Initialising ...
Initialising ...
Initialising ...
Initialising ...
Initialising ...
Initialising ...
Initialising ...
-tetraoctyl diglycolamide solvent induced by hydrogen ion beamNakahara, Masaumi; Ishii, Yasuyuki*; Yamagata, Ryohei*; Yamada, Naoto*; Koka, Masashi*
QST-M-52; QST Takasaki Annual Report 2023, P. 47, 2025/03
The development of an extractant and a separation process have been studied to recover Am and Cm from high-level liquid waste. To strip Am and Cm from loaded solvent effectively, the evaluation for complex structures is attempted with ion beam induced luminescence. In this study, Sm as a simulated material of minor actinide in the -tetraoctyl diglycolamide were irradiated by the H
ion beam, and the ion beam induced luminescence spectra of Sm complexes were measured to evaluate the structures of Sm complexes.
Nakahara, Masaumi; Watanabe, So; Ishii, Yasuyuki*; Yamagata, Ryohei*; Yuri, Yosuke*; Yuyama, Takahiro*; Ishizaka, Tomohisa*; Koka, Masashi*; Yamada, Naoto*; Hagura, Naoto*
Nuclear Instruments and Methods in Physics Research B, 554, p.165449_1 - 165449_5, 2024/09
Times Cited Count：0 Percentile：0.00(Instruments & Instrumentation)Ion beam induced luminescence analysis of lanthanide complexes in the organic solvents for minor actinides recovery process was carried out to investigate the structures of complexes. In this study, hydrogen ion beam obtained from the single-ended accelerator and argon ion beam obtained from the azimuthally varying field cyclotron were used in Takasaki Ion Accelerators for Advanced Radiation Application in National Institutes for Quantum Science and Technology. In the experiments, ion beam induced luminescence spectra of lanthanide complexes in the organic solvents were measured, and the relationship between the obtained spectra and the structures of complexes was studied.
Nakahara, Masaumi; Watanabe, So; Yuyama, Takahiro*; Ishizaka, Tomohisa*; Yuri, Yosuke*; Ishii, Yasuyuki*; Yamagata, Ryohei*; Yamada, Naoto*; Koka, Masashi*; Kada, Wataru*; et al.
QST-M-47; QST Takasaki Annual Report 2022, P. 64, 2024/03
An extraction chromatography method has been studied to recover minor actinides from high-level liquid waste. For effective elution of minor actinides in an adsorbent, the structures of complexes are attempted to be evaluated with ion beam induced luminescence. In this study, Eu complexes in the adsorbent were irradiated by Ar
ion beam, and the ion beam induced luminescence spectra of Eu complexes were measured to evaluate the structures of Eu complexes.
Nakahara, Masaumi; Watanabe, So; Takeuchi, Masayuki; Yuyama, Takahiro*; Ishizaka, Tomohisa*; Ishii, Yasuyuki*; Yamagata, Ryohei*; Yamada, Naoto*; Koka, Masashi*; Kada, Wataru*; et al.
Nuclear Instruments and Methods in Physics Research B, 542, p.144 - 150, 2023/09
Times Cited Count：5 Percentile：80.64(Instruments & Instrumentation)The structures of Eu complexes in the adsorbents prepared with various extractants were evaluated by ion beam induced luminescence analysis in an extraction chromatography for minor actinides recovery. The luminescence of Eu was measured with a proton beam obtained from the single-ended accelerator and an argon ion beam obtained from the azimuthally varying field cyclotron in Takasaki Ion Accelerators for Advanced Radiation Application in National Institutes for Quantum Science and Technology. In this study, it was confirmed that the spectral shape of Eu complexes in the adsorbents varied depending on the kinds of extractants, and the correlation between the change in the spectra and the structures of Eu complexes was investigated.
