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Journal Articles

Incorporation of a bromine atom into DNA-related molecules changes their electronic properties

Hirato, Misaki*; Yokoya, Akinari*; Baba, Yuji*; Mori, Seiji*; Fujii, Kentaro*; Wada, Shinichi*; Izumi, Yudai*; Haga, Yoshinori

Physical Chemistry Chemical Physics, 25(21), p.14836 - 14847, 2023/05

 Times Cited Count:0 Percentile:0.01(Chemistry, Physical)

Journal Articles

Design and actual performance of J-PARC 3 GeV rapid cycling synchrotron for high-intensity operation

Yamamoto, Kazami; Kinsho, Michikazu; Hayashi, Naoki; Saha, P. K.; Tamura, Fumihiko; Yamamoto, Masanobu; Tani, Norio; Takayanagi, Tomohiro; Kamiya, Junichiro; Shobuda, Yoshihiro; et al.

Journal of Nuclear Science and Technology, 59(9), p.1174 - 1205, 2022/09

 Times Cited Count:3 Percentile:84.2(Nuclear Science & Technology)

In the Japan Proton Accelerator Research Complex, the purpose of the 3 GeV rapid cycling synchrotron (RCS) is to accelerate a 1 MW, high-intensity proton beam. To achieve beam operation at a repetition rate of 25 Hz at high intensities, the RCS was elaborately designed. After starting the RCS operation, we carefully verified the validity of its design and made certain improvements to establish a reliable operation at higher power as possible. Consequently, we demonstrated beam operation at a high power, namely, 1 MW. We then summarized the design, actual performance, and improvements of the RCS to achieve a 1 MW beam.

Journal Articles

Development of ARKADIA-Safety for severe accident evaluation of sodium-cooled fast reactors

Aoyagi, Mitsuhiro; Sonehara, Masateru; Ishida, Shinya; Uchibori, Akihiro; Kawada, Kenichi; Okano, Yasushi; Takata, Takashi

Proceedings of Technical Meeting on State-of-the-art Thermal Hydraulics of Fast Reactors (Internet), 3 Pages, 2022/09

Journal Articles

Improvement construction for ground around High Active liquid Waste facility in Tokai Reprocessing Plant

Omori, Kazuki; Yamauchi, Sho; Yanagibashi, Futoshi; Sasaki, Shunichi; Wada, Takuya; Suzuki, Hisanori; Domura, Kazuyuki; Takeuchi, Kenji

Nihon Hozen Gakkai Dai-18-Kai Gakujutsu Koenkai Yoshishu, p.245 - 248, 2022/07

Tokai Reprocessing Plant (TRP), which is shifted to decommissioning stage, stores large amount of high-level radioactive liquid waste (HLLW). Although TRP is implementing vitrification of HLLW to reduce the risks related to HLLW storage, additional 20 years are required to complete vitrification of HLLW. Therefore, TRP is implementing safety countermeasure related to seismic resistance of HLLW storage facility as one of the top priorities. The results of the seismic evaluation indicate that although the facility itself is seismically resistant, there is a risk of insufficient binding force acting between the facility and the surrounding ground. Thus, replacement of the surrounding ground with concrete is performed. Since the countermeasures, to protect existing buries structure and coordinate with the other construction projects around the site, are required, the dedicated team was setup to handle the process and safety management of the concrete replacement construction.

Journal Articles

Long-term density-dependent groundwater flow analysis and its effect on nuclide migration for safety assessment of high-level radioactive waste disposal with consideration of interaction between fractures and matrix of rock formation in coastal crystalline groundwater systems

Park, Y.-J.*; Sawada, Atsushi; Ozutsumi, Takenori*; Tanaka, Tatsuya*; Hashimoto, Shuji*; Morita, Yutaka*

Proceedings of 3rd International Conference on Discrete Fracture Network Engineering (DFNE 2022) (Internet), 8 Pages, 2022/00

Safety analysis for underground disposal facilities for high-level radioactive waste requires thorough understanding of long-term groundwater flow and nuclide migration processes in geologic media. In the coastal subsurface systems, groundwater flow is defined by the complex interactions between freshwater of meteoric origin and denser saline water from the sea. In addition, sea levels are expected to fluctuate significantly due to a transgression and regression of the sea over the millions of years for safety analysis. This study presents long-term evolution of groundwater environment such as salinity concentration and flow velocity with focus of the interaction between fractures and matrix blocks in regional and near-field scale analysis framework for groundwater flow and nuclide migration for underground disposal facilities in hypothetical fractured crystalline coastal systems.

