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JAEA Reports

Aerial monitoring around TEPCO's Fukushima Daiichi Nuclear Power Station and development of radiation monitoring technology for unmanned vehicle in fiscal year 2024 (Contract research)

Futemma, Akira; Ochi, Kotaro; Sasaki, Miyuki; Nakama, Shigeo; Kawasaki, Yoshiharu*; Iwai, Takeyuki*; Hiraga, Shogo*; Haginoya, Masashi*; Matsunaga, Yuki*; Yamada, Tsutomu*; et al.

JAEA-Technology 2025-016, 253 Pages, 2026/03

JAEA-Technology-2025-016.pdf:20.16MB

Aerial Radiation Monitoring (ARM) has been used to quickly and widely measure radiation distribution caused by the TEPCO's Fukushima Daiichi Nuclear Power Station (FDNPS) accident resulted from the tsunami accompanying the Pacific coast of Tohoku Earthquake on March 11, 2011. Since the accident, As a commissioned project of the Nuclear Regulation Authority, the Japan Atomic Energy Agency (JAEA) has continuously conducted ARM around FDNPS. This report summarizes the results of the 2024 monitoring activities, evaluates temporal changes in ambient dose rates, and identifies factors contributing to these changes. A terrain-corrected analysis was applied to improve dose rates conversion accuracy, and results with and without this correction were compared. A radon-progeny discrimination method was also used to assess its impact on manned-helicopter measurements. Furthermore, development of unmanned airplane monitoring technologies was advanced to enhance the efficiency of wide-area surveys.

JAEA Reports

Introduction of classification considered as waste package for dismantling waste in JRTF

Nakajima, Ryota; Sakai, Tatsuya; Tani, Riku; Handa, Yuichi; Sunaoshi, Mizuho*; Inoue, Hidetaka*; Yamada, Satoshi; Shimizu, Osamu

JAEA-Technology 2025-012, 39 Pages, 2026/01

JAEA-Technology-2025-012.pdf:2.31MB

JAERI's Reprocessing Test Facility (JRTF) has transition to decommissioning since 1996 and inside the facility dismantled equipment and instrument. In the dismantling and removal work of glove boxes and other equipment, starting in October 2022, we prepared a "Manual for Separation of Dismantled Materials of JRTF" and carried out sorting and separation of the generated dismantled waste with the aim of producing waste package that meets the technical standards required for disposal to a landfill facility. This report describes the results and findings of sorting and separating the dismantled waste generated during the dismantling and removal work of glove boxes and other equipment in accordance with the "Manual for Separation of Dismantled Materials of JRTF".

Journal Articles

Improvement in legal compliance activities of nuclear security in JAEA

Hirata, Tomohiro; Hanawa, Kazutaka; Shibata, Ryodai; Yamada, Hiroyuki; Yamazaki, Katsuyuki

Dai-46-Kai Nihon Kaku Busshitsu Kanri Gakkai Nenji Taikai Kaigi Rombunshu (Internet), 4 Pages, 2025/12

no abstracts in English

Journal Articles

Summary of nuclear security culture development activities and long-term results of awareness surveys in JAEA

Hanawa, Kazutaka; Hirata, Tomohiro; Shibata, Ryodai; Yamada, Hiroyuki; Miyaji, Noriko

Dai-46-Kai Nihon Kaku Busshitsu Kanri Gakkai Nenji Taikai Kaigi Rombunshu (Internet), 4 Pages, 2025/12

no abstracts in English

Journal Articles

Freeze-crosslinked biomass-based chitosan sponge hydrogels with metal-induced mechanical enhancement for high-performance Cu$$^{2+}$$ and Pb$$^{2+}$$ adsorption

Nankawa, Takuya; Sugita, Asako; Fukakusa, Chihoko*; Yamada, Teppei*; Sekine, Yurina

Separation and Purification Technology, 378(3), p.134780_1 - 134780_9, 2025/12

 Times Cited Count:4 Percentile:0.00(Engineering, Chemical)

We report a sustainable and chemical free strategy to fabricate sponge like chitosan hydrogels via freeze induced physical crosslinking using mild alkaline solutions, without toxic crosslinkers or synthetic additives. The resulting freeze crosslinked biomass-based chitosan sponge hydrogels exhibited interconnected macropores, high water permeability, excellent compressibility, and mechanical recoverability. These features enabled outstanding adsorption of hazardous heavy metals, achieving far better maximum capacities for Cu$$^{2+}$$ and Pb$$^{2+}$$ markedly surpassing conventional hydrogels. Notably, Cu$$^{2+}$$ adsorption induced visible color changes and enhanced mechanical strength, attributed to metal induced secondary crosslinking between amino and hydroxyl groups and adsorbed ions. Cu$$^{2+}$$ adsorption also led to a measurable increase in the Youngs modulus of the hydrogels, likely due to coordination with chitosan functional groups.

