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Journal Articles

Downward terrestrial gamma-ray flash associated with collision of lightning leaders

Wada, Yuki*; Morimoto, Takeshi*; Wu, T.*; Wang, D.*; Kikuchi, Hiroshi*; Nakamura, Yoshitaka*; Yoshikawa, Eiichi*; Ushio, Tomoo*; Tsuchiya, Harufumi

Science Advances (Internet), 11(21), p.eads6906_1 - eads6906_10, 2025/05

 Times Cited Count:0

Journal Articles

Novel approach to explore hydrogen trapping sites in aluminum; Integrating Muon spin relaxation with first-principles calculations

Shimizu, Kazuyuki*; Nishimura, Katsuhiko*; Matsuda, Kenji*; Nunomura, Norio*; Namiki, Takahiro*; Tsuchiya, Taiki*; Akamaru, Satoshi*; Lee, S.*; Tsuru, Tomohito; Higemoto, Wataru; et al.

International Journal of Hydrogen Energy, 95, p.292 - 299, 2024/12

 Times Cited Count:1 Percentile:31.33(Chemistry, Physical)

Zero-field muon spin relaxation experiments were conducted on Al-0.06%Mn, Al-0.06%Cr, Al-0.02%Fe, and Al-0.02%Ni alloys (at.%) across the temperature ranging from 5 to 300 K. The temperature-dependent variations of the dipole field widths ($$Delta$$) elucidated four distinct peaks for the prepared alloys. Atomic configurations of the muon trapping sites corresponding to the observed $$Delta$$ peaks below 200 K were meticulously characterized utilizing first-principles calculations for the trapping energies of hydrogen in proximity to a solute and solute-vacancy pair. This comprehensive analysis facilitated the establishment of a linear correlation between the muon $$Delta$$ peak temperature and the hydrogen trapping energy. However, significant deviations from this linear relationship were observed for the fourth $$Delta$$ peaks above 200 K in Al-Mn, Al-Cr, Al-Fe, and Al-Ni alloys. This discrepancy can be interpreted by considering the disparate distribution functions of muon and hydrogen within the tetrahedral site, wherein two of the four Al atoms are substituted by the solute element and vacancy (solute-vacancy pair).

Journal Articles

Extraordinary $$^{99}$$Mo adsorption; Utilizing spray-dried mesoporous alumina for clinical-grade generator development

Alowasheeir, A.*; Eguchi, Miharu*; Fujita, Yoshitaka; Tsuchiya, Kunihiko; Wakabayashi, Ryutaro*; Kimura, Tatsuo*; Ariga, Katsuhiko*; Hatano, Kentaro*; Fukumitsu, Nobuyoshi*; Yamauchi, Yusuke*

Bulletin of the Chemical Society of Japan, 97(10), p.uoae099_1 - uoae099_7, 2024/10

 Times Cited Count:3 Percentile:37.20(Chemistry, Multidisciplinary)

no abstracts in English

Journal Articles

Morphology evolution of $$beta$$-phase in Al-Mg-Si alloys during aging treatment

Ahmed, A.*; Uttarasak, K.*; Tsuchiya, Taiki*; Lee, S.*; Nishimura, Katsuhiko*; Nunomura, Norio*; Shimizu, Kazuyuki*; Hirayama, Kyosuke*; Toda, Hiroyuki*; Yamaguchi, Masatake; et al.

Journal of Alloys and Compounds, 988, p.174234_1 - 174234_9, 2024/06

 Times Cited Count:10 Percentile:96.31(Chemistry, Physical)

This study aims to clarify the growth process of the$$beta$$-phase in Al-Mg-Si alloys from the point of view of morphology evolution. For this research, the $$beta$$-phase orientation relationship, shape, growth process, misfit value, and interfacial condition between the $$beta$$-phase and Al matrix were investigated using high-resolution transmission electron microscopy (HR-TEM), focus ion beam (FIB), and optical microscope (OM). Results include the identification of {111} $$beta$$ facets at the edges of the $$beta$$-phase, as well as the proposal of two new three-dimensional shapes for the $$beta$$-phase. We purposed the morphology evolution during the growth process of Mg$$_2$$Si crystal and calculated the misfit to understand the unstable (111)$$beta$$ facet has a higher misfit value as compared to the (001)$$beta$$ and (011)$$beta$$ facets. Our observations provide how they influence the behavior of Mg$$_2$$Si crystals.

