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JAEA Reports

Research plan on geosphere stability for long-term isolation of radioactive waste (Scientific program for fiscal year 2020)

Ishimaru, Tsuneari; Ogata, Nobuhisa; Shimada, Koji; Kokubu, Yoko; Niwa, Masakazu; Asamori, Koichi; Watanabe, Takahiro; Sueoka, Shigeru; Komatsu, Tetsuya; Yokoyama, Tatsunori; et al.

JAEA-Review 2020-010, 46 Pages, 2020/07

JAEA-Review-2020-010.pdf:1.89MB

This report is a plan of research and development (R&D) on geosphere stability for long-term isolation of high-level radioactive waste (HLW) in Japan Atomic Energy Agency (JAEA), in fiscal year 2020. The objectives and contents in fiscal year 2020 are described in detail based on the JAEA 3rd Medium- and Long-term Plan (fiscal years 2015-2021). In addition, the background of this research is described from the necessity and the significance for site investigation and safety assessment, and the past progress. The plan framework is structured into the following categories: (1) Development and systematization of investigation techniques, (2) Development of models for long-term estimation and effective assessment, (3) Development of dating techniques.

Journal Articles

The Chemistry of uranium (I); Basics and application

Sato, Nobuaki*; Kirishima, Akira*; Watanabe, Masayuki

Uran No Kagaku (I); Kiso To Oyo, 184 Pages, 2020/06

This particular book deals with fundamental items related with chemistry of Uranium and consists of basic section and practical section. In the basic section, inorganic and radiochemistry of Uranium was described. On the other hand, in the practical section, the process chemistry related with reprocessing of nuclear fuels and "debris" involved with Fukushima Daiichi Power Plant accident were described. This book is intended for use by scientists, engineers and students in the nuclear industry in their education and/or professional practice.

Journal Articles

Development of one-dimensional optical fiber type radiation distribution sensing method based on wavelength spectrum unfolding

Terasaka, Yuta; Watanabe, Kenichi*; Uritani, Akira*; Yamazaki, Atsushi*; Sato, Yuki; Torii, Tatsuo; Wakaida, Ikuo

Proceedings of International Youth Nuclear Congress 2020 (IYNC 2020) (Internet), 4 Pages, 2020/05

Journal Articles

Pulsed neutron imaging based crystallographic structure study of a Japanese sword made by Sukemasa in the Muromachi period

Oikawa, Kenichi; Kiyanagi, Yoshiaki*; Sato, Hirotaka*; Omae, Kazuma*; Pham, A.*; Watanabe, Kenichi*; Matsumoto, Yoshihiro*; Shinohara, Takenao; Kai, Tetsuya; Harjo, S.; et al.

Materials Research Proceedings, Vol.15, p.207 - 213, 2020/02

Journal Articles

Intercomparison of numerical atmospheric dispersion prediction models for emergency response to emissions of radionuclides with limited source information in the Fukushima Dai-ichi Nuclear Power Plant accident

Iwasaki, Toshiki*; Sekiyama, Tsuyoshi*; Nakajima, Teruyuki*; Watanabe, Akira*; Suzuki, Yasushi*; Kondo, Hiroaki*; Morino, Yu*; Terada, Hiroaki; Nagai, Haruyasu; Takigawa, Masayuki*; et al.

Atmospheric Environment, 214, p.116830_1 - 116830_11, 2019/10

 Times Cited Count:0 Percentile:100(Environmental Sciences)

The utilization of numerical atmospheric dispersion prediction (NDP) models for accidental discharge of radioactive substances was recommended by a working group of the Meteorological Society of Japan. This paper is to validate the recommendation through NDP model intercomparison in the accidental release from the Fukushima Dai-ichi Nuclear Power Plant in 2011. Emission intensity is assumed to be constant during the whole forecast period for the worst-case scenario unless time sequence of emission is available. We expect to utilize forecasts of surface air contaminations for preventions of inhalations of radioactive substances, and column-integrated amounts for mitigation of radiation exposure associated with wet deposition. Although NDP forecasts have ensemble spread, they commonly figure out relative risk in space and time. They are of great benefit to disseminating effective warnings to public without failure. The multi-model ensemble technique may be effective to improve the reliability.

