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U/
U isotopic analysis of trace uranium in safeguards environmental samples using multicollector inductively coupled plasma mass spectrometryTomita, Jumpei; Tomita, Ryohei; Suzuki, Daisuke; Yasuda, Kenichiro; Miyamoto, Yutaka
Journal of the American Society for Mass Spectrometry, 35(6), p.1178 - 1183, 2024/05
Times Cited Count：0 Percentile：0.00(Biochemical Research Methods)A sensitive analytical technique was investigated in order to determine 10
order of U/U ratio in the sub-ng of uranium using a multi-collector ICP-MS. First, the solution volume was concentrated to one tenth to obtain higher intensities. Next, data acquisition was started from the beginning of the solution uptake and continued until all solution was exhausted. Taking advantage of multi-collector measurement, all data were used with excepting the portion affected by air mixing at the beginning and end of sample introduction. The isotope ratios were calculated from the total counts of each isotope. This technique was applied to U isotope standard (IRMM-184) to measure the 10 order of U/U ratio in the sub-ng of uranium. Measured values were in good agreement with the certified value within the uncertainity (
=2). The uncertainties obtained with this new technique (32% on average) were revised to be 10 times smaller than those obtained with the conventionalmethod.
Tomita, Ryohei; Tomita, Jumpei; Suzuki, Daisuke; Yasuda, Kenichiro; Miyamoto, Yutaka
Hosha Kagaku, (48), p.1 - 15, 2023/09
Secondary Ion Mass Spectrometry (SIMS) is the method to detect secondary ions produced by the sputtering of primary ions. SIMS is one of effective method to measure isotopic composition of particles containing nuclear material in environmental sample for safeguards. We are a group member of the International Atomic Energy Agency (IAEA)'s network of analytical laboratories and have developed analytical techniques using SIMS and other mass spectrometers for nuclear safeguards. We will introduce the principle of SIMS and analytical techniques developed by our group to measure isotopic composition of uranium particles which having a particle diameter of micron order in environmental sample for safeguards.
Miyamoto, Yutaka; Suzuki, Daisuke; Tomita, Ryohei; Tomita, Jumpei; Yasuda, Kenichiro
Isotope News, (786), p.22 - 25, 2023/04
no abstracts in English
Tomita, Ryohei; Tomita, Jumpei; Yomogida, Takumi; Suzuki, Daisuke; Yasuda, Kenichiro; Esaka, Fumitaka; Miyamoto, Yutaka
KEK Proceedings 2022-2, p.108 - 113, 2022/11
Automated Particle Measurement (APM) is the first measurement of environmental sample for safeguard purpose. APM tells us the number of particles in sample, their enrichment and their location. Precision and accuracy of APM is easily affected by particle condition. We have investigated how influential baking temperature in sample preparation are for uranium secondary ion quantity, uranium hydride generation and particle crystallinity. Our experimental results showed that baking temperature of 800
C reduced uranium secondary ion quantity to 33% compared with baking at 350C. Uranium hydride generation ratio of the sample baked at 850C was also 4 times higher than the sample baked at 350C. Baking at 850C raised only crystallinity of uranium particles. Baking sample at too high temperature caused less uranium secondary ion generation and much more uranium hydride generation. It made precision and accuracy of APM worse. In our experiment, baking at 350C is suitable for uranium particles in the safeguards sample.
Tomita, Jumpei; Tomita, Ryohei; Suzuki, Daisuke; Yasuda, Kenichiro; Miyamoto, Yutaka
KEK Proceedings 2022-2, p.154 - 158, 2022/11
Precise determination of minor U isotopes (
U and U) of particles from the safeguard environmental samples is powerful method for detecting the undeclared nuclear activities. In this study, preparation method of U particle was examined to utilize for the minor U isotope determination. The porous silica particles were used as the particle matrix and lutetium was mixed to the impregnation solution as U impregnation indicator for the particle picking. The result of the Scanning Electron Microscope indicated that the contacting the solution with Si particles overnight gently could produce the impregnated particles effectively rather than the mixing them with PFA stick.
