Factors controlling dissolved Cs concentrations in east Japanese rivers

Tsuji, Hideki*; Ishii, Yumiko*; Shin, M.*; Taniguchi, Keisuke*; Arai, Hirotsugu*; Kurihara, Momo*; Yasutaka, Tetsuo*; Kuramoto, Takayuki*; Nakanishi, Takahiro; Lee, S*; et al.

Science of the Total Environment, 697, p.134093_1 - 134093_11, 2019/12

https://doi.org/10.1016/j.scitotenv.2019.134093

To investigate the main factors that control the dissolved radiocesium concentration in river water in the area affected by the Fukushima Daiichi Nuclear Power Plant accident, the correlations between the dissolved Cs concentrations at 66 sites normalized to the average Cs inventories for the watersheds with the land use, soil components, topography, and water quality factors were assessed. We found that the topographic wetness index is significantly and positively correlated with the normalized dissolved Cs concentration. Similar positive correlations have been found for European rivers because wetland areas with boggy organic soils that weakly retain Cs are mainly found on plains. However, for small Japanese river watersheds, the building area ratio in the watershed strongly affected the dissolved Cs concentration.

Development of fabrication technologies for ITER in-vessel components

Kuroda, Toshimasa*; Sato, Kazuyoshi; Akiba, Masato; Ezato, Koichiro; Enoeda, Mikio; Osaki, Toshio*; Kosaku, Yasuo; Sato, Satoshi; Sato, Shinichi*; Suzuki, Satoshi*; et al.

JAERI-Tech 2002-044, 25 Pages, 2002/03

JAERI-Tech-2002-044.pdf:2.68MB

no abstracts in English

Development of seismic assessment method toward the demonstration reactor of JSFR, 2; Analysis of vibration test of 1/2.5 scale test assembly in triangular arrangement

Monde, Masatsugu*; Iwasaki, Akihisa*; Sawa, Naoki*; Ikarimoto, Iwao*; Taniguchi, Yoshihiro*; Kitamura, Seiji

no journal, , 

The three-dimensional analysis method of a reactor core is developed. The outline of the analysis method and the applicability of the method by comparison with a vibration test of 1/2.5 scale test assembly are reported.

Reduction of Eu by multiphoton excitation in alcohol solutions

Matsuda, Shohei; Nakashima, Nobuaki*; Yokoyama, Keiichi; Yatsuhashi, Tomoyuki*; Chosrowjan, H.*; Taniguchi, Seiji*; Somekawa, Toshihiro*

no journal, , 

The photoredox reactions of lanthanides as a photochemical separative technique proposed in the 1970s are expected to be applied for recovery and recycling of rare metals and nuclear fuel reprocessing. In this study, Eu ions in methanol and ethanol solutions were reduced to Eu ions upon irradiation with nanosecond laser pulses. Eu was observed when the laser wavelength was tuned to f-f transition bands at 394 and 465 nm. The formation rate of Eu was proportional to the square of the incident laser intensity, indicating that the photoreduction is induced by a two-photon process. The efficiency of the photoreduction in ethanol was higher than that in methanol.

Factors controlling dissolved Cs concentrations in east Japanese rivers

Tsuji, Hideki*; Ishii, Yumiko*; Hayashi, Seiji*; Shin, M.*; Taniguchi, Keisuke*; Arai, Hirotsugu*; Kurihara, Momo*; Yasutaka, Tetsuo*; Kuramoto, Takayuki*; Nakanishi, Takahiro; et al.

no journal, , 

Controlling factor of dissolved Cs concentrations in 66 in East Japan rivers was investigated. Dissolved Cs concentrations decreased by one order of magnitude between 2012 and 2017. Normalized dissolved Cs concentrations correlated well with building area ratios. Topographic wetness index generally predicted dissolved Cs concentrations. The high concentration of dissolved Cs in urban area cannot be explained by water quality condition.

Radiocaesium dynamics in forested watersheds in Fukushima Prefecture

Taniguchi, Keisuke*; Takeuchi, Yukio*; Fujita, Kazuki*; Dohi, Terumi; Hayashi, Seiji*; Kuramoto, Takayuki*; Nomura, Naoki*; Aono, Tatsuo*

no journal, , 

In Fukushima Prefecture, although decontamination has been completed except for difficult-to-return areas, most of the forest has not been decontaminated yet. From the forest, radiocaesium may enter rivers and affect downstream areas. A survey was conducted in three forested watersheds of the Nanokazawa, Saruta, Nuno rivers located in Fukushima Prefecture to understand the amount and characteristics of radiocaesium flowing out. In each watershed, suspended solids (SS) were collected by a suspended sand sampler, water was collected every few months, and the water level and flow rate were measured. After freeze-drying the SS sample, the concentration of suspended Cs-137 was measured by a germanium semiconductor detector. The water sample was filtered through a membrane filter with a pore size of 0.45 m, then the dissolved Cs-137 was collected by the solid-phase extraction disk method or AMP coprecipitation method, and the dissolved Cs-137 concentration was measured by a germanium semiconductor detector. The ranges of dissolved Cs-137 concentration in FY2019 were 69-190 mBq/L in the Saruta River, 9.7-16 mBq/L in the Nanokazawa river, and ND-3.2 mBq/L in the Nuno River. In the poster, we will also present the results of SS measurements and flow observations.