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JAEA Reports

Utilization of gamma ray irradiation at the WASTEF Facility

Sano, Naruto; Yamashita, Naoki; Watanabe, Masaya; Tsukada, Manabu*; Hoshino, Kazutoyo*; Hirai, Koki; Ikegami, Yuta*; Tashiro, Shinsuke; Yoshida, Ryoichiro; Hatakeyama, Yuichi; et al.

JAEA-Technology 2023-029, 36 Pages, 2024/03

JAEA-Technology-2023-029.pdf:2.47MB

At the Waste Safety Testing Facility (WASTEF), the gamma ray irradiation device "Gamma Cell 220" was relocated from the 4th research building of the Nuclear Science Research Institute in FY2019, and the use of gamma ray irradiation has begun. Initially, Fuel Cycle Safety Research Group, Fuel Cycle Safety Research Division, Nuclear Safety Research Center, Sector of Nuclear Safety Research and Emergency Preparedness, the owner of this device, conducted the tests as the main user, but since 2022, other users, including those outside the organization, have started using it. The gamma ray irradiation device "Gamma Cell 220" is manufactured by Nordion International Inc. in Canada. Since it was purchased in 1989, the built-in 60Co radiation source has been updated once, and safety research related to nuclear fuel cycles, etc. It is still used for this purpose to this day. This report summarizes the equipment overview of the gamma ray irradiation device "Gamma Cell 220", its permits and licenses at WASTEF, usage status, maintenance and inspection, and future prospects.

Journal Articles

Present status of the JAEA-AMS-TONO (2022FY)

Fujita, Natsuko; Miyake, Masayasu; Matsubara, Akihiro*; Ishii, Masahiro*; Watanabe, Takahiro; Jinno, Satoshi; Nishio, Tomohiro*; Ogawa, Yumi; Kimura, Kenji; Shimada, Akiomi; et al.

Dai-35-Kai Tandemu Kasokuki Oyobi Sono Shuhen Gijutsu No Kenkyukai Hokokushu, p.17 - 19, 2024/03

The JAEA-AMS-TONO facility at the Tono Geoscience Center, JAEA has three accelerator mass spectrometers. We report the present status of the JAEA-AMS-TONO.

Journal Articles

Status report of JAEA-AMS-TONO; Research and technical development in the last four years

Kokubu, Yoko; Fujita, Natsuko; Watanabe, Takahiro; Matsubara, Akihiro; Ishizaka, Chika; Miyake, Masayasu*; Nishio, Tomohiro*; Kato, Motohisa*; Ogawa, Yumi*; Ishii, Masahiro*; et al.

Nuclear Instruments and Methods in Physics Research B, 539, p.68 - 72, 2023/06

 Times Cited Count:0 Percentile:0.02(Instruments & Instrumentation)

The JAEA-AMS-TONO facility at the Tono Geoscience Center, JAEA has an accelerator mass spectrometer (JAEA-AMS-TONO-5MV). The spectrometer enabled us to use a multi-nuclide AMS of carbon-14 ($$^{14}$$C), beryllium-10, aluminium-26 and iodine-129, and we have recently been proceeding test measurement of chlorine-36. In response to an increase of samples, we installed a state-of-the-art multi-nuclide AMS with a 300 kV Tandetron accelerator in 2020. Recently, we are driving the development of techniques of isobar separation in AMS and of sample preparation. Ion channeling is applied to remove isobaric interference and we are building a prototype AMS based on this technique for downsizing of AMS. The small sample graphitization for $$^{14}$$C has been attempted using an automated graphitization equipment equipped with an elemental analyzer.

Journal Articles

Present status of the JAEA-AMS-TONO (2021)

Matsubara, Akihiro*; Fujita, Natsuko; Miyake, Masayasu; Ishii, Masahiro*; Watanabe, Takahiro; Kokubu, Yoko; Nishio, Tomohiro*; Ogawa, Yumi; Jinno, Satoshi; Kimura, Kenji; et al.

JAEA-Conf 2022-002, p.55 - 62, 2023/03

We report the present status of the JAEA-AMS-TONO. Particularly, the destructions of varistors used in the beamline equipment will be presented. The cause of the destruction as well as implementation of the safety measures are mentioned.

Journal Articles

Present status of the JAEA-AMS-TONO (2022FY)

Fujita, Natsuko; Miyake, Masayasu; Matsubara, Akihiro*; Ishii, Masahiro*; Watanabe, Takahiro; Jinno, Satoshi; Nishio, Tomohiro*; Ogawa, Yumi; Yamamoto, Yusuke; Kimura, Kenji; et al.

