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Journal Articles

Revising the 4${it f}$ symmetry in CeCu$$_{2}$$Ge$$_{2}$$; Soft X-ray absorption and hard X-ray photoemission spectroscopy

Aratani, Hidekazu*; Nakatani, Yasuhiro*; Fujiwara, Hidenori*; Kawada, Moeki*; Kanai, Yuina*; Yamagami, Kohei*; Fujioka, Shuhei*; Hamamoto, Satoru*; Kuga, Kentaro*; Kiss, Takayuki*; et al.

Physical Review B, 98(12), p.121113_1 - 121113_6, 2018/09

AA2018-0352.pdf:1.16MB

 Times Cited Count:3 Percentile:24.8(Materials Science, Multidisciplinary)

Journal Articles

Three-dimensional electronic structures and the metal-insulator transition in Ruddlesden-Popper iridates

Yamasaki, Atsushi*; Fujiwara, Hidenori*; Tachibana, Shoichi*; Iwasaki, Daisuke*; Higashino, Yuji*; Yoshimi, Chiaki*; Nakagawa, Koya*; Nakatani, Yasuhiro*; Yamagami, Kohei*; Aratani, Hidekazu*; et al.

Physical Review B, 94(11), p.115103_1 - 115103_10, 2016/11

AA2016-0587.pdf:2.55MB

 Times Cited Count:14 Percentile:64.66(Materials Science, Multidisciplinary)

In this study, we systematically investigate three-dimensional(3D) momentum-resolved electronic structures of Ruddlesden-Popper-type iridium oxides Sr$$_{n+1}$$Ir$$_{n}$$O$$_{3n+1}$$ using soft-X-ray angle-resolved photoemission spectroscopy (SX-ARPES). Our results provide direct evidence of an insulator-to-metal transition that occurs upon increasing the dimensionality of the IrO$$_{2}$$-plane structure. This transition occurs when the spin-orbit-coupled $$j_{eff}$$ = 1/2 band changes its behavior in the dispersion relation and moves across the Fermi energy. By scanning the photon energy over 350 eV, we reveal the 3D Fermi surface in SrIrO$$_{3}$$ and $$k_{z}$$-dependent oscillations of photoelectron intensity in Sr$$_{3}$$Ir$$_{2}$$O$$_{7}$$. To corroborate the physics deduced using low-energy ARPES studies, we propose to utilize SX-ARPES as a powerful complementary technique, as this method surveys more than one whole Brillouin zone and provides a panoramic view of electronic structures.

Journal Articles

Thickness-dependent magnetic properties and strain-induced orbital magnetic moment in SrRuO$$_{3}$$ thin films

Ishigami, Keisuke*; Yoshimatsu, Kohei*; Toyota, Daisuke*; Takizawa, Masaru*; Yoshida, Teppei*; Shibata, Goro*; Harano, Takayuki*; Takahashi, Yukio*; Kadono, Toshiharu*; Verma, V. K.*; et al.

Physical Review B, 92(6), p.064402_1 - 064402_5, 2015/08

 Times Cited Count:29 Percentile:80.07(Materials Science, Multidisciplinary)

Journal Articles

Probing strongly correlated 4$$f$$-orbital symmetry of the ground state in Yb compounds by linear dichroism in core-level photoemission

Mori, Takeo*; Kitayama, Satoshi*; Kanai, Yuina*; Naimen, Sho*; Fujiwara, Hidenori*; Higashiya, Atsushi*; Tamasaku, Kenji*; Tanaka, Arata*; Terashima, Kensei*; Imada, Shin*; et al.

Journal of the Physical Society of Japan, 83(12), p.123702_1 - 123702_5, 2014/12

 Times Cited Count:15 Percentile:71.43(Physics, Multidisciplinary)

We show that the strongly correlated 4$$f$$-orbital symmetry of the ground state is revealed by linear dichroism in core-level photoemission spectra, as we have discovered for YbRh$$_{2}$$Si$$_{2}$$ and YbCu$$_{2}$$Si$$_{2}$$. Theoretical analysis shows us that the linear dichroism reflects the anisotropic charge distributions resulting from a crystalline electric field. We have successfully determined the ground-state 4$$f$$ symmetry for both compounds from the polarization-dependent angle resolved core-level spectra at a temperature well below the first excitation energy. The excited-state symmetry is also probed by temperature dependence of the linear dichroism where the high measurement temperatures are on the order of the crystal-field-splitting energies.

Journal Articles

Thickness-dependent ferromagnetic metal to paramagnetic insulator transition in La$$_{0.6}$$Sr$$_{0.4}$$MnO$$_3$$ thin films studied by X-ray magnetic circular dichroism

Shibata, Goro*; Yoshimatsu, Kohei*; Sakai, Enju*; Singh, V. R.*; Verma, V.*; Ishigami, Keisuke*; Harano, Takayuki*; Kadono, Toshiharu*; Takeda, Yukiharu; Okane, Tetsuo; et al.

Physical Review B, 89(23), p.235123_1 - 235123_5, 2014/06

AA2015-0419.pdf:0.33MB

 Times Cited Count:12 Percentile:53.39(Materials Science, Multidisciplinary)

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