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Al
through directional Compton profile measurement小泉 昭久*; 久保 康則*; 山本 悦嗣; 芳賀 芳範; 櫻井 吉晴*
Journal of the Physical Society of Japan, 88(3), p.034714_1 - 034714_6, 2019/03
パーセンタイル：100(Physics, Multidisciplinary)Directional Compton profiles of a heavy fermion compound UPdAl are measured in the basal plane of the hexagonal lattice. A remarkable change of the two-dimensional electron occupation number densities has been observed between 20 K and 100 K. Obtained results are attributed to the modification of the 5
electronic states.
and URhGe立岩 尚之; 芳賀 芳範; 山本 悦嗣
Physical Review B, 99(9), p.094417_1 - 094417_12, 2019/03
パーセンタイル：100(Materials Science, Multidisciplinary)ウラン系強磁性物質URhSiについて、強磁性転移温度
近辺で磁気測定を行い、臨界現象の研究を行った。自発磁化の温度依存に関する臨界指数
、磁化率の指数
、における磁化に関する指数
を、修正アロットプロットとスケーリング理論等を用いて決定した。URhSiの強磁性状態は一軸磁気異方性が大きいものの、臨界指数は三次元イジングモデルから期待されるもの( = 0.325, = 1.241, and = 4.82)とは異なることが明らかにされた。URhSiの臨界指数( = 0.300 
0.002, = 1.00 0.02, and = 4.32 0.04)は、ウラン系強磁性超伝導物質UGeとURhGeと類似している。URhSiの静的磁性と動的磁性をウラン系強磁性超伝導物質と対比させ議論する。
states of uranium compounds revealed by 4
-5 resonant photoelectron spectroscopy藤森 伸一; 小畠 雅明; 竹田 幸治; 岡根 哲夫; 斎藤 祐児; 藤森 淳; 山上 浩志; 芳賀 芳範; 山本 悦嗣; 大貫 惇睦*
Physical Review B, 99(3), p.035109_1 - 035109_5, 2019/01
パーセンタイル：100(Materials Science, Multidisciplinary)In the present study, we have elucidated the nature of the electron correlation effect in uranium compounds by imaging the partial 
density of states (pDOS) of typical itinerant, localized, and heavy fermion uranium compounds by using the 
4-5 resonant photoemission spectroscopy. Obtained 
pDOS exhibit a systematic trend depending on the physical properties of compounds: Although the coherent peak at the Fermi level can be explained by the band-structure calculation, an incoherent peak emerges on the higher binding energy side (
) in the cases of localized and heavy fermion compounds. The intensity and energy position of the incoherent peak is increased and shifted to a higher binding energy as the localization of the state increases. These behaviors are consistent with the prediction of the Mott metal-insulator transition, suggesting that the Hubbard-
type mechanism takes an essential role in the 
electronic structure of actinide materials.
立岩 尚之; 芳賀 芳範; 山本 悦嗣
Physical Review Letters, 121(23), p.237001_1 - 237001_6, 2018/12
被引用回数：1 パーセンタイル：47.22(Physics, Multidisciplinary)ウラン系強磁性超伝導物質UGeの高圧下磁化測定を行い、データをTakahashiによるスピンのゆらぎ理論を用いて解析した。強磁性相FM1とFM2の相境界
で、スピンゆらぎスペクトルの分布幅
に明確な異常が現れた。では、超伝導転移温度
が最大値を示す。このことは、近辺で発達する強磁性スピンのゆらぎが超伝導出現に役割を果たすことを示唆する。また、パラメーター
(ここで、
は強磁性転移温度)の圧力変化から、局在性の強いFM2から遍歴性の強いFM1へ基底状態は転移することが示唆された。との関係について、銅酸化物超伝導体等、他の超伝導物質と議論された。
electrons in actinide ferromagnets with spin fluctuation theory立岩 尚之; Posp
il, J.*; 芳賀 芳範; 酒井 宏典; 松田 達磨*; 山本 悦嗣
Progress in Nuclear Science and Technology (Internet), 5, p.104 - 107, 2018/12
ウラン系強磁性超伝導物質UGe, URhGe, UCoGeについて盛んに研究が行われてきた。最近、我々は69個のウラン化合物、7個のネプツニウム化合物、4個のプルトニウム化合物について、スピンゆらぎ理論の適用性を検討した。その結果、アクチノイド5電子の遍歴性を示唆する結果が得られた。会議では全強磁性化合物の解析結果と、UGeのスピンのゆらぎパラーメーターの圧力依存を議論する。
states in UPd
Al and valence crossover in the Vicinity of Heavy-Fermion superconductivity目時 直人; 芳賀 芳範; 山本 悦嗣; 松田 雅昌*
Journal of the Physical Society of Japan, 87(11), p.114712_1 - 114712_9, 2018/11
パーセンタイル：100(Physics, Multidisciplinary)ウラン金属間化合物UPdAlは、四価イオンU
の局在5(