Journal Articles

Nuclear quantum effect on the elasticity of ice VII under pressure; A Path-integral molecular dynamics study

Tsuchiya, Jun*; Shiga, Motoyuki; Tsuneyuki, Shinji*; Thompson, E. C.*

Physical Review Research (Internet), 6(2), p.023302_1 - 023302_6, 2024/06

We investigate the effect of nuclear quantum effects (NQEs) of hydrogen atoms on the elasticity of ice VII at high pressure and ambient temperature conditions using ab initio path-integral molecular dynamics (PIMD) calculations. We find that the NQEs of hydrogen contributes to the transition of ice VII from a static disordered structure to a dynamically disordered structure at pressures exceeding 40 GPa. This transition is marked by a discontinuous increase of the elastic constants. Comparison of ${it ab initio}$ molecular dynamics and PIMD calculations reveal that NQEs increase the elastic constants of ice by about 20% at 70 GPa and 300 K.

Journal Articles

Combining muon spin relaxation and DFT simulations of hydrogen trapping in Al$$_{6}$$Mn

Shimizu, Kazuyuki*; Nishimura, Katsuhiko*; Matsuda, Kenji*; Akamaru, Satoshi*; Nunomura, Norio*; Namiki, Takahiro*; Tsuchiya, Taiki*; Lee, S.*; Higemoto, Wataru; Tsuru, Tomohito; et al.

Scripta Materialia, 245, p.116051_1 - 116051_6, 2024/05

 Times Cited Count:2 Percentile:63.37(Nanoscience & Nanotechnology)

Hydrogen at the mass ppm level causes hydrogen embrittlement in metallic materials, but it is extremely difficult to experimentally elucidate the hydrogen trapping sites. We have taken advantage of the fact that positive muons can act as light isotopes of hydrogen to study the trapping state of hydrogen in matter. Zero-field muon spin relaxation experiments and the density functional theory (DFT) calculations for hydrogen trapping energy are carried out for Al$$_{6}$$Mn. The DFT calculations for hydrogen in Al$$_{6}$$Mn have found four possible trapping sites in which the hydrogen trapping energies are 0.168 (site 1), 0.312 (site 2), 0.364 (site 3), and 0.495 (site 4) in the unit of eV/atom. Temperature variations of the deduced dipole field width ($$Delta$$) indicated step-like changes at temperatures, 94, 193, and 236 K. Considering their site densities, the observed $$Delta$$ change temperatures are interpreted by trapping muons at sites 1, 3, and 4.

Journal Articles

Characterization of mineral insulated cables at the WWR-K reactor; First results

Shaimerdenov, A.*; Gizatulin, Sh.*; Sairanbayev, D.*; Bugybay, Zh.*; Silnyagin, P.*; Akhanov, A.*; Fuyushima, Takumi; Hirota, Noriaki; Tsuchiya, Kunihiko

Nuclear Instruments and Methods in Physics Research B, 548, p.165235_1 - 165235_6, 2024/03

 Times Cited Count:1 Percentile:58.81(Instruments & Instrumentation)

Compared to conditions in other types of installations, cable insulation in nuclear reactors is exposed to mixed conditions (high temperatures, radiation, pressure, humidity, aggressive environments) and at the same time they must maintain their performance characteristics for a long time (about 40-50 years). As a result of irradiation to such conditions, the electrical properties of the cable insulation are degraded, which leads to an increase in current loss. This is because the charge is induced by radiation into the insulator. At the WWR-K reactor, studies were started on the radiation resistance of signal cables with two types of mineral insulation (MgO and Al$$_{2}$$O$$_{3}$$). As part of these studies, new experimental data will be obtained on the behavior of signal cables with mineral insulation of two types in mixed operating conditions (radiation field and high temperature). It is planned to accumulate fluence of fast neutrons $$sim$$ 10$$^{20}$$cm$$^{-2}$$ in cables. The irradiation temperature will be (500 $$pm$$ 50)$$^{circ}$$C). The study of the degradation of the electrical properties of the insulation of signal cables will be carried out in real time (in-situ). For this, a special design of the experimental device and a technique for in-reactor measurement of electrical characteristics were developed. This paper presents a sketch of the capsule design, the results of complex calculations for the development of the capsule design, the expected neutron fluences, the dpa in steel, the technique for in-reactor measurement of electrical characteristics, and a work plan for the future indicating the expected results. The cable irradiation time until the target neutron fluence is reached will be about 100 effective days. This research is funded by the International Scientific-Technical Center.