Journal Articles

Development and validation of fuel stub motion model for the disrupted core of a sodium-cooled fast reactor

Kawada, Kenichi; Suzuki, Toru*

Nuclear Engineering and Technology, 53(12), p.3930 - 3943, 2021/12

 Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)

To improve the capability of the SAS4A code, which simulates the initiating phase of core disruptive accidents for MOX-fueled Sodium-cooled Fast Reactors (SFRs), the authors have investigated in detail the physical phenomena under unprotected loss-of-flow (ULOF) conditions in a previous paper. As the conclusion of the last article, fuel stub motion, in which the residual fuel pellets would move toward the core central region after fuel pin disruption, was identified as one of the key phenomena to be appropriately simulated for the initiating phase of ULOF. In the present paper, a simple model describing fuel stub motion, which was not modeled in the previous SAS4A code, was newly proposed. The applicability of the proposed model was validated through a series of analyses for the CABRI experiments, by which the stub motion would be represented with reasonable conservativeness for the reactivity evaluation of disrupted core.

Journal Articles

Prediction of stability constants for novel chelates design in minor actinides partitioning over lanthanides using density functional theory calculation

Kaneko, Masashi; Sasaki, Yuji; Wada, Eriko*; Nakase, Masahiko*; Takeshita, Kenji*

Chemistry Letters, 50(10), p.1765 - 1769, 2021/10

 Times Cited Count:0 Percentile:0(Chemistry, Multidisciplinary)

Density functional theory calculation is applied to predict the stability constants for Eu$$^{3+}$$ and Am$$^{3+}$$ complexes in aqueous solution for molecular modelling of novel separation agents for minor actinides over lanthanides. Logarithm of experimental stability constants correlates with calculated complex formation enthalpies with high reproducibility (R$$^{2}$$ $$>$$ 0.98). Prediction of stability constants of novel chelates is demonstrated and indicates a potential availability of the derivatives of diethylenetriaminepentaacetic acid type chelate in acidic condition and enhancement of Am$$^{3+}$$ selectivity over Eu$$^{3+}$$.

Journal Articles

Development of the analytical method using DPD simulation for molten fuel behaviour in a sodium-cooled fast reactor

Sonehara, Masateru; Uchibori, Akihiro; Aoyagi, Mitsuhiro; Kawada, Kenichi; Takata, Takashi; Ohshima, Hiroyuki

Dai-25-Kai Doryoku, Enerugi Gijutsu Shimpojiumu Koen Rombunshu (Internet), 3 Pages, 2021/07

In sodium-cooled fast reactors (SFRs), it has been pointed out that molten fuel may be discharged from the core during a severe accident (SA) accompanied by core damage, and may solidify into debri particles with diameters ranging from several millimeters to several hundred micrometers due to interaction with the sodium coolant and accumulate at the bottom of the reactor vessel. Therefore, it is necessary to understand the behavior of such debri particles appropriately to evaluate the SA event progression. To meet these requirements, a molten fuel behavior analysis code using dissipative particle dynamics (DPD), a kind of particle method, has been developed as a part of the SPECTRA code, tool for consistent analysis of in-vessel and ex-vessel events in sodium fast reactor accidents. In this study, it was found that the new analyses code can reproduce sedimentation behavior of particles by adding a new stress term in the shear direction.

Journal Articles

Study on dominant aspects of unprotected loss-of-flow to be evaluated in the initiating phase for a sodium-cooled fast reactor

Kawada, Kenichi; Suzuki, Toru*

Journal of Nuclear Science and Technology, 58(3), p.347 - 360, 2021/03

 Times Cited Count:1 Percentile:14.68(Nuclear Science & Technology)

SAS4A is presently the worldwide standard computer code for simulation of the initiating phase of the Core Disruptive Accident (CDA) in MOX-fueled Sodium-cooled Fast Reactors (SFR). In order to improve the capability of the computational code, SAS4A, to be applied to the safety assessment for SFRs, detailed investigations of physical phenomena under unprotected loss-of-flow (ULOF) conditions were conducted, and physical models to be developed and improved were identified using the Phenomena Identification and Ranking Table (PIRT) method. A fuel stub motion, in which the residual fuel pellets would move to the core central region after fuel pin disruption, was selected as one of the key phenomena to be simulated properly and a key concept of the fuel stub motion model was presented.

Journal Articles

Thermally altered subsurface material of asteroid (162173) Ryugu

Kitazato, Kohei*; Milliken, R. E.*; Iwata, Takahiro*; Abe, Masanao*; Otake, Makiko*; Matsuura, Shuji*; Takagi, Yasuhiko*; Nakamura, Tomoki*; Hiroi, Takahiro*; Matsuoka, Moe*; et al.