Journal Articles

Application of unstructured mesh-based sodium-water reaction analysis code SERAPHIM

Uchibori, Akihiro; Shiina, Yoshimi*; Watanabe, Akira*; Takata, Takashi

Proceedings of 18th International Topical Meeting on Nuclear Reactor Thermal Hydraulics (NURETH-18) (USB Flash Drive), p.5315 - 5324, 2019/08

A computational fluid dynamics code SERAPHIM for a sodium-water reaction phenomenon has been developed. An unstructured mesh-based analysis method has been integrated into this code for evaluation in a complex-shaped domain including multiple heat transfer tubes in our recent studies. In this study, a numerical analysis of an experiment on sodium-water reaction in a tube bundle domain was performed to investigate applicability of the unstructured mesh-based SERAPHIM code. The formulated high-temperature region and its temperature level agreed with an experimental result.

Journal Articles

The Surface composition of asteroid 162173 Ryugu from Hayabusa2 near-infrared spectroscopy

Kitazato, Kohei*; Milliken, R. E.*; Iwata, Takahiro*; Abe, Masanao*; Otake, Makiko*; Matsuura, Shuji*; Arai, Takehiko*; Nakauchi, Yusuke*; Nakamura, Tomoki*; Matsuoka, Moe*; et al.

Science, 364(6437), p.272 - 275, 2019/04

 Times Cited Count:79 Percentile:0.09(Multidisciplinary Sciences)

The near-Earth asteroid 162173 Ryugu, the target of Hayabusa2 sample return mission, is believed to be a primitive carbonaceous object. The Near Infrared Spectrometer (NIRS3) on Hayabusa2 acquired reflectance spectra of Ryugu's surface to provide direct measurements of the surface composition and geological context for the returned samples. A weak, narrow absorption feature centered at 2.72 micron was detected across the entire observed surface, indicating that hydroxyl (OH)-bearing minerals are ubiquitous there. The intensity of the OH feature and low albedo are similar to thermally- and/or shock-metamorphosed carbonaceous chondrite meteorites. There are few variations in the OH-band position, consistent with Ryugu being a compositionally homogeneous rubble-pile object generated from impact fragments of an undifferentiated aqueously altered parent body.

Journal Articles

Development of unstructured mesh-based numerical method for sodium-water reaction phenomenon

Uchibori, Akihiro; Watanabe, Akira*; Takata, Takashi; Ohshima, Hiroyuki

Nuclear Technology, 205(1-2), p.119 - 127, 2019/01

 Times Cited Count:0 Percentile:100(Nuclear Science & Technology)

To evaluate a sodium-water reaction phenomenon in a steam generator of sodium-cooled fast reactors, a computational fluid dynamics code SERAPHIM, in which a compressible multicomponent multiphase flow with sodium-water chemical reaction is computed, has been developed. The original SERAPHIM code is based on the difference method. In this study, unstructured mesh-based numerical method was developed to advance a numerical accuracy for the complex-shaped domain including multiple heat transfer tubes. Numerical analysis of an underexpanded jet experiment was performed as part of validation of the unstructured mesh-based numerical method. The calculated pressure profile and location of the Mach disk showed good agreement with the experimental data. Applicability of the numerical method for the actual situation was confirmed through the analysis of water vapor discharging into liquid sodium.

Journal Articles

Prediction of the drying behavior of debris in Fukushima Daiichi Nuclear Power Station for dry storage

Nakayoshi, Akira; Suzuki, Seiya; Okamura, Nobuo; Watanabe, Masayuki; Koizumi, Kenji

Journal of Nuclear Science and Technology, 55(10), p.1119 - 1129, 2018/10

 Times Cited Count:0 Percentile:100(Nuclear Science & Technology)

Journal Articles

First direct mass measurements of nuclides around $$Z$$ = 100 with a multireflection time-of-flight mass spectrograph

Ito, Yuta*; Schury, P.*; Wada, Michiharu*; Arai, Fumiya*; Haba, Hiromitsu*; Hirayama, Yoshikazu*; Ishizawa, Satoshi*; Kaji, Daiya*; Kimura, Sota*; Koura, Hiroyuki; et al.

