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Journal Articles

Overvoltage reduction in membrane Bunsen reaction for hydrogen production by using a radiation-grafted cation exchange membrane and porous Au anode

Sawada, Shinichi*; Kimura, Takehiro*; Nishijima, Haruyuki*; Kodaira, Takahide*; Tanaka, Nobuyuki; Kubo, Shinji; Imabayashi, Shinichiro*; Nomura, Mikihiro*; Yamaki, Tetsuya*

International Journal of Hydrogen Energy, 45(27), p.13814 - 13820, 2020/05

 Times Cited Count:0 Percentile:100(Chemistry, Physical)

An electrochemical membrane Bunsen reaction using a cation exchange membrane (CEM) is a key to achieving an iodine-sulfur (IS) thermochemical water splitting process for mass-production of hydrogen. In this study, we prepared both the radiation-grafted CEM with a high ion exchange capacity (IEC) and the highly-porous Au-electroplated anode, and then used them for the membrane Bunsen reaction to reduce the cell overvoltage. The high-IEC grafted CEM exhibited low resistivity for proton transport, while the porous Au anode had a large effective surface area for anodic SO$$_{2}$$ oxidation reaction. As a result, the cell overvoltage for the membrane Bunsen reaction was significantly reduced to 0.21 V at 200 mA/cm$$^{2}$$, which was only one-third of that of the previous test using the commercial CEM and non-porous anode. From the analysis of the current-voltage characteristics, employment of the grafted CEM was found to be more effective for the overvoltage reduction compared to the porous Au anode.

Journal Articles

Photoneutron detection in lightning by gadolinium orthosilicate scintillators

Wada, Yuki*; Nakazawa, Kazuhiro*; Enoto, Teruaki*; Furuta, Yoshihiro; Yuasa, Takayuki*; Makishima, Kazuo*; Tsuchiya, Harufumi

Physical Review D, 101(10), p.102007_1 - 102007_6, 2020/05

 Times Cited Count:0 Percentile:100(Astronomy & Astrophysics)

Journal Articles

Anomalous small-angle X-ray scattering (ASAXS) study of irradiation-induced nanostructure change in Fe-ion beam irradiated oxide dispersion-strengthened (ODS) steel

Kumada, Takayuki; Oba, Yojiro; Motokawa, Ryuhei; Morooka, Satoshi; Tominaga, Aki; Tanida, Hajime; Shobu, Takahisa; Konno, Azusa; Owada, Kenji*; Ono, Naoko*; et al.

Journal of Nuclear Materials, 528, p.151890_1 - 151890_7, 2020/01

 Times Cited Count:0 Percentile:100(Materials Science, Multidisciplinary)

We have developed an anomalous small-angle X-ray scattering (ASAXS) diffractometer in SPring-8 to investigate irradiation-induced nanostructural change in ion-beam irradiated stainless steel. A thermally-aged MA956 stainless steel sample displays power-law scattering that follows the Porod law at the magnitude of scattering vector, Q, below 0.5 nm$$^-1$$ and an overlapped shoulder around 0.7 nm$$^-1$$. After the ion-beam irradiation, the intensity of the shoulder remained unchanged, whereas that of the power-law scattering nearly doubled. This result indicates that none of the structural parameters of the Cr-rich nanoprecipitates, such as the number density, size, and interface roughness, were changed by the irradiation.

Journal Articles

Liquid film behavior and heat-transfer mechanism near the rewetting front in a single rod air-water system

Wada, Yuki; Le, T. D.; Satou, Akira; Shibamoto, Yasuteru; Yonomoto, Taisuke

Journal of Nuclear Science and Technology, 57(1), p.100 - 113, 2020/01

 Times Cited Count:0 Percentile:100(Nuclear Science & Technology)

Journal Articles

Study on dryout and rewetting during accidents including ATWS for the BWR at JAEA

Satou, Akira; Wada, Yuki; Shibamoto, Yasuteru; Yonomoto, Taisuke

Nuclear Engineering and Design, 354, p.110164_1 - 110164_10, 2019/12

 Times Cited Count:1 Percentile:50.57(Nuclear Science & Technology)

JAEA has conducted a series of experimental researches on the Post-boiling transition heat transfer, transient critical heat flux and rewetting for BWRs. Experimental data bases covering the anticipated operational conditions was developed; the significance of the precursor cooling was identified. This paper presents approaches of the present research focusing on the anticipated transient without scram, effects of the spacer and physical understanding of the phenomena for development of mechanistic model together with promising results obtained so far.

