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Yoshida, Takeru; Maeda, Koji; Sekio, Yoshihiro; Tomita, Hideki*; Iwata, Yoshihiro; Hirai, Mutsumi*; Mizokami, Masato*; Sakamoto, Tetsuo*
Scientific Reports (Internet), 16, p.9865_1 - 9865_8, 2026/03
Times Cited Count：0 Percentile：0.00(Multidisciplinary Sciences)Miyabe, Masabumi; Iwata, Yoshihiro; Tomita, Hideki*; Morita, Masato*; Sakamoto, Tetsuo*
Spectrochimica Acta, Part B, 221, p.107036_1 - 107036_12, 2024/11
Times Cited Count：7 Percentile：70.78(Spectroscopy)Two-color two-step resonance ionization spectroscopy of neodymium (Nd) was performed to identify more than 120 even-parity autoionizing levels and their candidate J-values. The analysis of the observed autoionizing Rydberg series yielded a value of 44560.11 (43)
(2)
cm
as a more accurate ionization potential of Nd. The saturation method was used to measure the transition cross-sections for some intense ionization transitions. From the measured cross-sections, the ionization efficiencies of some two-step ionization schemes were evaluated using the scheme cross-section formula to obtain several promising schemes.
-ray discrimination based on the property and thickness controls of scintillators using Li glass and LiCAF(Ce) in a -ray fieldKaburagi, Masaaki; Shimazoe, Kenji*; Terasaka, Yuta; Tomita, Hideki*; Yoshihashi, Sachiko*; Yamazaki, Atsushi*; Uritani, Akira*; Takahashi, Hiroyuki*
Nuclear Instruments and Methods in Physics Research A, 1046, p.167636_1 - 167636_8, 2023/01
Times Cited Count：8 Percentile：77.35(Instruments & Instrumentation)We focus on the thickness and property controls of inorganic scintillators used for thermal neutron detection in intense -ray fields without considering pulse shape discrimination techniques. GS20
(a lithium glass) and LiCaAlF
:Ce(LiCAF:Ce) cintillators with thicknesses of 0.5 and 1.0 mm, respectively, have been employed. Pulse signals generated by photomultiplier tubes, to which the scintillators were coupled, were inserted into a digital pulse processing unit with 1 Gsps, and the areas of waveforms were integrated for 360 ns. In a 
Co -ray field, the neutron detection for GS20 with a 0.5-mm thickness was possible at dose rates of up to 0.919 Gy/h; however, for LiCAF:Ce, neutron detection was possible at 0.473 Gy/h, and it failed at 0.709 Gy/h. Threfore, in a Co -ray field, the neutron/-ray discrimination of GS20 was better than that of LiCAF:Ce due to its better energy resolution and higher detection efficiency.
Miyabe, Masabumi; Satou, Yukihiko; Wakaida, Ikuo; Terabayashi, Ryohei*; Sonnenschein, V.*; Tomita, Hideki*; Zhao, Y.*; Sakamoto, Tetsuo*
Journal of Physics B; Atomic, Molecular and Optical Physics, 54(14), p.145003_1 - 145003_8, 2021/07
Times Cited Count：2 Percentile：12.94(Optics)Two-color two-step photoionization optogalvanic spectroscopy was performed using high-repetition-rate titanium sapphire lasers and a uranium hollow cathode lamp to find the two-step resonance ionization schemes of uranium. Many ionization transitions were observed by exciting uranium atoms in a ground state into five, even parity, excited levels with the first-step laser and by scanning the second-step laser wavelengths. By blocking the first-step laser, single-color, two-photon ionization transitions were also identified. From these results, we have found more than 50 odd-parity autoionizing levels of uranium in the energy, ranging from the ionization potential (49958.4 cm) to 51150 cm. The determined energy levels are within 1 cm of previously reported values.
Ito, Chikara; Maeda, Shigetaka; Inoue, Toshihiko; Tomita, Hideki*; Iguchi, Tetsuo*
Radiation Protection, 40(6), p.491 - 495, 2020/11
A highly accurate and precise technique for measurement of the 
Nb(n,n')
Nb reaction rate was established for the material surveillance tests, etc. in fast reactors. The self-absorption effect on the measurement of the characteristic X-rays emitted by Nb was decreased by the solution and evaporation to dryness of niobium dosimeter. A highly precise count of the number of Nb atoms was obtained by measuring the niobium solution concentration using inductively coupled plasma mass spectrometry. X-rays of Nb were measured accurately by means of comparing the X-ray intensity of irradiated niobium solution with that of the solution in which stable Nb was added. The difference between both intensities indicates the effect of 
Ta, which is generated from an impurity tantalum, and the intensity of X-rays from Nb was evaluated. Measurement error of the Nb(n,n')Nb reaction rate was reduced to be less than 4%, which was equivalent to the other reaction rate errors of dosimeters used for Joyo dosimetry. In addition, an advanced technique using Resonance Ionization Mass Spectrometry was proposed for the precise measurement of Nb yield, and Nb will be resonance-ionized selectively by discriminating the hyperfine splitting of the atomic energy levels between Nb and Nb at high resolution.
