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Journal Articles

Anomalous small-angle X-ray scattering (ASAXS) study of irradiation-induced nanostructure change in Fe-ion beam irradiated oxide dispersion-strengthened (ODS) steel

Kumada, Takayuki; Oba, Yojiro; Motokawa, Ryuhei; Morooka, Satoshi; Tominaga, Aki; Tanida, Hajime; Shobu, Takahisa; Konno, Azusa; Owada, Kenji*; Ono, Naoko*; et al.

Journal of Nuclear Materials, 528, p.151890_1 - 151890_7, 2020/01

 Times Cited Count:0 Percentile:100(Materials Science, Multidisciplinary)

We have developed an anomalous small-angle X-ray scattering (ASAXS) diffractometer in SPring-8 to investigate irradiation-induced nanostructural change in ion-beam irradiated stainless steel. A thermally-aged MA956 stainless steel sample displays power-law scattering that follows the Porod law at the magnitude of scattering vector, Q, below 0.5 nm$$^-1$$ and an overlapped shoulder around 0.7 nm$$^-1$$. After the ion-beam irradiation, the intensity of the shoulder remained unchanged, whereas that of the power-law scattering nearly doubled. This result indicates that none of the structural parameters of the Cr-rich nanoprecipitates, such as the number density, size, and interface roughness, were changed by the irradiation.

Journal Articles

Revising the 4${it f}$ symmetry in CeCu$$_{2}$$Ge$$_{2}$$; Soft X-ray absorption and hard X-ray photoemission spectroscopy

Aratani, Hidekazu*; Nakatani, Yasuhiro*; Fujiwara, Hidenori*; Kawada, Moeki*; Kanai, Yuina*; Yamagami, Kohei*; Fujioka, Shuhei*; Hamamoto, Satoru*; Kuga, Kentaro*; Kiss, Takayuki*; et al.

Physical Review B, 98(12), p.121113_1 - 121113_6, 2018/09

AA2018-0352.pdf:1.16MB

 Times Cited Count:3 Percentile:63.29(Materials Science, Multidisciplinary)

Journal Articles

Effect of $$B$$-site randomness on the antiferroelectric/relaxor nature of the ground state; Diffuse and inelastic X-ray scattering study of Pb(In$$_{1/2}$$Nb$$_{1/2}$$)O$$_3$$

Owada, Kenji*; Tsukada, Shinya*; Fukuda, Tatsuo; Tsutsui, Satoshi*; Baron, A. Q. R.*; Mizuki, Junichiro*; Owa, Hidehiro*; Yasuda, Naohiko*; Terauchi, Hikaru*

Physical Review B, 98(5), p.054106_1 - 054106_10, 2018/08

 Times Cited Count:0 Percentile:100(Materials Science, Multidisciplinary)

Journal Articles

Chemical form analysis of reaction products in Cs-adsorption on stainless steel by means of HAXPES and SEM/EDX

Kobata, Masaaki; Okane, Tetsuo; Nakajima, Kunihisa; Suzuki, Eriko; Owada, Kenji; Kobayashi, Keisuke*; Yamagami, Hiroshi; Osaka, Masahiko

Journal of Nuclear Materials, 498, p.387 - 394, 2018/01

 Times Cited Count:7 Percentile:11(Materials Science, Multidisciplinary)

In this study, for the understandings of Cesium (Cs) adsorption behavior on structure materials in severe accidents at a light water nuclear reactor, the chemical state of Cs and its distribution on the surface of SUS304 stainless steel (SS) with different Si concentration were investigated by hard X-ray photoelectron spectroscopy (HAXPES) and scanning electron microscope / energy dispersive X-ray spectroscopy (SEM/EDX). As a result, it was found that Cs is selectively adsorbed at the site where Si distributes with high concentration. CsFeSiO$$_{4}$$ is a dominant Cs products in the case of low Si content, mainly formed, while Cs$$_{2}$$Si$$_{2}$$O$$_{5}$$ and Cs$$_{2}$$Si$$_{4}$$O$$_{9}$$ are formed in addition to CsFeSiO$$_{4}$$ in the case of high Si content. The chemical forms of the Cs compounds produced in the adsorption process on the SS surface has a close correlation with the concentration and chemical states of Si originally included in SS.

