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Journal Articles

Radiochemical research for the advancement of $$^{99}$$Mo/$$^{rm 99m}$$Tc generator by (n, $$gamma$$) method, 3

Fujita, Yoshitaka; Seki, Misaki; Namekawa, Yoji*; Nishikata, Kaori; Daigo, Fumihisa; Ide, Hiroshi; Tsuchiya, Kunihiko; Sano, Tadafumi*; Fujihara, Yasuyuki*; Hori, Junichi*; et al.

KURNS Progress Report 2020, P. 136, 2021/08

no abstracts in English

Journal Articles

Effect on $$^{99}$$Mo-adsorption/$$^{99m}$$Tc-elution properties of alumina with different surface structures

Fujita, Yoshitaka; Seki, Misaki; Sano, Tadafumi*; Fujihara, Yasuyuki*; Kitagawa, Tomoya*; Matsukura, Minoru*; Hori, Junichi*; Suzuki, Tatsuya*; Tsuchiya, Kunihiko

Journal of Radioanalytical and Nuclear Chemistry, 327(3), p.1355 - 1363, 2021/03

 Times Cited Count:0 Percentile:0.02(Chemistry, Analytical)

We prepared three types of Al$$_{2}$$O$$_{3}$$ with different surface structures and investigated $$^{99}$$Mo-adsorption/$$^{99m}$$Tc-elution properties using [$$^{99}$$Mo]MoO$$_{3}$$ that was irradiated in the Kyoto University Research Reactor. Al$$_{2}$$O$$_{3}$$ adsorbed [$$^{99}$$Mo]molybdate ions in solutions at different pH; the lower was the pH, the higher was the Mo-adsorption capacity of Al$$_{2}$$O$$_{3}$$. The $$^{99m}$$Tc-elution properties of molybdate ion adsorbed Al$$_{2}$$O$$_{3}$$ were elucidated by flowing saline. Consequently, it was suggested that $$^{99}$$Mo-adsorption/desorption properties are affected by the specific surface of Al$$_{2}$$O$$_{3}$$ and $$^{99m}$$Tc-elution properties are affected by the crystal structure of Al$$_{2}$$O$$_{3}$$.

Journal Articles

Decommissioning of JMTR and study for construction of a new material testing reactor

Kaminaga, Masanori; Kusunoki, Tsuyoshi; Tsuchiya, Kunihiko; Hori, Naohiko; Naka, Michihiro

IAEA-TECDOC-1943, p.45 - 56, 2021/02

The JMTR operation was once stopped in order to have a check & review in August 2006, and the refurbishment and restart of JMTR was finally determined by the national discussion. The refurbishment was started from FY2007, and was finished in March 2011. However, at the end of the FY2010, the Great-Eastern-Japan-Earthquake occurred, and functional tests before the JMTR restart were delayed. On the other hand, based on the safety assessments considering the 2011 earthquake new regulatory requirements have established on Decmber18, 2013 by the NRA. The new regulatory requirements include the satisfaction of integrities for the updated earthquake forces, Tsunami, the consideration of natural phenomena, and the management of consideration in the Beyond Design Basis Accidents (BDBA) to protect fuel damage and to mitigate impact of the accidents. Analyses related to the new regulatory requirements have intensively been performed timely, and an application to the NRA had been submitted in March 27, 2015. After submission of application, seismic resistance assessment of JMTR reactor building was carried out by assuming the standard earthquake ground motion of 810 ga. As the results, it was found that seismic reinforcement work for reactor building and reactor pool wall were required. As a result, it became clear that at least 7 years of reinforcement work period and cost of about 40 billion yen are required for seismic reinforcement and to meet new regulatory standards. At the same time, it was made clear that high availability such as 8 operation cycles per year as originally planned cannot be expected due to aiging problem. For this reason, JAEA positioned JMTR as a decommissioning facility in the mid- and long-term plan of JAEA announced in April 2017. On the other hand, JAEA started to study the construction of a new material testing reactor. The examination results will be compiled by the end of FY2019. In this paper, outline of JMTR decommissioning plan is described.

Journal Articles

Two-step-pressurization method in pulsed electric current sintering of MoO$$_{3}$$ for production of $$^{99m}$$Tc radioactive isotope

Suematsu, Hisayuki*; Sato, Soma*; Nakayama, Tadachika*; Suzuki, Tatsuya*; Niihara, Koichi*; Nanko, Makoto*; Tsuchiya, Kunihiko

Journal of Asian Ceramic Societies (Internet), 8(4), p.1154 - 1161, 2020/12

 Times Cited Count:0 Percentile:0.01(Materials Science, Ceramics)

Pulsed electric current sintering of molybdenum trioxide (MoO$$_{3}$$) was carried out by one- and two-step pressuring methods for fabrication of irradiation target using production of $$^{99}$$Mo and $$^{rm 99m}$$Tc nuclear medicine. At 550$$^{circ}$$C by the two-step pressurizing method, a relative density of 93.1% was obtained while, by the one-step pressurization method, the relative density was 76.9%. Direct sample temperature measurements were conducted by inserting a thermocouple in a punch. By the two-step pressurizing method, the sample temperature was higher than that by the one-step pressurizing method even almost the same die temperature. From voltage and current waveforms, it was thought that the conductivity of the sample increased by the two-step pressurizing method to increase the sample temperature and the relative density. The two-step pressurization method enables us to prepare dense targets at a low temperature from recycled and coarse-grained $$^{98}$$Mo enriched MoO$$_{3}$$ powder.

