Chemical kinetic uncertainty quantification for Reynolds-Averaged Navier-Stokes simulations of turbulent premixed combustion

Motegi, Kosuke; Shiotsu, Hiroyuki; Matsumoto, Toshinori; Hibiki, Takashi*; Shibamoto, Yasuteru

International Journal of Heat and Mass Transfer, 258, p.128275_1 - 128275_15, 2026/05

https://doi.org/10.1016/j.ijheatmasstransfer.2025.128275

A Novel kinetic model for dissolution and precipitation of oxide on stainless-steel surface in stagnant liquid sodium

Kawaguchi, Munemichi*; Ikeda, Asuka; Saito, Junichi

Annals of Nuclear Energy, 226, p.111880_1 - 111880_9, 2026/02

https://doi.org/10.1016/j.anucene.2025.111880

Benchmarks of iron nuclear data for fusion neutron sources

Kwon, Saerom*; Konno, Chikara; Honda, Shogo*; Kenjo, Shunsuke*; Sato, Satoshi*

Fusion Engineering and Design, 223, p.115548_1 - 115548_8, 2026/02

https://doi.org/10.1016/j.fusengdes.2025.115548

In order to evaluate the accuracy of the iron data in the latest nuclear data libraries (FENDL-3.2b, JENDL-5, ENDF/B-VIII.0 and JEFF-3.3) used in the fusion neutron source design, we performed their benchmark tests by using QST/TIARA iron experiment with quasi mono-energy neutrons of 40 and 65 MeV and JAEA/FNS iron experiment with DT neutrons. From the test results, we have found the following issues; (1) The calculation results with FENDL-3.2b underestimate the measured neutron fluxes of the continuous energy range (10-60 MeV) by a factor of 0.6 in the TIARA experiment with 65 MeV neutrons; (2) The calculation results with FENDL-3.2b tend to underestimate the measured neutron flux above 10 MeV by a factor of 0.8 at depth of 70 cm and overestimate the measured ones below 10 keV by a factor of 1.3 up to depth of 40 cm in the FNS experiment. We investigated those issues in detail and clarified their reasons.

Validation of underwater radiation monitoring detector

Ji, W.*; Lee, E.*; Ji, Y.-Y.*; Ochi, Kotaro; Yoshimura, Kazuya; Funaki, Hironori; Sanada, Yukihisa

Nuclear Engineering and Technology, 58(2), p.103933_1 - 103933_6, 2026/02

https://doi.org/10.1016/j.net.2025.103933

We aimed to validate the performance of an in situ underwater radiation detector, MARK-U1 (Monitoring of Ambient Radiation of KAERI - Underwater), was used to estimate Cs activity concentration in river and reservoir sediment at predicted sites of contamination. Additionally, underwater core samples were collected to measure the radioactivity using a high-purity germanium (HPGe) detector. To estimate radioactivity, a conversion factor was derived by comparing the measured spectrum and Cs activity in the sample. A Monte Carlo N-Particle (MCNP) simulation was conducted to determine the effective source geometry for in situ measurement. The simulation results correlated well with the on-site MARK-U1 monitoring results, with a deviation of 31.62%. These findings validate the performance of the in situ detector. This device can therefore be used to estimate Cs activity concentration in the underwater sediment via on-site monitoring, without requiring sample collection.

Effects of melting and coagulating conditions on the structure of simulated waste glasses

Nagai, Takayuki; Aoyama, Yusuke; Okamoto, Yoshihiro; Hasegawa, Takehiko*; Sato, Seiichi*; Kikuchi, Tetsuya*; Hatakeyama, Kiyoshi*

JAEA-Research 2025-012, 43 Pages, 2026/01

JAEA-Research-2025-012.pdf:6.99MB

In the vitrification process study of high-level radioactive waste liquids, precipitates present in the simulated waste glasses are detected by X-ray diffraction (XRD), but due to the state of the precipitates (fine size, extremely small amount), precipitate peaks cannot be observed in the XRD pattern. We have evaluated the glass structure of simulated waste glasses prepared under different melting and coagulated conditions using Raman spectroscopy and other methods, in this study. The simulated waste glass, which does not show any precipitate peaks in the XRD pattern, was subjected to Raman spectroscopy, and it was confirmed that precipitate particles in the glass phase could be detected. And it was confirmed that in glass preparation, stirring the molten glass and increasing the cooling rate from the molten state are likely to suppress the formation of precipitate particles in the glass phase. The evaluation of the Si-O bridging structure of the glass revealed no difference in the Si-O bridging structure between areas with and without precipitates. The precipitates detected by Raman spectroscopy are not ceria (CeO) or calcium molybdate (CaMoO), but they are presumed to be compounds such as spinel. In experiments using synchrotron radiation, X-ray transmission images of the internal state of glasses were observed, and it was confirmed that stirring molten glass is effective in reducing bubbles present in the glass phase. The XAFS measurements of Mo K-edge, Ce L-edge, and Si K-edge confirmed that stirring the molten glass does not affect the chemical state of Mo, Ce, and Si contained in the glass.

