Ghys, L.*; Andreyev, A. N.; Huyse, M.*; Van Duppen, P.*; Antalic, S.*; Barzakh, A.*; Capponi, L.*; Cocolios, T. E.*; Cubiss, J.*; Derkx, X.*; et al.
Physical Review C, 100(5), p.054310_1 - 054310_13, 2019/11
The aim of this work was to investigate the -decay properties of Fr and daughter products. Neutron-deficient francium nuclei are produced at ISOLDE-CERN bombarding a UCx target with 1.4 GeV protons. Due to the very high statistics and the high beam purity, improved decay data for Fr and its daughters were obtained. The observation of crossover transitions positioned the isomeric high-spin level of At at an excitation energy of 265(3) keV. Half-life values of 4.47(5) s and 1.28(10) s were extracted for the ground state and isomeric state of At and 52(3) ms for the ground-state decay of Fr.
Barzakh, A. E.*; Cubiss, J. G.*; Andreyev, A. N.; Seliverstov, M. D.*; Andel, B.*; Antalic, S.*; Ascher, P.*; Atanasov, D.*; Beck, D.*; Biero, J.*; et al.
Physical Review C, 99(5), p.054317_1 - 054317_9, 2019/05
Hyperfine-structure parameters and isotope shifts for the 795-nm atomic transitions in At have been measured at CERN-ISOLDE, using the in-source resonance-ionization spectroscopy technique. Magnetic dipole and electric quadrupole moments, and changes in the nuclear mean-square charge radii, have been deduced. A large inverse odd-even staggering in radii, which may be associated with the presence of octupole collectivity, has been observed. Namely, the radius of the odd-odd isotope At has been found to be larger than the average.
Andel, B.*; Andreyev, A. N.; Antalic, S.*; Barzakh, A.*; Bree, N.*; Cocolios, T. E.*; Comas, V. F.*; Diriken, J.*; Elseviers, J.*; Fedorov, D. V.*; et al.
Physical Review C, 96(5), p.054327_1 - 054327_11, 2017/12
A detailed -decay spectroscopy study of Tl has been performed at ISOLDE (CERN). Z-selective ionization by the Resonance Ionization Laser Ion Source (RILIS) coupled to mass separation provided a high-purity beam of Tl. Fine-structure decays to excited levels in the daughter Au were identified and an -decay scheme of Tl was constructed based on an analysis of - and - - coincidences. Multipolarities of several -ray transitions deexciting levels in Au were determined. Based on the analysis of reduced -decay widths, it was found that all decays are hindered, which signifies a change of configuration between the parent and all daughter states.
Truesdale, V. L.*; Andreyev, A. N.; Ghys, L.*; Huyse, M.*; Van Duppen, P.*; Sels, S.*; Andel, B.*; Antalic, S.*; Barzakh, A.*; Capponi, L.*; et al.
Physical Review C, 94(3), p.034308_1 - 034308_11, 2016/09
A nuclear-decay spectroscopy study of the neutron-deficient isotope At is reported where an isotopically pure beam was produced using the selective Resonance Ionization Laser Ion Source and On-Line Isotope Mass Separator (CERN). The fine-structure decay of At allowed the low-energy excited states in the daughter nucleus Bi to be investigated. A -delayed fission study of At was also performed. A mixture of symmetric and asymmetric fission-fragment mass distributions of the daughter isotope Po (populated by decay of At) was deduced based on the measured fission-fragment energies. A DF probability (At) = 9(1)10 was determined.
Elseviers, J.*; Andreyev, A. N.*; Huyse, M.*; Van Duppen, P.*; Antalic, S.*; Barzakh, A.*; Bree, N.*; Cocolios, T. E.*; Comas, V. F.*; Diriken, J.*; et al.
Physical Review C, 88(4), p.044321_1 - 044321_13, 2013/10
The detailed analysis of the -delayed fission data of Tl is presented. The experiment was performed by producing a pure beam of Tl by means of highly selective resonance laser ionization followed by mass separation with the ISOLDE isotope separator. A surprising asymmetric mass distribution of fission fragments from Hg, the daughter of Tl decays, was obtained. Here, the energy calibration of the silicon detectors, which is crucial for a proper determination of the fission fragments' energy and mass split, is presented and the total kinetic energy and its dependence on the mass split ratio is discussed. A more precise -delayed fission probability of 3.2(2)10 was deduced.
Rothe, S.*; Andreyev, A. N.*; Antalic, S.*; Borschevsky, A.*; Capponi, L.*; Cocolios, T. E.*; De Witte, H.*; Eliav, E.*; Fedorov, D. V.*; Fedosseev, V. N.*; et al.
Nature Communications (Internet), 4, p.1835_1 - 1835_6, 2013/05
The radioactive element astatine exists only in trace amounts in nature. Its properties can therefore only be explored by study of smallest quantities of artificially produced isotopes or by performing theoretical calculations. One of the most important properties influencing the chemical behaviour is the energy required to remove one electron from the valence shell, referred to as the ionization potential (IP). Here we use laser spectroscopy to probe the optical spectrum of astatine near the ionization threshold. The observed series of Rydberg states allowed the deduction of the IP of the astatine atom for the first time. New ab initio calculations were performed to support the experimental result. The measured value of IP(At) serves as a benchmark for quantum chemistry calculations of the properties of astatine as well as for the theoretical prediction of the ionization potential of super-heavy element 117, the heaviest homologue of astatine.
Andreyev, A. N.*; Liberati, V.*; Antalic, S.*; Ackermann, D.*; Barzakh, A.*; Bree, N.*; Cocolios, T. E.*; Diriken, J.*; Elseviers, J.*; Fedorov, D.*; et al.
Physical Review C, 87(5), p.054311_1 - 054311_8, 2013/05
-decay studies of Tl and its dahghter products Au and Ir were carried out in two complementary experiments at the mass separator ISOLDE (CERN) and velocity filter SHIP (GSI). The nucluesu Au has decay properties of half-life 207 ms and -decay energy 6433 keV. The ground state spins and parities for Au and Ir were determined to be 1/2.
Andreyev, A. N.*; Elseviers, J.*; Huyse, M.*; Van Duppen, P.*; Antalic, S.*; Barzakh, A.*; Bree, N.*; Cocolios, T. E.*; Comas, V. F.*; Diriken, J.*; et al.
Physical Review Letters, 105(25), p.252502_1 - 252502_5, 2010/12
A very exotic process of -delayed fission of Tl is studied in detail by using resonant laser ionization with subsequent mass separation at ISOLDE (CERN). In contrast to common expectations, the fission-fragment mass distribution of the post--decay daughter nucleus Hg (/ = 1.25) is asymmetric. This asymmetry is more surprising since a mass-symmetric split of this extremely neutron-deficient nucleus would lead to two Zr fragments, with magic = 50 and semi-magic = 40. This is a new type of asymmetric fission, not caused by large shell effects related to fragment magic proton and neutron numbers, as observed in the actinide region. The newly-measured branching ratio for -delayed fission of Tl is 3.6(7)10 %.
西尾 勝久; Andreyev, A. N.*; Elseviers, J.*; Huyse, M.*; Van Duppen, P.*; Antalic, S.*; Barzakh, A.*; Bree, N.*; Cocolios, T. E.*; Comas, V. F.*; et al.
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