Journal Articles

Conceptual study on parasitic low-energy RI beam production with in-flight separator BigRIPS and the first stopping examination for high-energy RI beams in the parasitic gas cell

Sonoda, Tetsu*; Katayama, Ichiro*; Wada, Michiharu*; Iimura, Hideki; Sonnenschein, V.*; Iimura, Shun*; Takamine, Aiko*; Rosenbusch, M.*; Kojima, Takao*; Ahn, D. S.*; et al.

Progress of Theoretical and Experimental Physics (Internet), 2019(11), p.113D02_1 - 113D02_12, 2019/11

 Times Cited Count:0 Percentile:100(Physics, Multidisciplinary)

An in-flight separator, BigRIPS, at RIBF in RIKEN provides each experiment with specific nuclides separated from many nuclides produced by projectile fragmentation or in-flight fission. In this process, nuclides other than separated ones are discarded on the slits in BigRIPS, although they include many nuclides interested from the view point of nuclear structure. In order to extract these nuclides for parasitic experiments, we are developing a method using laser ion-source (PALIS). A test experiment with $$^{78}$$Se beam from RIBF has been performed by using a gas cell set in BigRIPS. Unstable nuclides around $$^{67}$$Se were stopped in the gas cell in accordance with a calculation using LISE code. The stopping efficiency has been estimated to be about 30%. As a next step, we will establish the technique for extracting reaction products from the gas cell.

Journal Articles

Contribution of membrane technology to hydrogen society; Development of membrane IS process

Inagaki, Yoshiyuki; Sakaba, Nariaki; Tanaka, Nobuyuki; Nomura, Mikihiro*; Sawada, Shinichi*; Yamaki, Tetsuya*

Nippon Kaisui Gakkai-Shi, 73(4), p.194 - 202, 2019/08

The thermochemical IS process is a promising hydrogen production method which can produce hydrogen in a large amount and stably with high efficiency by thermal splitting of water. Research and development on chemical reaction technology with membranes was conducted for the purpose of improving the efficiency of IS process and application of solar heat. The basic technology of ceramic membranes applied to decomposition reactions of hydrogen iodine and sulfuric acid was developed, and it is expected that the conversion rate on decomposition in each reaction can be remarkably improved. The basic technology of a cation exchange membrane applied to Bunsen reaction was developed with radiation-induced grafting technique, it is expected that the amount of iodine can be reduced to about one-fifth compared to the conventional method. These achievements are important technologies for practical use of the IS process.

Journal Articles

Downward terrestrial gamma-ray flash observed in a winter thunderstorm

Wada, Yuki*; Enoto, Teruaki*; Nakazawa, Kazuhiro*; Furuta, Yoshihiro; Yuasa, Takayuki*; Nakamura, Yoshitaka*; Morimoto, Takeshi*; Matsumoto, Takahiro*; Makishima, Kazuo*; Tsuchiya, Harufumi

Physical Review Letters, 123(6), p.061103_1 - 061103_6, 2019/08

 Times Cited Count:3 Percentile:25.77(Physics, Multidisciplinary)

Journal Articles

Ultrasound measurement of upward liquid film flow in vertical pipe

Wada, Yuki; Satou, Akira; Shibamoto, Yasuteru; Yonomoto, Taisuke; Sagawa, Jun*

Proceedings of 18th International Topical Meeting on Nuclear Reactor Thermal Hydraulics (NURETH-18) (USB Flash Drive), p.4518 - 4531, 2019/08

Liquid film detection under boiling transition (BT) condition is one of the important issues to develop models on dry out and rewet including physical characteristics of liquid film behavior. Although a heater surface temperature has been often used in previous studies to detect the position of liquid film front, it is difficult to accurately identify the position from the temperature measurement. Therefore, we are developing a nonintrusive measurement technique for detecting thin liquid film thickness under BT and rewet condition using ultrasound. In this study, we focus on high accuracy measurement for liquid film thinner than 0.1 mm by using high frequency ultrasound of 15 MHz and developing a signal processing method. Liquid film measurement results were found to agree with liquid film thickness correlations. Based on a comparison with constant current method, it is concluded that the present technique gives more reasonable liquid film thickness than constant current method.

