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Takahama, Ryusei*; Arizono, Mitsutoshi*; Indo, Daigo*; Yoshinaga, Taisei*; Terakura, Chieko*; Takeshita, Nao*; Shirasaki, Takumi*; Noda, Masaaki*; Kuwahara, Hideki*; Kajimoto, Ryoichi; et al.
JPS Conference Proceedings (Internet), 38, p.011114_1 - 011114_6, 2023/05
Tomita, Kana*; Kishi, Tetsuo*; Matsumura, Daiju; Yano, Tetsuji*
Journal of Non-Crystalline Solids, 597, p.121891_1 - 121891_10, 2022/12
Times Cited Count:1 Percentile:13.38(Materials Science, Ceramics)Shimada, Asako; Tsukahara, Takehiko*; Nomura, Masao*; Kim, M. S.*; Shimada, Taro; Takeda, Seiji; Yamaguchi, Tetsuji
Journal of Nuclear Science and Technology, 58(11), p.1184 - 1194, 2021/11
Times Cited Count:5 Percentile:64.12(Nuclear Science & Technology)Determining the completeness of nuclear reactor decommissioning is an important step in safely utilizing nuclear power. For example, Cs from the Fukushima Daiichi Nuclear Power Station (FDNPS) accident can be treated as background radioactivity, so determining the origin of Cs is essential. To accomplish this, measuring the Cs/Cs isotope ratio can be useful, so this study optimized a solvent extraction method, with calix[4]arene-bis(t-octylbenzo-crown-6) [BOBCalixC6] in 1-octanol, to purify radioactive Cs, radiocesium, from a solution of major environmental soil elements and mass spectrometry interference elements. This optimized method was applied to Cs purification in soil samples (40 g), and the final solutions contained a total of 10g/ml of the major soil elements and ng/ml concentrations at most of interfering elements. Soil samples collected near the FDNPS were then purified, and the Cs/Cs isotope ratios were measured, using both thermal ionization mass spectrometry (TIMS) and triple quadrupole induced coupled plasma mass spectrometry (ICP-QQQ). The results of each of these measurements were compared, and we found that Cs isotope ratios obtained by TIMS were more precise, by an order of magnitude, while the ICP-QQQ results possessed good abundance sensitivities. A slightly higher Cs/Cs ratio in the northwest area of the FDNPS was observed, while other areas exhibited similar values, all within the measurement error range, which indicated different origins of radiocesium. These results agreed with previously reported Cs/Cs activity distributions, suggesting that this ratio may be useful in identifying radiocesium origins for evaluating future nuclear reactor decommissions.
Kado, Rikiya*; Kishi, Tetsuo*; Lelong, G.*; Galoisy, L.*; Matsumura, Daiju; Calas, G.*; Yano, Tetsuji*
Journal of Non-Crystalline Solids, 539, p.120070_1 - 120070_8, 2020/07
Times Cited Count:5 Percentile:27.95(Materials Science, Ceramics)Takahama, Ryusei*; Ishii, Toi*; Indo, Daigo*; Arizono, Mitsutoshi*; Terakura, Chieko*; Tokura, Yoshinori*; Takeshita, Nao*; Noda, Masaaki*; Kuwahara, Hideki*; Saiki, Takuo*; et al.
Physical Review Materials (Internet), 4(7), p.074401_1 - 074401_11, 2020/07
Times Cited Count:10 Percentile:43.3(Materials Science, Multidisciplinary)Watanabe, So; Ogi, Hiromichi*; Arai, Yoichi; Aihara, Haruka; Takahatake, Yoko; Shibata, Atsuhiro; Nomura, Kazunori; Kamiya, Yuichi*; Asanuma, Noriko*; Matsuura, Haruaki*; et al.
Progress in Nuclear Energy, 117, p.103090_1 - 103090_8, 2019/11
Times Cited Count:12 Percentile:79.53(Nuclear Science & Technology)Kajimoto, Ryoichi; Nakamura, Mitsutaka; Murai, Naoki; Shamoto, Shinichi; Honda, Takashi*; Ikeda, Kazutaka*; Otomo, Toshiya*; Hata, Hiroto*; Eto, Takahiro*; Noda, Masaaki*; et al.