Dai-23-Kai AMS Shimpojiumu Hokokushu, p.1 - 4, 2022/12

The JAEA-AMS-TONO facility at the Tono Geoscience Center, JAEA has three accelerator mass spectrometers. We report the present status of the JAEA-AMS-TONO.

Journal Articles

Present status of the JAEA-AMS-TONO (2019-2020)

Fujita, Natsuko; Matsubara, Akihiro; Miyake, Masayasu*; Watanabe, Takahiro; Kokubu, Yoko; Nishio, Tomohiro*; Ogawa, Yumi*; Kato, Motohisa*; Shimada, Akiomi; Ogata, Nobuhisa

Dai-33-Kai Tandemu Kasokuki Oyobi Sono Shuhen Gijutsu No Kenkyukai Hokokushu, P. 48, 2022/04

no abstracts in English

Journal Articles

Measurement of double-differential thick-target neutron yields of the C($$d,n$$) reaction at 12, 20, and 30 MeV

Patwary, M. K. A*; Kin, Tadahiro*; Aoki, Katsumi*; Yoshinami, Kosuke*; Yamaguchi, Masaya*; Watanabe, Yukinobu*; Tsukada, Kazuaki; Sato, Nozomi*; Asai, Masato; Sato, Tetsuya; et al.

Journal of Nuclear Science and Technology, 58(2), p.252 - 258, 2021/02

 Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)

While designing deuteron accelerator neutron sources for radioisotopes production, nuclear data for light elements such as Li, Be, and C have been systematically measured in the deuteron energy range from a few MeV to around 50 MeV. Currently, the experimental data available on double-differential thick-target neutron yields (DDTTNYs) is insufficient, especially for deuteron energies between 18 and 33 MeV. In this study, we measured the DDTTNYs of ($$d,n$$) reactions on $$^{rm nat}$$C target for incident deuteron energies of 12, 20, and 30 MeV using the multiple-foils activation method to improve nuclear data insufficiency. We applied the GRAVEL code for the unfolding process to derive the DDTTNYs. The results were compared with the calculation by DEURACS. The present data were also used to confirm the systematics of the differential neutron yields at 0$$^{circ}$$ and total neutron yield per incident deuteron in the wide range of deuteron energy.

Journal Articles

Preliminary report on small-mass graphitization for radiocarbon dating using EA-AGE3 at JAEA-AMS-TONO

Watanabe, Takahiro; Fujita, Natsuko; Matsubara, Akihiro; Miyake, Masayasu*; Nishio, Tomohiro*; Ishizaka, Chika; Kokubu, Yoko

Geochemical Journal, 55(4), p.277 - 281, 2021/00

 Times Cited Count:2 Percentile:20.95(Geochemistry & Geophysics)

Small-mass radiocarbon dating less than 0.1 mg carbon has been developed by Accelerator mass spectrometry (AMS) and manual preparation techniques using the vacuum glass lines. Because geological samples are limited for the dating in many cases, preparation techniques should be improved for small samples and high efficiency analysis. For radiocarbon dating of geological and other organic samples, small-mass graphitization of international standard reference materials (ca. 0.1 and 0.05 mg carbon) was evaluated using the elemental analyzer and automated graphitization equipment 3 (EA-AGE3; IonPlus AG) in our study. Additionally, this paper presents the first data for the small samples by the EA-AGE3. The average radiocarbon concentration of the small-mass international standards (NIST-SRM4990C, IAEA-C5, and C7) prepared by the EA-AGE3 were agreement with the consensus values within $$pm$$ 2$$sigma$$. Therefore, small-mass graphitization using the EA-AGE3 can be adapted for AMS radiocarbon measurements in our case (down to ca. 0.05 mg carbon).

Journal Articles

Present status of the JAEA-AMS-TONO in 2019

Fujita, Natsuko; Matsubara, Akihiro; Miyake, Masayasu*; Watanabe, Takahiro; Kokubu, Yoko; Kato, Motohisa*; Okabe, Nobuaki*; Isozaki, Nobuhiro*; Ishizaka, Chika*; Nishio, Tomohiro; et al.

Proceedings of the 8th East Asia Accelerator Mass Spectrometry Symposium and the 22nd Japan Accelerator Mass Spectrometry symposium (EA-AMS 8 & JAMS-22), p.34 - 36, 2020/00

no abstracts in English

Journal Articles

Current status of JAEA-AMS-TONO in the 20th year

Kokubu, Yoko; Fujita, Natsuko; Miyake, Masayasu; Watanabe, Takahiro; Ishizaka, Chika; Okabe, Nobuaki; Ishimaru, Tsuneari; Matsubara, Akihiro*; Nishizawa, Akimitsu*; Nishio, Tomohiro*; et al.