He
excimer cluster tracers in superfluid helium-4 via neutron-
He absorption reactionSonnenschein, V.*; Tsuji, Yoshiyuki*; Kokuryu, Shoma*; Kubo, Wataru*; Suzuki, So*; Tomita, Hideki*; Kiyanagi, Yoshiaki*; Iguchi, Tetsuo*; Matsushita, Taku*; Wada, Nobuo*; et al.
Review of Scientific Instruments, 91(3), p.033318_1 - 033318_12, 2020/03
Times Cited Count：0 Percentile：0.00(Instruments & Instrumentation)Kurihara, Momo*; Yasutaka, Tetsuo*; Aono, Tatsuo*; Ashikawa, Nobuo*; Ebina, Hiroyuki*; Iijima, Takeshi*; Ishimaru, Kei*; Kanai, Ramon*; Karube, Jinichi*; Konnai, Yae*; et al.
Journal of Radioanalytical and Nuclear Chemistry, 322(2), p.477 - 485, 2019/11
Times Cited Count：8 Percentile：52.78(Chemistry, Analytical)We assessed the repeatability and reproducibility of methods for determining low dissolved radiocesium concentrations in freshwater in Fukushima. Twenty-one laboratories pre-concentrated three of 10 L samples by five different pre-concentration methods (prussian-blue-impregnated filter cartridges, coprecipitation with ammonium phosphomolybdate, evaporation, solid-phase extraction disks, and ion-exchange resin columns), and activity of radiocesium was measured. The z-scores for all of the 
Cs results were within 
2, indicating that the methods were accurate. The relative standard deviations (RSDs) indicating the variability in the results from different laboratories were larger than the RSDs indicating the variability in the results from each separate laboratory.
Sonoda, Tetsu*; Katayama, Ichiro*; Wada, Michiharu*; Iimura, Hideki; Sonnenschein, V.*; Iimura, Shun*; Takamine, Aiko*; Rosenbusch, M.*; Kojima, Takao*; Ahn, D. S.*; et al.
Progress of Theoretical and Experimental Physics (Internet), 2019(11), p.113D02_1 - 113D02_12, 2019/11
Times Cited Count：1 Percentile：8.89(Physics, Multidisciplinary)An in-flight separator, BigRIPS, at RIBF in RIKEN provides each experiment with specific nuclides separated from many nuclides produced by projectile fragmentation or in-flight fission. In this process, nuclides other than separated ones are discarded on the slits in BigRIPS, although they include many nuclides interested from the view point of nuclear structure. In order to extract these nuclides for parasitic experiments, we are developing a method using laser ion-source (PALIS). A test experiment with 
Se beam from RIBF has been performed by using a gas cell set in BigRIPS. Unstable nuclides around 
Se were stopped in the gas cell in accordance with a calculation using LISE code. The stopping efficiency has been estimated to be about 30%. As a next step, we will establish the technique for extracting reaction products from the gas cell.
He
clusters via neutron-He absorption reaction toward visualization of full velocity field in quantum turbulenceMatsushita, Taku*; Sonnenschein, V.*; Guo, W.*; Hayashida, Hirotoshi*; Hiroi, Kosuke; Hirota, Katsuya*; Iguchi, Tetsuo*; Ito, Daisuke*; Kitaguchi, Masaaki*; Kiyanagi, Yoshiaki*; et al.
Journal of Low Temperature Physics, 196(1-2), p.275 - 282, 2019/07
Times Cited Count：1 Percentile：3.36(Physics, Applied)Sakamoto, Tetsuo*; Morita, Masato*; Kanenari, Keita*; Tomita, Hideki*; Sonnenschein, V.*; Saito, Kosuke*; Ohashi, Masaya*; Kato, Kotaro*; Iguchi, Tetsuo*; Kawai, Toshihide*; et al.