Tomita, Ryohei; Tomita, Jumpei; Yomogida, Takumi; Suzuki, Daisuke; Yasuda, Kenichiro; Esaka, Fumitaka; Miyamoto, Yutaka
KEK Proceedings 2021-2, p.146 - 150, 2021/12
no abstracts in English
Suzuki, Daisuke; Tomita, Ryohei; Tomita, Jumpei; Esaka, Fumitaka; Yasuda, Kenichiro; Miyamoto, Yutaka
Journal of Radioanalytical and Nuclear Chemistry, 328(1), p.103 - 111, 2021/04
Times Cited Count：3 Percentile：37.09(Chemistry, Analytical)An analytical technique was developed to determine the age of uranium particles for safeguards. After the chemical separation of uranium and thorium, the 
Th/
U ratio was measured using single-collector inductively coupled plasma mass spectrometry and a U-based reference material comprising a certain amount of 
Th as a progeny nuclide of U. The results allowed us to determine the purification age of two certified materials, i.e., U-850 and U-100, which was in good agreement with the reference purification age (61 y). Moreover, the age of a single U-850 particle was determined with a difference of -28 to 2 years from the reference date.
collisions at 
= 200 and 62.4 GeVAdare, A.*; Afanasiev, S.*; Aidala, C.*; Ajitanand, N. N.*; Akiba, Yasuyuki*; Al-Bataineh, H.*; Alexander, J.*; Aoki, Kazuya*; Aphecetche, L.*; Armendariz, R.*; et al.
Physical Review C, 83(6), p.064903_1 - 064903_29, 2011/06
Times Cited Count：189 Percentile：99.42(Physics, Nuclear)Transverse momentum distributions and yields for 
, and 
in collisions at = 200 and 62.4 GeV at midrapidity are measured by the PHENIX experiment at the RHIC. We present the inverse slope parameter, mean transverse momentum, and yield per unit rapidity at each energy, and compare them to other measurements at different collisions. We also present the scaling properties such as 
and 
scaling and discuss the mechanism of the particle production in collisions. The measured spectra are compared to next-to-leading order perturbative QCD calculations.
and Au+Au collisions at 
= 200 GeVAdare, A.*; Afanasiev, S.*; Aidala, C.*; Ajitanand, N. N.*; Akiba, Yasuyuki*; Al-Bataineh, H.*; Alexander, J.*; Aoki, Kazuya*; Aphecetche, L.*; Aramaki, Y.*; et al.
Physical Review C, 83(4), p.044912_1 - 044912_16, 2011/04
Times Cited Count：9 Percentile：52.33(Physics, Nuclear)Measurements of electrons from the decay of open-heavy-flavor mesons have shown that the yields are suppressed in Au+Au collisions compared to expectations from binary-scaled collisions. Here we extend these studies to two particle correlations where one particle is an electron from the decay of a heavy flavor meson and the other is a charged hadron from either the decay of the heavy meson or from jet fragmentation. These measurements provide more detailed information about the interaction between heavy quarks and the quark-gluon matter. We find the away-side-jet shape and yield to be modified in Au+Au collisions compared to collisions.
+ collisions at = 200 GeV and scaling properties of hadron productionAdare, A.*; Afanasiev, S.*; Aidala, C.*; Ajitanand, N. N.*; Akiba, Y.*; Al-Bataineh, H.*; Alexander, J.*; Aoki, K.*; Aphecetche, L.*; Armendariz, R.*; et al.
Physical Review D, 83(5), p.052004_1 - 052004_26, 2011/03
Times Cited Count：180 Percentile：98.41(Astronomy & Astrophysics)The PHENIX experiment at RHIC has measured the invariant differential cross section for production of 
, 
, 
and 
mesons in collisions at = 200 GeV. The spectral shapes of all hadron transverse momentum distributions are well described by a Tsallis distribution functional form with only two parameters, 
and 
, determining the high 
and characterizing the low regions for the spectra, respectively. The integrated invariant cross sections calculated from the fitted distributions are found to be consistent with existing measurements and with statistical model predictions.