)電子状態を伴うことを中性子散乱による結晶場スペクトルから明らかにした。この電子状態は、最近研究した電子数と結晶構造が同じ希土類参照物質PrPdAlと同一であり、c軸方向に大きな磁気モーメントを伴う平べったい形状の軌道が、縦長の体心正方晶の持つ二次元結晶場ポテンシャルによって安定化されていることがわかった。ウランの5電子が金属状態において局在的な性格を持つことは非常に珍しい発見であり、やはり、結晶構造の特殊性に起因する。ウランが四価イオンであることは、三価のNpPdAlとの間に価数転移が存在することを意味し、この価数転移が結晶格子の異常や電気抵抗の増加によって観察されることを明らかにした。また、価数が不安定な領域で超伝導や磁気転移、重い電子系状態など多体効果の存在を示す数多くの現象が生じていることがわかった。
Si studied by photoelectron spectroscopy (INVITED)藤森 伸一; 竹田 幸治; 岡根 哲夫; 斎藤 祐児; 藤森 淳; 山上 浩志; 芳賀 芳範; 山本 悦嗣; 大貫 惇睦*
Progress in Nuclear Science and Technology (Internet), 5, p.82 - 85, 2018/11
One of the most remarkable properties of actinide compounds is the coexistence of superconductivity and magnetic ordering which has been realized in several strongly-correlated uranium based compounds. In these compounds, both superconductivity and magnetic ordering originate from U 5f states. To understand the origin of the coexistence as well as the mechanism of the superconductivity, it is essential to reveal their U 5f electronic structures. In this presentation, the U 5f electronic structures of heavy Fermion superconductors UPdAl and URuSi studied by photoelectron spectroscopy using soft X-rays from SPring-8 BL23SU are presented. For UPdAl, U 4d-5f resonant photoemission experiment was performed, and its partial U 5f spectrum was revealed experimentally. Furthermore, we have applied the three-dimentional ARPES to the hidden order compound URuSi, and revealed its complete 3D electronic structure in the paramagnetic phase. Their electronic structures are discussed based on these results.
中村 翔太*; 榊原 俊郎*; 清水 悠晴*; 橘高 俊一郎*; 河野 洋平*; 芳賀 芳範; Pospisil, J.; 山本 悦嗣
Progress in Nuclear Science and Technology (Internet), 5, p.123 - 127, 2018/11
Dc magnetization measurements have been performed on the orthorhombic Ising ferromagnet Urge. We observed a clear first-order reorientation transition with a small hysteresis and estimated the tricritical point to be around 4 K. The magnetization and the thermal expansion data indicate the presence of a characteristic temperature of about 1 K.
B小山田 明*; 猪原 崇生*; 山本 悦嗣; 芳賀 芳範
Progress in Nuclear Science and Technology (Internet), 5, p.128 - 131, 2018/11
We report the Hall effect measurements on a triangular-lattice antiferromagnet UNiB in the context of the proposed relevance of the ferroic order. Our measurements show that the Hall voltage is proportional to the square of the electric current and its coefficient increases significantly below the transition temperature, which supports the theoretical prediction.
竹田 幸治; 岡根 哲夫; 斎藤 祐児; 山上 浩志; 山本 悦嗣; 芳賀 芳範
Progress in Nuclear Science and Technology (Internet), 5, p.171 - 174, 2018/11
In order to investigate the electronic and magnetic states of UGe element-specifically, we have performed soft X-ray magnetic circular dichroism experiments at the U N
and Ge L
absorption edges. We have detected the XMCD signals at both the U and Ge sites and observed clear hysteresis loops in the ferromagnetic (FM) state at T = 5.5 K. From the branching ratio B, it is found that the occupation number of 5f electrons (n
) in UGe is close to 3. In addition, applying the magneto-optical sum rules analysis to the XMCD spectrum at the U N edges, the ratio of orbital magnetic moment to the spin magnetic moment (-M
/M
) is estimated to be 2.17. These values of B and -M/M are comparable compared with the results of other FM superconductors: URhGe and UCoGe
axisPospil, J.*; 芳賀 芳範; 小濱 芳允*; 三宅 厚志*; 神戸 振作; 立岩 尚之; Valika, M.*; Proschek, P.*; Prokleka, J.*; Sechovsk
, V.*; et al.