Results of environmental impact investigations as part of environmental monitoring investigation in backfilling of shafts and tunnels of Mizunami Underground Research Laboratory (FY2024)

Kokubu, Yoko; Takeuchi, Ryuji; Nishio, Kazuhisa*; Ikeda, Koki

JAEA-Data/Code 2025-013, 66 Pages, 2026/01

JAEA-Data-Code-2025-013.pdf:5.88MB

The Tono Geoscience Center of Japan Atomic Energy Agency (JAEA) has been conducting the environmental monitoring investigation to confirm the environmental impacts associated with the backfilling of shafts and tunnels at the Mizunami Underground Research Laboratory (MIU). This report summarizes the results of the environmental impact investigations conducted as part of the environmental monitoring investigation around the MIU Site in FY2024, which include groundwater level measurement in wells, river flow rate measurement, water analysis of Hazama river, noise and vibration surveys, and soil survey.

Neutron total and capture cross-section measurement and resolved resonance analysis of Er

Rovira Leveroni, G.; Kimura, Atsushi; Nakamura, Shoji; Endo, Shunsuke; Iwamoto, Osamu; Iwamoto, Nobuyuki; Katabuchi, Tatsuya*

Annals of Nuclear Energy, 225, p.111688_1 - 111688_18, 2026/01

https://doi.org/10.1016/j.anucene.2025.111688

Development of a new THINC/WLIC method based on a separate evaluation of the geometrical fidelity and the interface sharpness

Fukuda, Takanari; Yamashita, Susumu; Yoshida, Hiroyuki

Journal of Computational Physics, 545, p.114485_1 - 114485_32, 2026/01

https://doi.org/10.1016/j.jcp.2025.114485

This paper puts forward a novel approach for the evaluation of the geometrical fidelity and the interface sharpness of the VOF advection schemes separately and quantitatively. This new evaluation has elucidated the trade-off relationship of the geometrical fidelity and the interface sharpness between the existing schemes of the original THINC and the THINC/WLIC. By investigating and resolving this trade-off relationship, we have developed a novel THINC-based scheme that exhibits high performance with regard to both geometrical fidelity and interface sharpness, despite employing an algorithm as concise as those of the original THINC and the THINC/WLIC. The novel scheme, designated "THINC/Advanced WLIC (THINC/AWLIC)," has been developed by redefining the weight function of the preceding THINC/WLIC so that the contribution of the first-order upwind flux can be variably blended with the usage of the control parameter. The results of the multiple benchmark tests in two and three dimensions demonstrate that both the geometrical fidelity and the interface sharpness are significantly enhanced if the control parameter is appropriately determined. Furthermore, the associated error of THINC/AWLIC is comparable to that of the geometrical scheme, although the implementation complexity is unchanged from that of the simple THICN/WLIC.

Mutual separation of Ru, Rh, and Pd via reflux-assisted extraction and reverse-extraction using ion-pair and solvation with S- and amino-N-donor reagents

Sasaki, Yuji; Kaneko, Masashi; Matsumiya, Masahiko*; Kumagai, Yuta

Journal of Molecular Liquids, 441, p.129013_1 - 129013_10, 2026/01

https://doi.org/10.1016/j.molliq.2025.129013

This study determined extraction and back-extraction conditions for the mutual separation of three light PGMs, Ru, Rh, and Pd. Results revealed that reagents containing soft N and S donor atoms efficiently extract and strip Pd through solvation. In comparison, Ru and Rh undergo ion-pair extraction, requiring both anionic metal species and cationic extractants. These essential chlorinated PGM anions and protonated extractants having amino N atoms are present in HCl media. D(Ru) and D(Rh) values of approximately 100 and 10, respectively, were obtained using nitrilo-triacet-amide (NTAamide), which exhibits tetradentate coordination. Refluxing in 3-6 M HCl at 250 C, a condition that promotes the formation of highly chlorinated PGM anionic species, increased D(Ru) and D(Rh). Based on these findings, a flow diagram for the mutual separation of three PGMs was developed.

A Thermodynamic study of fluorite/bixbyite equilibria in the UO-PuO-PuO system

Vinograd, V. L.*; Vauchy, R.

Journal of Nuclear Materials, 619, p.156244_1 - 156244_16, 2026/01

https://doi.org/10.1016/j.jnucmat.2025.156244

Thermodynamic properties of (UPu)O fluorite (FCC) and (UPu)O bixbyite (BCC) in the UO-PuO-PuO system are assessed by considering phase equilibrium constraints and data on the variation of oxygen to metal ratio (O/M) as a function of the chemical potential of O. Thermodynamically, both BCC and FCC are described as ordered solid solutions allowing for a decrease in the configurational entropy of their oxygen/vacancy distributions at the specific values of = -0.5 and = -0.375 (O/M = 1.5 and O/M = 1.625). With this approach, fluorite/bixbyite equilibria in PuO-PuO and in UO-PuO-PuO are reproduced well with little effort. Moreover, we show that a large manifold of experimental data on the UO-PuO-PuO system is consistent with the assumption that Pu/(Pu+U) ratios in individual phases remain equal to the total Pu/(Pu+U) ratio in the system, i.e., no inter-phase U/Pu-partitioning occurs.