Sakuraba, Naotoshi; Numata, Masami; Komiya, Tomokazu; Ichise, Kenichi; Nishi, Masahiro; Tomita, Takeshi; Usami, Koji; Endo, Shinya; Miyata, Seiichi; Kurosawa, Tatsuya; et al.
JAEA-Technology 2009-071, 34 Pages, 2010/03
JAEA-Technology-2009-071.pdf:21.07MB
As a part of maintenance technology of a large-sized glove box for handling of TRU nuclides, we developed replacement technology for front acrylic panels using the bag-in/bag-out method and applied this technology to replace the deteriorated front acrylic panels at Waste Safety Testing Facility (WASTEF) in Nuclear Science Research Institute of Japan Atomic Energy Agency (JAEA). As a consequence, we could safely replace the front acrylic panels under the condition of continuous negative pressure only with partial decontamination of the glove box. We also demonstrated that the present technology is highly effective in points of safety, workability and cost as compared to the usual replacement technology for front acrylic panels of a glove box, where workers in an air-line suit replace directly the front acrylic panels in a green house.
Endo, Shinya; Numata, Masami; Ichise, Kenichi; Nishi, Masahiro; Komiya, Tomokazu; Sakuraba, Naotoshi; Usami, Koji; Tomita, Takeshi
Proceedings of 46th Annual Meeting of "Hot Laboratories and Remote Handling" Working Group (HOTLAB 2009) (CD-ROM), 6 Pages, 2009/09
For safety operation and maintenance of the large size glove box, the degraded acrylic panels of the box must be replaced by the new panels. As the conventional replacement technique, the decontamination of the glove box and installation of isolation tent are necessary to prevent the leak of contamination, because airtight condition of the box is broken down during replacement process. Therefore, the prerequisite works are required considerable manpower. The new replacement technique using bag-in / bag-out method was developed by JAEA. In this technique, for keeping the airtight condition of the box, the inside of degraded panel is covered with an airtight panel and the outside is covered over the large bag which is used to replace the acrylic panels. As the benefits of this technique, the prerequisite works are not required and the manpower is less than a third of the conventional technique.
Hato, Shinji; Terakado, Masato*; Tomita, Kenichi*; Homma, Toshimitsu
JAEA-Data/Code 2008-031, 75 Pages, 2009/03
JAEA-Data-Code-2008-031.pdf:3.73MB
This is the user's manual of DSYS-GUI, which calculates the internal dose coefficients by the models of International Commission on Radiological Protection (ICRP). The DSYS-GUI consists of two programs. One is a program for setting calculation conditions and executing. The other is a program for displaying results to figures and tables. The displaying them are used the Microsoft Excel. Anyone can easily calculate the internal dose coefficients and quickly display results as figures and tables with DSYS-GUI.
Endo, Satoru*; Tomita, Jumpei*; Tanaka, Kenichi*; Yamamoto, Masayoshi*; Fukutani, Satoshi*; Imanaka, Tetsuji*; Sakaguchi, Aya*; Amano, Hikaru; Kawamura, Hidehisa*; Kawamura, Hisao*; et al.
Radiation and Environmental Biophysics, 47(3), p.359 - 365, 2008/07
Times Cited Count：5 Percentile：20.74(Biology)Dolon village located about 60 km from the border of the Semipalatinsk Nuclear Test Site is known to be heavily contaminated by the first USSR atomic bomb test in August 1949. Soil samples around Dolon were taken in October 2005 in an attempt to evaluate internal thyroid dose arising from incorporation of radioiodine isotopes (mainly 
I). Iodine-129 in soil was measured by using the technique of Accelerator Mass Spectrometry. From the relationship between 
I and 
Cs (corrected for background and decay from 1949 to 2005) accumulated levels, the background level of I and the I/Cs ratio around Dolon were estimated to be (6.4 
0.4) 
10
atoms m
and 0.25 0.16, respectively. This I/Cs ratio is almost similar to the fission yield ratio for 
Pu fast fission (0.24).
