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JAEA Reports

Decommissioning report for Wastewater Treatment Facility (Part 2); Chapter on contamination inspection section

Yamamoto, Keisuke; Nakagawa, Takuya; Shimojo, Hiroto; Kijima, Jun; Miura, Daiya; Onose, Yoshihiko*; Namba, Koji*; Uchida, Hiroaki*; Sakamoto, Kazuhiko*; Ono, Chika*; et al.

JAEA-Technology 2024-019, 211 Pages, 2025/02

JAEA-Technology-2024-019.pdf:35.35MB

The uranium enrichment facilities at the Nuclear Fuel Cycle Engineering Laboratories of Japan Atomic Energy Agency (JAEA) were constructed sequentially to develop uranium enrichment technology with centrifugal separation method. The developed technologies were transferred to Japan Nuclear Fuel Limited until 2001. And the original purpose has been achieved. Wastewater Treatment Facility, one of the uranium enrichment facilities, was constructed in 1976 to treat radioactive liquid waste generated at the facilities, and it finished the role in 2008. In accordance with the Medium/Long-Term Management Plan of JAEA Facilities, interior equipment installed in this facility had been dismantled and removed since November 2021 to August 2023. This report summarizes the findings obtained through the work related to the contamination inspection methods cancellation the controlled area of Wastewater Treatment Facility from September 2023 to March 2024.

Journal Articles

Tracer diffusion coefficient measurements on NASICON-type Lithium-ion conductor LAGP using neutron radiography between 25$$^{circ}$$C and 500$$^{circ}$$C

Takagi, Honoka*; Yabutsuka, Takeshi*; Hayashida, Hirotoshi*; Song, F.; Kai, Tetsuya; Shinohara, Takenao; Kurita, Keisuke; Iikura, Hiroshi; Yamamoto, Norio*; Nakajima, Minoru*; et al.

Solid State Ionics, 417, p.116716_1 - 116716_7, 2024/12

 Times Cited Count:3 Percentile:43.46(Chemistry, Physical)

Journal Articles

Adsorption isotherm and kinetics of diffusion of water accumulated between polypropylene thin film and Si substrate; Neutron reflectivity investigation

Miyazaki, Tsukasa*; Miyata, Noboru*; Arima-Osonoi, Hiroshi*; Shimokita, Keisuke*; Yamamoto, Katsuhiro*; Takenaka, Mikihito*; Nakanishi, Yohei*; Shibata, Motoki*; Aoki, Hiroyuki; Yamada, Norifumi*; et al.

Colloids and Surfaces A; Physicochemical and Engineering Aspects, 701, p.134928_1 - 134928_8, 2024/11

 Times Cited Count:0 Percentile:11.70(Chemistry, Physical)

Journal Articles

Ca-induced phonon softening in BaTiO$$_{3}$$ revealed by inelastic X-ray and neutron scattering

Kimura, Koji*; Tsutsui, Satoshi*; Yamamoto, Yuta*; Nakano, Akitoshi*; Kawamura, Keisuke*; Kajimoto, Ryoichi; Kamazawa, Kazuya*; Martin, A.*; Webber, K. G.*; Kakimoto, Kenichi*; et al.

Physical Review B, 110(13), p.134314_1 - 134314_10, 2024/10

 Times Cited Count:1 Percentile:37.90(Materials Science, Multidisciplinary)

Journal Articles

Neutron reflectivity study on the adsorption layer of polyethylene grown on Si substrate

Shimokita, Keisuke*; Yamamoto, Katsuhiro*; Miyata, Noboru*; Shibata, Motoki*; Nakanishi, Yohei*; Arakawa, Masato*; Takenaka, Mikihito*; Kida, Takumitsu*; Tokumitsu, Katsuhisa*; Tanaka, Ryo*; et al.

Langmuir, 40(30), p.15758 - 15766, 2024/07

 Times Cited Count:2 Percentile:45.52(Chemistry, Multidisciplinary)

Journal Articles

Latent ion tracks were finally observed in diamond

Amekura, Hiroshi*; Chettah, A.*; Narumi, Kazumasa*; Chiba, Atsuya*; Hirano, Yoshimi*; Yamada, Keisuke*; Yamamoto, Shunya*; Leino, A. A.*; Djurabekova, F.*; Nordlund, K.*; et al.