Journal Articles

Low reactivity of stoichiometric FeS with hydrogen at high-pressure and high-temperature conditions

Takano, Masahiro*; Kagi, Hiroyuki*; Mori, Yuichiro*; Aoki, Katsutoshi*; Kakizawa, Sho*; Sano, Asami; Iizuka-Oku, Riko*; Tsuchiya, Taku*

Journal of Mineralogical and Petrological Sciences (Internet), 119(1), p.240122_1 - 240122_9, 2024/00

 Times Cited Count:0 Percentile:0.00(Mineralogy)

Hydrogenation of iron sulfide (FeS) under high-pressure and high-temperature conditions has attracted attention because hydrogen and sulfur are promising candidates as light elements in the cores of the Earth and other terrestrial planets. In earlier reports describing the hydrogenation of FeS, the chemical compositions of starting materials were not fully clarified. This study reports in-situ neutron and X-ray diffraction measurements under high-pressure and high-temperature conditions of an Fe-S-H system using a stochiometric Fe1.000S (troilite) as a starting material. The occupancies determined were significantly lower than those reported from earlier studies, indicating that the hydrogenation of FeS can be affected strongly by the stoichiometry of iron sulfide.

Journal Articles

Negative excursion of surface electric fields during gamma-ray glows in winter thunderstorms

Wada, Yuki*; Kamogawa, Masashi*; Kubo, Mamoru*; Enoto, Teruaki*; Hayashi, Shugo*; Sawano, Tatsuya*; Yonetoku, Daisuke*; Tsuchiya, Harufumi

Journal of Geophysical Research; Atmospheres, 128(21), p.e2023JD039354_1 - e2023JD039354_20, 2023/11

 Times Cited Count:1 Percentile:13.75(Meteorology & Atmospheric Sciences)

Journal Articles

Termination of downward-oriented gamma-ray glow by normal-polarity in-cloud discharge activity

Wada, Yuki*; Wu, T.*; Wang, D.*; Enoto, Teruaki*; Nakazawa, Kazuhiro*; Morimoto, Takeshi*; Nakamura, Yoshitaka*; Shinoda, Taro*; Tsuchiya, Harufumi

Journal of Geophysical Research; Atmospheres, 128(15), p.e2023JD038606_1 - e2023JD038606_9, 2023/08

 Times Cited Count:3 Percentile:40.74(Meteorology & Atmospheric Sciences)

Journal Articles

Citizen science observation of a gamma-ray glow associated with the initiation of a lightning flash

Tsurumi, Miwa*; Enoto, Teruaki*; Ikkatai, Yuko*; Wu, T.*; Wang, D.*; Shinoda, Taro*; Nakazawa, Kazuhiro*; Tsuji, Naoki*; Diniz, G.*; Kataoka, Jun*; et al.

Geophysical Research Letters, 50(13), p.e2023GL103612_1 - e2023GL103612_9, 2023/07

 Times Cited Count:7 Percentile:68.56(Geosciences, Multidisciplinary)

Journal Articles

Development of stabilization treatment technology for radioactive aluminum waste

Seki, Misaki; Fujita, Yoshitaka; Fujihara, Yasuyuki*; Zhang, J.*; Yoshinaga, Hisao*; Sano, Tadafumi*; Hori, Junichi*; Nagata, Hiroshi; Otsuka, Kaoru; Omori, Takazumi; et al.

