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Tanaka, Kazuya; Yamaji, Keiko*; Masuya, Hayato*; Tomita, Jumpei; Ozawa, Mayumi*; Yamasaki, Shinya*; Tokunaga, Kohei; Fukuyama, Kenjin*; Ohara, Yoshiyuki*; Maamoun, I.*; et al.
Chemosphere, 355, p.141837_1 - 141837_11, 2024/05
In this study, biogenic Mn(IV) oxide was applied to remove Ra from mine water collected from a U mill tailings pond in the Ningyo-toge center. Just 7.6 mg of biogenic Mn(IV) oxide removed more than 98% of the Ra from 3 L of mine water, corresponding to a distribution coefficient of 10
mL/g for Ra at pH 7. The obtained value was convincingly high for practical application of biogenic Mn(IV) oxide in water treatment.
Tomita, Jumpei; Tomita, Ryohei; Suzuki, Daisuke; Yasuda, Kenichiro; Miyamoto, Yutaka
Journal of the American Society for Mass Spectrometry, 35(6), p.1178 - 1183, 2024/05
Times Cited Count:0 Percentile:0.00(Biochemical Research Methods)A sensitive analytical technique was investigated in order to determine 10 order of
U/
U ratio in the sub-ng of uranium using a multi-collector ICP-MS. First, the solution volume was concentrated to one tenth to obtain higher intensities. Next, data acquisition was started from the beginning of the solution uptake and continued until all solution was exhausted. Taking advantage of multi-collector measurement, all data were used with excepting the portion affected by air mixing at the beginning and end of sample introduction. The isotope ratios were calculated from the total counts of each isotope. This technique was applied to U isotope standard (IRMM-184) to measure the 10
order of
U/
U ratio in the sub-ng of uranium. Measured values were in good agreement with the certified value within the uncertainity (
=2). The uncertainties obtained with this new technique (32% on average) were revised to be 10 times smaller than those obtained with the conventionalmethod.
Tomita, Ryohei; Tomita, Jumpei; Suzuki, Daisuke; Yasuda, Kenichiro; Miyamoto, Yutaka
Hosha Kagaku, (48), p.1 - 15, 2023/09
Secondary Ion Mass Spectrometry (SIMS) is the method to detect secondary ions produced by the sputtering of primary ions. SIMS is one of effective method to measure isotopic composition of particles containing nuclear material in environmental sample for safeguards. We are a group member of the International Atomic Energy Agency (IAEA)'s network of analytical laboratories and have developed analytical techniques using SIMS and other mass spectrometers for nuclear safeguards. We will introduce the principle of SIMS and analytical techniques developed by our group to measure isotopic composition of uranium particles which having a particle diameter of micron order in environmental sample for safeguards.
Miyamoto, Yutaka; Suzuki, Daisuke; Tomita, Ryohei; Tomita, Jumpei; Yasuda, Kenichiro
Isotope News, (786), p.22 - 25, 2023/04
no abstracts in English
Tomita, Ryohei; Tomita, Jumpei; Yomogida, Takumi; Suzuki, Daisuke; Yasuda, Kenichiro; Esaka, Fumitaka; Miyamoto, Yutaka
KEK Proceedings 2022-2, p.108 - 113, 2022/11
Automated Particle Measurement (APM) is the first measurement of environmental sample for safeguard purpose. APM tells us the number of particles in sample, their enrichment and their location. Precision and accuracy of APM is easily affected by particle condition. We have investigated how influential baking temperature in sample preparation are for uranium secondary ion quantity, uranium hydride generation and particle crystallinity. Our experimental results showed that baking temperature of 800C reduced uranium secondary ion quantity to 33% compared with baking at 350
C. Uranium hydride generation ratio of the sample baked at 850
C was also 4 times higher than the sample baked at 350
C. Baking at 850
C raised only crystallinity of uranium particles. Baking sample at too high temperature caused less uranium secondary ion generation and much more uranium hydride generation. It made precision and accuracy of APM worse. In our experiment, baking at 350
C is suitable for uranium particles in the safeguards sample.
Tomita, Jumpei; Tomita, Ryohei; Suzuki, Daisuke; Yasuda, Kenichiro; Miyamoto, Yutaka
KEK Proceedings 2022-2, p.154 - 158, 2022/11
Precise determination of minor U isotopes (U and
U) of particles from the safeguard environmental samples is powerful method for detecting the undeclared nuclear activities. In this study, preparation method of U particle was examined to utilize for the minor U isotope determination. The porous silica particles were used as the particle matrix and lutetium was mixed to the impregnation solution as U impregnation indicator for the particle picking. The result of the Scanning Electron Microscope indicated that the contacting the solution with Si particles overnight gently could produce the impregnated particles effectively rather than the mixing them with PFA stick.
Tomita, Ryohei; Tomita, Jumpei; Yomogida, Takumi; Suzuki, Daisuke; Yasuda, Kenichiro; Esaka, Fumitaka; Miyamoto, Yutaka
KEK Proceedings 2021-2, p.146 - 150, 2021/12
no abstracts in English
Tomita, Jumpei; Ozawa, Mayumi; Ohara, Yoshiyuki; Miyamoto, Yutaka
KEK Proceedings 2021-2, p.130 - 134, 2021/12
no abstracts in English
Suzuki, Daisuke; Tomita, Ryohei; Tomita, Jumpei; Esaka, Fumitaka; Yasuda, Kenichiro; Miyamoto, Yutaka
Journal of Radioanalytical and Nuclear Chemistry, 328(1), p.103 - 111, 2021/04
Times Cited Count:5 Percentile:49.08(Chemistry, Analytical)An analytical technique was developed to determine the age of uranium particles for safeguards. After the chemical separation of uranium and thorium, the Th/
U ratio was measured using single-collector inductively coupled plasma mass spectrometry and a
U-based reference material comprising a certain amount of
Th as a progeny nuclide of
U. The results allowed us to determine the purification age of two certified materials, i.e., U-850 and U-100, which was in good agreement with the reference purification age (61 y). Moreover, the age of a single U-850 particle was determined with a difference of -28 to 2 years from the reference date.