Journal Articles

Voltage drop analysis and leakage suppression design for mineral-insulated cables

Hirota, Noriaki; Shibata, Hiroshi; Takeuchi, Tomoaki; Otsuka, Noriaki; Tsuchiya, Kunihiko

Journal of Nuclear Science and Technology, 57(12), p.1276 - 1286, 2020/12

 Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)

The influence of materials of mineral-insulated (MI) cables on their electrical characteristics upon exposure to high-temperature conditions was examined via a transmission test, in the objective of achieving the stability of the potential distribution along the cable length. Occurrence of a voltage drop along the cable was confirmed for aluminum oxide (Al$$_{2}$$O$$_{3}$$) and magnesium oxide (MgO), as insulating materials of the MI cable. A finite-element method (FEM)-based analysis was performed to evaluate the leakage in the potentials, which was found at the terminal end. Voltage drop yields by the transmission test and the analysis were in good agreement for the MI cable of Al$$_{2}$$O$$_{3}$$ and MgO materials, which suggests the reproducibility of the magnitude relationship of the experimental results via the FEM analysis. To suppress the voltage drop, the same FEM analysis was conducted, the diameter of the core wires ($$d$$) and the distance between them ($$l$$) were varied. Considering the variation of $$d$$, the potential distribution in the MI cable produced a minimum voltage drop corresponding to a ratio $$d/D$$ of 0.35, obtained by dividing $$d$$ with that of the insulating material ($$D$$). In case of varying $$l$$, a minimum voltage drop was l/$$D$$ of 0.5.

Journal Articles

Development of the treatment method for difficult wastes aimed at decommissioning of JMTR; Structural materials of reactor and used ion-exchange resins

Seki, Misaki; Nakano, Hiroko; Nagata, Hiroshi; Otsuka, Kaoru; Omori, Takazumi; Takeuchi, Tomoaki; Ide, Hiroshi; Tsuchiya, Kunihiko

Dekomisshoningu Giho, (62), p.9 - 19, 2020/09

Japan Materials Testing Reactor (JMTR) has been contributing to various research and development activities such as the fundamental research of nuclear materials/fuels, safety research and development of power reactors, and radioisotope production since the beginning of the operation in 1968. JMTR, however, was decided as a one of decommission facilities in April 2017 and it is taken an inspection of a plan concerning decommissioning because the performance of JMTR does not confirm with the stipulated earthquake resistance. As aluminum and beryllium are used for the core structural materials in JMTR, it is necessary to establish treatment methods of these materials for the fabrication of stable wastes. In addition, a treatment method for the accumulated spent ion-exchange resins needs to be examined. This report describes the overview of these examination situations.

Journal Articles

Research on activation assessment of a reactor structural materials for decommissioning, 2

Seki, Misaki; Ishikawa, Koji*; Sano, Tadafumi*; Nagata, Hiroshi; Otsuka, Kaoru; Omori, Takazumi; Hanakawa, Hiroki; Ide, Hiroshi; Tsuchiya, Kunihiko; Fujihara, Yasuyuki*; et al.

KURNS Progress Report 2019, P. 279, 2020/08

no abstracts in English

Journal Articles

Radiochemical research for the advancement of $$^{99}$$Mo/$$^{rm 99m}$$Tc generator by (n,$$gamma$$) method, 2

Fujita, Yoshitaka; Seki, Misaki; Namekawa, Yoji*; Nishikata, Kaori; Kato, Yoshiaki; Sayato, Natsuki; Tsuchiya, Kunihiko; Sano, Tadafumi*; Fujihara, Yasuyuki*; Hori, Junichi*; et al.

KURNS Progress Report 2019, P. 157, 2020/08

no abstracts in English

Journal Articles

Research on activation assessment of a reactor structural materials for decommissioning

Seki, Misaki; Ishikawa, Koji*; Nagata, Hiroshi; Otsuka, Kaoru; Omori, Takazumi; Hanakawa, Hiroki; Ide, Hiroshi; Tsuchiya, Kunihiko; Sano, Tadafumi*; Fujihara, Yasuyuki*; et al.

KURNS Progress Report 2018, P. 257, 2019/08

no abstracts in English

Journal Articles

Radiochemical research for the advancement of $$^{99}$$Mo/$$^{rm 99m}$$Tc generator by (n,$$gamma$$) method

Fujita, Yoshitaka; Seki, Misaki; Namekawa, Yoji*; Nishikata, Kaori; Kimura, Akihiro; Shibata, Akira; Sayato, Natsuki; Tsuchiya, Kunihiko; Sano, Tadafumi*; Fujihara, Yasuyuki*; et al.