Journal Articles

Mineralogical characterization of radioactive particles from Fukushima soil using $$mu$$-XRD with synchrotron radiation

Motai, Satoko*; Mukai, Hiroki*; Watanuki, Tetsu; Owada, Kenji; Fukuda, Tatsuo; Machida, Akihiko; Kuramata, Chisaki*; Kikuchi, Ryosuke*; Yaita, Tsuyoshi; Kogure, Toshihiro*

Journal of Mineralogical and Petrological Sciences, 111(5), p.305 - 312, 2016/10

 Times Cited Count:11 Percentile:37.29(Mineralogy)

no abstracts in English

Journal Articles

Negative correlation between electrical response and domain size in a Ti-composition-gradient Pb[(Mg$$_{1/3}$$Nb$$_{2/3}$$)$$_{1-x}$$Ti$$_{x}$$]O$$_{3}$$ crystal near the morphotropic phase boundary

Shimizu, Daisuke*; Tsukada, Shinya*; Matsuura, Masato*; Sakamoto, Junya*; Kojima, Seiji*; Namikawa, Kazumichi*; Mizuki, Junichiro; Owada, Kenji

Physical Review B, 92(17), p.174121_1 - 174121_5, 2015/11

 Times Cited Count:8 Percentile:57.71(Materials Science, Multidisciplinary)

The phase diagram and the relationship between the crystal coherence length and electrical response of Pb[(Mg$$_{1/3}$$Nb$$_{2/3}$$)$$_{1-x}$$Ti$$_{x}$$]O$$_{3}$$ (PMN-xPT) near the morphotropic phase boundary (MPB) have been precisely investigated using a single crystal with a Ti composition gradient by synchrotron X-ray diffraction and inelastic light scattering at room temperature. The crystal has two boundaries at Ti compositions of 29.0 mol% and 34.7 mol% which correspond to the phase boundaries between the monoclinic B (MB) and C (MC) phases and between the MC and tetragonal (T) phases, respectively. It is shown that there is a strong negative correlation between the electrical response and the crystal coherence length at the sub-$$mu$$m scale. The results are explained by the size effects of domains near the MPB.

Journal Articles

Progress and status of the gyrotron development for the JT-60SA ECH/CD system

Kobayashi, Takayuki; Sawahata, Masayuki; Terakado, Masayuki; Hiranai, Shinichi; Ikeda, Ryosuke; Oda, Yasuhisa; Wada, Kenji; Hinata, Jun; Yokokura, Kenji; Hoshino, Katsumichi; et al.

Proceedings of 40th International Conference on Infrared, Millimeter, and Terahertz Waves (IRMMW-THz 2015) (USB Flash Drive), 3 Pages, 2015/08

A gyrotron for electron cyclotron heating and current drive (ECH/CD) has been developed for JT-60SA (Super-Advanced). In high-power, long-pulse operations, oscillations of 1 MW/100 s have been demonstrated at both 110 GHz and 138 GHz, for the first time. These results fully satisfied the requirements for JT-60SA. Moreover, it was experimentally shown that the higher power operation at each frequency is expected to be acceptable for this gyrotron from the viewpoint of heat load at the cavity resonator, collector, and stray radiation absorbers. An oscillation at 82 GHz, which is an additional frequency, has been demonstrated up to 2 s at the output power of 0.4 MW, so far. High power experiments toward higher power of 1.5 MW (110/138 GHz) and 1 MW (82 GHz) are ongoing.

Journal Articles

Spontaneous formation of suboxidic coordination around Co in ferromagnetic rutile Ti$$_{0.95}$$Co$$_{0.05}$$O$$_2$$ film

Hu, W.*; Hayashi, Koichi*; Fukumura, Tomoteru*; Akagi, Kazuto*; Tsukada, Masaru*; Happo, Naohisa*; Hosokawa, Shinya*; Owada, Kenji; Takahashi, Masamitsu; Suzuki, Motohiro*; et al.

Applied Physics Letters, 106(22), p.222403_1 - 222403_5, 2015/06

 Times Cited Count:28 Percentile:16.33(Physics, Applied)

Journal Articles

Gyrotron development for high-power, long-pulse electron cyclotron heating and current drive at two frequencies in JT-60SA and its extension toward operation at three frequencies

Kobayashi, Takayuki; Moriyama, Shinichi; Yokokura, Kenji; Sawahata, Masayuki; Terakado, Masayuki; Hiranai, Shinichi; Wada, Kenji; Sato, Yoshikatsu; Hinata, Jun; Hoshino, Katsumichi; et al.