Nuclear Instruments and Methods in Physics Research B, 456, p.271 - 275, 2019/10

 Times Cited Count:5 Percentile:48.18(Instruments & Instrumentation)

JAEA-AMS-TONO has been in operation at the Tono Geoscience Center, Japan Atomic Energy Agency since 1998 and 20 years have passed from the beginning of its utilization. The AMS system is a versatile system based on a 5 MV tandem Pelletron type accelerator. The system has been used to measure carbon-14 ($$^{14}$$C), beryllium-10 ($$^{10}$$Be) and aluminium-26 ($$^{26}$$Al). In addition, the development of measurement of iodine-129 ($$^{129}$$I) has been started. The main use is measurement of $$^{14}$$C in geological samples for dating studies in neotectonics and hydrogeology. In order to increase the speed of sample preparation, we introduced the automated graphitization equipment and made a gas-strip line to collect dissolved inorganic carbon in groundwater samples. Measurement of $$^{10}$$Be and $$^{26}$$Al has been used for geoscience studies and the detection limit in the measurement of $$^{10}$$Be was improved by $$^{7}$$Be-counting suppression. Recently tuning of measurement condition of $$^{129}$$I has been progressed.

Journal Articles

The present status of the AGE3 automated graphitization equipment for radiocarbon dating at the JAEA-AMS-TONO

Watanabe, Takahiro; Kokubu, Yoko; Fujita, Natsuko; Ishizaka, Chika*; Nishio, Tomohiro; Matsubara, Akihiro*; Miyake, Masayasu; Kato, Motohisa*; Isozaki, Nobuhiro*; Torazawa, Hitoshi*; et al.

JAEA-Conf 2018-002, p.116 - 119, 2019/02

AMS is widely used for radiocarbon dating of geological samples. However, improvement in efficiency of sample preparation techniques are needed for high-time resolution dataset. In 2016, automated graphitization equipment (AGE3, IonPlus AG) has been installed in Toki Research Institute of Isotope Geology and Geochronology, Tono Geoscience Center, JAEA. Background values and carbon recovery rates during preparation process of AGE3 should be estimated before application in radiocarbon dating. In this study, the AGE3 system was evaluated using the international standard materials (IAEA-C1, C4, C5, C6, C7, C9 and NIST-SRM4990C) at JAEA-AMS-TONO. Graphite samples was prepared by the AGE3 system and radiocarbon concentration of these standards was measured by AMS. The results were agreement with the consensus values. Background values were 0.15$$pm$$0.01 pMC (IAEA-C1) using the AGE3 system. Therefore, we concluded that the system can be adapted for radiocarbon dating of geological samples.

Journal Articles

Improvement of methods for measurement of $$^{129}$$I/$$^{127}$$I ratio at JAEA-AMS-TONO

Okabe, Nobuaki; Fujita, Natsuko; Matsubara, Akihiro*; Miyake, Masayasu; Nishio, Tomohiro*; Nishizawa, Akimitsu*; Isozaki, Nobuhiro*; Watanabe, Takahiro; Kokubu, Yoko

JAEA-Conf 2018-002, p.51 - 54, 2019/02

no abstracts in English

Journal Articles

The Twenty years of JAEA-AMS-TONO

Kokubu, Yoko; Fujita, Natsuko; Matsubara, Akihiro*; Nishizawa, Akimitsu*; Nishio, Tomohiro; Miyake, Masayasu; Ishimaru, Tsuneari; Watanabe, Takahiro; Ogata, Nobuhisa; Shimada, Akiomi; et al.

JAEA-Conf 2018-002, p.5 - 8, 2019/02

no abstracts in English

Journal Articles

Present status of the accelerator facility at the JAEA-AMS-TONO; 2016

Fujita, Natsuko; Miyake, Masayasu; Watanabe, Takahiro; Kokubu, Yoko; Ishimaru, Tsuneari; Matsubara, Akihiro*; Nishio, Tomohiro*; Kato, Motohisa*; Isozaki, Nobuhiro*; Torazawa, Hitoshi*; et al.

JAEA-Conf 2018-013, p.96 - 99, 2019/02

no abstracts in English

Journal Articles

Present status of the accelerator facility at the JAEA-AMS-TONO; 2017

Fujita, Natsuko; Miyake, Masayasu; Watanabe, Takahiro; Kokubu, Yoko; Matsubara, Akihiro*; Kato, Motohisa*; Okabe, Nobuaki; Isozaki, Nobuhiro*; Ishizaka, Chika*; Torazawa, Hitoshi*; et al.