Journal Articles

Development of the beam separation test device to evaluate the electric field of non-destructive electrostatic septum

Nagayama, Shota; Kinsho, Michikazu; Harada, Hiroyuki; Yamada, Ippei; Chimura, Motoki; Kojima, Kunihiro; Yamamoto, Kazami; Shimogawa, Tetsushi*; Sato, Atsushi*

Proceedings of 16th International Particle Accelerator Conference (IPAC25) (Internet), p.1025 - 1028, 2025/11

Slow extraction method of synchrotrons is used in nuclear and particle physics experiments, radiation therapy, and many other applications. In the slow extraction process, beam loss at the septum electrode, which separates the extracted beam from the circumferential side, induces activation and damage to the device. To solve this problem, we have devised an electric field measurement device named "Beam separation test device" to evaluate the two-dimensional electric field distribution of the nondestructive electrostatic septum that we are developing. The device consists of a prototype septum, horizontal and vertical wire scanners, and an electron gun installed on a movable stage fixed to a drive unit. This device measures the electric field by injecting an electron beam into the electric field and measuring the bending angle of the beam orbit. In developing this device, an additional optics system was designed to make a narrow electron beam to improve the measurement accuracy of the electric field distribution. In addition, we designed a beam dump that reduces secondary electron emission by utilizing energy loss when particles collide with materials. According to calculations of secondary electron emission, this beam dump can reduce secondary-emission into the chamber by up to 98%.

Journal Articles

Development of a phoswich detector for low-energy gamma rays emitted from alpha emitters

Morishita, Yuki; Yamada, Tsutomu*; Nakasone, Takamasa*; Kanno, Marina*; Sasaki, Miyuki; Sanada, Yukihisa; Torii, Tatsuo*

Radiation Measurements, 188, p.107502_1 - 107502_7, 2025/11

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

The decommissioning of the Fukushima Daiichi Nuclear Power Station requires thorough inspection of piping for contamination, including alpha nuclides. Since external alpha particle measurements are impractical, detection relies on gamma-rays emitted by the alpha nuclides. Therefore, a phoswich detector for detecting low-energy gamma-rays was developed and experimentally validated. The detector was designed with consideration of energy deposition characteristics and consists of YAP:Ce or HR-GAGG scintillators in combination with BGO scintillators, employing a photomultiplier tube for signal amplification. Validation procedures included Monte Carlo simulations and measurements using actual radiation sources. Both measurement and simulation results demonstrate a correlation in scintillator energy depositions across different gamma-ray energies. Pulse Shape Discrimination (PSD) plots effectively differentiate between low-energy and high-energy gamma-rays, thereby confirming the predictions from simulations. These results suggest promising potential for developing a sensitive low-energy gamma-ray detector utilizing various scintillator combinations. The phoswich detector shows promise for effectively detecting low-energy gamma-rays emitted by alpha nuclides in piping.

Journal Articles

Development of the performance evaluation method for small multicopter vertical mobility in a narrow environment

Yamada, Taichi; Suzuki, Soichiro; Ito, Rintaro; Ota, Yua*; Kaneko, Eiichiro*; Ogane, Katsuji*; Kawabata, Kuniaki

Advanced Robotics, 12 Pages, 2025/10

 Times Cited Count:0 Percentile:0.00(Robotics)

We develop a test method to evaluate the vertical moving performance of an unmanned aircraft system (UAS) in a narrow environment, specifically performance for ascending through a narrow aperture. This research aims to boost the UAS industry by pushing for the expansion of UAS use into various places and situations. UAS users should know whether the UAS performance is enough to achieve their objectives and what UAS suits them. However, discussing what/how much UASs can do is complex, especially in a place or situation affecting some UAS functions. Thus, the test method provides an easy-to-understand evaluation of UAS performance for mobility to access a destination in a narrow environment, even for UAS users without technical knowledge. To develop an acceptable test method for the UAS industry, we repeatedly held demonstrations and discussions with UAS manufacturers and users to incorporate their opinions from the early stages of this research. In addition, the experiments show that the test method appropriately indicates the difference in UAS performance. This paper describes the approach of UAS performance evaluation to promote the UAS industry, the development along with UAS users' opinions, and the result of the experiments to compare the type of UAS and consideration.

