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Journal Articles

Impact of fluvial discharge on $$^{137}$$Cs in the ocean following the Fukushima Daiichi Nuclear Power Station accident

Tsumune, Daisuke*; Tsubono, Takaki*; Misumi, Kazuhiro*; Sakuma, Kazuyuki; Onda, Yuichi*

Pure and Applied Chemistry, 16 Pages, 2024/00

 Times Cited Count:0

Twelve years after the Fukushima Daiichi Nuclear Power Station (F1NPS) accident, $$^{137}$$Cs activity concentrations have not yet decreased to pre-accident levels because of direct release from the site and fluvial discharges of $$^{137}$$Cs deposited on land. It is necessary to consider dispersion processes in the coastal area to understand the impact of multiple river discharges and direct release. To achieve this goal, we carried out oceanic dispersion simulations that considered direct release and fluvial discharges and compared the results with the annual averages of observed data. We assumed that particulate $$^{137}$$Cs discharged from rivers to the ocean quickly resuspended and re-leached after coagulation and precipitation and that all of the $$^{137}$$Cs were dispersed. The reproducibility of results was improved by considering fluvial discharges of particulate $$^{137}$$Cs at all sites between 2013 and 2016, except near the F1NPS. In other words, particulate $$^{137}$$Cs discharged from rivers was found to influence the results of ocean surface activity concentrations within a relatively short period of time. The impact of direct release was dominant for the observed $$^{137}$$Cs activity concentrations adjacent to the F1NPS, which was used to estimate direct releases.

Journal Articles

Factors controlling the spatiotemporal variation of $$^{137}$$Cs in seabed sediment off the Fukushima coast; Implications from numerical simulations

Misumi, Kazuhiro*; Tsumune, Daisuke*; Tsubono, Takaki*; Tateda, Yutaka*; Aoyama, Michio*; Kobayashi, Takuya; Hirose, Katsumi*

Journal of Environmental Radioactivity, 136, p.218 - 228, 2014/10

 Times Cited Count:22 Percentile:54.1(Environmental Sciences)

Major controls on spatiotemporal variations of $$^{137}$$Cs activity in seabed sediments derived from the Fukushima Dai-ichi Nuclear Power Plant accident during the first year after the accident were investigated by using numerical simulations. The model successfully reproduced major features of the observed spatiotemporal variations of $$^{137}$$Cs activity in sediments. The spatial pattern of $$^{137}$$Cs in sediments, which mainly reflected the history of $$^{137}$$Cs activity in the bottom water overlying the sediment and the sediment particle size distribution, became established during the first several months after the accident. Taking $$^{137}$$Cs activities in sediments in the coastal area and in the vicinity of the power plant into account, increased the simulated total inventory of $$^{137}$$Cs in sediments off the Fukushima coast to a value on the order of 10$$^{14}$$ Bq.

Journal Articles

Oceanic dispersion simulations of $$^{137}$$Cs released from the Fukushima Daiichi Nuclear Power Plant

Masumoto, Yukio*; Miyazawa, Yasumasa*; Tsumune, Daisuke*; Tsubono, Takaki*; Kobayashi, Takuya; Kawamura, Hideyuki; Estournel, C.*; Marsaleix, P.*; Lanerolle, L.*; Mehra, A.*; et al.

Elements, 8(3), p.207 - 212, 2012/06

 Times Cited Count:82 Percentile:92.24(Geochemistry & Geophysics)

Present status of oceanic dispersion simulations of cesium 137 ($$^{137}$$Cs) directly discharged from Fukushima Daiichi Nuclear Power Plant are reviewed using five model outputs and other available informations, focusing on estimations of discharged amount of $$^{137}$$Cs and subsequent dispersion in a region off Fukushima during March and April, 2011. Common aspects and discrepancies among the simulated results are described. While the discharged amount spreads from about 1 to 27 P Bq of $$^{137}$$Cs among the estimates, the values obtained from the five models indicate 2 to 4 P Bq. With these total amounts and time evolutions of the discharge rate, mimicking observed $$^{137}$$Cs concentration near FDNPP, as a source for the dispersion calculation, all the five models simulated the $$^{137}$$Cs dispersion in the ocean reasonably well corresponding to the observed distributions.

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