Nuclear Fusion, 55(6), p.063008_1 - 063008_8, 2015/06

 Times Cited Count:17 Percentile:20.44(Physics, Fluids & Plasmas)

A gyrotron enabling high-power, long-pulse oscillations at both 110 GHz and 138 GHz has been developed for electron cyclotron heating (ECH) and current drive (CD) in JT-60SA. Oscillations of 1 MW for 100 s have been demonstrated at both frequencies, for the first time as a gyrotron operating at two frequencies. The optimization of the anode voltage, or the electron pitch factor, using a triode gun was a key to obtain high power and high efficiency at two frequencies. It was also confirmed that the internal losses in the gyrotron were sufficiently low for expected long pulse operation at the higher power level of $$sim$$1.5 MW. Another important result is that an oscillation at 82 GHz, which enables to use fundamental harmonic waves in JT-60SA while the other two frequencies are used as second harmonics waves, was demonstrated up to 0.4 MW for 2 s. These results of the gyrotron development significantly contribute to enhancing operation regime of the ECH/CD system in JT-60SA.

JAEA Reports

Research on engineering technology in the full-scale demonstration of EBS and operation technology for HLW disposal; Research report in 2013 (Joint research)

Fujita, Tomoo; Tanai, Kenji; Nakayama, Masashi; Sawada, Sumiyuki*; Asano, Hidekazu*; Saito, Masahiko*; Yoshino, Osamu*; Kobayashi, Masato*

JAEA-Research 2014-031, 44 Pages, 2015/03

JAEA-Research-2014-031.pdf:16.11MB

Japan Atomic Energy Agency (JAEA) and Radioactive Waste Management Funding and Research Center (RWMC) concluded the letter of cooperation agreement on the research and development of radioactive waste disposal in April, 2005, and have been carrying out the collaboration work based on the agreement. JAEA have been carrying out the Horonobe Underground Research Laboratory (URL) Project which is intended for a sedimentary rock in the Horonobe town, Hokkaido, since 2001. In the project, geoscientific research and research and development on geological disposal technology are being promoted. Meanwhile, the government (the Agency for Natural Resources and Energy, Ministry of Economy, Trade and Industry) has been promoting construction of equipments for the full-scale demonstration of engineered barrier system (EBS) and operation technology for high-level radioactive waste (HLW) disposal since 2008, to enhance public's understanding to the geological disposal of HLW, e.g. using underground facility. RWMC received an order of the project in fiscal year 2012 (2011/2012) continuing since fiscal year 2008 (2008/2009). Since topics in this project are included in the Horonobe URL Project, JAEA carried out this project as collaboration work continuing since fiscal year 2008. This report summarizes the results of engineering technology carried out in this collaboration work in fiscal year 2013. In fiscal year 2013, emplacement tests using buffer material block for the vertical emplacement concept were carried out and visualization tests for water penetration in buffer material were carried out.

Journal Articles

Development of a dual frequency (110/138 GHz) gyrotron for JT-60SA and its extension to an oscillation at 82 GHz

Kobayashi, Takayuki; Moriyama, Shinichi; Isayama, Akihiko; Sawahata, Masayuki; Terakado, Masayuki; Hiranai, Shinichi; Wada, Kenji; Sato, Yoshikatsu; Hinata, Jun; Yokokura, Kenji; et al.

EPJ Web of Conferences, 87, p.04008_1 - 04008_5, 2015/03

 Times Cited Count:4 Percentile:13.79

A dual-frequency gyrotron, which can generate 110 GHz and 138 GHz waves independently, is being developed in JAEA to enable electron cyclotron heating (ECH) and current drive (ECCD) in a wider range of plasma discharge conditions of JT-60SA. Operation for the gyrotron conditioning and parameter optimization toward 1 MW for 100 s, which is the target output power and pulse length for JT-60SA, is in progress without problems. Oscillations of 1 MW for 10 s and 0.51 MW for 198 s were obtained, so far, at both frequencies. In addition, an oscillation (0.3 MW for 20 ms) at 82 GHz was demonstrated as an additional frequency of the dual-frequency gyrotron which shows a possibility of the use of fundamental harmonic wave in JT-60SA.

