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Journal Articles

Chemical characterization of a volatile dubnium compound, DbOCl$$_3$$

Chiera, N. M.*; Sato, Tetsuya; Eichler, R.*; Tomitsuka, Tomohiro; Asai, Masato; Adachi, Sadia*; Dressler, R.*; Hirose, Kentaro; Inoue, Hiroki*; Ito, Yuta; et al.

Angewandte Chemie; International Edition, 60(33), p.17871 - 17874, 2021/08

 Times Cited Count:2 Percentile:14.88(Chemistry, Multidisciplinary)

The formation and the chemical characterization of single atoms of dubnium (Db, element 105), in the form of its volatile oxychloride, was investigated using the on-line gas phase chromatography technique, in the temperature range 350 - 600 $$^circ$$C. Under the exact same chemical conditions, comparative studies with the lighter homologs of group-5 in the Periodic Table clearly indicate the volatility sequence being NbOCl$$_3 > $$ TaOCl$$_3 geq$$ DbOCl$$_3$$. From the obtained experimental results, thermochemical data for DbOCl$$_3$$ were derived. The present study delivers reliable experimental information for theoretical calculations on the chemical properties of transactinides.

Journal Articles

Thermally altered subsurface material of asteroid (162173) Ryugu

Kitazato, Kohei*; Milliken, R. E.*; Iwata, Takahiro*; Abe, Masanao*; Otake, Makiko*; Matsuura, Shuji*; Takagi, Yasuhiko*; Nakamura, Tomoki*; Hiroi, Takahiro*; Matsuoka, Moe*; et al.

Nature Astronomy (Internet), 5(3), p.246 - 250, 2021/03

 Times Cited Count:43 Percentile:96.93(Astronomy & Astrophysics)

Here we report observations of Ryugu's subsurface material by the Near-Infrared Spectrometer (NIRS3) on the Hayabusa2 spacecraft. Reflectance spectra of excavated material exhibit a hydroxyl (OH) absorption feature that is slightly stronger and peak-shifted compared with that observed for the surface, indicating that space weathering and/or radiative heating have caused subtle spectral changes in the uppermost surface. However, the strength and shape of the OH feature still suggests that the subsurface material experienced heating above 300 $$^{circ}$$C, similar to the surface. In contrast, thermophysical modeling indicates that radiative heating does not increase the temperature above 200 $$^{circ}$$C at the estimated excavation depth of 1 m, even if the semimajor axis is reduced to 0.344 au. This supports the hypothesis that primary thermal alteration occurred due to radiogenic and/or impact heating on Ryugu's parent body.

Journal Articles

Role of advection in atmospheric ammonia; A Case study at a Japanese lake basin influenced by agricultural ammonia sources

Kubota, Tomohiro; Kuroda, Hisao*; Watanabe, Mirai*; Takahashi, Akiko*; Nakazato, Ryoji*; Tarui, Mika*; Matsumoto, Shunichi*; Nakagawa, Keita*; Numata, Yasuko*; Ouchi, Takao*; et al.

Atmospheric Environment, 243, p.117856_1 - 117856_9, 2020/12

 Times Cited Count:3 Percentile:15.82(Environmental Sciences)

The dry and wet depositions of atmospheric ammonia (NH$$_{3}$$) is one of the important pathways of nitrogen loads to aquatic ecosystems. Crop and livestock agriculture, one of the largest emitters of NH$$_{3}$$ in Asian countries, are known to cause high spatial and seasonal variation of NH$$_{3}$$ and influence the surrounding lake basin areas via its dry and wet deposition. However, the spatial characteristics of the NH$$_{3}$$ concentration in basin scale are not completely understood for regulation in NH$$_{3}$$ emission. Here we aim to clarify dominant factors of spatial and seasonal variations of the NH$$_{3}$$ concentration in a eutrophic lake basin surrounded by agricultural areas in Japan. Passive sampling over various land use categories in the basin was conducted at 36 sites in total from October 2018 to January 2020. Interestingly, the observed NH$$_{3}$$ concentration near the livestock houses were higher in winter than summer, which was inconsistent with knowledge of seasonal changes of current NH$$_{3}$$ emission inventory based on temperature-driven volatilization process. Comparing monthly NH$$_{3}$$ concentrations with various meteorological factors, we suggested the importance of seasonal advection of NH$$_{3}$$ from high emission sources to which has been rarely paid attention by the previous past studies. As for this, should be considered for lake ecosystem management since deposition of NH$$_{3}$$ is known to be closely related to the ecological processes such as phytoplankton blooming.