Analytical Sciences, 34(11), p.1265 - 1270, 2018/11
Times Cited Count：12 Percentile：36.55(Chemistry, Analytical)Sonoda, Tetsu*; Iimura, Hideki; Reponen, M.*; Wada, Michiharu*; Katayama, Ichiro*; Sonnenschein, V.*; Takamatsu, Takahide*; Tomita, Hideki*; Kojima, Takao*
Nuclear Instruments and Methods in Physics Research A, 877, p.118 - 123, 2018/01
Times Cited Count：4 Percentile：29.89(Instruments & Instrumentation)In order to produce low-energy RI beams at RIKEN RIBF, a laser ion source, PALIS, is under construction. This ion source is based on resonance ionization of RI atoms captured in Ar gas. Because the ion source is located 70m away from lasers, we have developed an optical system for laser beam transport. This system can be controlled remotely when the ion source is not accessible because of high radiation level. The position of laser beam after transport is reasonably stable, and the transport efficiency is about 50%.
Tomita, Masanori*; Matsumoto, Hideki*; Funayama, Tomoo; Yokota, Yuichiro; Otsuka, Kensuke*; Maeda, Munetoshi*; Kobayashi, Yasuhiko
Life Sciences in Space Research, 6, p.36 - 43, 2015/07
A radiation-induced bystander response is generally known as a cellular response induced in unirradiated cell by receiving bystander signaling factors released from directly irradiated cells of a cell population. Bystander responses induced by high-LET heavy ions at low fluence are an important problem concerning the health of astronauts in the space environment. Here we set out NO-mediated bystander signal transductions induced by high-LET heavy-ion microbeam irradiation in normal human fibroblasts. Our findings suggest that Akt- and NF-
B-dependent signaling pathway involving COX-2 plays an important role in the NO-mediated high-LET heavy-ion-induced bystander responses. Additionally, COX-2 may be used as a molecular marker of high-LET heavy-ion-induced bystander cells, which are distinguish form directly irradiated cells.
Tomita, Masanori*; Matsumoto, Hideki*; Otsuka, Kensuke*; Funayama, Tomoo; Yokota, Yuichiro; Suzuki, Michiyo; Sakashita, Tetsuya; Kobayashi, Yasuhiko
JAEA-Review 2014-050, JAEA Takasaki Annual Report 2013, P. 77, 2015/03
Radiation-induced bystander responses are defined as responses in cells that have not been directly targeted by radiation but are in the neighborhood of cells that have been directly exposed. In this study, we aim to clarify a role of bystander response to sustain the homeostasis of damaged tissue using heavy-ion microbeams. We established the heavy-ion microbeam irradiation method to a 3D cultured human epidermis. Using this method, a viable cell rate of the 3D cultured human epidermis irradiated with 260 MeV 
Ne-ion microbeams or broadbeams was analyzed by the MTT method.
Matsumoto, Hideki*; Tomita, Masanori*; Otsuka, Kensuke*; Hatashita, Masanori*; Maeda, Munetoshi*; Funayama, Tomoo; Yokota, Yuichiro; Suzuki, Michiyo; Sakashita, Tetsuya; Ikeda, Hiroko; et al.
JAEA-Review 2014-050, JAEA Takasaki Annual Report 2013, P. 76, 2015/03
The objective of this project is to elucidate molecular mechanisms for the induction of radioadaptive response through radiation-induced bystander responses induced by irradiation with heavy ion microbeams in JAEA. We found that the adaptive response was induced by Ar (520 MeV 
Ar
) microbeam-irradiation of a limited number of cells, followed by the broad beam-irradiation and that the adaptive response was almost completely suppressed by the addition of carboxy-PTIO, as a nitric oxide (NO) scavenger. In addition, we found several genes induced specifically and preferentially when radioadaptive response could be induced. We confirmed that 
expression was specifically induced only when radioadaptive response could be induced. Our findings strongly suggested that radioadaptive response can be induced by NO-mediated bystander responses evoked by irradiation with heavy ion microbeams.
-ray for improvement neutron emission profile measurementUchida, Yuki*; Takada, Eiji*; Fujisaki, Akihiro*; Isobe, Mitsutaka*; Ogawa, Kunihiro*; Shinohara, Koji; Tomita, Hideki*; Kawarabayashi, Jun*; Iguchi, Tetsuo*
Review of Scientific Instruments, 85(11), p.11E118_1 - 11E118_4, 2014/11
Times Cited Count：14 Percentile：48.75(Instruments & Instrumentation)Ishihara, Kohei*; Kawarabayashi, Jun*; Tomita, Hideki*; Naka, Tatsuhiro*; Asada, Takashi*; Morishima, Kunihiro*; Nakamura, Mitsuhiro*; Maeda, Shigetaka; Iguchi, Tetsuo*
Progress in Nuclear Science and Technology (Internet), 4, p.661 - 664, 2014/04
Spent fuel emits not only neutrons but also lots of -rays by its included fission products (for example, neutron/ ratio is in the order of 10
). For its safety handling, it is important to investigate the neutron characteristics such as an emission rate, emission profile and energy spectrum. But it is difficult to measure the neutron characteristics with high precision because of lots of -rays. So the neutron characteristics are estimated by an evaluation based on its burning history. It is necessary to measure them for estimate of adequacy of the simulated result. Also, a direct measurement of the neutron characteristics is essential in the case that each spent fuel has different burning history and is mixed (for example the accident of the Fukushima Dai-ichi Nuclear Power Plant). Therefore, we develop a new nuclear emulsion in order to measure neutrons under high -rays field in our study.
