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Journal Articles

Three-dimensional bulk Fermi surfaces and Weyl crossings of Co$$_2$$MnGa thin films underneath a protection layer

Kono, Takashi*; Kakoki, Masaaki*; Yoshikawa, Tomoki*; Wang, X.*; Sumida, Kazuki; Muro, Takayuki*; Goto, Kazuki*; Sakuraba, Yuya*; Umetsu, Rie*; Kimura, Akio*

Physical Review B, 104(19), p.195112_1 - 195112_8, 2021/11

Angle-resolved photoelectron spectroscopy utilizing soft X-ray synchrotron radiation was applied to Heusler-type Co$$_2$$MnGa thin films that have a 1-nm Al capping layer. The bulk Fermi surfaces and band structures varied along the out-of-plane momentum, stemming from the three-dimensional crystal structure, in the absence of any in situ surface treatment. In addition, there were characteristic intersecting bands (Weyl cones), with crossing points near the Fermi level, which were consistent with computed results. The Weyl cones are of bulk origin and are responsible for the high anomalous Nernst and the anomalous Hall coefficients. A close comparison of the experimental band structures in Co$$_2$$MnGe and Co$$_2$$MnGa indicated that the rigid band picture is valid in both alloys and that fine carrier tuning is possible by replacing Ga with Ge to improve the anomalous conductivity.

Journal Articles

Detecting halfmetallic electronic structures of spintronic materials in a magnetic field

Fujiwara, Hidenori*; Umetsu, Rie*; Kuroda, Fumiaki*; Miyawaki, Jun*; Kashiuchi, Toshiyuki*; Nishimoto, Kohei*; Nagai, Kodai*; Sekiyama, Akira*; Irizawa, Akinori*; Takeda, Yukiharu; et al.

Scientific Reports (Internet), 11(1), p.18654_1 - 18654_9, 2021/09

 Times Cited Count:0

Journal Articles

Electronic structure and magnetic properties of the half-metallic ferrimagnet Mn$$_{2}$$VAl probed by soft X-ray spectroscopies

Nagai, Kodai*; Fujiwara, Hidenori*; Aratani, Hidekazu*; Fujioka, Shuhei*; Yomosa, Hiroshi*; Nakatani, Yasuhiro*; Kiss, Takayuki*; Sekiyama, Akira*; Kuroda, Fumiaki*; Fujii, Hitoshi*; et al.

Physical Review B, 97(3), p.035143_1 - 035143_8, 2018/01

AA2017-0644.pdf:1.01MB

 Times Cited Count:13 Percentile:63.24(Materials Science, Multidisciplinary)

We have studied the electronic structure of ferrimagnetic Mn$$_{2}$$VAl single crystals by means of soft X-ray absorption spectroscopy (XAS), X-ray absorption magnetic circular dichroism (XMCD), and resonant soft X-ray inelastic scattering (RIXS). We have successfully observed the XMCD signals for all the constituent elements. The Mn L$$_{2,3}$$ XAS and XMCD spectra are reproduced by spectral simulations based on density-functional theory, indicating the itinerant character of the Mn 3$$d$$ states. On the other hand, the V 3$$d$$ electrons are rather localized since the ionic model can qualitatively explain the V L$$_{2,3}$$ XAS and XMCD spectra. This picture is consistent with local $$dd$$ excitations revealed by the V L$$_{3}$$ RIXS.

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