Nature Communications (Internet), 15, p.1786_1 - 1786_10, 2024/02

 Times Cited Count:2 Percentile:37.90(Multidisciplinary Sciences)

Injecting high-energy heavy ions in the electronic stopping regime into solids can create cylindrical damage zones called latent ion tracks. Although these tracks form in many materials, none have ever been observed in diamond, even when irradiated with high-energy GeV uranium ions. Here we report the first observation of ion track formation in diamond irradiated with 2-9 MeV C$$_{60}$$ fullerene ions. Depending on the ion energy, the mean track length (diameter) changed from 17 (3.2) nm to 52 (7.1) nm. High resolution scanning transmission electron microscopy (HR-STEM) indicated the amorphization in the tracks, in which $$pi$$-bonding signal from graphite was detected by the electron energy loss spectroscopy (EELS).

Journal Articles

Neutron reflectivity study on the nanostructure of PMMA chains near substrate interfaces based on contrast variation accompanied with small molecule sorption

Shimokita, Keisuke*; Yamamoto, Katsuhiro*; Miyata, Noboru*; Nakanishi, Yohei*; Shibata, Motoki*; Takenaka, Mikihito*; Yamada, Norifumi*; Seto, Hideki*; Aoki, Hiroyuki; Miyazaki, Tsukasa*

Soft Matter, 19(11), p.2082 - 2089, 2023/03

 Times Cited Count:5 Percentile:59.91(Chemistry, Physical)

Journal Articles

Neutron reflectivity study on the suppression of interfacial water accumulation between a polypropylene thin film and Si substrate using a silane-coupling agent

Shimokita, Keisuke*; Yamamoto, Katsuhiro*; Miyata, Noboru*; Arima-Osonoi, Hiroshi*; Nakanishi, Yohei*; Takenaka, Mikihito*; Shibata, Motoki*; Yamada, Norifumi*; Seto, Hideki*; Aoki, Hiroyuki; et al.

Langmuir, 38(41), p.12457 - 12465, 2022/10

 Times Cited Count:3 Percentile:17.20(Chemistry, Multidisciplinary)

Journal Articles

Investigation of physical properties of glove for glove-box and estimation of its life-time

Kobayashi, Daisuke; Yamamoto, Masahiko; Nishida, Naoki; Miyoshi, Ryuta; Nemoto, Ryo*; Hayashi, Hiroyuki*; Kato, Keisuke; Nishino, Saki; Kuno, Takehiko; Kitao, Takahiko; et al.

Nihon Hozen Gakkai Dai-18-Kai Gakujutsu Koenkai Yoshishu, p.237 - 240, 2022/07

All gloves attached to glove-box in Tokai Reprocessing Plant have a fixed expiration date and have to be replaced every 4-year. However, degrees of glove deterioration are different depending on its usage environment (frequency, chemicals, radiation, etc.), because of rubber products. Therefore, physical properties such as tensile strength, elongation, hardness of gloves are measured, and the life-time of gloves are estimated. As a result, gloves without any defects in its appearance have enough physical property for acceptance criteria of new glove. The extrapolated physical property of glove is sufficiently larger than the reported values of damaged glove. No deterioration in physical properties of gloves, that are periodically replaced without any defects in its appearance, is observed and the usable life-time of the glove is estimated to be 8 years.

Journal Articles

Sodium-cooled Fast Reactors

Ohshima, Hiroyuki; Morishita, Masaki*; Aizawa, Kosuke; Ando, Masanori; Ashida, Takashi; Chikazawa, Yoshitaka; Doda, Norihiro; Enuma, Yasuhiro; Ezure, Toshiki; Fukano, Yoshitaka; et al.

Sodium-cooled Fast Reactors; JSME Series in Thermal and Nuclear Power Generation, Vol.3, 631 Pages, 2022/07

This book is a collection of the past experience of design, construction, and operation of two reactors, the latest knowledge and technology for SFR designs, and the future prospects of SFR development in Japan. It is intended to provide the perspective and the relevant knowledge to enable readers to become more familiar with SFR technology.

