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Journal Articles

Evaluating the effect of temporal variations in wind speed on sheltering effectiveness and developing a simplified correction method to account for these variations

Hirouchi, Jun; Takahara, Shogo; Watanabe, Masatoshi*

Journal of Radiological Protection, 45(2), p.021506_1 - 021506_13, 2025/05

 Times Cited Count:0 Percentile:0.00(Environmental Sciences)

Sheltering is a key countermeasure for mitigating radiation exposures during nuclear power plant accidents. The effectiveness of sheltering in minimizing inhalation exposure is commonly expressed using the reduction factor, which is the ratio of indoor to outdoor cumulative doses. The indoor dose is primarily influenced by the air exchange rate, penetration factor, and indoor deposition rate. Additionally, the air exchange rate is dependent on wind speed. In previous studies, the reduction factor was often treated as a constant value or calculated under constant wind speed conditions. However, wind speed varies in reality. This study investigated the effect of temporal variations in wind speed on the reduction factor and developed a simplified correction method to account for these variations. The results revealed that temporal variations in wind speed caused the reduction factor to differ by a factor of approximately two. Using the simplified correction method, the corrected reduction factors agreed, on average, within 10% of those calculated using a method that explicitly considers temporal variations in actual wind speed. Additionally, the computational cost was reduced by more than 20 times.

JAEA Reports

Evaluation of exposure doses and reduction factor for sheltering for each nuclear site under each accident scenario (Contract research)

Hirouchi, Jun; Watanabe, Masatoshi*; Hayashi, Naho; Nagakubo, Azusa; Takahara, Shogo

JAEA-Research 2024-015, 114 Pages, 2025/03

JAEA-Research-2024-015.pdf:10.03MB

The public living in areas contaminated by nuclear accidents is exposed to radiation in the early phase and over the long term. Even under the same accident scenario, the exposure doses and the effectiveness of sheltering, which is one of the protective measures, vary depending on the meteorological condition and the surrounding environment. The exposure doses and sheltering effectiveness in the early phase are important information for the public and the national and local governments planning a nuclear emergency preparedness. In this report, we evaluate the exposure doses and sheltering effectiveness at sites with nuclear facilities in Japan using OSCAAR, one of the probabilistic risk assessment codes, for five accident scenarios: three scenarios from past severe accident studies; a scenario defined by the Nuclear Regulatory Authority; and a scenario assuming the Fukushima Daiichi Nuclear Power Station accident. The sheltering effectiveness differed by approximately 20% among the sites. This was due to the differences in wind speed among the sites.

Journal Articles

Effects of different accident scenarios and sites on the reduction factor used for expressing sheltering effectiveness

Hirouchi, Jun; Watanabe, Masatoshi*; Hayashi, Naho; Nagakubo, Azusa; Takahara, Shogo

Journal of Radiological Protection, 45(1), p.011506_1 - 011506_11, 2025/03

 Times Cited Count:0 Percentile:0.00(Environmental Sciences)

Public living in areas contaminated by nuclear accidents is exposed to radiation in the early phase and over the long term. Even under similar accident scenarios, radiation doses and sheltering effectiveness, which is one of the protective measures, depend on meteorological conditions and the surrounding environment. Radiation doses and sheltering effectiveness in the early phase of nuclear accidents are crucial information for the public as well as national and local governments planning a nuclear emergency preparedness. In this study, we assessed radiation doses and sheltering effectiveness at sites with nuclear facilities in Japan using the Off-Site Consequence Analysis code for Atmospheric Release accidents, which is one of the level-3 probabilistic risk assessment codes, for five accident scenarios: three scenarios from past severe accident studies, a scenario defined by the Nuclear Regulation Authority in Japan, and a scenario corresponding to the Fukushima-Daiichi Nuclear Power Station accident. The sheltering effectiveness differed by up to approximately 50% among the accident scenarios at the same sites and by approximately 20%$$sim$$50% among sites under the same accident scenario. Differences in the radionuclide composition among the accident scenarios and the differences in wind speeds among the sites primarily caused these differences in sheltering effectiveness.