KURNS Progress Report 2018, P. 155, 2019/08

no abstracts in English

Journal Articles

Development of radiation resistant monitoring system in light water reactor

Takeuchi, Tomoaki; Otsuka, Noriaki; Nakano, Hiroko; Iida, Tatsuya*; Ozawa, Osamu*; Shibagaki, Taro*; Komanome, Hirohisa*; Tsuchiya, Kunihiko

QST-M-16; QST Takasaki Annual Report 2017, P. 67, 2019/03

no abstracts in English

Journal Articles

Status of JMTR decommissioning plan formulation, 2

Otsuka, Kaoru; Ide, Hiroshi; Nagata, Hiroshi; Omori, Takazumi; Seki, Misaki; Hanakawa, Hiroki; Nemoto, Hiroyoshi; Watanabe, Masao; Iimura, Koichi; Tsuchiya, Kunihiko; et al.

UTNL-R-0499, p.12_1 - 12_8, 2019/03

no abstracts in English

Journal Articles

Preliminary analysis for demolition of secondary cooling system and pool canal cycling system secondary piping

Hanakawa, Hiroki; Kawamata, Takanori; Ogasawara, Yasushi; Otsuka, Kaoru; Omori, Takazumi; Ide, Hiroshi; Tsuchiya, Kunihiko

UTNL-R-0499, p.11_1 - 11_7, 2019/03

no abstracts in English

Journal Articles

Development of novel alumina adsorbent applying mesoporous process

Fukumitsu, Nobuyoshi*; Yamauchi, Yusuke*; Saptiama, I.*; Ariga, Katsuhiko*; Hatano, Kentaro*; Kumada, Hiroaki*; Fujita, Yoshitaka; Tsuchiya, Kunihiko

Isotope News, (760), p.15 - 18, 2018/12

no abstracts in English

Journal Articles

Development of radiation resistant monitoring camera system

Takeuchi, Tomoaki; Otsuka, Noriaki; Watanabe, Takashi*; Tanaka, Shigeo*; Ozawa, Osamu*; Komanome, Hirohisa*; Ueno, Shunji*; Tsuchiya, Kunihiko

Proceedings of 2017 IEEE Nuclear Science Symposium and Medical Imaging Conference (NSS/MIC 2017) (Internet), 3 Pages, 2018/11

no abstracts in English

Journal Articles

Evaluation of in-water wireless transmission system under the conditions simulated the severe accident

Otsuka, Noriaki; Takeuchi, Tomoaki; Tsuchiya, Kunihiko; Shibagaki, Taro*; Komanome, Hirohisa*

Proceedings of 2017 IEEE Nuclear Science Symposium and Medical Imaging Conference (NSS/MIC 2017) (Internet), 3 Pages, 2018/11

no abstracts in English

Journal Articles

Neutron irradiation effect of high-density MoO$$_{3}$$ pellets for Mo-99 production

Fujita, Yoshitaka; Nishikata, Kaori; Namekawa, Yoji*; Kimura, Akihiro; Shibata, Akira; Sayato, Natsuki; Tsuchiya, Kunihiko; Sano, Tadafumi*; Fujihara, Yasuyuki*; Zhang, J.*

KURRI Progress Report 2017, P. 126, 2018/08

no abstracts in English

Journal Articles

Template-free fabrication of mesoporous alumina nanospheres using post-synthesis water-ethanol treatment of monodispersed aluminium glycerate nanospheres for molybdenum adsorption

Saptiama, I.*; Kaneti, Y. V.*; Suzuki, Yoshitaka; Tsuchiya, Kunihiko; Fukumitsu, Nobuyoshi*; Sakae, Takeji*; Kim, J.*; Kang, Y.-M.*; Ariga, Katsuhiko*; Yamauchi, Yusuke*

Small, 14(21), p.1800474_1 - 1800474_14, 2018/05

 Times Cited Count:32 Percentile:90(Chemistry, Multidisciplinary)

no abstracts in English

Journal Articles

High-temperature oxidation of sheath materials using mineral-insulated cables for a simulated severe accident

Nakano, Hiroko; Hirota, Noriaki; Shibata, Hiroshi; Takeuchi, Tomoaki; Tsuchiya, Kunihiko

Mechanical Engineering Journal (Internet), 5(2), p.17-00594_1 - 17-00594_12, 2018/04

no abstracts in English

Journal Articles

Molybdenum adsorption and desorption properties of alumina with different surface structures for $$^{99}$$Mo/$$^{99m}$$Tc generators

Suzuki, Yoshitaka; Kitagawa, Tomoya*; Namekawa, Yoji*; Matsukura, Minoru*; Nishikata, Kaori; Mimura, Hitoshi*; Tsuchiya, Kunihiko

Transactions of the Materials Research Society of Japan, 43(2), p.75 - 80, 2018/04

no abstracts in English

368 (Records 1-20 displayed on this page)