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Journal Articles

Fluorous and organic extraction systems; A Comparison from the perspectives of coordination structures, interfaces, and bulk extraction phases

Ueda, Yuki; Micheau, C.; Akutsu, Kazuhiro*; Tokunaga, Kohei; Yamada, Masako*; Yamada, Norifumi*; Bourgeois, D.*; Motokawa, Ryuhei

Langmuir, 40(46), p.24257 - 24271, 2024/11

 Times Cited Count:0 Percentile:0.00(Chemistry, Multidisciplinary)

Microscopic structures in liquid-liquid extraction, such as structuration between extractants or extracted complexes in bulk organic phases and at interfaces, can influence macroscopic phenomena, such as the distribution behavior of solutes, including extraction efficiency, selectivity, and phase separation of the organic phase. In this study, we correlated the macroscopic behavior of the extraction of Zr(IV) ions from nitric acid solutions with microscopic structural information in order to understand at the molecular level the key factors contributing to the higher metal ion extraction performance in the fluorous extraction system comprising fluorous phosphate (TFP) in perfluorohexane as compared to the analogous organic extraction system comprising organic phosphate (THP) in n-hexane. Extended X-ray absorption fine structure, neutron reflectometry, and small-angle neutron scattering revealed the local coordination structure around the Zr(IV) ion, the accumulation of extractant molecules at the interface, and the structuration of extractant molecules in the bulk extraction phase, respectively. In the fluorous extraction system, extractant aggregates with were formed after contact with nitric acid. In contrast, in the organic extraction system, only extractant dimers were formed. We speculate that differences in the local coordination structure around the Zr(IV) ion and the structuration of the extractant molecules in the bulk extraction phase contribute to the high Zr(IV) extraction performance in the fluorous extraction system. In particular, the size of the aggregates hardly changed with increasing Zr(IV) concentration in the fluorous phase, which may be closely related to the absence of phase splitting in the fluorous extraction system.

Journal Articles

Uncovering the characteristics of plastic-associated biofilm from the inland river system of Mongolia

Battulga, B.; Munkhbat, D.*; Matsueda, Makoto; Atarashi-Andoh, Mariko; Oyuntsetseg, B.*; Koarashi, Jun; Kawahigashi, Masayuki*

Environmental Pollution, 357, p.124427_1 - 124427_10, 2024/09

 Times Cited Count:0 Percentile:0.00(Environmental Sciences)

The occurrence and characteristics of plastic debris in aquatic and terrestrial environments have been extensively studied. However, there is still limited information on the properties and dynamic behavior of plastic-associated biofilms in the environment. In this study, we collected plastic samples from an inland river system in Mongolia and extracted biofilms from the plastics to uncover the characteristics of the biofilms using analytical, isotopic, and thermogravimetric techniques. Mixtures of organic and mineral particles were detected from extracted biofilms, revealing the plastic as a carrier for exogenous substances including contaminants in the river ecosystem. The present study provides insights into the characteristics and environmental behavior of biofilms which are useful to elucidate the impact of plastic-associated biofilms on organic matter and material cycling in the aquatic ecosystems.

Journal Articles

None

Ueda, Yuki; Micheau, C.; Motokawa, Ryuhei

Shiki, 64, p.2 - 6, 2024/09

no abstracts in English

Journal Articles

Globular pattern formation of hierarchical ceria nanoarchitectures

Aoyagi, Noboru; Motokawa, Ryuhei; Okumura, Masahiko; Ueda, Yuki; Saito, Takumi*; Nishitsuji, Shotaro*; Taguchi, Tomitsugu*; Yomogida, Takumi; Sazaki, Gen*; Ikeda, Atsushi

Communications Chemistry (Internet), 7, p.128_1 - 128_13, 2024/06

 Times Cited Count:0 Percentile:0.00(Chemistry, Multidisciplinary)

Journal Articles

Impact of branching position and degree on uranium extraction by amines; A Supramolecular and thermodynamic study

Guerinoni, E.*; Giusti, F.*; Dourdain, S.*; Dufr$^e$che, J.-F.*; Motokawa, Ryuhei; Ueda, Yuki; Aoyagi, Noboru; Zemb, T.*; Pellet-Rostaing, S.*

Journal of Molecular Liquids, 403, p.124820_1 - 124820_11, 2024/06

 Times Cited Count:0 Percentile:0.00(Chemistry, Physical)

Journal Articles

Current numbers of qubits and their uses

Ichikawa, Tsubasa*; Hakoshima, Hideaki*; Inui, Koji*; Ito, Kosuke*; Matsuda, Ryo*; Mitarai, Kosuke*; Miyamoto, Koichi*; Mizukami, Wataru*; Mizuta, Kaoru*; Mori, Toshio*; et al.

