outermost pins and the duct. The bundle compression test analyses by BAMBOO equipped with the model showed that the local deformation of claddings of outermost pins reproduced the similar trend to the compression test results.

Transverse asymmetry of individual rays in the La()La reaction

Okuizumi, Mao*; Auton, C. J.*; Endo, Shunsuke; Fujioka, Hiroyuki*; Hirota, Katsuya*; Ino, Takashi*; Ishizaki, Kohei*; Kimura, Atsushi; Kitaguchi, Masaaki*; Koga, Jun*; et al.

Physical Review C, 111(3), p.034611_1 - 034611_6, 2025/03

https://doi.org/10.1103/PhysRevC.111.034611

Solvent extraction of tin in nitric acids; Evaluation of multiple extractants

Ito, Kengo*; Takahashi, Shin*; Kato, Chizu*; Fukutani, Satoshi*; Matsumura, Tatsuro; Fujii, Toshiyuki*

Journal of Radioanalytical and Nuclear Chemistry, 334, p.2467 - 2475, 2025/02

https://doi.org/10.1007/s10967-025-10003-7

In this study, the solvent extraction behavior of tin (Sn), specifically Sn, from high-level radioactive waste was evaluated using six different extractants in a HNO system. Among the tested extractants, N,N-Didodecyl-2-hydroxyacetoamide (HAA) exhibited higher efficiency, still not sufficient for industrial implementation. In systems where HCl was added to HNO, both tributyl phosphate (TBP) and N,N,N,N'-tetra-2-ethylhexyl diglycolamide (TEHDGA) achieved D values greater than 1 at 1 M HCl. However, due to practical challenges in industrial applications, HAA extraction in HNO systems, particularly at low Sn concentrations (0.0008 M), may provide a more effective solution for Sn recovery.

Solvent extraction behaviors of rhodium and palladium in nitric acid solutions using amide extractants

Ito, Kengo*; Morita, Misaki*; Araki, Yuta*; Kato, Chizu*; Fukutani, Satoshi*; Matsumura, Tatsuro; Fujii, Toshiyuki*

Solvent Extraction Research and Development, Japan, 32(1), p.53 - 62, 2025/00

https://doi.org/10.15261/serdj.32.53

Rhodium (Rh) and Palladium (Pd) in high-level radioactive waste are primarily fission products. This Study focused on understanding the extraction behavior of these platinum group elements (PGEs) using the novel extractants -hexaoctylnitriloacetamide (HONTA) and alkyl diamideamine (ADAAM). Both extractants showed affinity for Pd, with distribution coefficients significantly exceeding 1, demonstrating their effectiveness in Pd separation. In contrast, the distribution coefficients for Rh were consistently below 10 , indicating low extraction efficiency from nitric acid. However, by leveraging the salting-out effect with calcium nitrate hydrate, a distribution coefficient of 570 for Rh was achieved using HONTA. To overcome the difficult back-extraction of PGEs with HONTA, experiments were conducted using HEDTA and thiourea. Back-extraction with HEDTA in high-concentration nitric acid (2M) resulted in 90% extraction of Pd, while thiourea-based back-extraction with nitric acid yielded over 40% extraction for Rh, with the maximum of 62.7% achieved using hydrochloric acid.

Effect of neutron beam properties on dose distributions in a water phantom for boron neutron capture therapy

Ishikawa, Akihisa; Tanaka, Hiroki*; Nakamura, Satoshi*; Kumada, Hiroaki*; Sakurai, Yoshinori*; Watanabe, Kenichi*; Yoshihashi, Sachiko*; Tanagami, Yuki*; Uritani, Akira*; Kiyanagi, Yoshiaki*

Journal of Radiation Research (Internet), 65(6), p.765 - 775, 2024/11

https://doi.org/10.1093/jrr/rrae076

Isotope-dependent site occupation of hydrogen in epitaxial titanium hydride nanofilms

Ozawa, Takahiro*; Fukutani, Katsuyuki; 7 of others*

Nature Communications (Internet), 15, p.9558_1 - 9558_8, 2024/11

https://doi.org/10.1038/s41467-024-53838-6

Solvent extraction of selenium in nitric acid; Evaluation of multiple extractants and proposal of a novel separation process

Ito, Kengo*; Kawakami, Takahiro*; Kato, Chizu*; Fukutani, Satoshi*; Matsumura, Tatsuro; Fujii, Toshiyuki*

Journal of Radioanalytical and Nuclear Chemistry, 333(10), p.5183 - 5189, 2024/10

https://doi.org/10.1007/s10967-024-09681-6

Solvent extraction behaviors of Se (VI) from nitric acid solutions were investigated with multiple extractants used for uranium, plutonium, minor actinides, and rare earthelements separation processes from high-level liquid waste. During the processes, Se remained in the residual aqueous solutions, as all extractants showed distributionratios 1. In contrast, Se showed distribution ratios 1 with -phenylenediamine in dilute nitric acid ( 2 M HNO), octanol as the organic phase, and concentrated nitric acid (8 M HNO) for back extraction, suggesting a potential new single separation process and recovery of Se.

Benchmark analysis on pipe support structures for establishing inelastic seismic design

Nakamura, Izumi*; Takito, Kiyotaka; Shimazu, Ryuya*; Okuda, Yukihiko; Sakai, Michiya*; Otani, Akihito*; Watakabe, Tomoyoshi; Okuda, Takahiro; Shibutani, Tadahiro*; Shiratori, Masaki*

Proceedings of ASME 2024 Pressure Vessels & Piping Conference (PVP 2024) (Internet), 9 Pages, 2024/07

First demonstration of a single-end readout position-sensitive optical fiber radiation sensor inside the Fukushima Daiichi Nuclear Power Station based on wavelength-resolving analysis

Terasaka, Yuta; Sato, Yuki; Uritani, Akira*

Nuclear Instruments and Methods in Physics Research A, 1062, p.169227_1 - 169227_6, 2024/05

https://doi.org/10.1016/j.nima.2024.169227

Revealing the role of high-valence elementary substitution in the hydrogen-induced Mottronic transitions of vanadium dioxide

Zhou, X.*; Fukutani, Katsuyuki; 9 of others*

Applied Physics Letters, 124(8), p.082103_1 - 082103_7, 2024/02

https://doi.org/10.1063/5.0189271