Nature Astronomy (Internet), 5(3), p.246 - 250, 2021/03

 Times Cited Count:30 Percentile:96.52(Astronomy & Astrophysics)

Here we report observations of Ryugu's subsurface material by the Near-Infrared Spectrometer (NIRS3) on the Hayabusa2 spacecraft. Reflectance spectra of excavated material exhibit a hydroxyl (OH) absorption feature that is slightly stronger and peak-shifted compared with that observed for the surface, indicating that space weathering and/or radiative heating have caused subtle spectral changes in the uppermost surface. However, the strength and shape of the OH feature still suggests that the subsurface material experienced heating above 300 $$^{circ}$$C, similar to the surface. In contrast, thermophysical modeling indicates that radiative heating does not increase the temperature above 200 $$^{circ}$$C at the estimated excavation depth of 1 m, even if the semimajor axis is reduced to 0.344 au. This supports the hypothesis that primary thermal alteration occurred due to radiogenic and/or impact heating on Ryugu's parent body.

Journal Articles

Validation study of SAS4A code for the unprotected loss-of-flow accident in an SFR

Ishida, Shinya; Kawada, Kenichi; Fukano, Yoshitaka

Mechanical Engineering Journal (Internet), 7(3), p.19-00523_1 - 19-00523_17, 2020/06

The Phenomena Identification and Ranking Table (PIRT) approach was applied to the validation of SAS4A code in order to indicate the reliability of SAS4A code sufficiently and objectively. Based on this approach, issue and objective were clarified, plant design and scenario were defined, FOM and key phenomena were selected, and the code validation test matrix was completed with the results of investigation about analysis models and test cases. The results of the test analysis corresponding to this matrix show that the SAS4A models required for the IP evaluation were sufficiently validated. Furthermore, the validation with this matrix is highly reliable, since this matrix represents the comprehensive validation that also considers the relation between physical phenomena. In this study, the reliability and validity of SAS4A code were significantly enhanced by using PIRT approach to the sufficient level for CDA analyses in SFR.

Journal Articles

An Experimental setup for creating and imaging $$^{4}$$He$$_{2}$$$$^{ast}$$ excimer cluster tracers in superfluid helium-4 via neutron-$$^{3}$$He absorption reaction

Sonnenschein, V.*; Tsuji, Yoshiyuki*; Kokuryu, Shoma*; Kubo, Wataru*; Suzuki, So*; Tomita, Hideki*; Kiyanagi, Yoshiaki*; Iguchi, Tetsuo*; Matsushita, Taku*; Wada, Nobuo*; et al.

Review of Scientific Instruments, 91(3), p.033318_1 - 033318_12, 2020/03

 Times Cited Count:0 Percentile:0(Instruments & Instrumentation)

Journal Articles

Anomalous small-angle X-ray scattering (ASAXS) study of irradiation-induced nanostructure change in Fe-ion beam irradiated oxide dispersion-strengthened (ODS) steel

Kumada, Takayuki; Oba, Yojiro; Motokawa, Ryuhei; Morooka, Satoshi; Tominaga, Aki; Tanida, Hajime; Shobu, Takahisa; Konno, Azusa; Owada, Kenji*; Ono, Naoko*; et al.

Journal of Nuclear Materials, 528, p.151890_1 - 151890_7, 2020/01

 Times Cited Count:1 Percentile:14.68(Materials Science, Multidisciplinary)

We have developed an anomalous small-angle X-ray scattering (ASAXS) diffractometer in SPring-8 to investigate irradiation-induced nanostructural change in ion-beam irradiated stainless steel. A thermally-aged MA956 stainless steel sample displays power-law scattering that follows the Porod law at the magnitude of scattering vector, Q, below 0.5 nm$$^-1$$ and an overlapped shoulder around 0.7 nm$$^-1$$. After the ion-beam irradiation, the intensity of the shoulder remained unchanged, whereas that of the power-law scattering nearly doubled. This result indicates that none of the structural parameters of the Cr-rich nanoprecipitates, such as the number density, size, and interface roughness, were changed by the irradiation.

