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Journal Articles

Hydrogen absorption and diffusion behaviors in cube-shaped palladium nanoparticles revealed by ambient-pressure X-ray photoelectron spectroscopy

Tang, J.*; Seo, O.*; Rivera Rocabado, D. S.*; Koitaya, Takanori*; Yamamoto, Susumu*; Namba, Yusuke*; Song, C.*; Kim, J.*; Yoshigoe, Akitaka; Koyama, Michihisa*; et al.

Applied Surface Science, 587, p.152797_1 - 152797_8, 2022/06

The hydrogen absorption and diffusion mechanisms on cube-shaped Pd nanoparticles (NPs) which are important hydrogen-storage materials were studied using X-ray photoelectron spectroscopy and DFT calculations. In the surface region, hydrogen absorption showed almost similar behavior regardless of the NPs size. It was found that the octahedral sites are more favorable than the tetrahedral sites for hydrogen occupation. We also clarified that the hydrogen atoms absorbing on the smaller-sized Pd NPs diffuse to the subsurface more actively because of the weakened Pd-H bond by the surface disordering, which plays an important role in hydrogen adsorption at a low H$$_{2}$$ pressure.

Journal Articles

Effect of uranium deficiency on normal and superconducting properties in unconventional superconductor UTe$$_2$$

Haga, Yoshinori; Opletal, P.; Tokiwa, Yoshifumi; Yamamoto, Etsuji; Tokunaga, Yo; Kambe, Shinsaku; Sakai, Hironori

Journal of Physics; Condensed Matter, 34(17), p.175601_1 - 175601_7, 2022/04

Journal Articles

Electronic structure of ThPd$$_2$$Al$$_3$$; Impact of the U $$5f$$ states on the electronic structure of UPd$$_2$$Al$$_3$$

Fujimori, Shinichi; Takeda, Yukiharu; Yamagami, Hiroshi; Posp$'i$$v{s}$il, J.*; Yamamoto, Etsuji; Haga, Yoshinori

Physical Review B, 105(11), p.115128_1 - 115128_6, 2022/03

Journal Articles

Design and actual performance of J-PARC 3 GeV rapid cycling synchrotron for high-intensity operation

Yamamoto, Kazami; Kinsho, Michikazu; Hayashi, Naoki; Saha, P. K.; Tamura, Fumihiko; Yamamoto, Masanobu; Tani, Norio; Takayanagi, Tomohiro; Kamiya, Junichiro; Shobuda, Yoshihiro; et al.

Journal of Nuclear Science and Technology, 32 Pages, 2022/02

In the Japan Proton Accelerator Research Complex, the purpose of the 3 GeV rapid cycling synchrotron (RCS) is to accelerate a 1 MW, high-intensity proton beam. To achieve beam operation at a repetition rate of 25 Hz at high intensities, the RCS was elaborately designed. After starting the RCS operation, we carefully verified the validity of its design and made certain improvements to establish a reliable operation at higher power as possible. Consequently, we demonstrated beam operation at a high power, namely, 1 MW. We then summarized the design, actual performance, and improvements of the RCS to achieve a 1 MW beam.

Journal Articles

Comparison of sodium fast reactor core assembly seismic evaluation using the Japanese and French simulation tools

Yamamoto, Tomohiko; Matsubara, Shinichiro*; Harada, Hidenori*; Saunier, P.*; Martin, L.*; Gentet, D.*; Dirat, J.-F.*; Collignon, C.*

Nuclear Engineering and Design, 383, p.111406_1 - 111406_14, 2021/11

 Times Cited Count:0

Japan-France collaboration on ASTRID (Advanced Sodium Technological Reactor for Industrial Demonstration) project is launched in 2014. In this project, Japan-France evaluates core assemblies with interferences on seismic event. The object of this study is to verify the seismic evaluation method on core assemblies between Japan and France by comparing the results. The analysis of this benchmark calculation shows a satisfactory agreement between the Japanese and French tools and the figures show a good behavior of the core in horizontal direction under French seismic condition.

Journal Articles

Anisotropic physical properties of layered antiferromagnet U$$_2$$Pt$$_6$$Ga$$_{15}$$

Matsumoto, Yuji*; Haga, Yoshinori; Yamamoto, Etsuji; Takeuchi, Tetsuya*; Miyake, Atsushi*; Tokunaga, Masashi*

Journal of the Physical Society of Japan, 90(7), p.074707_1 - 074707_6, 2021/07

 Times Cited Count:0 Percentile:0(Physics, Multidisciplinary)

Journal Articles

Observation of longitudinal magnetic fluctuations at a first-order ferromagnetic quantum phase transition in UGe$$_2$$

Noma, Yuichiro*; Kotegawa, Hisashi*; Kubo, Tetsuro*; To, Hideki*; Harima, Hisatomo*; Haga, Yoshinori; Yamamoto, Etsuji; Onuki, Yoshichika*; Ito, Kohei*; Nakamura, Ai*; et al.