Physical Review Letters, 120(15), p.152501_1 - 152501_6, 2018/04

 Times Cited Count:29 Percentile:3.45(Physics, Multidisciplinary)

Masses of $$^{246}$$Es, $$^{251}$$Fm and the transfermium nuclei $$^{249-252}$$Md, and $$^{254}$$No, produced by hot- and cold-fusion reactions, in the vicinity of the deformed $$N=152$$ neutron shell closure, have been directly measured using a multi-reflection time-of-flight mass spectrograph. The masses of $$^{246}$$Es and $$^{249,250,252}$$Md were measured for the first time. Using the masses of $$^{249,250}$$Md as anchor points for $$alpha$$ decay chains, the masses of heavier nuclei, up to $$^{261}$$Bh and $$^{266}$$Mt, were determined. These new masses were compared with theoretical global mass models and demonstrated to be in good agreement with macroscopic-microscopic models in this region. The empirical shell gap parameter $$delta_{2n}$$ derived from three isotopic masses was updated with the new masses and corroborate the existence of the deformed $$N=152$$ neutron shell closure for Md and Lr.

Journal Articles

Application of unstructured mesh-based numerical method to sodium-water reaction phenomenon analysis code SERAPHIM

Uchibori, Akihiro; Watanabe, Akira*; Takata, Takashi; Ohshima, Hiroyuki

Nippon Kikai Gakkai Rombunshu (Internet), 84(859), p.17-00394_1 - 17-00394_6, 2018/03

For assessment of the wastage environment under tube failure accident in a steam generator of sodium-cooled fast reactors, a mechanistic computer code called SERAPHIM calculating compressible multicomponent multiphase flow with sodium-water chemical reaction has been developed. The original SERAPHIM code is based on the finite difference method. In this study, unstructured mesh-based numerical method was developed and introduced into the SERAPHIM code to advance a numerical accuracy for the complex-shaped domain including multiple heat transfer tubes. Validity of the unstructured mesh-based SERAPHIM code was investigated through the analysis of an underexpanded jet experiment. The calculated pressure profile showed good agreement with the experimental data. Numerical analysis of water vapor discharging into liquid sodium was also performed. It was demonstrated that the proposed numerical method could be applicable to evaluation of the sodium-water reaction phenomenon.

Journal Articles

Determination of fusion barrier distributions from quasielastic scattering cross sections towards superheavy nuclei synthesis

Tanaka, Taiki*; Narikiyo, Yoshihiro*; Morita, Kosuke*; Fujita, Kunihiro*; Kaji, Daiya*; Morimoto, Koji*; Yamaki, Sayaka*; Wakabayashi, Yasuo*; Tanaka, Kengo*; Takeyama, Mirei*; et al.

Journal of the Physical Society of Japan, 87(1), p.014201_1 - 014201_9, 2018/01

 Times Cited Count:5 Percentile:32.14(Physics, Multidisciplinary)

Excitation functions of quasielastic scattering cross sections for the $$^{48}$$Ca + $$^{208}$$Pb, $$^{50}$$Ti + $$^{208}$$Pb, and $$^{48}$$Ca + $$^{248}$$Cm reactions were successfully measured by using the gas-filled recoil-ion separator GARIS. Fusion barrier distributions were extracted from these data, and compared with the coupled-channels calculations. It was found that the peak energies of the barrier distributions for the $$^{48}$$Ca + $$^{208}$$Pb and $$^{50}$$Ti + $$^{208}$$Pb systems coincide with those of the 2n evaporation channel cross sections for the systems, while that of the $$^{48}$$Ca + $$^{248}$$Cm is located slightly below the 4n evaporation ones. This results provide us helpful information to predict the optimum beam energy to synthesize superheavy nuclei.