Journal Articles

Electronic properties of DNA-related molecules containing a bromine atom

Hirato, Misaki*; Onizawa, Misato*; Baba, Yuji*; Haga, Yoshinori; Fujii, Kentaro*; Wada, Shinichi*; Yokoya, Akinari*

International Journal of Radiation Biology, 7 Pages, 2020/00

 Times Cited Count:2 Percentile:28.65(Biology)

Journal Articles

Validation study of initiating phase evaluation method for the core disruptive accident in an SFR

Ishida, Shinya; Kawada, Kenichi; Fukano, Yoshitaka

Proceedings of 27th International Conference on Nuclear Engineering (ICONE-27) (Internet), 10 Pages, 2019/05

Core Disruptive Accident (CDA) has been considered as one of the important safety issues in the severe accident evaluation of Sodium-cooled Fast Reactor (SFR), and SAS4A code is developed for Initiating Phase (IP) of CDA. Phenomena Identification and Ranking Table (PIRT) approach was applied to the validation of SAS4A code in order to enhance its reliability in this study. SAS4A was validated in the following steps: (1) selection of the figure of merit (FOM) corresponding to Unprotected Loss Of Flow (ULOF) which is one of the most important and typical events in CDA, (2) identification of the phenomena involved in ULOF, (3) ranking the important phenomena, (4) development of the code validation test matrix, and (5) test analyses for validation corresponding to the test matrix. The reliability and validity of SAS4A code were significantly enhanced by this validation with PIRT approach.

Journal Articles

The Surface composition of asteroid 162173 Ryugu from Hayabusa2 near-infrared spectroscopy

Kitazato, Kohei*; Milliken, R. E.*; Iwata, Takahiro*; Abe, Masanao*; Otake, Makiko*; Matsuura, Shuji*; Arai, Takehiko*; Nakauchi, Yusuke*; Nakamura, Tomoki*; Matsuoka, Moe*; et al.

Science, 364(6437), p.272 - 275, 2019/04

 Times Cited Count:233 Percentile:99.74(Multidisciplinary Sciences)

The near-Earth asteroid 162173 Ryugu, the target of Hayabusa2 sample return mission, is believed to be a primitive carbonaceous object. The Near Infrared Spectrometer (NIRS3) on Hayabusa2 acquired reflectance spectra of Ryugu's surface to provide direct measurements of the surface composition and geological context for the returned samples. A weak, narrow absorption feature centered at 2.72 micron was detected across the entire observed surface, indicating that hydroxyl (OH)-bearing minerals are ubiquitous there. The intensity of the OH feature and low albedo are similar to thermally- and/or shock-metamorphosed carbonaceous chondrite meteorites. There are few variations in the OH-band position, consistent with Ryugu being a compositionally homogeneous rubble-pile object generated from impact fragments of an undifferentiated aqueously altered parent body.

Journal Articles

Machine-learning guided discovery of a new thermoelectric material

Iwasaki, Yuma*; Takeuchi, Ichiro*; Stanev, V.*; Gilad Kusne, A.*; Ishida, Masahiko*; Kirihara, Akihiro*; Ihara, Kazuki*; Sawada, Ryoto*; Terashima, Koichi*; Someya, Hiroko*; et al.

Scientific Reports (Internet), 9, p.2751_1 - 2751_7, 2019/02

 Times Cited Count:50 Percentile:92.47(Multidisciplinary Sciences)

Journal Articles

SAS4A simulations of selected CABRI-1 oxide fuel experiments

Karahan, A.*; Kawada, Kenichi; Tentner, A.*

Proceedings of 2018 ANS Winter Meeting and Nuclear Technology Expo; Embedded Topical International Topical Meeting on Advances in Thermal Hydraulics (ATH 2018) (USB Flash Drive), 4 Pages, 2018/11

Journal Articles

Revising the 4${it f}$ symmetry in CeCu$$_{2}$$Ge$$_{2}$$; Soft X-ray absorption and hard X-ray photoemission spectroscopy

Aratani, Hidekazu*; Nakatani, Yasuhiro*; Fujiwara, Hidenori*; Kawada, Moeki*; Kanai, Yuina*; Yamagami, Kohei*; Fujioka, Shuhei*; Hamamoto, Satoru*; Kuga, Kentaro*; Kiss, Takayuki*; et al.

Physical Review B, 98(12), p.121113_1 - 121113_6, 2018/09


 Times Cited Count:4 Percentile:22.49(Materials Science, Multidisciplinary)

Journal Articles

Effect of $$B$$-site randomness on the antiferroelectric/relaxor nature of the ground state; Diffuse and inelastic X-ray scattering study of Pb(In$$_{1/2}$$Nb$$_{1/2}$$)O$$_3$$

Owada, Kenji*; Tsukada, Shinya*; Fukuda, Tatsuo; Tsutsui, Satoshi*; Baron, A. Q. R.*; Mizuki, Junichiro*; Owa, Hidehiro*; Yasuda, Naohiko*; Terauchi, Hikaru*

Physical Review B, 98(5), p.054106_1 - 054106_10, 2018/08

 Times Cited Count:3 Percentile:16.9(Materials Science, Multidisciplinary)

454 (Records 1-20 displayed on this page)