Journal of the Physical Society of Japan, 90(7), p.073707_1 - 073707_5, 2021/07

 Times Cited Count:0 Percentile:0(Physics, Multidisciplinary)

Journal Articles

Evaluation of Tsunami debris impact on Tokai Reprocessing Plant

Nishino, Saki; Tsuboi, Masatoshi; Okada, Jumpei; Saegusa, Yu; Omori, Kazuki; Yasuo, Kiyoshi; Seshimo, Kazuyoshi; Domura, Kazuyuki; Yamamoto, Masahiko

Nihon Hozen Gakkai Dai-17-Kai Gakujutsu Koenkai Yoshishu, p.541 - 548, 2021/07

no abstracts in English

Journal Articles

Study on the predictive evaluation method for loads acting on roof and sidewall of cylindrical tank in nonlinear sloshing based on simplified equations

Ikesue, Shunichi*; Morita, Hideyuki*; Ishii, Hidekazu*; Sago, Hiromi*; Yokoi, Shinobu*; Yamamoto, Tomohiko

Proceedings of ASME 2021 Pressure Vessels and Piping Conference (PVP 2021) (Internet), 8 Pages, 2021/07

In this paper, a new method is proposed for the nonlinear sloshing condition of a cylindrical tank, which can evaluate the vertical load acting on the roof and the horizontal load acting on the sidewall. This method is a combination of simplified equations for the liquid surface level and velocity proposed in the past study and the new pressure model modified from the existing model. A long calculation time as CFD analysis is not needed, because this method is consisted of simplified equations. The validity of this method was confirmed by comparing them with the CFD and the test. And future issues on the improvement of this method were clarified from the result.

Journal Articles

Electronic structure of URu$$_2$$Si$$_2$$ in paramagnetic phase; Three-dimensional angle resolved photoelectron spectroscopy study

Fujimori, Shinichi; Takeda, Yukiharu; Yamagami, Hiroshi; Yamamoto, Etsuji; Haga, Yoshinori

Electronic Structure (Internet), 3(2), p.024008_1 - 024008_8, 2021/06

JAEA Reports

Development of fireproof sheet on glove box panels

Kawasaki, Kohei; Shinada, Kenta; Okamoto, Naritoshi; Kageyama, Tomio; Eda, Takashi; Okazaki, Hiro; Suzuki, Hiromichi; Yamamoto, Kazuya; Otabe, Jun

JAEA-Technology 2020-025, 80 Pages, 2021/03


Plutonium Fuel Production Facility was built in 1988 for the purpose of mainly producing MOX fuel of the prototype fast breeder reactor MONJU, and large glove boxes were installed for handling unsealed nuclear fuel material remotely. The panels of these glove boxes are made of acrylic, except for those installed after December 2013. For fires inside the glove box, automatic fire extinguishing systems using halides have been introduced since the beginning of construction, but for fires outside the glove box, there have been issues with direct measures for acrylic. Therefore, we have developed a fireproof sheet that mitigates the effect of fire outside the glove box on the panels as much as possible. As a result, fire-retardant sheets have been selected and attached to the glove box panels. We conducted a flammability test of the acrylic plate attached with these fireproof sheets and a usage environment influence test of fireproof sheets, and obtained good results. In addition, we set up a working group in the Plutonium Fuel Development Center in view of reducing external exposure during the work of attaching fireproof sheets, in which we discussed and examined the work procedure, and summarized it in the basic procedure manual.

Journal Articles

Development of ${it spatiotemporal}$ measurement and analysis techniques in X-ray photoelectron spectroscopy; From NAP-HARPES to 4D-XPS

Toyoda, Satoshi*; Yamamoto, Tomoki*; Yoshimura, Masashi*; Sumida, Hirosuke*; Mineoi, Susumu*; Machida, Masatake*; Yoshigoe, Akitaka; Suzuki, Satoru*; Yokoyama, Kazushi*; Ohashi, Yuji*; et al.

Vacuum and Surface Science, 64(2), p.86 - 91, 2021/02

We have developed ${it spatiotemporal}$ measurement and analysis techniques in X-ray photoelectron spectroscopy. To begin with, time-division depth profiles of gate stacked film interfaces have been achieved by NAP-HARPES (Near Ambient Pressure Hard X-ray Angle-Resolved Photo Emission Spectroscopy) data. We then have promoted our methods to quickly perform peak fittings and depth profiling from time-division ARPES data, which enables us to realize 4D-XPS analysis. It is found that the traditional maximum entropy method (MEM) combined with Jackknife averaging of sparse modeling in NAP-HARPES data is effective to perform dynamic measurement of depth profiles with high precision.