Scientific Reports (Internet), 8(1), p.9651_1 - 9651_8, 2018/06
Times Cited Count:6 Percentile:30.02(Multidisciplinary Sciences)Hemmi, Ko; Yamaguchi, Tetsuji; Takeda, Seiji; Kimura, Hideo
Genshiryoku Bakkuendo Kenkyu (CD-ROM), 24(1), p.3 - 14, 2017/06
Conditions of contaminated sources and ranges of forest decontamination that significantly reduce the air dose rate in residential areas were investigated by means of a sensitivity analysis related to the decontamination of the forest contaminated by radiocesium deriving from the accident at Fukushima Daiichi Nuclear Power Station. The contaminated sources including Cs and Cs were assumed to be a layer of sedimented organic matter (the A layer) and surface soils (the A layer). The air dose rates were calculated using the three-dimensional Monte Carlo transport code MCNP. A slope number of the forest, angles, state of contaminant distribution, radiocesium content in the forest soils, decontamination ranges, distance from the forest boundary to an evaluation point, and height at the evaluation point were adopted as the parameters. The decontamination of a litter (A) layer within the distance of 20 m from the forest boundary was revealed to be effective in reducing the air dose rate when the source distribution was homogeneous. The air dose rates were significantly reduced by the decontamination of the A layer within a distance of 40 m from the forest boundary on condition that the radiocesium content of the A layer was larger than that of the A layer and the source distribution was non-homogeneous, such as the forest areas beyond 20 m from the forest boundary, which were more heavily contaminated than those within 20 m.
Okuda, Tetsuji*; Hata, Hiroto*; Eto, Takahiro*; Sobaru, Shogo*; Oda, Ryosuke*; Kaji, Hiroki*; Nishina, Kosuke*; Kuwahara, Hideki*; Nakamura, Mitsutaka; Kajimoto, Ryoichi
Journal of the Physical Society of Japan, 85(9), p.094717_1 - 094717_6, 2016/09
Times Cited Count:5 Percentile:39.89(Physics, Multidisciplinary)Kajimoto, Ryoichi; Tomiyasu, Keisuke*; Nakajima, Kenji; Kawamura, Seiko; Inamura, Yasuhiro; Okuda, Tetsuji*
Journal of the Physical Society of Japan, 84(7), p.074708_1 - 074708_6, 2015/07
Times Cited Count:9 Percentile:55.76(Physics, Multidisciplinary)Okuda, Tetsuji*; Hata, Hiroto*; Eto, Takahiro*; Nishina, Kosuke*; Kuwahara, Hideki*; Nakamura, Mitsutaka; Kajimoto, Ryoichi
Journal of Physics; Conference Series, 568(Part 2), p.022035_1 - 022035_5, 2014/12
Times Cited Count:8 Percentile:91.23(Physics, Applied)Yamaguchi, Tetsuji; Takeda, Seiji; Nishimura, Yuki; Iida, Yoshihisa; Tanaka, Tadao
Radiochimica Acta, 102(11), p.999 - 1008, 2014/11
Times Cited Count:1 Percentile:8.82(Chemistry, Inorganic & Nuclear)An attempt was made to select thermodynamic data with uncertainties and to evaluate the solubility of radioelements with uncertainties considering variation in groundwater chemistry. The thermodynamic data was selected by reviewing the JAEA-TDB released in 2012. Data for Nb, Pd and Pa were revised from the viewpoint of the consistency of the data selection process. Data for Se, U and Pa were revised from the viewpoint of the conservativeness. Up-to-date ternary calcium-metal(IV)-OH complexes were adopted for Zr, Th, U, Np and Pu. A Monte Carlo-based probabilistic calculation code, PA-SOL, was used for probabilistic analysis of the solubility.
Kajimoto, Ryoichi; Nakajima, Kenji; Kawamura, Seiko; Inamura, Yasuhiro; Okuda, Tetsuji*; Tomiyasu, Keisuke*
JPS Conference Proceedings (Internet), 3, p.014018_1 - 014018_5, 2014/06
Abe, Sosuke*; Ono, Shinya*; Kanemura, Rui*; Yoshigoe, Akitaka; Teraoka, Yuden; Ogata, Shoichi*; Yasuda, Tetsuji*; Tanaka, Masatoshi*
Applied Physics Express, 6(11), p.115701_1 - 115701_4, 2013/11
Times Cited Count:4 Percentile:18.28(Physics, Applied)Kajimoto, Ryoichi; Nakajima, Kenji; Kawamura, Seiko; Inamura, Yasuhiro; Kakurai, Kazuhisa; Hokazono, Takahisa*; Ozono, Akira*; Okuda, Tetsuji*
Journal of the Physical Society of Japan, 82(5), p.054702_1 - 054702_6, 2013/05
Times Cited Count:5 Percentile:38.94(Physics, Multidisciplinary)Onoue, Tetsuji*; Sato, Honami*; Nakamura, Tomoki*; Noguchi, Takaaki*; Hidaka, Yoshihiro*; Shirai, Naoki*; Ebihara, Mitsuru*; Osawa, Takahito; Hatsukawa, Yuichi; Toh, Yosuke; et al.