Nakahara, Masaumi; Watanabe, So; Ishii, Yasuyuki*; Yamagata, Ryohei*; Yamada, Naoto*; Koka, Masashi*; Yuyama, Takahiro*; Ishizaka, Tomohisa*; Kada, Wataru*; Hagura, Naoto*
QST-M-39; QST Takasaki Annual Report 2021, P. 62, 2023/02
In an extraction chromatography method for minor actinides recovery, analysis for the structure of complex in a silica-based adsorbent has been studied to separate minor actinides efficiently. In this study, Eu was used as simulated material of minor actinides, and silica-based adsorbents containing Eu complex were prepared. The ion beam induced luminescence spectra of Eu complexes in silica-based adsorbents were measured, and the basic data for the structures of Eu complexes were obtained.
Yamagata, Kazuhito*; Ouchi, Kazuki; Marumo, Kazuki*; Tasaki-Handa, Yuiko*; Haraga, Tomoko; Saito, Shingo*
Inorganic Chemistry, 62(2), p.730 - 738, 2023/01
Times Cited Count：3 Percentile：42.77(Chemistry, Inorganic & Nuclear)The inert NpO
complex with a fluorescein-modified phenanthroline-2,9-dicarboxylic acid was found by kinetic selection using polyacrylamide gel electrophoresis (PAGE) from a small chemical library. The small spontaneous dissociation rate constant of 8
10
s
(the half-life of 23 hours) was determined. This is the singly-charged NpO complex exhibiting unusual kinetic inertness in aqueous solution, one million times slower than widely accepted fast kinetics of neptunyl complexes. Selective fluorescence detection of NpO was achieved in PAGE with a detection limit of 68 pmol dm
(17 fg). This system was successfully applied to simulated spent nuclear fuel and high-level radioactive waste samples.
Kureta, Masatoshi; Yamagata, Yoji*; Miyakoshi, Ken*; Mashii, Tatsuya*; Miura, Yoshiaki*; Takahashi, Kazunori*
JAEA-Research 2022-007, 28 Pages, 2022/09
JAEA-Research-2022-007.pdf:8.17MB
To enhance energy separation in a counter-current Ranque-Hilsch vortex tube, a newly designed hollow helical fin was inserted into the hot tube of the vortex tube. In this study, the effect of the fin on the energy separation was investigated using three types of the vortex tube, and then computational fluid dynamics (CFD) simulation has been conducted to understand the experimental results and discuss the flow structure in the vortex tube with the hollow helical fin. As a result, it was found from the experimental data that the fin effectively enhanced energy separation, and that the tube length could be shorten. When the inlet air pressure was 0.5 MPa, the maximum temperature difference from the inlet to the cold exit was 62.2
C. The CFD code employing the Reynolds Stress Model (RSM) turbulence model was used to analyze the fluid dynamics in the vortex tube. As a result, it was confirmed that the temperature, velocity, and pressure distributions changed significantly at the stagnation point, and that the distributions in the tube with the fin were completely different from those without the fin. It was thought that a strong reversing helical vortex flow with small recirculating vortex structure formed between the fin end and the stagnation point on the cold exit side would enhance energy separation in the vortex tube with the hollow helical fin.
Yoshimoto, Masahiro; Nakanoya, Takamitsu; Yamazaki, Yoshio; Saha, P. K.; Kinsho, Michikazu; Yamamoto, Shunya*; Okazaki, Hiroyuki*; Taguchi, Tomitsugu*; Yamada, Naoto*; Yamagata, Ryohei*
Proceedings of 18th Annual Meeting of Particle Accelerator Society of Japan (Internet), p.850 - 854, 2021/10
no abstracts in English
Fe and 
Pu deposited on Earth constrain the r-process yields of recent nearby supernovaeWallner, A.*; Froehlich, M. B.*; Hotchkis, M. A. C.*; Kinoshita, N.*; Paul, M.*; Martschini, M.*; Pavetich, S.*; Tims, S. G.*; Kivel, N.*; Schumann, D.*; et al.
Science, 372(6543), p.742 - 745, 2021/05
Times Cited Count：66 Percentile：97.00(Multidisciplinary Sciences)Half of the chemical elements heavier than iron are produced by the rapid neutron capture process (r-process). The sites and yields of this process are disputed, with candidates including some types of supernovae (SNe) and mergers of neutron stars. We search for two isotopic signatures in a sample of Pacific Ocean crust-iron-60 (Fe) (half-life, 2.6 million years), which is predominantly produced in massive stars and ejected in supernova explosions, and Pu (half-life, 80.6 million years), which is produced solely in r-process events. We detect two distinct influxes of Fe to Earth in the last 10 million years and accompanying lower quantities of Pu. The Pu/Fe influx ratios are similar for both events. The Pu influx is lower than expected if SNe dominate r-process nucleosynthesis, which implies some contribution from other sources.