Journal Articles

The Surface composition of asteroid 162173 Ryugu from Hayabusa2 near-infrared spectroscopy

Kitazato, Kohei*; Milliken, R. E.*; Iwata, Takahiro*; Abe, Masanao*; Otake, Makiko*; Matsuura, Shuji*; Arai, Takehiko*; Nakauchi, Yusuke*; Nakamura, Tomoki*; Matsuoka, Moe*; et al.

Science, 364(6437), p.272 - 275, 2019/04

 Times Cited Count:259 Percentile:99.73(Multidisciplinary Sciences)

The near-Earth asteroid 162173 Ryugu, the target of Hayabusa2 sample return mission, is believed to be a primitive carbonaceous object. The Near Infrared Spectrometer (NIRS3) on Hayabusa2 acquired reflectance spectra of Ryugu's surface to provide direct measurements of the surface composition and geological context for the returned samples. A weak, narrow absorption feature centered at 2.72 micron was detected across the entire observed surface, indicating that hydroxyl (OH)-bearing minerals are ubiquitous there. The intensity of the OH feature and low albedo are similar to thermally- and/or shock-metamorphosed carbonaceous chondrite meteorites. There are few variations in the OH-band position, consistent with Ryugu being a compositionally homogeneous rubble-pile object generated from impact fragments of an undifferentiated aqueously altered parent body.

Journal Articles

Analysis of bystander effect induced by cell membrane response in glioma cells

Wada, Seiichi*; Ando, Tatsuhiko*; Watanabe, Aya*; Kakizaki, Takehiko*; Natsuhori, Masahiro*; Funayama, Tomoo; Sakashita, Tetsuya; Yokota, Yuichiro; Kobayashi, Yasuhiko

JAEA-Review 2014-050, JAEA Takasaki Annual Report 2013, P. 79, 2015/03

So far, we clarified that X-ray irradiation induced cell killing by bystander effect mediated-secreted factor. This phenomenon was related with sphingomyelinase (SMase). In this study we analyzed mechanism of secreted SMase from irradiated cells after irradiation. SMase was detected in the culture medium after irradiation by SDS-PAGE. Then, SMase was detected in the exosome of culture medium, but not out of exosome after irradiation. This result indicates that SMase was secreted as exosome from the irradiated cells.

Journal Articles

Investigation of fission properties and evaporation residue measurement in the reactions using $$^{238}$$U target nucleus

Nishio, Katsuhisa; Ikezoe, Hiroshi; Hofmann, S.*; Ackermann, D.*; Antalic, S.*; Aritomo, Yoshihiro; Comas, V. F.*; D$"u$llmann, Ch. E.*; Gorshkov, A.*; Graeger, R.*; et al.

EPJ Web of Conferences, 17, p.09005_1 - 09005_4, 2011/10

 Times Cited Count:1 Percentile:47.57(Physics, Nuclear)

Journal Articles

Observation of ion cyclotron emission owing to DD fusion product H ions in JT-60U

Sato, Shoichi*; Ichimura, Makoto*; Yamaguchi, Yusuke*; Katano, Makoto*; Imai, Yasutaka*; Murakami, Tatsuya*; Miyake, Yuichiro*; Yokoyama, Takuro*; Moriyama, Shinichi; Kobayashi, Takayuki; et al.

Plasma and Fusion Research (Internet), 5, p.S2067_1 - S2067_4, 2010/12

Ion cyclotron emissions (ICEs) due to deuterium-deuterium fusion-product (FP) ions on JT-60U are studied. ICE due to H-ions is identified from the difference of the toroidal wave number of 2nd ICE(D). The parameter dependence for the appearance of ICE(H) is investigated from the experimental conditions and also is studied by using "Escape Particle Orbit analysis Code (EPOC)".

Journal Articles

Nuclear orientation in the reaction $$^{34}$$S+$$^{238}$$U and synthesis of the new isotope $$^{268}$$Hs

Nishio, Katsuhisa; Hofmann, S.*; He${ss}$berger, F. P.*; Ackermann, D.*; Antalic, S.*; Aritomo, Yoshihiro; Comas, V. F.*; D$"u$llmann, Ch. E.*; Gorshkov, A.*; Graeger, R.*; et al.

