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Journal Articles

Two-step-pressurization method in pulsed electric current sintering of MoO$$_{3}$$ for production of $$^{99m}$$Tc radioactive isotope

Suematsu, Hisayuki*; Sato, Soma*; Nakayama, Tadachika*; Suzuki, Tatsuya*; Niihara, Koichi*; Nanko, Makoto*; Tsuchiya, Kunihiko

Journal of Asian Ceramic Societies (Internet), 8(4), p.1154 - 1161, 2020/12

 Times Cited Count:0 Percentile:100(Materials Science, Ceramics)

Pulsed electric current sintering of molybdenum trioxide (MoO$$_{3}$$) was carried out by one- and two-step pressuring methods for fabrication of irradiation target using production of $$^{99}$$Mo and $$^{rm 99m}$$Tc nuclear medicine. At 550$$^{circ}$$C by the two-step pressurizing method, a relative density of 93.1% was obtained while, by the one-step pressurization method, the relative density was 76.9%. Direct sample temperature measurements were conducted by inserting a thermocouple in a punch. By the two-step pressurizing method, the sample temperature was higher than that by the one-step pressurizing method even almost the same die temperature. From voltage and current waveforms, it was thought that the conductivity of the sample increased by the two-step pressurizing method to increase the sample temperature and the relative density. The two-step pressurization method enables us to prepare dense targets at a low temperature from recycled and coarse-grained $$^{98}$$Mo enriched MoO$$_{3}$$ powder.

Journal Articles

Voltage drop analysis and leakage suppression design for mineral-insulated cables

Hirota, Noriaki; Shibata, Hiroshi; Takeuchi, Tomoaki; Otsuka, Noriaki; Tsuchiya, Kunihiko

Journal of Nuclear Science and Technology, 57(12), p.1276 - 1286, 2020/12

 Times Cited Count:0 Percentile:100(Nuclear Science & Technology)

The influence of materials of mineral-insulated (MI) cables on their electrical characteristics upon exposure to high-temperature conditions was examined via a transmission test, in the objective of achieving the stability of the potential distribution along the cable length. Occurrence of a voltage drop along the cable was confirmed for aluminum oxide (Al$$_{2}$$O$$_{3}$$) and magnesium oxide (MgO), as insulating materials of the MI cable. A finite-element method (FEM)-based analysis was performed to evaluate the leakage in the potentials, which was found at the terminal end. Voltage drop yields by the transmission test and the analysis were in good agreement for the MI cable of Al$$_{2}$$O$$_{3}$$ and MgO materials, which suggests the reproducibility of the magnitude relationship of the experimental results via the FEM analysis. To suppress the voltage drop, the same FEM analysis was conducted, the diameter of the core wires ($$d$$) and the distance between them ($$l$$) were varied. Considering the variation of $$d$$, the potential distribution in the MI cable produced a minimum voltage drop corresponding to a ratio $$d/D$$ of 0.35, obtained by dividing $$d$$ with that of the insulating material ($$D$$). In case of varying $$l$$, a minimum voltage drop was l/$$D$$ of 0.5.

Journal Articles

Development of the treatment method for difficult wastes aimed at decommissioning of JMTR; Structural materials of reactor and used ion-exchange resins

Seki, Misaki; Nakano, Hiroko; Nagata, Hiroshi; Otsuka, Kaoru; Omori, Takazumi; Takeuchi, Tomoaki; Ide, Hiroshi; Tsuchiya, Kunihiko

Dekomisshoningu Giho, (62), p.9 - 19, 2020/09

Japan Materials Testing Reactor (JMTR) has been contributing to various research and development activities such as the fundamental research of nuclear materials/fuels, safety research and development of power reactors, and radioisotope production since the beginning of the operation in 1968. JMTR, however, was decided as a one of decommission facilities in April 2017 and it is taken an inspection of a plan concerning decommissioning because the performance of JMTR does not confirm with the stipulated earthquake resistance. As aluminum and beryllium are used for the core structural materials in JMTR, it is necessary to establish treatment methods of these materials for the fabrication of stable wastes. In addition, a treatment method for the accumulated spent ion-exchange resins needs to be examined. This report describes the overview of these examination situations.

Journal Articles

Research on activation assessment of a reactor structural materials for decommissioning, 2

Seki, Misaki; Ishikawa, Koji*; Sano, Tadafumi*; Nagata, Hiroshi; Otsuka, Kaoru; Omori, Takazumi; Hanakawa, Hiroki; Ide, Hiroshi; Tsuchiya, Kunihiko; Fujihara, Yasuyuki*; et al.