Ma, B.*; Teshigawara, Makoto; Wakabayashi, Yasuo*; Yan, M.*; Hashiguchi, Takao*; Yamagata, Yutaka*; Wang, S.*; Ikeda, Yujiro*; Otake, Yoshie*
Nuclear Instruments and Methods in Physics Research A, 995, p.165079_1 - 165079_7, 2021/04
Times Cited Count：2 Percentile：25.50(Instruments & Instrumentation)We have optimized a cold neutron moderator to be operated at the RIKEN accelerator-driven compact neutron source. We selected a safe and easy to manage material, mesitylene, as the RANS cold moderator. An efficient moderator system was designed by studying and optimizing a coupled cold neutron moderator of mesitylene at 20 K with a polyethylene (PE) pre-moderator at room temperature in the slab geometry with Particle and Heavy Ion Transport code System (PHITS) simulations. The parameters of mesitylene and PE thickness, the reflector, and the shielding configuration were studied to increase cold neutron intensities. Consequently, an integrated cold neutron intensity of 1.1510
n/cm
/
A at 2 m from the neutron-producing target was finally achieved, which was 12 times higher than that of the current PE moderator. The results showed attractive application prospect of mesitylene as cold neutron moderator material.
Yoshimoto, Masahiro; Nakanoya, Takamitsu; Yamazaki, Yoshio; Saha, P. K.; Kinsho, Michikazu; Yamamoto, Shunya*; Okazaki, Hiroyuki*; Taguchi, Tomitsugu*; Yamada, Naoto*; Yamagata, Ryohei*
JPS Conference Proceedings (Internet), 33, p.011019_1 - 011019_7, 2021/03
The multi-turn charge-exchange H
beam injection scheme with stripper foils is one of the key techniques to achieve a MW-class high power proton beam. The J-PARC RCS adopts Hybrid type Boron-doped Carbon (HBC) stripper foil, which was developed in KEK to improve the lifetime. Indeed, the RCS user operation confirmed that HBC foil has the great advantage of a longer lifetime against high beam irradiation. To examine characteristics of the HBC foils, various beam studies were performed, such as the stripping efficiency measurement and long-term observation with an H beam in the J-PARC RCS, foil analysis using RBS, EDR and PIXE methods, and SEM and TEM observation after the ion beam irradiation in Takasaki Ion Accelerators for Advanced Radiation Application (TIARA) on National Institutes for Quantum and Radiological Science and Technology (QST). Recently, the deposition apparatus for the HBC foils from the KEK Tsukuba-site was relocated to the JAEA Tokai-site, and we started fabrication of new HBC foil in 2017. (The new one fabricated in JAEA we call J-HBC foil.) And, we continue investigations in TIARA with the J-HBC foils. Furthermore, in-depth researches by changing the process parameters of the foil deposition are carried on. Recent results suggest that the amount of the boron doped in the foil is more important parameter than the ratio of the discharge amount of carbon from cathode and anode electrodes. In this presentation, we will report the details of recent analysis of the J-HBC foil.
-rays after neutron capture by 
La for a T-violation searchOkudaira, Takuya; Shimizu, Hirohiko*; Kitaguchi, Masaaki*; Hirota, Katsuya*; Haddock, C. C.*; Ito, Ikuya*; Yamamoto, Tomoki*; Endo, Shunsuke*; Ishizaki, Kohei*; Sato, Takumi*; et al.
