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Journal Articles

Production of $$^{88}$$Nb and $$^{170}$$Ta for chemical studies of element 105, Db, using the GARIS gas-jet system

Huang, M.*; Haba, Hiromitsu*; Murakami, Masashi*; Asai, Masato; Kaji, Daiya*; Kanaya, Jumpei*; Kasamatsu, Yoshitaka*; Kikunaga, Hidetoshi*; Kikutani, Yuki*; Komori, Yukiko*; et al.

Journal of Radioanalytical and Nuclear Chemistry, 304(2), p.845 - 849, 2015/05

 Times Cited Count:3 Percentile:24.31(Chemistry, Analytical)

A technique to utilize radioisotopes of Nb and Ta was developed for chemical studies of element 105, Db, by coupling a gas-jet transport system to the RIKEN gas-filled recoil ion separator (GARIS). The short-lived $$^{88}$$Nb and $$^{170}$$Ta were produced with nuclear reactions using a $$^{19}$$F beam whose energy was the same as that to produce $$^{262}$$Db. Then, they were separated with GARIS and extracted to a chemistry laboratory with the gas-jet transport system. By changing only magnetic field of GARIS and inserting an energy degrader and a shutter for recoil ions, we could deliver the $$^{88}$$Nb and $$^{170}$$Ta to a chemistry device for $$^{262}$$Db without changing other experimental conditions.

Journal Articles

Production of $$^{262}$$Db in the $$^{248}$$Cm($$^{19}$$F,5$$n$$)$$^{262}$$Db reaction and decay properties of $$^{262}$$Db and $$^{258}$$Lr

Haba, Hiromitsu*; Huang, M.*; Kaji, Daiya*; Kanaya, Jumpei*; Kudo, Yuki*; Morimoto, Koji*; Morita, Kosuke*; Murakami, Masashi*; Ozeki, Kazutaka*; Sakai, Ryutaro*; et al.

Physical Review C, 89(2), p.024618_1 - 024618_11, 2014/02

 Times Cited Count:26 Percentile:81.76(Physics, Nuclear)

Journal Articles

New result in the production and decay of an isotope, $$^{278}$$113 of the 113th element

Morita, Kosuke*; Morimoto, Koji*; Kaji, Daiya*; Haba, Hiromitsu*; Ozeki, Kazutaka*; Kudo, Yuki*; Sumita, Takayuki*; Wakabayashi, Yasuo*; Yoneda, Akira*; Tanaka, Kengo*; et al.

Journal of the Physical Society of Japan, 81(10), p.103201_1 - 103201_4, 2012/10

 Times Cited Count:175 Percentile:97.25(Physics, Multidisciplinary)

An isotope of the 113th element, $$^{278}$$113, was produced in a nuclear reaction with a $$^{70}$$Zn beam on a $$^{209}$$Bi target. We observed six consecutive $$alpha$$ decays following the implantation of a heavy particle in nearly the same position in the semiconductor detector, in extremely low background condition. The fifth and sixth decays are fully consistent with the sequential decays of $$^{262}$$Db and $$^{258}$$Lr both in decay energies and decay times. This indicates that the present decay chain consisted of $$^{278}$$113, $$^{274}$$Rg (Z = 111), $$^{270}$$Mt (Z = 109), $$^{266}$$Bh (Z = 107), $$^{262}$$Db (Z = 105), and $$^{258}$$Lr (Z = 103) with firm connections. This result, together with previously reported results from 2004 and 2007, conclusively leads the unambiguous production and identification of the isotope $$^{278}$$113, of the 113th element.

Oral presentation

Production and decay properties of $$^{277}$$Cn produced in the reaction of $$^{208}$$Pb+$$^{70}$$Zn

Sumita, Takayuki*; Morimoto, Koji*; Kaji, Daiya*; Ozeki, Kazutaka*; Katori, Kenji*; Sakai, Ryutaro*; Hasebe, Hiroo*; Haba, Hiromitsu*; Yoneda, Akira*; Yoshida, Atsushi*; et al.

no journal, , 

The decay property of $$^{277}$$Cn (atomic number, $$Z=112$$) produced in the $$^{208}$$Pb($$^{70}$$Zn, $$n$$) reaction was studied. The experiment was performed using the gas-filled recoil ion separator (GARIS) at the RIKEN liner accelerator facility (RILAC). The $$^{208}$$Pb target with about 630 $$mu$$g/cm$$^{2}$$ thickness was bombarded with 347.5, 351.5, and 355.5 MeV $$^{70}$$Zn beam. At the beam energy of 351.5 MeV, we observed one $$alpha$$-decay chain from $$^{277}$$Cn. The $$alpha$$-particle energy of $$^{277}$$Cn was $$11.07 pm 0.08$$ MeV and its lifetime was measured to be 0.370 ms. Including our previous result of the $$^{277}$$Cn production in 2004, the cross section of the $$^{208}$$Pb($$^{70}$$Zn, $$n$$) reaction is deduced to be $$0.17^{+0.16}_{-0.10}$$ pb.

Oral presentation

Development of mesoporous alumina for enabling domestic production of $$^{99}$$Mo/$$^{99m}$$Tc

Alowasheeir, A.*; Eguchi, Miharu*; Fujita, Yoshitaka; Tsuchiya, Kunihiko; Wakabayashi, Ryutaro*; Kimura, Tatsuo*; Ariga, Katsuhiko*; Hatano, Kentaro*; Fukumitsu, Nobuyoshi*; Yamauchi, Yusuke*

no journal, , 

In this study, we investigate the influence of surface properties of mesoporous Al$$_{2}$$O$$_{2}$$ on $$^{99}$$Mo adsorption and $$^{99m}$$Tc elution properties for practical $$^{99}$$Mo/$$^{99m}$$Tc generators. It is clarified that the quantity of -OH groups on the surface of mesoporous walls affects the adsorbed $$^{99}$$Mo amount. Our mesoporous Al$$_{2}$$O$$_{2}$$ demonstrates two times higher the $$^{99}$$Mo adsorption capacity than commercial Al$$_{2}$$O$$_{3}$$.

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