Tomita, Jumpei
Zusetsu Nihon No Onsen No, 170 Onsen No Saiensu, P. 111, 2020/03
no abstracts in English
Tomita, Jumpei; Takeuchi, Erina
Applied Radiation and Isotopes, 150, p.103 - 109, 2019/08
Times Cited Count:19 Percentile:86.32(Chemistry, Inorganic & Nuclear)A rapid analytical method for determining Sr in urine samples (1-2 L) was developed to assess the internal exposure of workers in a radiological emergency. Strontium in a urine sample was rapidly separated by phosphate co-precipitation, followed by extraction chromatography with a tandem column of Pre-filter, TRU and Sr resin, and the
Sr activity was determined by ICP-MS/MS. Measurement in the MS/MS mode with an O
reaction gas flow rate 1 mL min
showed no tailing of
Sr at m/z = 90 up to 50 mg-Sr L
. The interferences of Ge, Se and Zr at m/z = 90 were successfully removed by chemical separation. This analytical method was validated by the results of the analyses of synthetic urine samples (1.2-1.6 L) containing a known amount of
Sr along with 1 mg of each of Ge, Se, Sr and Zr. The turnaround time for analysis was about 10 h, and the detection limit of
Sr was approximately 1 Bq per urine sample.
Tomita, Jumpei
Bunseki, 2019(3), p.112 - 113, 2019/03
no abstracts in English
Tomita, Jumpei; Abe, Takuya
JAEA-Research 2016-026, 12 Pages, 2017/03
An analytical method of low-level Ra isotopes in freshwater samples with combination of pre-concentration from large volume of water sample (
170 L) using Powdex resin and
-ray spectrometry followed by simple coprecipitation of Ra was developed.
pre-concentration of Ra by batch method using Powder resin was examined, and it was shown that the amount of the resin required collecting Ra in the water sample could be determined by measuring the electric conductivity (EC) of water sample. It was found that coprecipitation of Ra with barium sulfate could remove more than 96% of potassium that increases the background. The validation of this method was confirmed by the analyses of 170 L of water sample containing the known amount of Ra isotopes with different EC. Among the analyses, the recovery of Ra was 98% in average and detection limits of
Ra and
Ra were achieved to be approximately 0.3 and 0.5 mBq L
, respectively.
Tanimura, Yoshihiko; Tomita, Jumpei; Yoshitomi, Hiroshi; Yoshizawa, Michio; Hakozaki, Ryozo*; Takahashi, Sohei*
Hoken Butsuri, 51(3), p.141 - 146, 2016/09
Photon spectra were measured inside and outside a house in Minami-Soma city by using a NaI(Tl) scintillation spectrometer. The photons were categorized into three groups according to their energy. The groups were (1) scattered photons, which include low energy photons, (2) direct photons from Cs and
Cs sources and (3) the other photons. Then the ratios of the ambient dose equivalents H
(10) of the scattered photons to those of the direct photons from the
Cs and
Cs sources have been evaluated from the measured photon spectra. The ratios are high inside the house compared with those out of the house. It was found that the scattered photons contribute to the H
(10) by more than 50
inside the house. The ambient dose equivalent average energies of the scattered photons are around 0.25 MeV both inside and outside the house. These data is worthwhile to design the optimum shielding for the protection against the public radiation exposure.
Tomita, Jumpei; Yamamoto, Masayoshi*; Nozaki, Teo; Tanimura, Yoshihiko*; Oishi, Tetsuya
Journal of Environmental Radioactivity, 146, p.88 - 93, 2015/08
Times Cited Count:16 Percentile:40.90(Environmental Sciences)Yamamoto, Masayoshi*; Tomita, Jumpei
Onsen Kagaku, 64(4), p.388 - 401, 2015/03
no abstracts in English
Endo, Satoru*; Tomita, Jumpei*; Tanaka, Kenichi*; Yamamoto, Masayoshi*; Fukutani, Satoshi*; Imanaka, Tetsuji*; Sakaguchi, Aya*; Amano, Hikaru; Kawamura, Hidehisa*; Kawamura, Hisao*; et al.
Radiation and Environmental Biophysics, 47(3), p.359 - 365, 2008/07
Times Cited Count:5 Percentile:20.44(Biology)Dolon village located about 60 km from the border of the Semipalatinsk Nuclear Test Site is known to be heavily contaminated by the first USSR atomic bomb test in August 1949. Soil samples around Dolon were taken in October 2005 in an attempt to evaluate internal thyroid dose arising from incorporation of radioiodine isotopes (mainly I). Iodine-129 in soil was measured by using the technique of Accelerator Mass Spectrometry. From the relationship between
I and
Cs (corrected for background and decay from 1949 to 2005) accumulated levels, the background level of
I and the
I/
Cs ratio around Dolon were estimated to be (6.4
0.4)
10
atoms m
and 0.25
0.16, respectively. This
I/
Cs ratio is almost similar to the fission yield ratio for
Pu fast fission (0.24).
Tomita, Jumpei
no journal, ,
no abstracts in English
Tomita, Jumpei; Takeuchi, Erina
no journal, ,
no abstracts in English