Journal Articles

Development of unstructured mesh-based numerical method for sodium-water reaction phenomenon in steam generators of sodium-cooled fast reactors

Uchibori, Akihiro; Watanabe, Akira*; Takata, Takashi; Ohshima, Hiroyuki

Journal of Nuclear Science and Technology, 54(10), p.1036 - 1045, 2017/10

 Times Cited Count:3 Percentile:47.53(Nuclear Science & Technology)

To evaluate a sodium-water reaction phenomenon in a steam generator of sodium-cooled fast reactors, a computational fluid dynamics code SERAPHIM, in which a compressible multicomponent multiphase flow with sodium-water chemical reaction is computed, has been developed. The original SERAPHIM code is based on the difference method. In this study, unstructured mesh-based numerical method was developed to advance a numerical accuracy for the complex-shaped domain including multiple heat transfer tubes. Numerical analysis of an underexpanded jet experiment was performed as part of validation of the unstructured mesh-based numerical method. The calculated pressure profile showed good agreement with the experimental data. Applicability of the numerical method for the actual situation was confirmed through the analysis of water vapor discharging into liquid sodium. The effect of use of the unstructured mesh was also investigated by the two analyses using structured and unstructured mesh.

Journal Articles

Development of unstructured mesh-based numerical method for sodium-water reaction phenomenon

Uchibori, Akihiro; Takata, Takashi; Ohshima, Hiroyuki; Watanabe, Akira*

Proceedings of 17th International Topical Meeting on Nuclear Reactor Thermal Hydraulics (NURETH-17) (USB Flash Drive), 12 Pages, 2017/09

To evaluate a sodium-water reaction phenomenon in a steam generator of sodium-cooled fast reactors, a computational fluid dynamics code SERAPHIM, in which a compressible multicomponent multiphase flow with sodium-water chemical reaction is computed, has been developed. The original SERAPHIM code is based on the difference method. In this study, unstructured mesh-based numerical method was developed to advance a numerical accuracy for the complex-shaped domain including multiple heat transfer tubes. Numerical analysis of an underexpanded jet experiment was performed as part of validation of the unstructured mesh-based numerical method. The calculated pressure profile and location of the Mach disk showed good agreement with the experimental data. Applicability of the numerical method for the actual situation was confirmed through the analysis of water vapor discharging into liquid sodium.

Journal Articles

Observation of doubly-charged ions of francium isotopes extracted from a gas cell

Schury, P.*; Wada, Michiharu*; Ito, Yuta*; Kaji, Daiya*; Haba, Hiromitsu*; Hirayama, Yoshikazu*; Kimura, Sota*; Koura, Hiroyuki; MacCormick, M.*; Miyatake, Hiroari*; et al.

Nuclear Instruments and Methods in Physics Research B, 407, p.160 - 165, 2017/06

 Times Cited Count:5 Percentile:29.13(Instruments & Instrumentation)

Various isotopes of Ac, Ra, Fr, and Rn were produced by fusion-evaporation reactions using a $$^{48}$$Ca beam. The energetic ions were stopped in and extracted from a helium gas cell. The extracted ions were identified using a multi-reflection time-of-fight mass spectrograph. In all cases, it was observed that the predominant charge state for the extracted ions, including the alkali Fr, was 2+.

Journal Articles

Numerical study on modeling of liquid film flow under countercurrent flow limitation in volume of fluid method

Watanabe, Taro*; Takata, Takashi; Yamaguchi, Akira*

Nuclear Engineering and Design, 313, p.447 - 457, 2017/03

 Times Cited Count:1 Percentile:78.69(Nuclear Science & Technology)

Countercurrent flow limitation (CCFL) in a heat transfer tube at a steam generator (SG) of pressurized water reactor (PWR) is one of the important issues on the core cooling under a loss of coolant accident(LOCA). In order to improve the prediction accuracy of the CCFL characteristics in numerical simulations using the volume of fluid (VOF) method with less computational cost, a thin liquid film flow in a countercurrent flow is modeled independently and is coupled with the VOF method. Then, we have carried out numerical simulations of a countercurrent flow in a vertical tube so as to investigate the CCFL characteristics and compare them with the previous experimental results. As a result, it has been concluded that the effect of liquid film entrainment by upward gas flux will cause the difference in the experiments.