Nature Reviews Physics (Internet), 6(6), p.345 - 347, 2024/06

 Times Cited Count:2 Percentile:51.04(Physics, Applied)

Journal Articles

Organization of malonamides from the interface to the organic bulk phase

Micheau, C.; Ueda, Yuki; Motokawa, Ryuhei; Akutsu, Kazuhiro*; Yamada, Norifumi*; Yamada, Masako*; Moussaoui, S. A.*; Makombe, E.*; Meyer, D.*; Berthon, L.*; et al.

Journal of Molecular Liquids, 401, p.124372_1 - 124372_12, 2024/05

 Times Cited Count:1 Percentile:62.80(Chemistry, Physical)

Journal Articles

Synthesis of heat-resistant living polymer particles by one-step reversible addition-fragmentation chain transfer precipitation polymerization of styrene and $$N$$-phenylmaleimide

Yamazaki, Shun*; Kaneko, Naoya*; Kato, Atsuya*; Watanabe, Kohei*; Aoki, Daisuke*; Taniguchi, Tatsuo*; Karatsu, Takashi*; Ueda, Yuki; Motokawa, Ryuhei; Okura, Koki*; et al.

Polymer, 298, p.126846_1 - 126846_11, 2024/04

 Times Cited Count:3 Percentile:86.77(Polymer Science)

Journal Articles

Benchmark analysis by Beremin model and GTN model in CAF Subcommittee

Nagoshi, Yasuto*; Fukahori, Takuya*; Okada, Hiroshi*; Takahashi, Akiyuki*; Shimodaira, Masaki; Ueda, Takashi*; Ogawa, Takuya*; Yashirodai, Kenji*; Takahashi, Yukio*; Ohata, Mitsuru*

Transactions of the 27th International Conference on Structural Mechanics in Reactor Technology (SMiRT 27) (Internet), 9 Pages, 2024/03

no abstracts in English

Journal Articles

Upgrade of the small-angle neutron scattering diffractometer SANS-J at JRR-3

Kumada, Takayuki; Motokawa, Ryuhei; Oba, Yojiro; Nakagawa, Hiroshi; Sekine, Yurina; Micheau, C.; Ueda, Yuki; Sugita, Tsuyoshi; Birumachi, Atsushi; Sasaki, Miki; et al.

Journal of Applied Crystallography, 56(6), p.1776 - 1783, 2023/12

 Times Cited Count:11 Percentile:96.87(Chemistry, Multidisciplinary)

The combination of the existing position-sensitive photomultiplier and the $$^{3}$$He main detector with focusing devices, and the newly installed front detectors in SANS-J at JRR-3 covers small-angle neutron scattering signals in the range of the magnitude of the scattering vector Q from 0.002 to 6 nm-1 gaplessly with three standard device layouts. The installation of the front detector and a graphical user interface system largely improved the usability of SANS-J.

Journal Articles

Occurrence of radioactive cesium-rich micro-particles (CsMPs) in a school building located 2.8 km south-west of the Fukushima Daiichi Nuclear Power Plant

Fueda, Kazuki*; Komiya, Tatsuki*; Minomo, Kenta*; Horie, Kenji*; Takehara, Mami*; Yamasaki, Shinya*; Shiotsu, Hiroyuki; Onuki, Toshihiko*; Grambow, B.*; Law, G. T. W.*; et al.

Chemosphere, 328, p.138566_1 - 138566_12, 2023/07

 Times Cited Count:4 Percentile:31.19(Environmental Sciences)

Journal Articles

Foam flotation of clay particles using a bifunctional amine surfactant

Micheau, C.; Ueda, Yuki; Motokawa, Ryuhei; Bauduin, P.*; Girard, L.*; Diat, O.*

Langmuir, 39(31), p.10965 - 10977, 2023/07

 Times Cited Count:8 Percentile:72.72(Chemistry, Multidisciplinary)

Journal Articles

A Novel method for processing noisy magnetotelluric data based on independence of signal sources and continuity of response functions

Ogawa, Hiroki; Asamori, Koichi; Negi, Tateyuki*; Ueda, Takumi*

Journal of Applied Geophysics, 213, p.105012_1 - 105012_17, 2023/06

 Times Cited Count:2 Percentile:47.92(Geosciences, Multidisciplinary)