Proceedings of the National Academy of Sciences of the United States of America, 109(47), p.19134 - 19139, 2012/11
Times Cited Count:40 Percentile:72.55(Multidisciplinary Sciences)The 34 million year (My) interval of the Late Triassic is marked by the formation of several large impact structures on Earth. As with the Chicxulub impact event at the Cretaceous/Paleogene boudary, the Late Triassic impact events have been considered a factor in biotic extinction events in the Late Triassic (e.g., the Triassic/Jurassic boundary). However, the causal link between these impact events and a mass extinction event in the Late Triassic remains controversial because of a lack of stratigraphic records of their ejecta deposits. Here we report evidence for an impact event (platinum group elements anomaly, nickel-rich magnetite and microspherules) deposited within a Paleo-Pacific basin in the middle Norian (Upper Triassic) deep-sea sediment in Japan. This includes anomalously high abundances of iridium, up to 41.5 parts per billion (ppb), in the ejecta deposit, which suggests that the iridium anomaly may be found on a global scale. The middle Norian age of the ejecta deposit suggests that the impact event that produced the 100-km-wide Manicouagan crater in Canada8 is most likely related to its deposition. Our analysis of siliceous microfossils shows no evidence of a mass extinction event across the impact event horizon, and no contemporaneous faunal turnover is seen in other marine fossils. However, such an event has been reported among terrestrial tetrapods and floras in North America. We therefore hypothesize that the Manicouagan impact caused the catastrophic collapse of terrestrial ecosystems near the impact site, but not within the marine realm.
Kume, Tetsuji*; Oura, Hiroyuki*; Takeichi, Tomoo*; Omura, Ayako*; Machida, Akihiko; Watanuki, Tetsu; Aoki, Katsutoshi; Sasaki, Shigeo*; Shimizu, Hiroyasu*; Takemura, Kenichi*
Physical Review B, 84(6), p.064132_1 - 064132_7, 2011/08
Times Cited Count:19 Percentile:61.17(Materials Science, Multidisciplinary)Raman, IR, and visible absorption spectra of scandium trihydride (ScH) have been measured at high pressures up to 50 GPa at room temperature. The structural and electronic phase transitions were investigated. Successive hcp-intermediate-fcc phase transitions took place at 25 and 46 GPa. It was suggested that the intermediate phase of ScH has the same structure as that of YH. The energy gap of ScH is 1.7 eV at the ambient condition and is closed around 50 GPa, at which the crystal structure transforms to fcc.
Okuda, Tetsuji*; Uto, Kazuma*; Seki, Shinichiro*; Onose, Yoshinori*; Tokura, Yoshinori*; Kajimoto, Ryoichi; Matsuda, Masaaki*
Journal of the Physical Society of Japan, 80(1), p.014711_1 - 014711_7, 2011/04
Times Cited Count:26 Percentile:76.16(Physics, Multidisciplinary)Kajimoto, Ryoichi; Nakajima, Kenji; Kawamura, Seiko; Inamura, Yasuhiro; Kakurai, Kazuhisa; Arai, Masatoshi; Hokazono, Takahisa*; Ozono, Akira*; Okuda, Tetsuji*
Journal of the Physical Society of Japan, 79(12), p.123705_1 - 123705_4, 2010/12
Times Cited Count:21 Percentile:71.73(Physics, Multidisciplinary)Amamoto, Ippei; Mitamura, Naoki*; Tsuzuki, Tatsuya*; Takasaki, Yasushi*; Shibayama, Atsushi*; Yano, Tetsuji*; Nakada, Masami; Okamoto, Yoshihiro
Proceedings of 13th International Conference on Environmental Remediation and Radioactive Waste Management (ICEM 2010) (CD-ROM), p.503 - 508, 2010/10
The main objective of this development is to recycle the purified eutectic medium of the pyroreprocessing, delaying its disposal for as long as possible. We have introduced the simple filtration method to remove the rare earth element (REE) particles which were formed due to the conversion of REE chlorides to phosphates. Here, the iron phosphate glass is used as a filtration medium for the removal of FP particles. However, some soluble FP such as compounds of alkali-metals, alkaline-earth metals, etc. still remain in the eutectic medium. This time around, on an experimental basis, the iron phosphate glass has been used as a sorbent instead, to remove the soluble FP. We have obtained some positive results and have intention to incorporate it into the spent electrolyte recycle process as a part of the FP separation and immobilization system.