Journal Articles

Heterophase fluctuations near $$T_{rm c}$$ in the relaxor ferroelectrics (1-x)Pb(Zn$$_{1/3}$$Nb$$_{2/3}$$)O$$_{3}$$-xPbTiO$$_{3}$$ ($$x$$ = 0.09) studied by X-ray diffuse scattering and coherent X-ray scattering

Owada, Kenji; Mizuki, Junichiro*; Matsushita, Mitsuyoshi*; Namikawa, Kazumichi*

Physical Review B, 90(10), p.104109_1 - 104109_12, 2014/09

 Times Cited Count:5 Percentile:69.29(Materials Science, Multidisciplinary)

The paraelectric (PE) to ferroelectric (FE) first-order phase transition of 0.91Pb(Zn$$_{1/3}$$Nb$$_{2/3}$$)O$$_{3}$$-0.09PbTiO$$_{3}$$ ($$T_{c}^{c}$$ = 455 K on cooling) has been studied by the complementary use of X-ray diffuse scattering (XDS) and coherent X-ray scattering (CXS). XDS was mainly used to investigate the FE regions, while CXS was mainly used to investigate the PE regions above $$T_{c}^{c}$$ on cooling. The diffuse scattering intensity due to the appearance of FE regions shows a maximum at $$T_{rm max}= 460$$ K. The diffuse scattering is dynamic in nature and the softening trend changes to a hardening trend at $$T_{rm max}$$. This means that the FE instability is maximum at $$T_{rm max}$$ and therefore the FE regions are well stabilized below $$T_{rm max} $$. The spatial autocorrelation function obtained by CXS, corresponding to the texture of PE regions, starts to rapidly change at about $$T_{rm max}$$ and is most unstable at $$T_{c}^{c}$$. We conclude that a heterophase fluctuation occurs between $$T_{c}^{c}$$ and $$T_{rm max}$$ near the phase transition. The heterophase fluctuation can be expected to correlate to the low-frequency dielectric dispersion and contribute to the phase transition as a precursor phenomenon of the first-order phase transition.

Journal Articles

Acute and obtuse rhombohedrons in the local structures of relaxor ferroelectric Pb(Mg$$_{1/3}$$Nb$$_{2/3}$$)O$$_3$$

Hu, W.*; Hayashi, Koichi*; Owada, Kenji; Chen, J.*; Happo, Naohisa*; Hosokawa, Shinya*; Takahashi, Masamitsu; Bokov, A.*; Ye, Z.-G*

Physical Review B, 89(14), p.140103_1 - 140103_5, 2014/04

 Times Cited Count:33 Percentile:14.32(Materials Science, Multidisciplinary)

JAEA Reports

Development of instrument to measure transmission power density distribution using dielectric disk in millimeter waveguide

Yokokura, Kenji; Moriyama, Shinichi; Kobayashi, Takayuki; Hiranai, Shinichi; Sawahata, Masayuki; Terakado, Masayuki; Hinata, Jun; Wada, Kenji; Sato, Yoshikatsu; Hoshino, Katsumichi; et al.

JAEA-Technology 2014-002, 64 Pages, 2014/03

JAEA-Technology-2014-002.pdf:6.83MB

A new instrument has been developed to measure spatial distribution of power density and total power of the millimeter wave, by measuring temperature rise of dielectric material inserted in the waveguide. For a measurement, a dielectric disk with thermally insulated support is inserted into the few millimeters gap in the waveguide. The disk is heated by the millimeter wave pulse for 0.1$$sim$$0.2 s, and immediately after the pulse, it is pulled up and its temperature distribution is measured by an infrared camera to estimate the spatial power density distribution of the millimeter wave. In the other hand, total transmission power is estimated by the disk temperature reached equilibrium. In the measurement test, deformation of the power density distribution was successfully detected when the mirror angle was intentionally changed in the matching optics unit (MOU) at the waveguide input from the gyrotron. The test result shows that the instrument is effective for both adjustment of MOU without opening the vacuum boundary and to detect any abnormal transmission during operation of the ECH system. The test also shows high reliability of the instrument which stands with 1 MW high power transmission without any arcing or pressure rise in vacuum region. The instrument will be contributed to keep good condition of high power long pulse ECH system by detecting abnormal transmission in the waveguide in operation without open vacuum boundary.