Genshiryoku Bakkuendo Kenkyu (CD-ROM), 29(1), p.2 - 9, 2022/06

no abstracts in English

Journal Articles

Mechanisms responsible for adsorption of molybdate ions on alumina for the production of medical radioisotopes

Fujita, Yoshitaka; Niizeki, Tomotake*; Fukumitsu, Nobuyoshi*; Ariga, Katsuhiko*; Yamauchi, Yusuke*; Malgras, V.*; Kaneti, Y. V.*; Liu, C.-H.*; Hatano, Kentaro*; Suematsu, Hisayuki*; et al.

Bulletin of the Chemical Society of Japan, 95(1), p.129 - 137, 2022/01

 Times Cited Count:10 Percentile:61.73(Chemistry, Multidisciplinary)

In this work, the mechanisms responsible for the adsorption of molybdate ions on alumina are investigated using in-depth surface analyses carried out on alumina specimens immersed in solutions containing different molybdate ions at different pH values. The obtained results reveal that when alumina is immersed in an acidic solution containing molybdate ions, the hydroxyl groups present on the surface are removed to generate positively charged sites, and molybdate ions (MoO$$_{4}$$$$^{2-}$$ or AlMo$$_{6}$$O$$_{24}$$H$$_{6}$$$$^{3-}$$) are adsorbed by electrostatic interaction. Alumina dissolves slightly in an acidic solution to form AlMo$$_{6}$$O$$_{24}$$H$$_{6}$$$$^{3-}$$, which is more easily desorbed than MoO$$_{4}$$$$^{2-}$$. Furthermore, the enhancement in the Mo adsorption or desorption property may be achieved by enriching the surface of the alumina adsorbent with many -OH groups and optimizing Mo solution to adsorb molybdate ions on alumina as MoO$$_{4}$$$$^{2-}$$ ions. These findings will assist researchers in engineering more efficient and stable alumina-based adsorbents for molybdenum adsorption used in medical radioisotope ($$^{99}$$Mo/$$^{99m}$$Tc) generators.

Journal Articles

Dynamic properties on $$^{99}$$Mo adsorption and $$^{rm 99m}$$Tc elution with alumina columns

Fujita, Yoshitaka; Seki, Misaki; Sano, Tadafumi*; Fujihara, Yasuyuki*; Suzuki, Tatsuya*; Yoshinaga, Hisao*; Hori, Junichi*; Suematsu, Hisayuki*; Tsuchiya, Kunihiko

Journal of Physics; Conference Series, 2155, p.012018_1 - 012018_6, 2022/01

BB2021-0617.pdf:0.77MB

Technetium-99m ($$^{rm 99m}$$Tc), the daughter nuclide of Molybdenum-99 ($$^{99}$$Mo), is the most commonly used radioisotope in radiopharmaceuticals. The research and development (R&D) for the production of $$^{99}$$Mo by the neutron activation method ((n, $$gamma$$) method) has been carried out from viewpoints of no-proliferation and nuclear security, etc. Since the specific activity of $$^{99}$$Mo produced by the (n, $$gamma$$) method is extremely low, developing Al$$_{2}$$O$$_{3}$$ with a large Mo adsorption capacity is necessary to adapt (n, $$gamma$$)$$^{99}$$Mo to the generator. In this study, three kinds of Al$$_{2}$$O$$_{3}$$ specimens with different raw materials were prepared and compared their adaptability to generators by static and dynamic adsorption. MoO$$_{3}$$ pellet pieces (1.5g) were irradiated with 5 MW for 20 min in the Kyoto University Research Reactor (KUR). Irradiated MoO$$_{3}$$ pellet pieces were dissolved in 6M-NaOH aq. In dynamic adsorption, 1 g of Al$$_{2}$$O$$_{3}$$ was filled into a PFA tube ($$phi$$1.59 mm). The $$^{99}$$Mo adsorption capacity of Al$$_{2}$$O$$_{3}$$ specimens under dynamic condition was slightly reduced compared to that under static condition. The $$^{rm 99m}$$Tc elution rate was about 100% at 1.5 mL of milking in dynamic adsorption, while it was around 56-87% in static adsorption. The $$^{99}$$Mo/$$^{rm 99m}$$Tc ratio of dynamic condition was greatly reduced compared to that of static condition. Therefore, the $$^{rm 99m}$$Tc elution property is greatly affected by the method of adsorbing Mo, e.g., the column shape, the linear flow rate, etc.