Homma, Toshimitsu; Matsubara, Takeshi; Tomita, Kenichi*
Proceedings of International Symposium on Environmental Modeling and Radioecology, p.196 - 203, 2007/03
This paper presents the results obtained from the application of OSCAAR to the Iput dose reconstruction scenario of BIOMASS and also to the Chernobyl I fallout scenario of EMRAS, both organized by International Atomic Energy Agency. The Iput Scenario deals with Cs contamination of the catchment basin and agricultural area in the Bryansk Region of Russia, which was heavily contaminated after the Chernobyl accident. This exercise was used to test the chronic exposure pathway models in OSCAAR with actual measurements and to identify the most important sources of uncertainty with respect to each part of the assessment. The OSCAAR chronic exposure pathway models almost successfully reconstructed the whole 10-year time course of Cs activity concentrations in most requested types of agricultural products and natural foodstuffs. The Plavsk scenario provides an good opportunity to test not only the food chain transfer model of I but also the method of assessing I thyroid burden. OSCAAR showed in general good capabilities for assessing the important I exposure pathways, but also limitations using constant isotopic ratio I /Cs provided by the scenario to estimate I deposition for whole Plavsk district.
Homma, Toshimitsu; Tomita, Kenichi*; Hato, Shinji*
Nuclear Engineering and Technology, 37(3), p.245 - 258, 2005/06
This paper addresses two types of uncertainty: stochastic uncertainty and subjective uncertainty in probabilistic accident consequence assessments. The off-site consequence assessment code OSCAAR has been applied to uncertainty and sensitivity analyses on the individual risks of early fatality and latent cancer fatality in the population due to a severe accident. A new stratified meteorological sampling scheme was successfully implemented into the trajectory model for atmospheric dispersion and the statistical variability of the probability distributions of the consequence was examined. A total of 65 uncertain input parameters was considered and 128 runs of OSCAAR were performed in the parameter uncertainty analysis. The study provided the range of uncertainty for the expected values of individual risks of early and latent cancer fatality close to the site. In the sensitivity analyses, the correlation/regression measures were useful for identifying those input parameters whose uncertainty makes an important contribution to the overall uncertainty for the consequence.
Liu, X.*; Tomita, Kenichi*; Homma, Toshimitsu
JAERI-Research 2002-004, 37 Pages, 2002/03
JAERI-Research-2002-004.pdf:2.14MB
One important step in Level 3 Probabilistic Safety Assessment is meteorological sequence sampling, on which the previous studies were mainly related to code systems using straight line plume model and more efforts are needed for trajectory puff model such as the OSCAAR code system. This report describes the development of a new meteorological sampling scheme for the OSCAAR code system that explicitly considers population distribution. A group of principles was set forth for the development of this new sampling scheme, including completeness, stratification, sample allocation, practicability and so on. The calculation results illustrate that although it is quite difficult to idealize stratification of meteorological sequences based on a few environmental parameters the new scheme do gather the most inverse conditions in a single subset of meteorological sequences. The size of this subset may be as small as a few dozens, so that the tail of a CCDF curve is possible to remain relatively static in different trials of the PCA code system.
Homma, Toshimitsu; Ishikawa, Jun; Tomita, Kenichi*; Muramatsu, Ken
JAERI-Research 2000-060, 80 Pages, 2000/12
JAERI-Research-2000-060.pdf:4.49MB
no abstracts in English
Homma, Toshimitsu; Inoue, Yoshihisa*; Tomita, Kenichi*
JAERI-Research 2000-049, 101 Pages, 2000/10
JAERI-Research-2000-049.pdf:3.03MB
no abstracts in English
Homma, Toshimitsu; Liu, X.; Tomita, Kenichi*
Proceedings of 5th International Conference on Probabilistic Safety Assessment and Management (PSAM-5), p.2753 - 2758, 2000/00
no abstracts in English