Journal Articles

Research and development on membrane IS process for hydrogen production using solar heat

Myagmarjav, O.; Iwatsuki, Jin; Tanaka, Nobuyuki; Noguchi, Hiroki; Kamiji, Yu; Ioka, Ikuo; Kubo, Shinji; Nomura, Mikihiro*; Yamaki, Tetsuya*; Sawada, Shinichi*; et al.

International Journal of Hydrogen Energy, 44(35), p.19141 - 19152, 2019/07

 Times Cited Count:6 Percentile:23.71(Chemistry, Physical)

Journal Articles

Turbulence intensity profile in high Reynolds number pipe flow

Wada, Yuki; Furuichi, Noriyuki*; Kusano, Eisuke*; Tsuji, Yoshiyuki*

Proceedings of 11th International Symposium on Turbulence and Shear Flow Phenomena (TSFP-11) (Internet), 6 Pages, 2019/07

This paper reports characteristics of turbulence intensity profile obtained in high Reynolds number actual flow facility in Japan. The experiments were performed in a pipe flow with water, and the friction Reynolds number was varied up to $$Re_{tau}$$ = 2.0 $$times$$ 10$$^{4}$$. The streamwise velocity was measured by laser Doppler velocimetry (LDV). The new procedure to correct the measurement volume effect of LDV is suggested and we discuss turbulence intensity issues such as the inner peak Reynolds number dependence and the outer logarithmic behavior, it was found that these characteristic behaviors are consistent with previous turbulence studies.

Journal Articles

Gamma-ray glow preceding downward terrestrial gamma-ray flash

Wada, Yuki*; Enoto, Teruaki*; Nakamura, Yoshitaka*; Furuta, Yoshihiro; Yuasa, Takayuki*; Nakazawa, Kazuhiro*; Morimoto, Takeshi*; Sato, Mitsuteru*; Matsumoto, Takahiro*; Yonetoku, Daisuke*; et al.

Communications Physics (Internet), 2(1), p.67_1 - 67_9, 2019/06

 Times Cited Count:3 Percentile:25.77(Physics, Multidisciplinary)

Journal Articles

High-energy atmospheric phenomena initiated by lightning

Enoto, Teruaki*; Wada, Yuki*; Tsuchiya, Harufumi

Nippon Butsuri Gakkai-Shi, 74(4), p.192 - 200, 2019/04

no abstracts in English

Journal Articles

The Surface composition of asteroid 162173 Ryugu from Hayabusa2 near-infrared spectroscopy

Kitazato, Kohei*; Milliken, R. E.*; Iwata, Takahiro*; Abe, Masanao*; Otake, Makiko*; Matsuura, Shuji*; Arai, Takehiko*; Nakauchi, Yusuke*; Nakamura, Tomoki*; Matsuoka, Moe*; et al.

Science, 364(6437), p.272 - 275, 2019/04

 Times Cited Count:79 Percentile:0.09(Multidisciplinary Sciences)

The near-Earth asteroid 162173 Ryugu, the target of Hayabusa2 sample return mission, is believed to be a primitive carbonaceous object. The Near Infrared Spectrometer (NIRS3) on Hayabusa2 acquired reflectance spectra of Ryugu's surface to provide direct measurements of the surface composition and geological context for the returned samples. A weak, narrow absorption feature centered at 2.72 micron was detected across the entire observed surface, indicating that hydroxyl (OH)-bearing minerals are ubiquitous there. The intensity of the OH feature and low albedo are similar to thermally- and/or shock-metamorphosed carbonaceous chondrite meteorites. There are few variations in the OH-band position, consistent with Ryugu being a compositionally homogeneous rubble-pile object generated from impact fragments of an undifferentiated aqueously altered parent body.