Journal Articles

Recent status of the cryogenic sample environment at the MLF, J-PARC

Ishikado, Motoyuki*; Takahashi, Ryuta*; Yamauchi, Yasuhiro*; Nakamura, Masatoshi*; Ishimaru, Sora*; Yamauchi, Sara*; Kawamura, Seiko; Kira, Hiroshi*; Sakaguchi, Yoshifumi*; Watanabe, Masao; et al.

JPS Conference Proceedings (Internet), 41, p.011010_1 - 011010_7, 2024/05

Journal Articles

Nature of the physicochemical process in water photolysis uncovered by a computer simulation

Kai, Takeshi; Toigawa, Tomohiro; Ukai, Masatoshi*; Fujii, Kentaro*; Watanabe, Ritsuko*; Yokoya, Akinari*

Journal of Chemical Physics, 158(16), p.164103_1 - 164103_8, 2023/04

 Times Cited Count:7 Percentile:57.06(Chemistry, Physical)

New insight into water radiolysis and photolysis is indispensable in the dramatic progress of sciences and technologies in various research areas. In the radiation field, reactive hydrated electrons are considerably produced along radiation tracks. Although the formation results from a transient dynamic correlation between ejected electrons and water, the individual mechanisms of electron thermalization, delocalization, and polarization are unknown. Using a dynamic Monte Carlo code, we show herein that the ejected electrons are immediately delocalized by molecular excitations in parallel with phonon polarization and gradually thermalized by momentum transfer with an orientation polarization in a simultaneous manner. Our results show that these mechanisms heavily depend on the intermolecular vibration and rotation modes peculiar to water. We expect our approach to be a powerful technique for connecting physical and chemical processes in various solvents.

Journal Articles

Measurements of thermal conductivity for near stoichiometric (U$$_{0.7-z}$$Pu$$_{0.3}$$Am$$_{z}$$)O$$_{2}$$ (z = 0.05, 0.10, and 0.15)

Yokoyama, Keisuke; Watanabe, Masashi; Tokoro, Daishiro*; Sugimoto, Masatoshi*; Morimoto, Kyoichi; Kato, Masato; Hino, Tetsushi*

Nuclear Materials and Energy (Internet), 31, p.101156_1 - 101156_7, 2022/06

 Times Cited Count:6 Percentile:56.04(Nuclear Science & Technology)

In current nuclear fuel cycle systems, to reduce the amount of high-level radioactive waste, minor actinides (MAs) bearing MOX fuel is one option for burning MAs using fast reactor. However, the effects of Am content in fuel on thermal conductivity are unclear because there are no experimental data on thermal conductivity of high Am bearing MOX fuel. In this study, The thermal conductivities of near stoichiometric (U$$_{0.7-z}$$Pu$$_{0.3}$$Am$$_{z}$$)O$$_{2}$$ solid solutions(z = 0.05, 0.10, and 0.15) have been measured between room temperature (RT) and 1473 K. The thermal conductivities decreased with increasing Am content and satisfied the classical phonon transport model ((A+BT)$$^{-1}$$) up to about 1473 K. A values increased linearly with increasing Am content because the change in ionic radius affects the conduction of the phonon due to the solid solution in U$$^{5+}$$ and Am$$^{3+}$$. B values were independent of Am content.

Journal Articles

A Storm-induced flood and associated nearshore dispersal of the river-derived suspended $$^{137}$$Cs

Uchiyama, Yusuke*; Tokunaga, Natsuki*; Azuma, Kohei*; Kamidaira, Yuki; Tsumune, Daisuke*; Iwasaki, Toshiki*; Yamada, Masatoshi*; Tateda, Yutaka*; Ishimaru, Takashi*; Ito, Yukari*; et al.