Journal Articles

An Automotive intelligent catalyst that contributes to hydrogen safety for the Decommissioning of Fukushima Daiichi Nuclear Power Station (1FD)

Tanaka, Hirohisa*; Masaki, Sayaka*; Aotani, Takuro*; Inagawa, Kohei*; Iwata, Sogo*; Aida, Tatsuya*; Yamamoto, Tadasuke*; Kita, Tomoaki*; Ono, Hitomi*; Takenaka, Keisuke*; et al.

SAE Technical Paper 2022-01-0534 (Internet), 10 Pages, 2022/03

Journal Articles

Measurements of intensity of produced light in water during irradiations of electron beams with energies above and below the Cerenkov-light threshold

Yamamoto, Seiichi*; Nagao, Yuto*; Kurita, Keisuke; Yamaguchi, Mitsutaka*; Kawachi, Naoki*

Journal of Instrumentation (Internet), 16(1), p.P01007_1 - P01007_9, 2021/01

 Times Cited Count:0 Percentile:0.00(Instruments & Instrumentation)

Luminescence of water during irradiation with particles having energies below the Cerenkov-light threshold was recently found for various types of radiations. However, the relation between the intensities of Cerenkov light and of the luminescence of water at the beam energy below the Cherenkov threshold is not well known. To clarify this point, we measured the produced light irradiating a water sample with electron beams having maximum energies above and below the Cerenkov-light threshold.

Journal Articles

Ion tracks in silicon formed by much lower energy deposition than the track formation threshold

Amekura, Hiroshi*; Toulemonde, M.*; Narumi, Kazumasa*; Li, R.*; Chiba, Atsuya*; Hirano, Yoshimi*; Yamada, Keisuke*; Yamamoto, Shunya*; Ishikawa, Norito; Okubo, Nariaki; et al.

Scientific Reports (Internet), 11(1), p.185_1 - 185_11, 2021/01

 Times Cited Count:15 Percentile:66.13(Multidisciplinary Sciences)

We report the track formation of 10 nm in diameter in silicon irradiated with 6 MeV C$$_{60}$$, i.e., much lower energy than the previously reported energy threshold.

Journal Articles

Neutron reflectivity on the mobile surface and immobile interfacial layers in the poly(vinyl acetate) adsorption layer on a Si substrate with deuterated toluene vapor-induced swelling

Miyazaki, Tsukasa*; Shimokita, Keisuke*; Yamamoto, Katsuhiro*; Aoki, Hiroyuki; Yamada, Norifumi*; Miyata, Noboru*

Langmuir, 36(49), p.15181 - 15188, 2020/12

 Times Cited Count:11 Percentile:39.56(Chemistry, Multidisciplinary)

Journal Articles

Magnetic and electronic properties of B-site-ordered double-perovskite oxide La$$_{2}$$CrMnO$$_{6}$$ thin films

Yoshimatsu, Kohei*; Ishimaru, Junya*; Watarai, Keisuke*; Yamamoto, Kohei*; Hirata, Yasuyuki*; Wadachi, Hiroki*; Takeda, Yukiharu; Horiba, Koji*; Kumigashira, Hiroshi*; Sakata, Osami*; et al.

Physical Review B, 99(23), p.235129_1 - 235129_8, 2019/06

 Times Cited Count:17 Percentile:58.73(Materials Science, Multidisciplinary)

Journal Articles

Defect structure analysis of heterointerface between Pt and CeO$$_{rm x}$$ promoter on Pt electro-catalyst

Fugane, Keisuke*; Mori, Toshiyuki*; Yan, P.*; Masuda, Takuya*; Yamamoto, Shunya; Ye, F.*; Yoshikawa, Hideki*; Auchterlonie, G.*; Drennan, J.*

ACS Applied Materials & Interfaces, 7(4), p.2698 - 2707, 2015/02

 Times Cited Count:31 Percentile:63.98(Nanoscience & Nanotechnology)

no abstracts in English

Journal Articles

Sensitivity analyses of initial compositions and cross sections for activation products of in-core structure materials

Yamamoto, Kento; Okumura, Keisuke; Kojima, Kensuke; Okamoto, Tsutomu

Nuclear Back-end and Transmutation Technology for Waste Disposal, p.233 - 249, 2015/00