JAEA Reports

Study on the advancement of LWR MOX Fuel; Study on fuel concept for effective Pu utilization and reduction of spent fuel assemblies

Naganuma, Masayuki; Ikusawa, Yoshihisa; Shuji, Yoshiyuki; Suzuki, Kiichi; Yamada, Yoshikazu; Kamiya, Masayoshi

JAEA-Research 2025-006, 165 Pages, 2025/09

JAEA-Research-2025-006.pdf:5.93MB

As a study for advancing LWR MOX fuel, the fuel concept that can contribute to effective plutonium utilization (e.g. reduction of the number of plu-thermal plants required) and reduction of spent fuel subassemblies (interim storage subassemblies) by using existing reactors was investigated. Specifically, since an increase of Pu loading is effective for the above purposes, MOX fuel candidate concepts with the potential to increase Pu loading in the range of the current MOX fuel guidelines (Pu content: $$leqq$$ 13 wt%, burnup: $$leqq$$ 45 GWd/t, MOX fuel loading: $$leqq$$ 1/3) for PWRs were identified and compared in terms of "core and fuel design", "front-end", and "back-end", and the promising fuel concept was selected. Consequently, it was found that placing fuel elements with burnable poisons in the periphery (mainly in the corners) and adjusting the power peaking in the subassembly can increase the Pu content of the fuel elements in the periphery compared to the existing MOX fuel, which is effective in increasing the total Pu loading. Based on this measures, several fuel candidate concepts were devised, then each fuel specification that maintain criticality and power peaking equivalent to the existing MOX fuel were evaluated. As a result of the comparison of the characteristics of each candidate, the fuel concept in which UO$$_{2}$$-Gd fuel is loaded near the corners was conclusively selected as the most promising concept, because it can increase Pu loading by approximately 15% compared to the existing MOX fuel core and has a lower development burden. Moreover, schematic evaluations were conducted for this fuel concept using the Nuclear Material Balance Analysis Code, confirming the quantitative prospect on how much the above increase in Pu loading would actually affect the number of required plu-thermal plants and the material balance of nuclear fuel cycle.

Journal Articles

Speciation of cesium in a radiocesium-bearing microparticle emitted from Unit 1 during the Fukushima nuclear accident by XANES spectroscopy using transition edge sensor

Takahashi, Yoshio*; Miura, Hikaru*; Yamada, Shinya*; Sekizawa, Oki*; Nitta, Kiyofumi*; Hashimoto, Tadashi*; Yomogida, Takumi; Yamaguchi, Akiko; Okada, Shinji*; Itai, Takaaki*; et al.

Journal of Hazardous Materials, 495, p.139031_1 - 139031_19, 2025/09

 Times Cited Count:1 Percentile:0.00(Engineering, Environmental)

In this presentation, we analyzed the chemical state of cesium in radiocesium-bearing microparticles (CsMPs) released during the 2011 Fukushima Daiichi Nuclear Power Plant accident using high-resolution X-ray absorption spectroscopy (XANES) and micro X-ray fluorescence ($$mu$$-XRF). The results identified two forms of cesium: one dissolved in glass and the other enriched on the surfaces of internal voids. The latter is considered to have originally existed as a gas and became concentrated during the cooling and solidification of the molten glass. These findings are crucial for understanding the formation process of CsMPs during the accident, as well as for future decommissioning and safety assessments.

Journal Articles

Development of scientific communication in the field of human factors and ergonomics

Yamada, Yasuyuki*; Ebara, Takeshi*; Oba, Kyoko; Shoji, Naoto*; Toriizuka, Takashi*; Yagi, Eko*; Yoshitake, Ryoji*

Ningen Kogaku, 61(4), p.252 - 261, 2025/08

This review aims to summarize the human factors and ergonomic understanding of science communication and to present future perspectives, based on discussions within the Science Communication Research Committee of the Japan Human Factors and Ergonomics Society. It first reviewed the definitions, trends, and approaches to science communication, and introduced practices in the field of human factors and ergonomics (HFE) based on its various types. It then discussed the roles of science communication in the context of risk management, outlined key considerations for effective interventions, presented HFE approaches tailored to participants' human traits, and identified the competencies required of science communicators. Finally, it summarized issues for practice and research, and proposed directions for advancing science communication within the domain of HFE. We hope this review contributes to a shared understanding of science communication in HFE and serves as a foundation for its future development.