Dai-31-Kai Tandemu Kasokuki Oyobi Sono Shuhen Gijutsu No Kenkyukai Hokokushu, p.92 - 95, 2018/12

no abstracts in English

Journal Articles

Present status of the JAEA-AMS-TONO; 2016

Fujita, Natsuko; Miyake, Masayasu; Watanabe, Takahiro; Kokubu, Yoko; Ishimaru, Tsuneari; Matsubara, Akihiro*; Isozaki, Nobuhiro*; Nishio, Tomohiro*; Kato, Motohisa*; Torazawa, Hitoshi*; et al.

Dai-19-Kai AMS Shimpojiumu, 2016-Nendo "Jumoku Nenrin" Kenkyukai Kyodo Kaisai Shimpojiumu Hokokushu, p.68 - 71, 2017/06

no abstracts in English

Journal Articles

Present status of the tandem accelerator at the JAEA-AMS-TONO; 2015

Fujita, Natsuko; Matsubara, Akihiro*; Watanabe, Takahiro; Kokubu, Yoko; Umeda, Koji*; Ishimaru, Tsuneari; Nishizawa, Akimitsu*; Miyake, Masayasu; Owaki, Yoshio*; Nishio, Tomohiro*; et al.

Dai-29-Kai Tandemu Kasokuki Oyobi Sono Shuhen Gijutsu No Kenkyukai Hokokushu, p.39 - 42, 2017/03

no abstracts in English

Journal Articles

Present status of the JAEA-AMS-TONO; 2015

Fujita, Natsuko; Matsubara, Akihiro; Watanabe, Takahiro; Kokubu, Yoko; Umeda, Koji; Nishizawa, Akimitsu*; Miyake, Masayasu*; Owaki, Yoshio*; Nishio, Tomohiro*; Kato, Motohisa*

Dai-18-Kai AMS Shimpojiumu Hokokushu, p.85 - 90, 2016/12

no abstracts in English

Journal Articles

Evaluation of dark current profile for prediction of voltage holding capability on multi-aperture multi-grid accelerator for ITER

Nishikiori, Ryo; Kojima, Atsushi; Hanada, Masaya; Kashiwagi, Mieko; Watanabe, Kazuhiro; Umeda, Naotaka; Tobari, Hiroyuki; Yoshida, Masafumi; Ichikawa, Masahiro; Hiratsuka, Junichi; et al.

Plasma and Fusion Research (Internet), 11, p.2401014_1 - 2401014_4, 2016/03

One of critical issues for high-energy high-current beam acceleration in ITER and JT-60SA is the high voltage holding which is dominated by vacuum discharges. The past results suggest that vacuum discharge occurs beyond the threshold of the dark current. The dark current can be derived from F-N theory where electric field enhancement factor beta is included. Though, beta could only be evaluated from the experiment previously. Therefore, the method to decide beta without experiment is required. This time dark currents were measured at three different areas to compare beta in different electric field. As a result, the effective electric field $$beta$$E, where E is average electric field, were found to be almost constant for different areas although the beta is largely different. By applying $$beta$$E, beta can be evaluated analytically, leading to the analytical prediction of the dark current and voltage holding capability without the measurements.

Journal Articles

Measurement of heat load density profile on acceleration grid in MeV-class negative ion accelerator

Hiratsuka, Junichi; Hanada, Masaya; Kojima, Atsushi; Umeda, Naotaka; Kashiwagi, Mieko; Miyamoto, Kenji*; Yoshida, Masafumi; Nishikiori, Ryo; Ichikawa, Masahiro; Watanabe, Kazuhiro; et al.

Review of Scientific Instruments, 87(2), p.02B137_1 - 02B137_3, 2016/02

 Times Cited Count:4 Percentile:21.61(Instruments & Instrumentation)

To understand the physics of the negative ion extraction/acceleration, the heat load density profile on the acceleration grid has been firstly measured in the ITER prototype accelerator where the negative ions are accelerated to 1 MeV with five acceleration stages. In order to clarify the profile, the peripheries around the apertures on the acceleration grid were separated into thermally insulated 34 blocks with thermocouples. The spatial resolution is as low as 3 mm and small enough to measure the tail of the beam profile with a beam diameter of 16 mm. It was found that there were two peaks of heat load density around the aperture. These two peaks were also clarified to be caused by the intercepted negative ions and secondary electrons from detailed investigation by changing the beam optics and gas density profile. This is the first experimental result, which is useful to understand the trajectories of these particles.

221 (Records 1-20 displayed on this page)