JAEA Reports

Research on engineering technology in the full-scale demonstration of EBS and operation technology for HLW disposal; Research report in 2012 (Joint research)

Nakatsuka, Noboru; Sato, Haruo; Tanai, Kenji; Nakayama, Masashi; Sawada, Sumiyuki*; Asano, Hidekazu*; Saito, Masahiko*; Yoshino, Osamu*; Tsukahara, Shigeki*; Hishioka, Sosuke*; et al.

JAEA-Research 2013-034, 70 Pages, 2014/01

JAEA-Research-2013-034.pdf:9.11MB

Japan Atomic Energy Agency (JAEA) and Radioactive Waste Management Funding and Research Center (RWMC) concluded the letter of cooperation agreement on the research and development of radioactive waste disposal in April, 2005, and have been carrying out the collaboration work based on the agreement. JAEA have been carrying out the Horonobe Underground Research Laboratory (URL) Project which is intended for a sedimentary rock in the Horonobe town, Hokkaido, since 2001. In the project, geoscientific research and research and development on geological disposal technology are being promoted. Meanwhile, the government (the Agency for Natural Resources and Energy, Ministry of Economy, Trade and Industry) has been promoting construction of equipments for the full-scale demonstration of engineered barrier system and operation technology for high-level radioactive waste (HLW) disposal since 2008, to enhance public's understanding to the geological disposal of HLW, e.g. using underground facility. RWMC received an order of the project in fiscal year 2012 (2011/2012) continuing since fiscal year 2008 (2008/2009). Since topics in this project are included in the Horonobe URL Project, JAEA carried out this project as collaboration work continuing in fiscal year 2008. This report summarizes the results of engineering technology carried out in this collaboration work in fiscal year 2012. In fiscal year 2012, part of the equipments for emplacement of buffer material was produced and visualization test for water penetration in buffer material were carried out.

Journal Articles

Verification and validation procedures of calculation codes for determining corrosive conditions in the BWR primary cooling system based on water radiolysis and mixed potential models

Uchida, Shunsuke*; Wada, Yoichi*; Yamamoto, Seiji*; Takagi, Junichi*; Hisamune, Kenji*

Journal of Nuclear Science and Technology, 51(1), p.24 - 36, 2014/01

 Times Cited Count:4 Percentile:59.06(Nuclear Science & Technology)

ECP in the BWR primary cooling system can be measured only in the restricted region. In order to determine ECP at any location, ECP should be evaluated by computer simulation codes consisting of water radiolysis models to determine the concentrations of corrosive radiolytic species and mixed potential models to determine ECP based on corrosive species. Mitigation of SCC crack growth rate due to decreasing ECP can be authorized by the JSME Standards, while mitigation of ECP due to hydrogen addition has not been authorized yet. In the paper, standard procedures to authorize the computer simulation codes based on the verification and validation method are proposed. The numerical justification of every code applied as a standard code should be verified and its accuracy and applicability for plant analysis should be validated. Benchmark problems for verification processes are proposed and comparison of the calculated results with the measured ones for the plant of evaluation is required.

JAEA Reports

Research on engineering technology in the full-scale demonstration of EBS and operation technology for HLW disposal; Research report in 2011 (Joint research)

Nakatsuka, Noboru; Sato, Haruo; Tanai, Kenji; Sugita, Yutaka; Nakayama, Masashi; Sawada, Sumiyuki*; Niinuma, Hiroaki*; Asano, Hidekazu*; Saito, Masahiko*; Yoshino, Osamu*; et al.