EPJ Web of Conferences, 219, p.09001_1 - 09001_6, 2019/12
Parity violating effects enhanced by up to 10
times have been observed in several neutron induced compound nuclei. There is a theoretical prediction that time reversal (T) violating effects can also be enhanced in these nuclei implying that T-violation can be searched for by making very sensitive measurements. However, the enhancement factor has not yet been measured in all nuclei. The angular distribution of the (n,) reaction was measured with La by using a germanium detector assembly at J-PARC, and the enhancement factor was obtained. From the result, the measurement time to achieve the most sensitive T-violation search was estimated as 1.4 days, and a 40% polarized La target and a 70% polarized 
He spin filter whose thickness is 70 atm
cm are needed. Therefore high quality He spin filter is developed in JAEA. The measurement result of the (n,) reaction at J-PARC and the development status of the He spin filter will be presented.
Sato, Yuji*; Tsukamoto, Masahiro*; Shobu, Takahisa; Yamashita, Yoshihiro*; Yamagata, Shuto*; Nishi, Takaya*; Higashino, Ritsuko*; Okubo, Tomomasa*; Nakano, Hitoshi*; Abe, Nobuyuki*
Applied Physics A, 124(4), p.288_1 - 288_6, 2018/04
Times Cited Count：19 Percentile：62.04(Materials Science, Multidisciplinary)The dynamics of titanium (Ti) melted by laser irradiation was investigated in a synchrotron radiation experiment. As an indicator of wettability, the contact angle between a selective laser melting (SLM) baseplate and the molten Ti was measured by synchrotron X-rays at 30 keV during laser irradiation. As the baseplate temperature increased, the contact angle decreased, down to 28 degrees at a baseplate temperature of 500C. Based on this result, the influence of wettability of a Ti plate fabricated by SLM in a vacuum was investigated. It was revealed that the improvement of wettability by preheating suppressed sputtering generation, and a surface having a small surface roughness was fabricated by SLM in a vacuum.
Sekio, Yoshihiro; Yamagata, Ichiro; Akasaka, Naoaki; Sakaguchi, Norihito*
Proceedings of International Conference on Fast Reactors and Related Fuel Cycles; Next Generation Nuclear Systems for Sustainable Development (FR-17) (USB Flash Drive), 8 Pages, 2017/06
The widths of void denuded zones (VDZs) which were formed near random grain boundaries by neutron irradiation were analyzed in order to perform quantitative evaluations for the irradiation-induced point defect behavior in the modified 316 stainless steel (PNC316) having been developed by JAEA. Namely, the temperature dependence of VDZ width was investigated and vacancy migration energy of the PNC316 steel was estimated from the VDZ width analysis for the neutron-irradiated specimens. The obtained value of vacancy migration energy was estimated as 1.46 eV, which was consistent with that from the exiting method using electron in-situ examination. This indicates that VDZ analysis could be effective method to evaluate especially vacancy migration energy during irradiation, and this would be realized from not in-situ observation but post-irradiation examination in the case of neutron irradiation.
Co -ray irradiation facilitiesUno, Sadanori; Hanaya, Hiroaki; Yamagata, Ryohei; Seito, Hajime; Nagao, Yuto; Yamasaki, Shota; Agematsu, Takashi; Kawashima, Ikuo*; Yagi, Norihiko*; Takagi, Masahide*; et al.
JAEA-Review 2015-022, JAEA Takasaki Annual Report 2014, P. 172, 2016/02
This paper reports on the operation status of the -ray irradiation facilities and the electron accelerator in fiscal 2014 at the Takasaki Advanced Radiation Research Institute of JAEA. The -ray irradiation facilities were operated smoothly, whereas the electron accelerator stopped for five months because of successive troubles of discharge due to deterioration of equipment over thirty-four years. The annual operation times of the -ray irradiation facilities of the first, second and food buildings were 19,907, 13,831 and 7,293 hours, respectively, and that of the electron accelerator was 746 hours. The -ray irradiation facilities were replenished with new five sources of 2.22 PBq, and twenty old sources were removed for disposal. The electron accelerator was repaired for each trouble, however, the complete recovery has not yet been achieved.
-ray irradiation facilitiesAgematsu, Takashi; Uno, Sadanori; Hanaya, Hiroaki; Yamagata, Ryohei; Seito, Hajime; Nagao, Yuto; Yamasaki, Shota; Kawashima, Ikuo*; Yagi, Norihiko*; Takagi, Masahide*; et al.