To improve the prediction accuracy of concentrations of activation products (APs) in the field of nuclear back-end, it is important to investigate the elements and the nuclear reactions leading to generation of APs. To clarify quantitatively the source elements and the nuclear reactions dominating generation of APs, sensitivity analyses of initial compositions and cross sections were conducted using ORIGEN2.2 code and ORLIBJ40, which is a set of the 1-group cross section libraries based on JENDL-4.0. Activations of cladding tubes, end-plugs and spacers of fuel assemblies and channel boxes in BWR, whose materials are zirconium alloy, stainless steel, and nickel-chromium-based alloy, were analyzed. The results clarified quantitatively the source elements and the nuclear reactions dominating generation of APs. It was remarkable that the dominant generation pathways were clarified even for the nuclides generated through complicated pathways. In conclusion, the results of sensitivity analyses could be utilized to select the objective of elements for measurements of impurities in the materials and of nuclear data for improvement of accuracy.

Journal Articles

Accurate structure analyses of polymer crystals on the basis of wide-angle X-ray and neutron diffractions

Tashiro, Koji*; Hanesaka, Makoto*; Yamamoto, Hiroko*; Wasanasuk, K.*; Jayaratri, P.*; Yoshizawa, Yoshinori*; Tanaka, Ichiro*; Niimura, Nobuo*; Kusaka, Katsuhiro*; Hosoya, Takaaki*; et al.

Kobunshi Rombunshu, 71(11), p.508 - 526, 2014/11

 Times Cited Count:7 Percentile:23.22(Polymer Science)

The crystal structure analysis of various polymer substances has been reviewed on the basis of wide-angle high-energy X-ray and neutron diffraction data. The progress in structural analytical techniques of polymer crystals have been reviewed at first. The structural models proposed so far were reinvestigated and new models have been proposed for various kinds of polymer crystals including polyethylene, poly(vinyl alcohol), poly(lactic acid) and its stereocomplex etc. The hydrogen atomic positions were also clarified by the quantitative analysis of wide-angle neutron diffraction data, from which the physical properties of polymer crystals have been evaluated theoretically. The bonded electron density distribution has been estimated for a polydiacetylene single crystal on the basis of the so-called X-N method or by the combination of structural information derived from X-ray and neutron diffraction data analysis. Some comments have been added about future developments in the field of structure-property relationship determination.

Journal Articles

Orbital magnetic moment and coercivity of SiO$$_2$$-coated FePt nanoparticles studied by X-ray magnetic circular dichroism

Takahashi, Yukio*; Kadono, Toshiharu*; Yamamoto, Shimpei*; Singh, V. R.*; Verma, V.*; Ishigami, Keisuke*; Shibata, Goro*; Harano, Takayuki*; Takeda, Yukiharu; Okane, Tetsuo; et al.

Physical Review B, 90(2), p.024423_1 - 024423_5, 2014/07

AA2015-0417.pdf:0.45MB

 Times Cited Count:11 Percentile:41.72(Materials Science, Multidisciplinary)

Journal Articles

A Study of the generation of $$^{232}$$U in UO$$_{2}$$ and MOX fuels

Yamamoto, Kento; Okumura, Keisuke

Journal of Nuclear Science and Technology, 51(4), p.568 - 573, 2014/04

 Times Cited Count:3 Percentile:21.44(Nuclear Science & Technology)

To clarify the generation pathway of $$^{232}$$U in burned fuels, which is an important nuclide for dose evaluation at various stages in fuel cycle, concentrations of $$^{232}$$U generated through various pathways were evaluated for UO$$_{2}$$ and MOX fuels at 45 GWd/t using the ORIGEN2.2 code. It was found that the difference of $$^{232}$$U concentrations in UO$$_{2}$$ and MOX fuel are mainly derived from the difference of the initial compositions of $$^{234}$$U, $$^{235}$$U and $$^{236}$$U and the contribution of plutonium and americium isotopes in MOX fuels is not so large compared with that of uranium isotopes. The results clarified that the capture cross sections of $$^{230}$$Th, $$^{231}$$Pa, $$^{235}$$U and $$^{236}$$U and ($$n$$,2$$n$$) cross sections of $$^{232}$$Np and $$^{238}$$U have a large effect on generation of $$^{232}$$U. The additional investigation showed that not only time after irradiation but also time before irradiation has a strong effect on $$^{232}$$U concentration.

103 (Records 1-20 displayed on this page)