Physical Review B, 98(1), p.014430_1 - 014430_7, 2018/07
被引用回数：1 パーセンタイル：55.95(Materials Science, Multidisciplinary)The metamagnetic transition between the antiferromagnetic and paramagnetic state in UIrGe has been studied at various temperatures by magnetization, heat capacity, and magnetocaloric effect measurements on a single crystal in static and pulsed magnetic fields applied along the orthorhombic axis. The first-order transition is accompanied by a dramatic increase of the Sommerfeld coefficient. A tentative scenario explaining these anomalies by antiferromagnetic correlations or short-range order in the paramagnetic state is discussed.
竹田 幸治; 斎藤 祐児; 岡根 哲夫; 山上 浩志; 松田 達磨*; 山本 悦嗣; 芳賀 芳範; 大貫 惇睦*
Physical Review B, 97(18), p.184414_1 - 184414_7, 2018/05
パーセンタイル：100(Materials Science, Multidisciplinary)We have performed soft X-ray magnetic circular dichroism (XMCD) experiments on the itinerant-electron metamagnet UCoAl at the U 4-5 (
) and Co 2
-3 (
) absorption edges in order to investigate the magnetic properties of the U 5 and Co 3 electrons separately. From the line shape of the XMCD spectrum, it is deduced that the orbital magnetic moment of the Co 3 electrons is unusually large. Through the systematic temperature (
)- and magnetic field (
)-dependent XMCD measurements, we have obtained two types of the magnetization curve as a function of and (M-H curve and M-T curve, respectively). The metamagnetic transition from a paramagnetic state to a field-induced ferromagnetic state was observed clearly under 15 K at 
. The value of the and its -dependence agree well between the U and Co sites, and the bulk magnetization. Whereas, we have discovered the remarkable differences in the M-H and M-T curves between the U and Co sites. The present findings show clearly that the role of the Co 3 electrons should be considered more carefully in order to understand the origin of the magnetic ordering in UCoAl.
; 
Ge-NQR study at ambient pressure野間 雄一郎*; 小手川 恒*; 久保 徹郎*; 藤 秀樹*; 播磨 尚朝*; 芳賀 芳範; 山本 悦嗣; 大貫 惇睦*; 伊藤 公平*; Haller, E. E.*; et al.
Journal of the Physical Society of Japan, 87(3), p.033704_1 - 033704_5, 2018/03
被引用回数：1 パーセンタイル：47.22(Physics, Multidisciplinary)Ge nuclear quadrupole resonance study of ferromagnetic superconductor UGe is reported. Detailed analyses successfully assigned crystallographic sites of Ge atoms. The measurement of the nuclear spin-lattice relaxation rate revealed highly anisotropic magnetic fluctuations.
松本 裕司*; 芳賀 芳範; 立岩 尚之; 山本 悦嗣; Fisk, Z.*
Journal of the Physical Society of Japan, 87(2), p.024706_1 - 024706_4, 2018/02
パーセンタイル：100(Physics, Multidisciplinary)Single crystal samples of UPtIn with the hexagonal structure are grown from indium flux. Strong uniaxial magnetic anisotropy is revealed from magnetic property measurements. Specific heat measurement reveals a significant deviation from -linear behavior, indicating the smaller electronic specific heat than the previous study.
立岩 尚之; Pospisil, J.*; 芳賀 芳範; 山本 悦嗣
Physical Review B, 97(6), p.064423_1 - 064423_10, 2018/02
被引用回数：1 パーセンタイル：55.95(Materials Science, Multidisciplinary)強磁性体URhAlの磁気臨界現象を研究した。自発磁化の臨界指数、磁化率の指数、強磁性転移温度における磁化の臨界指数を求めた。それぞれ=0.2870.005, =1.470.02, =6.080.04と決定された。これらの臨界指数はWidomのスケーリング則(
)を満たしている。得られた結果は、二次元イジングモデルについての繰り込み群を用いた理論モデルで説明される。
Al; New polymorphic phase in Al-Pd-Sc systemPospisil, J.; 芳賀 芳範; 中島 邦久; 石川 法人; Csa
ov
, I.*; 立岩 尚之; 山本 悦嗣; 山村 朝雄*
Solid State Communications, 268, p.12 - 14, 2017/12
パーセンタイル：100(Physics, Condensed Matter)A new compound of the composition ScPdAl showing polymorphism has been discovered. At room temperature, it crystalizes in the orthorhombic structure, but it transforms into a cubic phase above 1053
C. ScPdAl exists as a very stable intermetallic phase just in the vicinity of the icosahedral quasicrystal Al
Pd
Sc
.