Science of the Total Environment, 816, p.151573_1 - 151573_13, 2022/04

 Times Cited Count:12 Percentile:53.76(Environmental Sciences)

no abstracts in English

Journal Articles

Assessment of radiation doses to off-site responders in TEPCO Fukushima Daiichi Nuclear Power Station Accident

Shimada, Kazumasa; Iijima, Masashi*; Watanabe, Masatoshi*; Takahara, Shogo

Proceedings of Asian Symposium on Risk Assessment and Management 2021 (ASRAM 2021) (Internet), 17 Pages, 2021/10

The radiation doses received by the off-site responders in the Fukushima Daiichi Nuclear Power Station accident were assessed. Atmospheric dispersion simulation was conducted with the source term of the previous research to calculate the atmospheric concentration and ground surface deposition in the municipalities where off-site responders actives. The external exposure dose from cloudshine and groundshine, the internal exposure dose due to inhalation of radioactive plume and resuspended radio nuclei, and the temporal and spatial distribution within each municipality were assessed. As a result of comparing the assessed values of the external exposure dose with the measured values of the personal dosimeter, the measured values were within the assessed range. As a result of our assessment with internal dose exposure, if the exposures occurred without protective measures, the potential daily effective dose in the period between 12 and 31 March 2011 were several tens mSv per day or more in the relatively high dose area. Therefore, to keep the doses received by the responders below the reference level of 20 mSv recommended by the ICRP, it is necessary to ensure that the protective measures for internal exposures such as masks are taken, and to manage the time spent for their activity at least daily.

Journal Articles

Assessment model of radiation doses from external exposure to the public after the Fukushima Daiichi Nuclear Power Plant accident

Takahara, Shogo; Iijima, Masashi*; Watanabe, Masatoshi*

Health Physics, 118(6), p.664 - 677, 2020/06

 Times Cited Count:12 Percentile:68.94(Environmental Sciences)

Assessment model of radiation doses from external exposures was developed based on the actual measurement of individual doses and ambient dose equivalent rate inside and outside of a house in Fukushima city. The survey on behavioral pattern was also carried out under the same purpose. In addition to the actual measurement and survey by ourselves, we also took into account the latest insights from the Fukushima Dai-ichi Nuclear Power Plant (FDNPP) accident. Comparisons between the assessed results and the measured ones revealed that the time dependences of doses obtained using the developed models were in good agreement with the results of actual measurements. In addition, we were able to reproduce the distribution of doses for indoor and outdoor workers. Therefore, our probabilistic approach was validated. According to our assessment and actual measurement, no participants received 1 mSv/y or higher in Fukushima city in eight years after the FDNPP accident.

Journal Articles

Assessment of radiation doses from ingestion pathway to the public in Fukushima prefecture after the Fukushima Dai-ichi Nuclear Power Plant accident

Takahara, Shogo; Watanabe, Masatoshi*

Proceedings of Asian Symposium on Risk Assessment and Management 2019 (ASRAM 2019) (USB Flash Drive), 9 Pages, 2019/09

Internal exposure from ingestion pathway is one of most concerned contributor to the received doses to the public after the Fukushima Dai-ichi Nuclear Power Plant (FDNPP) accident. In the present study, we developed the dose prediction model taking into account the ecological half-lives of radionuclides in foodstuffs and the reduction effects on concentration of radionuclides in cooking-process based on the experiences and the latest insights of the FDNPP accident. From comparison of the retrospective assessment results in Fukushima city between our models and the previous models (market bascket, duplicate, sewer sludge method), no contradictions were observed. In addition, it was found that the potential annual effective doses, which were assessed using the developed model, is several tens micro Sieverts in the first year after the FDNPP accident, and subsequent years the doses is also not exceeding several micro Sv for the future in Fukushima city.

Journal Articles

Present status of personnel protection system at J-PARC

Kikuzawa, Nobuhiro; Niki, Kazuaki*; Yamamoto, Noboru*; Hayashi, Naoki; Adachi, Masatoshi*; Watanabe, Kazuhiko*

Proceedings of 16th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.877 - 880, 2019/07

Interlock system of J-PARC is classified into a personnel protection system (PPS) for human safety and a machine protection system (MPS) for protecting equipment. The PPS of the J-PARC accelerator started from the operation at Linac in 2006 and was completed by the MR operation in 2008. In the next 10 years, some improvements have been made, such as updating video monitoring systems and establishing new interlocks. In addition to describing recent operations including these updatings, this paper reports the current status of inspections and maintenance conducted to maintain and improve reliability.