A number of schemes for processing magnetotelluric (MT) data have been reported aiming at suppressing the strong effect of artificial electromagnetic noise, especially coherent noise that is correlated between electric and magnetic time series. Many of the recent denoising schemes are based on decomposing MT data into the responses of the natural signal and noise. Meanwhile, it is crucial to distinguish the natural signal from noise stably without depending on any empirical choice of parameter setting. In addition, improper subtraction of values from the separated signal can lead to the loss of useful values of the natural signal or missing noise-affected values, which may result in failure in deriving the true MT responses. We propose a novel data-processing method that applies frequency-domain independent component analysis (FDICA) to both the local MT data and the reference magnetic data. Among the separated signal, the proposed method can quantitatively distinguish the natural signal from the noise-affected components by calculating the ratio of cross-power spectrum with the reference data to the auto-power spectrum for each component. When determining which values to subtract from the separated signal, we introduce an evaluation index with respect to two characteristics of the MT response function: stationary in the time domain and smoothness in the frequency domain. We conduct the experiments both with MT time series severely contaminated by synthetic coherent noises and with MT field data interfered with DC (direct current) railways. Consequently, we confirm the superiority of the proposed method in the noise-suppression performance over the conventional methods of MT data processing.

Journal Articles

Investigation of niobium surface roughness and hydrogen content with different polishing conditions for performance recovery of superconducting QWRs in JAEA Tokai-Tandem Accelerator

Kamiya, Junichiro; Nii, Keisuke*; Kabumoto, Hiroshi; Kondo, Yasuhiro; Tamura, Jun; Harada, Hiroyuki; Matsui, Yutaka; Matsuda, Makoto; Moriya, Katsuhiro; Ida, Yoshiaki*; et al.

e-Journal of Surface Science and Nanotechnology (Internet), 21(4), p.344 - 349, 2023/05

no abstracts in English

Journal Articles

Hierarchical aggregation in a complex fluid; The Role of isomeric interconversion

Massey, D.*; Williams, C. D.*; Mu, J.*; Masters, A. J.*; Motokawa, Ryuhei; Aoyagi, Noboru; Ueda, Yuki; Antonio, M. R.*

Journal of Physical Chemistry B, 127(9), p.2052 - 2065, 2023/03

 Times Cited Count:2 Percentile:22.86(Chemistry, Physical)

Journal Articles

Deuterated malonamide synthesis for fundamental research on solvent extraction systems

Micheau, C.; Ueda, Yuki; Akutsu, Kazuhiro*; Bourgeois, D.*; Motokawa, Ryuhei

Solvent Extraction and Ion Exchange, 41(2), p.221 - 240, 2023/02

 Times Cited Count:4 Percentile:53.75(Chemistry, Multidisciplinary)

Journal Articles

Reports of electro-polishing implementation for quarter-wave resonators, 2

Nii, Keisuke*; Ida, Yoshiaki*; Ueda, Hideki*; Yamaguchi, Takanori*; Kabumoto, Hiroshi; Kamiya, Junichiro; Kondo, Yasuhiro; Tamura, Jun; Harada, Hiroyuki; Matsui, Yutaka; et al.

Proceedings of 19th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.601 - 604, 2023/01

no abstracts in English

Journal Articles

Tough yet flexible superelastic alloys meet biomedical needs

Xu, X.*; Odaira, Takumi*; Xu, S.*; Hirata, Kenji*; Omori, Toshihiro*; Ueki, Kosuke*; Ueda, Kyosuke*; Narushima, Takayuki*; Nagasako, Makoto*; Kainuma, Ryosuke*; et al.

Advanced Materials & Processes, 180(7), p.35 - 37, 2022/10

Journal Articles

Flexible and tough superelastic Co-Cr alloys for biomedical applications

Odaira, Takumi*; Xu, S.*; Hirata, Kenji*; Xu, X.*; Omori, Toshihiro*; Ueki, Kosuke*; Ueda, Kyosuke*; Narushima, Takayuki*; Nagasako, Makoto*; Harjo, S.; et al.

Advanced Materials, 34(27), p.2202305_1 - 2202305_11, 2022/07

 Times Cited Count:23 Percentile:89.93(Chemistry, Multidisciplinary)

Journal Articles

Polymer photonic crystals prepared by triblock copolymerization-induced ${it in situ}$ microphase separation

Isozaki, Yuka*; Higashiharaguchi, Seiya*; Kaneko, Naoya*; Yamazaki, Shun*; Taniguchi, Tatsuo*; Karatsu, Takashi*; Ueda, Yuki; Motokawa, Ryuhei

Chemistry Letters, 51(6), p.625 - 628, 2022/06

 Times Cited Count:3 Percentile:25.39(Chemistry, Multidisciplinary)

257 (Records 1-20 displayed on this page)