Journal Articles

A Correction method based on probability density function and measurement volume for turbulence intensity profile measured by LDV in turbulent pipe flow

Wada, Yuki; Furuichi, Noriyuki*; Kusano, Eisuke*; Tsuji, Yoshiyuki*

Proceedings of 15th International Conference on Flow Dynamics (ICFD 2018) (USB Flash Drive), p.778 - 779, 2018/11

Spatial resolution effect of LDV (Laser Doppler Velocimetry) on the time-averaged statistics is presented in high Reynolds number turbulent pipe flow. Employing PDF (Probability Density Function) of streamwise velocity, we report the study of overestimation of time-averaged statistics based on the size of measurement volume. We proposed a simple equation to estimate their spatial resolution effect. Using the proposed equation, the measurement position and the measurement volume calculated precisely based on experimental setup, it was found that the correction for spatial resolution effect is possible. Analyzing the pipe flow data measured by LDV, we estimated the expected turbulence intensity profile. The validity of the present correction method was confirmed by comparing the correction result based on the low-resolution experimental result with the high-resolution experimental result.

Journal Articles

Development of ion-exchange membranes for the membrane Bunsen reaction in thermochemical hydrogen production by iodine-sulfur process

Nomura, Mikihiro*; Kodaira, Takahide*; Ikeda, Ayumi*; Naka, Yasuhito*; Nishijima, Haruyuki*; Imabayashi, Shinichiro*; Sawada, Shinichi*; Yamaki, Tetsuya*; Tanaka, Nobuyuki; Kubo, Shinji

Journal of Chemical Engineering of Japan, 51(9), p.726 - 731, 2018/09

 Times Cited Count:2 Percentile:75.37(Engineering, Chemical)

Thermochemical hydrogen production by the iodine-sulfur process decomposes water into hydrogen and oxygen by combining the chemical reactions of iodine and sulfur. Two types of acids are produced through the Bunsen reaction. To improve the performance of this reaction, ion-exchange membranes for the membrane Bunsen reaction should be developed. In the present study, a cation-exchange membrane was prepared by using a radiation-graft polymerization method. It was found that a divinylbenzene crosslinking procedure was very effective in reducing water permeation through the membrane, and the membrane Bunsen reaction was successfully carried out by using the developed crosslinked membrane. Therefore, the developed crosslinked membrane is a potential candidate for cation-exchange membranes for the membrane Bunsen reaction.

Journal Articles

Revising the 4${it f}$ symmetry in CeCu$$_{2}$$Ge$$_{2}$$; Soft X-ray absorption and hard X-ray photoemission spectroscopy

Aratani, Hidekazu*; Nakatani, Yasuhiro*; Fujiwara, Hidenori*; Kawada, Moeki*; Kanai, Yuina*; Yamagami, Kohei*; Fujioka, Shuhei*; Hamamoto, Satoru*; Kuga, Kentaro*; Kiss, Takayuki*; et al.

Physical Review B, 98(12), p.121113_1 - 121113_6, 2018/09


 Times Cited Count:3 Percentile:60.22(Materials Science, Multidisciplinary)

Journal Articles

On the liquid film flow characteristics during the rewetting in the single rod air-water system

Wada, Yuki; Le, T. D.; Satou, Akira; Shibamoto, Yasuteru; Yonomoto, Taisuke

Proceedings of 26th International Conference on Nuclear Engineering (ICONE-26) (Internet), 10 Pages, 2018/07

Journal Articles

Termination of electron acceleration in thundercloud by intracloud/intercloud discharge

Wada, Yuki*; Bowers, G. S.*; Enoto, Teruaki*; Kamogawa, Masashi*; Nakamura, Yoshitaka*; Morimoto, Takeshi*; Smith, D.*; Furuta, Yoshihiro*; Nakazawa, Kazuhiro*; Yuasa, Takayuki*; et al.

Geophysical Research Letters, 45(11), p.5700 - 5707, 2018/06

 Times Cited Count:10 Percentile:13.82(Geosciences, Multidisciplinary)

Journal Articles

Further experiments for mean velocity profile of pipe flow at high Reynolds number

Furuichi, Noriyuki*; Terao, Yoshiya*; Wada, Yuki; Tsuji, Yoshiyuki*

Physics of Fluids, 30(5), p.055101_1 - 055101_7, 2018/05

 Times Cited Count:0 Percentile:100(Mechanics)

697 (Records 1-20 displayed on this page)