Journal Articles

Modeling the extraction of bound rubber from silica-filled styrene-butadiene rubber with toluene

Tamura, Yukiko*; Arakawa, Masato*; Takenaka, Mikihito*; Nakanishi, Yohei*; Fujinami, So*; Shibata, Motoki*; Yamamoto, Katsuhiro*; Miyata, Noboru*; Yamada, Masako*; Seto, Hideki*; et al.

Polymer, 333, p.128662_1 - 128662_8, 2025/08

 Times Cited Count:1 Percentile:43.42(Polymer Science)

Journal Articles

Effect of potassium doping on the electrical properties of stacked graphene layers

Yamada, Takatoshi*; Ogawa, Shuichi*; Yoshigoe, Akitaka; Tsuda, Yasutaka; Masuzawa, Tomoaki*; Okada, Mitsuhiro*; Kobashi, Kazufumi*; Okigawa, Yuki*

Japanese Journal of Applied Physics, 64(7), p.07SP17_1 - 07SP17_5, 2025/07

 Times Cited Count:0 Percentile:0.00(Physics, Applied)

Journal Articles

Nanoconfinement-driven energy-efficient CO$$_{2}$$ capture and release at high pressures on a unique large-pore mesoporous carbon

Szab$'o$, L.*; Inoue, Mizuki*; Sekine, Yurina; Motokawa, Ryuhei; Matsumoto, Yusuke*; Nge, T. T.*; Ismail, E.*; Ichinose, Izumi*; Yamada, Tatsuhiko*

ChemSusChem, 18(10), p.e202402034_1 - e202402034_13, 2025/05

 Times Cited Count:0 Percentile:0.00(Chemistry, Multidisciplinary)

Here, we developed a large-pore mesoporous carbon with pore sizes centered around 20-30 nm using a templated technical lignin. During the soft-templating process, unique cylindrical supramolecular assemblies form from the copolymer template, distinct from other systems reported thus far. This peculiar nanostructuring takes place due to the presence of polyethylene glycol (PEG) segments on both the Pluronic template and the PEG- grafted lignin derivative (glycol lignin). A large increase in CO$$_{2}$$ uptake occurs on the resulting large-pore mesoporous carbon at 270 K close to the saturation pressure, owing to capillary condensation.

Journal Articles

Linking combustion-derived magnetite and black carbon; Insights from magnetic characterization of PM$$_{2.5}$$ in downwind East Asia

Nozomu, Tsuchiya*; Ikemori, Fumikazu*; Kawasaki, Kazuo*; Yamada, Rena*; Hata, Mitsuhiko*; Furuuchi, Masami*; Iwamoto, Yoko*; Kaneyasu, Naoki*; Sadanaga, Yasuhiro*; Watanabe, Takahiro; et al.

Environmental Science & Technology, 59(21), p.10400 - 10410, 2025/05

 Times Cited Count:1 Percentile:47.55(Engineering, Environmental)

Black carbon (BC) is a typical primary aerosol emitted from combustion. While its co-existence with iron oxides (FeO$$_{x}$$) has recently been reported, the extent of bias caused by FeO$$_{x}$$ mixing to the BC observations is largely unknown. To identify the dominant FeO$$_{x}$$ emission sources and associated overestimation of BC, magnetics properties of PM$$_{2.5}$$ collected at a remote site in East Asia was investigated in combination with detailed isotopic and chemical analyses. Consequently, biomass burning events did not enhance aerosol magnetism as they did for the mass concentration of BC, whereas coal burning events coincided with periods of high magnetization. Therefore, magnetization/BC ratio is proposed as a highly selective indicator for identifying combustion sources (i.e. coal, oil or biomass burning).

Journal Articles

Development of a compact detector for measurement of alpha contamination in piping

Morishita, Yuki; Peschet, L.; Yamada, Tsutomu*; Nakasone, Takamasa*; Kanno, Marina*; Sasaki, Miyuki; Sanada, Yukihisa; Torii, Tatsuo*

Radiation Measurements, 183, p.107414_1 - 107414_6, 2025/04

 Times Cited Count:2 Percentile:64.08(Nuclear Science & Technology)

In the decommissioning nuclear facilities, it is crucial to inspect piping for contamination to prevent worker exposure to alpha-emitting nuclides. Traditional methods using gamma rays and neutrons are inadequate for detecting small amounts of alpha nuclides due to the short range (approximately 4 cm) of alpha particles in air. To address this, we developed a compact detector capable of distinguishing between alpha particles for direct measurement within pipes. This detector, comprising a ZnS(Ag) scintillator for alpha particles and a plastic scintillator for beta particles (gamma rays), was coupled to a small photomultiplier tube. The system demonstrated high accuracy in differentiating between alpha and beta radiation through pulse shape discrimination (PSD). Monte Carlo simulations and empirical measurements confirmed the detector's effectiveness, achieving a 51.3% detection efficiency for alpha particles with negligible sensitivity to beta and gamma radiation. This innovation presents a significant advancement for direct alpha contamination measurement in environments with high beta and gamma backgrounds, such as the Fukushima Daiichi Nuclear Power Plant decommissioning site.