KURNS Progress Report 2019, P. 279, 2020/08

no abstracts in English

Journal Articles

Radiochemical research for the advancement of $$^{99}$$Mo/$$^{rm 99m}$$Tc generator by (n,$$gamma$$) method, 2

Fujita, Yoshitaka; Seki, Misaki; Namekawa, Yoji*; Nishikata, Kaori; Kato, Yoshiaki; Sayato, Natsuki; Tsuchiya, Kunihiko; Sano, Tadafumi*; Fujihara, Yasuyuki*; Hori, Junichi*; et al.

KURNS Progress Report 2019, P. 157, 2020/08

no abstracts in English

Journal Articles

Research on activation assessment of a reactor structural materials for decommissioning

Seki, Misaki; Ishikawa, Koji*; Nagata, Hiroshi; Otsuka, Kaoru; Omori, Takazumi; Hanakawa, Hiroki; Ide, Hiroshi; Tsuchiya, Kunihiko; Sano, Tadafumi*; Fujihara, Yasuyuki*; et al.

KURNS Progress Report 2018, P. 257, 2019/08

no abstracts in English

Journal Articles

Radiochemical research for the advancement of $$^{99}$$Mo/$$^{rm 99m}$$Tc generator by (n,$$gamma$$) method

Fujita, Yoshitaka; Seki, Misaki; Namekawa, Yoji*; Nishikata, Kaori; Kimura, Akihiro; Shibata, Akira; Sayato, Natsuki; Tsuchiya, Kunihiko; Sano, Tadafumi*; Fujihara, Yasuyuki*; et al.

KURNS Progress Report 2018, P. 155, 2019/08

no abstracts in English

Journal Articles

Development of radiation resistant monitoring system in light water reactor

Takeuchi, Tomoaki; Otsuka, Noriaki; Nakano, Hiroko; Iida, Tatsuya*; Ozawa, Osamu*; Shibagaki, Taro*; Komanome, Hirohisa*; Tsuchiya, Kunihiko

QST-M-16; QST Takasaki Annual Report 2017, P. 67, 2019/03

no abstracts in English

Journal Articles

Status of JMTR decommissioning plan formulation, 2

Otsuka, Kaoru; Ide, Hiroshi; Nagata, Hiroshi; Omori, Takazumi; Seki, Misaki; Hanakawa, Hiroki; Nemoto, Hiroyoshi; Watanabe, Masao; Iimura, Koichi; Tsuchiya, Kunihiko; et al.

UTNL-R-0499, p.12_1 - 12_8, 2019/03

no abstracts in English

Journal Articles

Preliminary analysis for demolition of secondary cooling system and pool canal cycling system secondary piping

Hanakawa, Hiroki; Kawamata, Takanori; Ogasawara, Yasushi; Otsuka, Kaoru; Omori, Takazumi; Ide, Hiroshi; Tsuchiya, Kunihiko

UTNL-R-0499, p.11_1 - 11_7, 2019/03

no abstracts in English

Journal Articles

Development of novel alumina adsorbent applying mesoporous process

Fukumitsu, Nobuyoshi*; Yamauchi, Yusuke*; Saptiama, I.*; Ariga, Katsuhiko*; Hatano, Kentaro*; Kumada, Hiroaki*; Fujita, Yoshitaka; Tsuchiya, Kunihiko

Isotope News, (760), p.15 - 18, 2018/12

no abstracts in English

Journal Articles

Development of radiation resistant monitoring camera system

Takeuchi, Tomoaki; Otsuka, Noriaki; Watanabe, Takashi*; Tanaka, Shigeo*; Ozawa, Osamu*; Komanome, Hirohisa*; Ueno, Shunji*; Tsuchiya, Kunihiko

Proceedings of 2017 IEEE Nuclear Science Symposium and Medical Imaging Conference (NSS/MIC 2017) (Internet), 3 Pages, 2018/11

no abstracts in English

Journal Articles

Evaluation of in-water wireless transmission system under the conditions simulated the severe accident

Otsuka, Noriaki; Takeuchi, Tomoaki; Tsuchiya, Kunihiko; Shibagaki, Taro*; Komanome, Hirohisa*

Proceedings of 2017 IEEE Nuclear Science Symposium and Medical Imaging Conference (NSS/MIC 2017) (Internet), 3 Pages, 2018/11

no abstracts in English

Journal Articles

Neutron irradiation effect of high-density MoO$$_{3}$$ pellets for Mo-99 production