JAEA-Review 2015-022, JAEA Takasaki Annual Report 2014, P. 173, 2016/02
The electron accelerator and the three -ray irradiation facilities of Takasaki Advanced Radiation Research Institute were operated for various research subjects according to the operation plan in FY 2014. The number of research subjects in FY 2014 decreased at the electron accelerator with operation stop by accelerator trouble, and increased slightly at the -ray irradiation facilities as compared with FY 2013, and research subjects were 205 and 857, respectively. Among these research subjects, 35 and 172 related to recovery from the Fukushima Daiichi Nuclear disaster, respectively, were performed at the electron accelerator and the -ray irradiation facilities, respectively.
Uno, Sadanori; Hanaya, Hiroaki; Yamasaki, Shota; Yamagata, Ryohei; Seito, Hajime; Nagao, Yuto; Agematsu, Takashi; Kawashima, Ikuo*; Yagi, Norihiko*; Takagi, Masahide*; et al.
Dai-28-Kai Tandemu Kasokuki Oyobi Sono Shuhen Gijutsu No Kenkyukai Hokokushu, p.121 - 123, 2015/12
no abstracts in English
-ray irradiation facilitiesAgematsu, Takashi; Hanaya, Hiroaki; Yamagata, Ryohei; Seito, Hajime; Nagao, Yuto; Kaneko, Hirohisa; Yamaguchi, Toshiyuki*; Kawashima, Ikuo*; Yagi, Norihiko*; Takagi, Masahide*; et al.
JAEA-Review 2014-050, JAEA Takasaki Annual Report 2013, P. 182, 2015/03
The electron accelerator and the -ray irradiation facility have been operated approximately smoothly. The annual operation time in FY 2013 for the electron accelerator, the first, the second cobalt irradiation facility and food irradiation facility are 1242 h, 18,900 h, 11,804 h and 6,587 h, respectively. Typically repairs were next ones. The SF
gas withdrawal system was renewed at the electron accelerator. The 600 m water storage tank was installed to keep pool-water for the cobalt facilities maintenance. New pieces of Co sources were purchased and loaded to the first and the second irradiation facility. The maintenance check was done for the food irradiation facility.
-ray irradiation facilitiesAgematsu, Takashi; Hanaya, Hiroaki; Yamagata, Ryohei; Seito, Hajime; Nagao, Yuto; Kaneko, Hirohisa; Yamaguchi, Toshiyuki*; Kawashima, Ikuo*; Yagi, Norihiko*; Takagi, Masahide*; et al.
JAEA-Review 2014-050, JAEA Takasaki Annual Report 2013, P. 183, 2015/03
The electron accelerator and the three -ray irradiation facilities were operated for various research subjects according to the operation plan in FY 2013. The number of research subjects at the electron accelerator and at the -ray irradiation facilities kept constant from FY 2012. Among these research subjects, 47 and 91 ones respectively performed at the electron accelerator and the -ray irradiation facilities were relevant to recovery from the Fukushima Daiichi nuclear disaster.
Sekio, Yoshihiro; Yamagata, Ichiro; Yamashita, Shinichiro; Inoue, Masaki; Maeda, Koji
Proceedings of 2014 Nuclear Plant Chemistry Conference (NPC 2014) (USB Flash Drive), 10 Pages, 2014/10
In the Fukushima Dai-ichi Nuclear Power Plant accident, seawater was temporarily injected into the spent fuel pools since water cooling and feeding functions were lost. For fuel assemblies which experienced seawater immersion, surface corrosion due to seawater constituents and the resultant degradation of mechanical property are of concern. Therefore, in order to assess the integrity of fuel assemblies (especially cladding tubes), the effects of seawater immersion on corrosion behavior and mechanical properties for as-recieved and irradiated Zircaloy-2 cladding tubes were investigated in the present study. As a result, no obvious surface corrosion and no significant degradation in the tensile strength property were observed after both artificial and natural seawater immersion tests for both steels. This suggests that the effects of seawater immersions on corrosion behavior and mechanical property (especially tensile property) for Zircaloy-2 cladding tubes are probably negligible.