Physical Review C, 82(2), p.024611_1 - 024611_9, 2010/08

 Times Cited Count:79 Percentile:96.03(Physics, Nuclear)

Journal Articles

Effects of nuclear orientation on fusion and fission process for reactions using uranium target nuclei

Nishio, Katsuhisa; Ikezoe, Hiroshi; Mitsuoka, Shinichi; Nishinaka, Ichiro; Makii, Hiroyuki; Watanabe, Yutaka*; Nagame, Yuichiro; Otsuki, Tsutomu*; Hirose, Kentaro*; Hofmann, S.*

AIP Conference Proceedings 1224, p.301 - 310, 2010/04

 Times Cited Count:5 Percentile:84.69(Physics, Nuclear)

Journal Articles

Effects of nuclear orientation on fission fragment mass distributions in the reactions using actinide target nuclei

Nishio, Katsuhisa; Ikezoe, Hiroshi; Mitsuoka, Shinichi; Nishinaka, Ichiro; Makii, Hiroyuki; Watanabe, Yutaka*; Nagame, Yuichiro; Otsuki, Tsutomu*; Hirose, Kentaro*; Hofmann, S.*

AIP Conference Proceedings 1175, p.111 - 118, 2009/10

Journal Articles

Effects of nuclear orientation on fission fragment mass distributions in the reactions using actinide target nuclei

Nishio, Katsuhisa; Ikezoe, Hiroshi; Mitsuoka, Shinichi; Nishinaka, Ichiro; Makii, Hiroyuki; Watanabe, Yutaka*; Nagame, Yuichiro; Otsuki, Tsutomu*; Hirose, Kentaro*; Hofmann, S.*

AIP Conference Proceedings 1175, p.111 - 118, 2009/10

Journal Articles

Effects of nuclear orientation on fusion and fission process in heavy ion reactions

Nishio, Katsuhisa; Ikezoe, Hiroshi; Mitsuoka, Shinichi; Nishinaka, Ichiro; Watanabe, Yutaka*; Nagame, Yuichiro; Otsuki, Tsutomu*; Hirose, Kentaro*; Hofmann, S.*

AIP Conference Proceedings 1120 (Internet), p.275 - 279, 2009/05

Journal Articles

Effects of nuclear orientation on fission fragment mass distributions in the reactions of $$^{34,36}$$S+$$^{238}$$U

Nishio, Katsuhisa; Ikezoe, Hiroshi; Mitsuoka, Shinichi; Nishinaka, Ichiro; Watanabe, Yutaka*; Nagame, Yuichiro; Otsuki, Tsutomu*; Hirose, Kentaro*; Hofmann, S.*

AIP Conference Proceedings 1098, p.289 - 294, 2009/03

Journal Articles

Temporal and spatial variations of radiocarbon in Japan Sea Bottom Water

Kumamoto, Yuichiro*; Aramaki, Takafumi*; Watanabe, Shuichi*; Yoneda, Minoru*; Shibata, Yasuyuki*; Togawa, Orihiko; Morita, Masatoshi*; Shitashima, Kiminori*

Journal of Oceanography, 64(3), p.429 - 441, 2008/06

 Times Cited Count:11 Percentile:25.5(Oceanography)

In 1995 and 2000, radiocarbon ratio ($$Delta$$$$^{14}$$C) of total dissolved inorganic carbon was measured in the Japan Sea, a semi-closed marginal sea in the western North Pacific, where deep and bottom waters are formed in itself. Compiling them with historical radiocarbon data in the Japan Sea, temporal and spatial variations of the radiocarbon in the bottom water below 2000 m depth were elucidated. $$Delta$$$$^{14}$$C in the bottom waters in the western Japan and Yamato Basins increased by about 20 ‰ between 1977/79 and 1995 and did not changed between 1995 and 1999/2000, suggesting penetration of surface bomb-produced radiocarbon into the bottom waters due to bottom ventilation in the earlier period and stagnation of the bottom ventilation in the following period, respectively. In the eastern Japan Basin, the bottom $$Delta$$$$^{14}$$C increased by about 10 ‰ between 1977/79 and 2002, suggesting less ventilation of the bottom water in the basin. The temporal changes of the radiocarbon, tritium, and dissolved oxygen suggest sporadic occurrences of the bottom ventilation between 1979 and 1984 and its stagnation between 1984 and 2004 in the eastern Japan and Yamato Basins. The former is probably due to spreading of a newly ventilated bottom water in the western Japan Basin in the severe winter of 1976-1977 along the abyssal circulation in the Japan Sea. The latter does not conflict with temporal changes of bomb-produced $$^{137}$$Cs and chlorofluorocarbon-11 in the bottom water.