Journal Articles

MIRS: an imaging spectrometer for the MMX mission

Barucci, M. A.*; Reess, J.-M.*; Bernardi, P.*; Doressoundiram, A.*; Fornasier, S.*; Le Du, M.*; Iwata, Takahiro*; Nakagawa, Hiromu*; Nakamura, Tomoki*; Andr$'e$, Y.*; et al.

Earth, Planets and Space (Internet), 73(1), p.211_1 - 211_28, 2021/12

 Times Cited Count:24 Percentile:81.16(Geosciences, Multidisciplinary)

The MMX InfraRed Spectrometer (MIRS) is an imaging spectrometer on board of MMX JAXA mission. MIRS is built at LESIA-Paris Observatory in collaboration with four other French laboratories, collaboration and financial support of CNES and close collaboration with JAXA and MELCO. The instrument is designed to fully accomplish MMX's scientific and measurement objectives. MIRS will remotely provide near-infrared spectral maps of Phobos and Deimos containing compositional diagnostic spectral features that will be used to analyze the surface composition and to support the sampling site selection. MIRS will also study Mars atmosphere, in particular to spatial and temporal changes such as clouds, dust and water vapor.

Journal Articles

Catalog of gamma-ray glows during four winter seasons in Japan

Wada, Yuki*; Matsumoto, Takahiro*; Enoto, Teruaki*; Nakazawa, Kazuhiro*; Yuasa, Takayuki*; Furuta, Yoshihiro*; Yonetoku, Daisuke*; Sawano, Tatsuya*; Okada, Go*; Nanto, Hidehito*; et al.

Physical Review Research (Internet), 3(4), p.043117_1 - 043117_31, 2021/12

Journal Articles

Multiple gamma-ray glows and a downward TGF observed from nearby thunderclouds

Hisadomi, Shohei*; Nakazawa, Kazuhiro*; Wada, Yuki*; Tsuji, Yuna*; Enoto, Teruaki*; Shinoda, Taro*; Morimoto, Takeshi*; Nakamura, Yoshitaka*; Yuasa, Takayuki*; Tsuchiya, Harufumi

Journal of Geophysical Research; Atmospheres, 126(18), p.e2021JD034543_1 - e2021JD034543_12, 2021/09

 Times Cited Count:20 Percentile:77.40(Meteorology & Atmospheric Sciences)

Journal Articles

Radiochemical research for the advancement of $$^{99}$$Mo/$$^{rm 99m}$$Tc generator by (n, $$gamma$$) method, 3

Fujita, Yoshitaka; Seki, Misaki; Namekawa, Yoji*; Nishikata, Kaori; Daigo, Fumihisa; Ide, Hiroshi; Tsuchiya, Kunihiko; Sano, Tadafumi*; Fujihara, Yasuyuki*; Hori, Junichi*; et al.

KURNS Progress Report 2020, P. 136, 2021/08

no abstracts in English

Journal Articles

Microstructures and interface magnetic moments in Mn$$_{2}$$VAl/Fe layered films showing exchange bias

Kubota, Takahide*; Shimada, Yusuke*; Tsuchiya, Tomoki*; Yoshikawa, Tomoki*; Ito, Keita*; Takeda, Yukiharu; Saito, Yuji; Konno, Toyohiko*; Kimura, Akio*; Takanashi, Koki*

Nanomaterials (Internet), 11(7), p.1723_1 - 1723_11, 2021/07

 Times Cited Count:2 Percentile:10.80(Chemistry, Multidisciplinary)

Journal Articles

Gamma-ray observations at the coastal area of Japan Sea in winter seasons

Tsuchiya, Harufumi; Enoto, Teruaki*; Wada, Yuki*; Furuta, Yoshihiro; Nakazawa, Kazuhiro*; Yuasa, Takayuki*; Umemoto, Daigo*; Makishima, Kazuo*; GROWTH Collaboration*

Proceedings of Science (Internet), 358, p.1163_1 - 1163_6, 2021/07

357 (Records 1-20 displayed on this page)