Maeda, Shigetaka; Ito, Chikara; Ishihara, Kohei*; Takagi, Keisuke*; Minato, Haruna*; Sakai, Yosuke*; Kawarabayashi, Jun*; Tomita, Hideki*; Iguchi, Tetsuo*
Progress in Nuclear Science and Technology (Internet), 4, p.665 - 669, 2014/04
In order to realize neutron spectroscopy in high-intensity ray fields, an advanced nuclear emulsion based on a non-sensitized OPERA film with AgBr grain sizes of 60 nm has been developed together with a neutron spectrum unfolding method. The response functions were evaluated in the neutron energy range between 0.1 and 4.5 MeV by Monte Carlo calculations. To realize a highly reliable unfolding method that does not require an initial guess spectrum, an algorithm was formulized based on the maximum entropy principle and the maximum likelihood method, and the new unfolding code MEALU was developed. Through analyses of mock-up data, its performance was checked. The neutron spectrum from fresh fuel from the experimental fast reactor Joyo was estimated and track lengths were simulated using the calculated response function and the estimated spectrum. Comparison between the assumed neutron spectrum and the unfolded one confirmed the effectiveness of the proposed technique.
-ray fields with novel nuclear emulsion techniqueIshihara, Kohei*; Takagi, Keisuke*; Minato, Haruna*; Kawarabayashi, Jun*; Tomita, Hideki*; Maeda, Shigetaka; Naka, Tatsuhiro*; Morishima, Kunihiro*; Nakano, Toshiyuki*; Nakamura, Mitsuhiro*; et al.
Radiation Measurements, 55, p.79 - 82, 2013/08
Times Cited Count：2 Percentile：16.52(Nuclear Science & Technology)In order to measure the neutron under a condition of high intensity of -ray background, we made new nuclear emulsion based on non-sensitized OPERA emulsion which had small AgBr grain size (AgBr grain size of 60, 90 and 160 nm). The sensitivity of this new emulsion, which was a correlation between stopping power and grain density, was estimated experimentally by irradiating neutrons with several energies. We also simulated the response to -ray induced electrons and compared with some experimental results by using Co source. The results showed that there might be a threshold energy deposited in one AgBr grain under which it was impossible to develop. We estimated efficiency to the -ray and the neutron with this obtained response of the new emulsion.
Sonoda, Tetsu*; Wada, Michiharu*; Tomita, Hideki*; Sakamoto, Chika*; Takatsuka, Takaaki*; Furukawa, Takeshi*; Iimura, Hideki; Ito, Yuta*; Kubo, Toshiyuki*; Matsuo, Yukari*; et al.
Nuclear Instruments and Methods in Physics Research B, 295, p.1 - 10, 2013/01
Times Cited Count：22 Percentile：80.93(Instruments & Instrumentation)no abstracts in English
field using new type of nuclear emulsionKawarabayashi, Jun*; Ishihara, Kohei*; Takagi, Keisuke*; Tomita, Hideki*; Iguchi, Tetsuo*; Naka, Tatsuhiro*; Morishima, Kunihiro*; Maeda, Shigetaka
Journal of ASTM International (Internet), 9(3), 5 Pages, 2012/03
In order to measure the neutron from a spent fuel assembly in fast breeder reactor precisely, we made new nuclear emulsion based on non-sensitized OPERA film with AgBr grain size of 60, 90 and 160 nm. The efficiency for 
Cf neutron of the new emulsion was calculated to be 0.7
10
which energy ranged from 0.3 to 2 MeV that agrees with preliminary estimated value from experimental results. The sensitivity of the new emulsion was also estimated experimentally by irradiating 565 KeV and 14 MeV neutrons and found that the emulsion with the AgBr grain size of 60 nm showed the lowest sensitivity among these three emulsions but still had enough sensitivity for proton. Also, there was a suggestion from the experimental data that there was a threshold LET of 15 KeV/
m for our new emulsion below which no silver cluster was developed. Further development of the response of nuclear emulsion with a few tens of nano-meter AgBr size is next step of this study.