Journal Articles

Cryogenic sample environments shared at the MLF, J-PARC

Kawamura, Seiko; Takahashi, Ryuta*; Ishikado, Motoyuki*; Yamauchi, Yasuhiro*; Nakamura, Masatoshi*; Ouchi, Keiichi*; Kira, Hiroshi*; Kambara, Wataru*; Aoyama, Kazuhiro*; Sakaguchi, Yoshifumi*; et al.

Journal of Neutron Research, 21(1-2), p.17 - 22, 2019/05

The Cryogenics and Magnets group in the Sample Environment team is responsible for operation of cryostats and magnets for user's experiments at the MLF in J-PARC. We have introduced a top-loading $$^4$$He cryostat, a bottom-loading $$^3$$He cryostat, a dilution refrigerator insert and a superconducting magnet. The frequency of use of them dramatically becomes higher in these two years, as the beam power and the number of proposal increase. To respond such situation, we have made efforts to enhance performance of these equipment as follows. The $$^3$$He cryostat originally involves an operation software for automatic initial cooling down to the base temperature and automatic re-charge of $$^3$$He. Recently we made an additional program for automatic temperature control with only the sorb heater. Last year, a new outer vacuum chamber of the magnet with an oscillating radial collimator (ORC) was fabricated. The data quality was drastically improved by introducing this ORC so that the magnet can be used even for the inelastic neutron scattering experiments.

Journal Articles

Dose-reduction effects of vehicles against gamma radiation in the case of a nuclear accident

Takahara, Shogo; Watanabe, Masatoshi*; Hirouchi, Jun; Iijima, Masashi*; Munakata, Masahiro

Health Physics, 114(1), p.64 - 72, 2018/01

AA2017-0033.pdf:0.55MB

 Times Cited Count:2 Percentile:16.54(Environmental Sciences)

Journal Articles

A Significant role of non-thermal equilibrated electrons in the formation of deleterious complex DNA damage

Kai, Takeshi; Yokoya, Akinari*; Ukai, Masatoshi*; Fujii, Kentaro*; Toigawa, Tomohiro; Watanabe, Ritsuko*

Physical Chemistry Chemical Physics, 20(4), p.2838 - 2844, 2018/01

 Times Cited Count:30 Percentile:78.25(Chemistry, Physical)

It is thought that complex DNA damage which induces in radiation biological effects is formed at radiation track end. Thus, the earliest stage of water radiolysis at the electron track end was studied to predict DNA damage. These results indicate that DNA damage sites comprising multiple nucleobase lesions with a single strand breaks can therefore be formed by multiple collisions of the electrons within three base pairs (3bp) of a DNA strand. This multiple damage site cannot be processed by base excision repair enzymes. However, pre-hydrated electrons can also be produced resulting in an additional base lesion more than 3bp away from the multi-damage site. This clustered damage site may be finally converted into a double strand break (DSB) when base excision enzymes process the additional base lesions. These DSBs include another base lesion(s) at their termini that escape from the base excision process and which may result in biological effects such as mutation in surviving cells.

Journal Articles

Factors affecting the effectiveness of sheltering in reducing internal exposure

Hirouchi, Jun; Takahara, Shogo; Komagamine, Hiroshi*; Watanabe, Masatoshi*; Munakata, Masahiro

Proceedings of Asian Symposium on Risk Assessment and Management 2017 (ASRAM 2017) (USB Flash Drive), 11 Pages, 2017/11

no abstracts in English

Journal Articles

Identification of penetration path and deposition distribution of radionuclides in houses by experiments and numerical model

Hirouchi, Jun; Takahara, Shogo; Iijima, Masashi; Watanabe, Masatoshi; Munakata, Masahiro