JAEA-Research 2013-027, 34 Pages, 2013/11

JAEA-Research-2013-027.pdf:5.84MB

Japan Atomic Energy Agency (JAEA) and Radioactive Waste Management Funding and Research Center (RWMC) concluded the letter of cooperation agreement on the research and development of radioactive waste disposal in April, 2005, and have been carrying out the collaboration work based on the agreement. JAEA have been carrying out the Horonobe Underground Research Laboratory (URL) Project which is intended for a sedimentary rock in the Horonobe town, Hokkaido, since 2001. In the project, geoscientific research and research and development on geological disposal technology are being promoted. Meanwhile, the government (the Agency for Natural Resources and Energy, Ministry of Economy, Trade and Industry) has been promoting construction of equipments for the full-scale demonstration of engineered barrier system and operation technology for high-level radioactive waste (HLW) disposal since 2008, to enhance public's understanding to the geological disposal of HLW, e.g. using underground facility. RWMC received an order of the project in fiscal year 2010 (2010/2011) continuing since fiscal year 2008 (2008/2009). Since topics in this project are included in the Horonobe URL Project, JAEA carried out this project as collaboration work continuing in fiscal year 2008. This report summarizes the results of engineering technology carried out in this collaboration work in fiscal year 2011. In fiscal year 2011, part of the equipments for emplacement of buffer material was produced and visualization test for water penetration in buffer material were carried out.

Journal Articles

Development of a linear motion antenna for the JT-60SA ECRF system

Moriyama, Shinichi; Kobayashi, Takayuki; Isayama, Akihiko; Hoshino, Katsumichi; Suzuki, Sadaaki; Hiranai, Shinichi; Yokokura, Kenji; Sawahata, Masayuki; Terakado, Masayuki; Hinata, Jun; et al.

Fusion Engineering and Design, 88(6-8), p.935 - 939, 2013/10

 Times Cited Count:4 Percentile:59.76(Nuclear Science & Technology)

An antenna having a first mirror driven in the linear motion (LM) and a fixed second mirror was proposed for electron cyclotron range of frequency (ECRF) heating and current drive system, to minimize the risk of cooling-water-leakage. Basic mechanical feasibilities of the bellows covering the movable structures of the antenna were previously investigated using a mock-up. This time, a support structure of the shaft has been designed using a metallic sliding bearing with solid lubricant. The sliding bearing can support combination of linear and rotational motions while a ball bearing supports either linear or rotational motion. We have newly installed the sliding bearing into the mock-up. A vacuum pumping test has been carried out paying attention to the influence of the solid lubricant by mass analysis. To design the LM antenna for JT-60SA in detail, heating and current drive characteristics for typical experimental scenarios of JT-60SA has been investigated by calculation.

Journal Articles

Effect of salt-containing filter paper attached to osmotic membrane

Sano, Kenji*; Yamada, Arisa*; Matsui, Akihiro*; Tsuji, Hideyuki*; Hasegawa, Shin; Sawada, Shinichi; Maekawa, Yasunari

Desalination, 324, p.34 - 36, 2013/09

 Times Cited Count:1 Percentile:92.03(Engineering, Chemical)

Anchored osmotic pressure inducer was examined. Salt-containing filter paper attached to an osmotic membrane increased the water flux to more than 10% at 1 MPa. The salt-containing filter paper was fabricated via graft polymerization of acrylic acid onto a filter paper followed by alkaline treatment. The filter paper was characterized by thermo gravimetric analysis (TGA), attenuated total reflection Fourier transform infrared spectroscopy (ATR-FTIR), scanning electronic microscopy-energy dispersive X-ray spectrometry(SEM-EDS).

Journal Articles

Full-coherent free electron laser seeded by 13th- and 15th-order harmonics of near-infrared femtosecond laser pulses

Sato, Takahiro*; Iwasaki, Atsushi*; Owada, Shigeki*; Yamanouchi, Kaoru*; Takahashi, Eiji*; Midorikawa, Katsumi*; Aoyama, Makoto; Yamakawa, Koichi; Togashi, Tadashi*; Fukami, Kenji*; et al.

Journal of Physics B; Atomic, Molecular and Optical Physics, 46(16), p.164006_1 - 164006_6, 2013/08

 Times Cited Count:3 Percentile:76.91(Optics)

By introducing 13th- (61.7 nm) and 15th-order harmonics (53.4 nm) of femtosecond laser pulses at 800 nm into an undulator of SCSS (SPring-8 Compact SASE Source) test accelerator at RIKEN, these harmonic pulses were amplified by a factor of more than 10$$^{2}$$ with a high contrast ratio through the interaction between accelerated electron bunches and the harmonic pulses. From numerical simulations of the amplification processes of high-order harmonic pulses in the undulator, optimum conditions of the electron bunch duration interacting with the high-order harmonic pulses were investigated for generating full-coherent and intense pulses in the extreme ultraviolet wavelength region.

236 (Records 1-20 displayed on this page)