Journal Articles

Three-dimensional electronic structures and the metal-insulator transition in Ruddlesden-Popper iridates

Yamasaki, Atsushi*; Fujiwara, Hidenori*; Tachibana, Shoichi*; Iwasaki, Daisuke*; Higashino, Yuji*; Yoshimi, Chiaki*; Nakagawa, Koya*; Nakatani, Yasuhiro*; Yamagami, Kohei*; Aratani, Hidekazu*; et al.

Physical Review B, 94(11), p.115103_1 - 115103_10, 2016/11

AA2016-0587.pdf:2.55MB

 Times Cited Count:12 Percentile:32.31(Materials Science, Multidisciplinary)

In this study, we systematically investigate three-dimensional(3D) momentum-resolved electronic structures of Ruddlesden-Popper-type iridium oxides Sr$$_{n+1}$$Ir$$_{n}$$O$$_{3n+1}$$ using soft-X-ray angle-resolved photoemission spectroscopy (SX-ARPES). Our results provide direct evidence of an insulator-to-metal transition that occurs upon increasing the dimensionality of the IrO$$_{2}$$-plane structure. This transition occurs when the spin-orbit-coupled $$j_{eff}$$ = 1/2 band changes its behavior in the dispersion relation and moves across the Fermi energy. By scanning the photon energy over 350 eV, we reveal the 3D Fermi surface in SrIrO$$_{3}$$ and $$k_{z}$$-dependent oscillations of photoelectron intensity in Sr$$_{3}$$Ir$$_{2}$$O$$_{7}$$. To corroborate the physics deduced using low-energy ARPES studies, we propose to utilize SX-ARPES as a powerful complementary technique, as this method surveys more than one whole Brillouin zone and provides a panoramic view of electronic structures.

Journal Articles

Development of unstructured mesh-based numerical method for sodium-water reaction phenomenon in steam generators of sodium-cooled fast reactors

Uchibori, Akihiro; Watanabe, Akira*; Takata, Takashi; Ohno, Shuji; Ohshima, Hiroyuki

Proceedings of OECD/NEA & IAEA Workshop on Application of CFD/CMFD Codes to Nuclear Reactor Safety and Design and their Experimental Validation (CFD4NRS-6) (Internet), 11 Pages, 2016/09

For assessment of the wastage environment under tube failure accident in a steam generator of sodium-cooled fast reactors, a mechanistic computer code called SERAPHIM calculating compressible multicomponent multiphase flow with sodium-water chemical reaction has been developed. The original SERAPHIM code is based on the finite difference method. In this study, unstructured mesh-based numerical method was developed and introduced into the SERAPHIM code to advance a numerical accuracy for the complex-shaped domain including multiple heat transfer tubes. Validity of the unstructured mesh-based SERAPHIM code was investigated through the analysis of an under expanded jet experiment. The calculated pressure profile showed good agreement with the experimental data. Numerical analysis of water vapor discharging into liquid sodium was also performed. It was demonstrated that the proposed numerical method could be applicable to evaluation of the sodium-water reaction phenomenon.

Journal Articles

Preparation and evaluation of an astatine-211-labeled sigma receptor ligand for $$alpha$$ radionuclide therapy

Ogawa, Kazuma*; Mizuno, Yoshiaki*; Washiyama, Koshin*; Shiba, Kazuhiro*; Takahashi, Naruto*; Kozaka, Takashi*; Watanabe, Shigeki; Shinohara, Atsushi*; Odani, Akira*

Nuclear Medicine and Biology, 42(11), p.875 - 879, 2015/11

 Times Cited Count:12 Percentile:34.4(Radiology, Nuclear Medicine & Medical Imaging)

Journal Articles

Optical properties of tetravalent uranium complexes in non-aqueous media

Aoyagi, Noboru; Watanabe, Masayuki; Kirishima, Akira*; Sato, Nobuaki*; Kimura, Takaumi

Journal of Radioanalytical and Nuclear Chemistry, 303(2), p.1095 - 1098, 2015/02

 Times Cited Count:3 Percentile:62.23(Chemistry, Analytical)

152 (Records 1-20 displayed on this page)