Si studied by angle-resolved photoelectron spectroscopy; Elucidating the contribution of U 5 states in URuSi藤森 伸一; 小畠 雅明; 竹田 幸治; 岡根 哲夫; 斎藤 祐児; 藤森 淳; 山上 浩志; 松本 裕司*; 山本 悦嗣; 立岩 尚之; et al.
Physical Review B, 96(12), p.125117_1 - 125117_9, 2017/09
被引用回数：1 パーセンタイル：80.59(Materials Science, Multidisciplinary)The Fermi surface and band structure of 
have been studied by angle resolved photoelectron spectroscopy (ARPES) with the incident photon energies of 
= 665-735 eV. Detailed band structure and the three-dimensional shape of the Fermi surface were derived experimentally, and they are quantitatively explained by the band-structure calculation based on the density functional approximation. Comparison of the experimental ARPES spectra of with those of 
shows that they have considerably different spectral profiles particularly in the energy range of 
- 1 eV. Some energy bands with their energy dispersions of about 1 eV observed in are missing in the ARPES spectra of measured along the same high symmetry line of Brillouin zone, suggesting that U 5 states form these bands in . The relationship between the ARPES spectra of and is very different from the case between 
and 
where their intrinsic difference is limited only in the very vicinity of the Fermi energy. The present result argues that the U 5 electrons in have strong hybridization with ligand states, and essentially have an itinerant character.
(
=Al, Ga, and In) studied by photoelectron spectroscopy藤森 伸一; 小畠 雅明; 竹田 幸治; 岡根 哲夫; 斎藤 祐児; 藤森 淳; 山上 浩志; 芳賀 芳範; 山本 悦嗣; 大貫 惇睦*
Physical Review B, 96(11), p.115126_1 - 115126_10, 2017/09
被引用回数：2 パーセンタイル：64.92(Materials Science, Multidisciplinary)The electronic structures of U (=Al, Ga, and In) were studied by photoelectron spectroscopy to understand the the relationship between their electronic structure and magnetic properties. The band structures and Fermi surfaces of UAl and UGa were revealed experimentally by angle-resolved photoelectron spectroscopy (ARPES), and they were compared with the result of band structure calculations. The topologies of the Fermi surfaces and the band structures of UAl and UGa were explained reasonably well by the calculation, although bands near the Fermi level (
) were renormalized owing to the finite electron correlation effect. The topologies of the Fermi surfaces of UAl and UGa are very similar to each other, except for some minor differences. Such minor differences in their Fermi surface or electron correlation effect might take an essential role in their magnetism.
-electron systems; Phenomenological analysis with spin fluctuation theory立岩 尚之; Pospil, J.*; 芳賀 芳範; 酒井 宏典; 松田 達磨*; 山本 悦嗣
Physical Review B, 96(3), p.035125_1 - 035125_15, 2017/07
被引用回数：7 パーセンタイル：24.2(Materials Science, Multidisciplinary)我々は69個のウラン強磁性物質、7個のネプツニウム強磁性物質、4個のプルトニウム強磁性物質について、Takahashiらによって提案されたスピンのゆらぎ理論(Y. Takahashi, J. Phys. Soc. Jpn. 
, 3553 (1986))を用いた解析を行った。基本的な磁気的パラメーターと、スピンのゆらぎパラメータを決定し、アクチノイド電子系に対するスピンのゆらぎ理論の適用を考察した。
電子系の遍歴強磁性物質は一般化されたRhodes-Wohlfarthの関係式(
)を満たす。ここで
は自発磁化、
は有効磁気モーメント、は強磁性転移温度である。はスピンのゆらぎスペクトルのエネルギー空間における分布幅である。同じ関係式が、アクチノイド電子系でも基本的に成立することが明らかにされた。
芳賀 芳範; 松本 裕司*; Pospisil, J.; 立岩 尚之; 山本 悦嗣; 山村 朝雄*; Fisk, Z.*
Journal of Physics; Conference Series, 807(1), p.012015_1 - 012015_4, 2017/04
Transport characteristics of an antiferromagnetic uranium compound URhIn are studied. The antiferromagnetic transition leads to a formation of a gap on the Fermi surface as demonstrated by a hump in the resistivity behavior as a function of temperature. Hall effect, magnetoresistance and de Haas-van Alphen study consistently demonstrate a small carrier concentration in the antiferromagnetic state suggesting that majority of the Fermi surface vanishes.