JAEA Reports

Environmental radiation monitoring data from 10 years after the accident at the Fukushima Daiichi Nuclear Power Station, conducted by Oarai Nuclear Engineering Institute, JAEA

Inoue, Yuki; Yamada, Junya; Hamaguchi, Takumi; Seya, Natsumi; Muto, Yasunobu; Nohara, Naofumi; Oishi, Tetsuya; Hashimoto, Makoto

JAEA-Data/Code 2024-017, 109 Pages, 2025/03

JAEA-Data-Code-2024-017.pdf:4.54MB

This report presents the results of environmental radiation monitoring at Oarai Nuclear Engineering Institute, JAEA for 10 years from 2011 to 2021 after the accident at the Fukushima Daiichi Nuclear Power Station. Database of monitoring results are included as an appendix. Environmental transfer parameters, deposition velocity, resuspension factor, concentration factor and distribution coefficient, are calculated as an Appendix.

Journal Articles

Luminescence of samarium complexes in ${it N,N,N',N'}$-tetraoctyl diglycolamide solvent induced by hydrogen ion beam

Nakahara, Masaumi; Ishii, Yasuyuki*; Yamagata, Ryohei*; Yamada, Naoto*; Koka, Masashi*

QST-M-52; QST Takasaki Annual Report 2023, P. 47, 2025/03

The development of an extractant and a separation process have been studied to recover Am and Cm from high-level liquid waste. To strip Am and Cm from loaded solvent effectively, the evaluation for complex structures is attempted with ion beam induced luminescence. In this study, Sm as a simulated material of minor actinide in the ${it N,N,N',N'}$-tetraoctyl diglycolamide were irradiated by the H$$^{+}$$ ion beam, and the ion beam induced luminescence spectra of Sm complexes were measured to evaluate the structures of Sm complexes.

Journal Articles

Assessment of individual external exposure doses based on environmental radiation in areas affected by the Fukushima Daiichi Nuclear Power Station accident

Sato, Rina; Yoshimura, Kazuya; Sanada, Yukihisa; Mikami, Satoshi; Yamada, Tsutomu*; Nakasone, Takamasa*; Kanaizuka, Seiichi*; Sato, Tetsuro*; Mori, Tsubasa*; Takagi, Marie*

Environment International, 194, p.109148_1 - 109148_8, 2024/12

 Times Cited Count:6 Percentile:53.54(Environmental Sciences)

Assessment of individual external doses from ambient dose equivalents is used for predictive and retrospective assessments where personal dosimeters are not applicable. However, it tends to contain more errors than assessment by personal dosimetry due to various parameters. Therefore, in order to accurately assess the individual dose from ambient dose equivalents, a model that estimates effective doses considering life patterns and the shielding effects by buildings and vehicles, were developed in this study. The model parameters were examined using robust datasets of environmental radiation measured in the areas affected by the Fukushima Daiichi Nuclear Power Station accident in 2020 to 2021. The accuracy of the model was validated by comparison with 106 daily personal doses measured in Fukushima Prefecture in 2020. The measured personal dose was well reproduced by the model-estimated effective dose, showing that the model can be used to assess the individual exposure dose, similar to personal dosimetry. Furthermore, this model is an effective tool for radiation protection, as it can estimate the individual dose predictively and retrospectively by using environmental radiation data.

Journal Articles

Surface depth analysis of chemical changes in random copolymer thin films composed of hydrophilic and hydrophobic silicon-based monomers induced by plasma treatment as studied by hard X-ray photoelectron spectroscopy and neutron reflectivity measurements

Yamamoto, Katsuhiro*; Imai, Tatsuya*; Kawai, Atsuki*; Ito, Eri*; Miyazaki, Tsukasa*; Miyata, Noboru*; Yamada, Norifumi*; Seto, Hideki*; Aoki, Hiroyuki

ACS Applied Materials & Interfaces, 16(48), p.66782 - 66791, 2024/11

 Times Cited Count:1 Percentile:9.72(Nanoscience & Nanotechnology)

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