Journal Articles

Effects of nuclear orientation on the mass distribution of fission fragments in the reaction of $$^{36}$$S + $$^{238}$$U

Nishio, Katsuhisa; Ikezoe, Hiroshi; Mitsuoka, Shinichi; Nishinaka, Ichiro; Nagame, Yuichiro; Watanabe, Yutaka*; Otsuki, Tsutomu*; Hirose, Kentaro*; Hofmann, S.*

Physical Review C, 77(6), p.064607_1 - 064607_5, 2008/06

 Times Cited Count:121 Percentile:98.15(Physics, Nuclear)

Journal Articles

Heavy-ion microbeam system at JAEA-Takasaki for microbeam biology

Funayama, Tomoo; Wada, Seiichi*; Yokota, Yuichiro; Fukamoto, Kana; Sakashita, Tetsuya; Taguchi, Mitsumasa; Kakizaki, Takehiko*; Hamada, Nobuyuki*; Suzuki, Michiyo; Furusawa, Yoshiya*; et al.

Journal of Radiation Research, 49(1), p.71 - 82, 2008/01

 Times Cited Count:47 Percentile:78.7(Biology)

Research concerning cellular responses to low dose irradiation, radiation-induced bystander effects, and the biological track structure of charged particles has recently received particular attention in the field of radiation biology. Target irradiation employing a microbeam represents a useful means of advancing this research by obviating some of the disadvantages associated with the conventional irradiation strategies. The heavy-ion microbeam system at JAEA-Takasaki can provide target irradiation of heavy charged particles to biological material at atmospheric pressure using a minimum beam size 5 $$mu$$m in diameter. The system can be applied to the investigation of mechanisms within biological organisms not only in the context of radiation biology, but also in the fields of general biology such as physiology, developmental biology and neurobiology, and should help to establish and contribute to the field of "microbeam biology".

Journal Articles

Breeding of stress-tolerant variety series in ornamentals by ion beam irradiation

Okamura, Masachika*; Momose, Masayuki*; Watanabe, Satomi*; Shimizu, Akira*; Hase, Yoshihiro; Yokota, Yuichiro; Tanaka, Atsushi

JAEA-Review 2006-042, JAEA Takasaki Annual Report 2005, P. 82, 2007/02

no abstracts in English

Journal Articles

${it Klavier}$ (${it klv}$), a novel hypernodulation mutant of ${it Lotus japonicus}$ affected in vascular tissue organization and floral induction

Kira, Erika*; Tateno, Kumiko*; Miura, Kinichiro*; Haga, Tatsuya*; Hayashi, Masaki*; Harada, Kyuya*; Sato, Shusei*; Tabata, Satoshi*; Shikazono, Naoya; Tanaka, Atsushi; et al.

Plant Journal, 44(3), p.505 - 515, 2005/11

 Times Cited Count:90 Percentile:86.71(Plant Sciences)

no abstracts in English

Journal Articles

Rare earth element distribution in the acetic acid soluble fraction of combusted coals; Its implication as a proxy for the original coal-forming plants

Fu, F.; Akagi, Tasuku*; Suzuki, Yuichiro*; Watanabe, Kazuo; Yabuki, Sadayo*

Geochemical Journal, 38(4), p.333 - 343, 2004/08

 Times Cited Count:9 Percentile:20.33(Geochemistry & Geophysics)

no abstracts in English

JAEA Reports

The First loading fuel elements and power-up for JRR-2

JRR-2 Control Office; Kambara, Toyozo; Shoda, Katsuhiko; Hirata, Yutaka; Shoji, Tsutomu; Kohayakawa, Toru; Morozumi, Minoru; Kambayashi, Yuichiro; Shitomi, Hajimu; Kokanezawa, Takashi; et al.

JAERI 1027, 57 Pages, 1962/09

JAERI-1027.pdf:4.76MB

no abstracts in English

36 (Records 1-20 displayed on this page)