Fujita, Yoshitaka; Nishikata, Kaori; Namekawa, Yoji*; Kimura, Akihiro; Shibata, Akira; Sayato, Natsuki; Tsuchiya, Kunihiko; Sano, Tadafumi*; Fujihara, Yasuyuki*; Zhang, J.*

KURRI Progress Report 2017, P. 126, 2018/08

no abstracts in English

Journal Articles

Template-free fabrication of mesoporous alumina nanospheres using post-synthesis water-ethanol treatment of monodispersed aluminium glycerate nanospheres for molybdenum adsorption

Saptiama, I.*; Kaneti, Y. V.*; Suzuki, Yoshitaka; Tsuchiya, Kunihiko; Fukumitsu, Nobuyoshi*; Sakae, Takeji*; Kim, J.*; Kang, Y.-M.*; Ariga, Katsuhiko*; Yamauchi, Yusuke*

Small, 14(21), p.1800474_1 - 1800474_14, 2018/05

 Times Cited Count:18 Percentile:12.49(Chemistry, Multidisciplinary)

no abstracts in English

Journal Articles

High-temperature oxidation of sheath materials using mineral-insulated cables for a simulated severe accident

Nakano, Hiroko; Hirota, Noriaki; Shibata, Hiroshi; Takeuchi, Tomoaki; Tsuchiya, Kunihiko

Mechanical Engineering Journal (Internet), 5(2), p.17-00594_1 - 17-00594_12, 2018/04

no abstracts in English

Journal Articles

Molybdenum adsorption and desorption properties of alumina with different surface structures for $$^{99}$$Mo/$$^{99m}$$Tc generators

Suzuki, Yoshitaka; Kitagawa, Tomoya*; Namekawa, Yoji*; Matsukura, Minoru*; Nishikata, Kaori; Mimura, Hitoshi*; Tsuchiya, Kunihiko

Transactions of the Materials Research Society of Japan, 43(2), p.75 - 80, 2018/04

no abstracts in English

Journal Articles

Status of JMTR decommissioning plan formulation

Otsuka, kaoru; Hanakawa, Hiroki; Nagata, Hiroshi; Omori, Takazumi; Takeuchi, Tomoaki; Tsuchiya, Kunihiko

UTNL-R-0496, p.13_1 - 13_11, 2018/03

no abstracts in English

JAEA Reports

Degradation behavior of optical components by gamma irradiation (Contract research)

Takeuchi, Tomoaki; Shibata, Hiroshi; Hanakawa, Hiroki; Uehara, Toshiaki*; Ueno, Shunji*; Tsuchiya, Kunihiko; Kumahara, Hajime*; Shibagaki, Taro*; Komanome, Hirohisa*

JAEA-Technology 2017-026, 26 Pages, 2018/02

JAEA-Technology-2017-026.pdf:4.0MB

Under severe accidents, high-integrity transmission techniques are necessary so as to monitor the situation of the nuclear power plant. In this study, effects of gamma irradiation up to 10$$^{6}$$Gy on properties of optical devices were evaluated toward the development of a radiation-resistant in-water wireless transmission system using visible light. After the irradiation, for the LEDs, the total luminous flux decreased and the browning of resin lenses occurred. Meanwhile, the current-voltage characteristics hardly changed. For the PDs, the light sensitivity decreased and the browning of resin window occurred. The dark currents of PDs did not become large enough to adversely affect transmission. These results indicated that both the decreases of the total luminous flux of the LEDs and the light sensitivity of the PDs were mainly caused by not the degradation of the semiconductor parts but the browning of the resin parts by the irradiation. In addition, basic decrease behaviors of light transmission of several different types of glasses by gamma irradiation were also obtained so as to select the suitable optical windows and filters for the developing radiation-resistant in-water wireless transmission system.

Journal Articles

Molybdenum adsorption properties of alumina-embedded mesoporous silica for medical radioisotope production

Saptiama, I.*; Kaneti, Y. V.*; Oveisi, H.*; Suzuki, Yoshitaka; Tsuchiya, Kunihiko; Takai, Kimiko*; Sakae, Takeji*; Pradhan, S.*; Hossain, M. S. A.*; Fukumitsu, Nobuyoshi*; et al.

Bulletin of the Chemical Society of Japan, 91(2), p.195 - 200, 2018/02

 Times Cited Count:31 Percentile:7.8(Chemistry, Multidisciplinary)

no abstracts in English

364 (Records 1-20 displayed on this page)