Radiation Physics and Chemistry, 140, p.127 - 131, 2017/11

BB2016-0282.pdf:0.39MB

 Times Cited Count:3 Percentile:23.14(Chemistry, Physical)

Journal Articles

Oxygen potentials, oxygen diffusion coefficients and defect equilibria of nonstoichiometric (U,Pu)O$$_{2pm x}$$

Kato, Masato; Watanabe, Masashi; Matsumoto, Taku; Hirooka, Shun; Akashi, Masatoshi

Journal of Nuclear Materials, 487, p.424 - 432, 2017/04

 Times Cited Count:24 Percentile:87.00(Materials Science, Multidisciplinary)

Oxygen potential of (U,Pu)O$$_{2pm x}$$ was evaluated based on defect chemistry using an updated experimental data set. The relationship between oxygen partial pressure and deviation $$x$$ in (U,Pu)O$$_{2pm x}$$ was analyzed, and equilibrium constants of defect formation were determined as functions of Pu content and temperature. Brouwer's diagrams were constructed using the determined equilibrium constants, and a relational equation to determine O/M ratio was derived as functions of O/M ratio, Pu content and temperature. In addition, relationship between oxygen potential and oxygen diffusion coefficients were described.

JAEA Reports

Survey on evacuation facilities in case of nuclear emergency in Shimane prefecture (Contract research)

Takahara, Shogo; Watanabe, Masatoshi; Oguri, Tomomi; Kimura, Masanori; Hirouchi, Jun; Munakata, Masahiro; Homma, Toshimitsu

JAEA-Data/Code 2016-016, 65 Pages, 2017/02

JAEA-Data-Code-2016-016.pdf:2.32MB

We surveyed on structural and material data on 22 facilities which are listed in local disaster management plan in Matsue city. These facilities can be divided into educational facilities, communal facilities and gymnastic hall. Height and floor-area of rooms, as well as window-area were collected as the structural data. We also collected information on constructional materials, and density of those. In addition, mass-thicknesses of the constructional materials were evaluated based on our surveys, and compared to the previous studies which were made in Japan, U.S., and European countries. Consequently, it was found that there is no significant difference of mass-thickness of constructional materials between the results of our surveys and the previous studies. However, for gymnastic hall, since thin metal plates are used for roofs, we can point out that the mass-thickness of roofs are much lower than those for other concrete facilities and clay tile roofing wooden houses.

Journal Articles

Deceleration processes of secondary electrons produced by a high-energy Auger electron in a biological context

Kai, Takeshi; Yokoya, Akinari; Ukai, Masatoshi; Fujii, Kentaro; Watanabe, Ritsuko

International Journal of Radiation Biology, 92(11), p.654 - 659, 2016/11

 Times Cited Count:14 Percentile:72.42(Biology)

Journal Articles

Dynamic behavior of secondary electrons in liquid water at the earliest stage upon irradiation; Implications for DNA damage localization mechanism

Kai, Takeshi; Yokoya, Akinari*; Ukai, Masatoshi*; Fujii, Kentaro*; Watanabe, Ritsuko*

Journal of Physical Chemistry A, 120(42), p.8228 - 8233, 2016/10

 Times Cited Count:27 Percentile:70.96(Chemistry, Physical)

Low energy secondary electrons produced by an ionizing radiation in a living cell may involve in formation of complexed DNA damage. We performed theoretical study for numerical calculation of dynamic behavior of the electrons to imply a formation of radiation damage to DNA. The decelerating electrons are gradually attracted to their parent cations by the Coulombic force within hundreds of fs, and about 12.6 % of electrons are finally distributed within 2 nm from the cations. The collision fraction of the ionization and excitation within 1 nm from the cation was estimated to be about 40 %. From those analyses, we suggested a process of DNA damage that the secondary electrons may cause highly localized lesions around a cation in DNA molecule through additional dissociative electron transfer as well as the ionization or the excitation if the electrons are ejected from DNA. The localized damage may involve ultimately in biological effects such as cell death or mutation induction.

117 (Records 1-20 displayed on this page)