Journal Articles

Internal event level-1 PRA for sodium-cooled fast reactor considering safety measures of defense-in-depth level 1 to 3

Nishino, Hiroyuki; Kurisaka, Kenichi; Naruto, Kenichi*; Gondai, Yoji; Yamamoto, Masaya; Yamano, Hidemasa

Proceedings of Asian Symposium on Risk Assessment and Management 2020 (ASRAM 2020) (Internet), 12 Pages, 2020/11

The objective of this study is to evaluate the occurrence frequency of accident sequences which may lead to core damage if provisions in defense in depth (DiD) level 1 to 3 are the only safety measures. For this objective, the existing safety measures in this SFR are categorized into those for the DiD level 1-3 and those for the DiD level 4. The safety measures for the DiD level 1-3 are as follows; (1) main reactor shutdown system, (2) double boundary structure in the primary main and auxiliary cooling system and the reactor vessel, which maintain the reactor coolant level sufficient for coolant circulation in the primary main cooling system, (3) decay heat removal in a forced circulation mode. Accident sequences are categorized into typical SFR-specific groups and station blackout (SBO) in this study. The SFR-specific groups are unprotected loss of flow, unprotected transient over power, unprotected loss of heat sink, loss of reactor level, and protected loss of heat sink (PLOHS). The occurrence frequency of these accident sequence groups was quantified to identify major contributors. As the result, PLOHS excluding SBO was indicated as the dominant contribution of 80% or more in the all accident sequence groups and the annual occurrence frequency of the PLOHS was 1.0E-4 order of magnitude. For the PLOHS, loss of offsite power (LOOP) was indicated as major contribution of 30% in initiating events. In the accident sequences of the PLOHS initiated from LOOP, a dominant sequence was combination of common cause failure of primary pumps in the main cooling system and failure-to-start of the auxiliary cooling system after LOOP. The second dominant contribution (15% or more) in the all accident sequence groups is PLOHS in SBO (i.e., decay heat removal failure due to SBO). Each of the other accident sequence groups was 1%.

Journal Articles

Development and application of a $$^3$$He neutron spin filter at J-PARC

Okudaira, Takuya; Oku, Takayuki; Ino, Takashi*; Hayashida, Hirotoshi*; Kira, Hiroshi*; Sakai, Kenji; Hiroi, Kosuke; Takahashi, Shingo*; Aizawa, Kazuya; Endo, Hitoshi*; et al.

Nuclear Instruments and Methods in Physics Research A, 977, p.164301_1 - 164301_8, 2020/10

 Times Cited Count:4 Percentile:76.41(Instruments & Instrumentation)

Journal Articles

The $$f$$-electron state of the heavy fermion superconductor NpPd$$_5$$Al$$_2$$ and the isostructural family

Metoki, Naoto; Aczel, A. A.*; Aoki, Dai*; Chi, S.*; Fernandez-Baca, J. A.*; Griveau, J.-C.*; Hagihara, Masato*; Hong, T.*; Haga, Yoshinori; Ikeuchi, Kazuhiko*; et al.

JPS Conference Proceedings (Internet), 30, p.011123_1 - 011123_6, 2020/03

Rare earths (4$$f$$) and actinides (5$$f$$) provide variety of interesting states realized with competing interactions between the increasing number of $$f$$ electrons. Since crystal field splitting of many-body $$f$$ electron system is smaller than the bandwidth, (1) high resolution experiments are needed, (2) essentially no clear spectrum with well defined peaks is expected in itinerant Ce and U compounds, and (3) Np and Pu is strictly regulated. Therefore, systematic research on magnetic excitations by neutron scattering experiments of localized compounds and rare earth iso-structural reference is useful. We describe the $$f$$ electron states of heavy electron compounds NpPd$$_5$$Al$$_2$$ and actinide and rare earth based iso-structural family.

Journal Articles

Structural characterization and magnetic behavior of uranium compound U$$_2$$Pt$$_6$$Al$$_{15}$$

Haga, Yoshinori; Sugai, Takashi*; Matsumoto, Yuji*; Yamamoto, Etsuji

JPS Conference Proceedings (Internet), 29, p.013003_1 - 013003_5, 2020/02

Journal Articles

Development of the neutron polarizer for the T-violation search using compound nuclei

Okudaira, Takuya; Oku, Takayuki; Sakai, Kenji; Ino, Takashi*; Hayashida, Hirotoshi*; Hiroi, Kosuke; Shinohara, Takenao; Kakurai, Kazuhisa*; Aizawa, Kazuya; Shimizu, Hirohiko*; et al.

Proceedings of Science (Internet), 356, 5 Pages, 2019/12

The technology development section carries out the development of the neutron polarization device: $$^{3}$$He Spin Filter. It is often used for the fundamental physics region. In order to explain the matter-dominated universe, a time reversal violation is necessary and searches for new physics are conducted in the world. The T-violation search using a polarized neutron beam is planned at J-PARC. A large $$^{3}$$He spin filter is needed to polarize high energy neutrons for the experiment and is developed in JAEA. Recently, we developed the accurate measurement system to evaluate the polarization of $$^{3}$$He and a vacuum system to make the $$^{3}$$He spin filter, and large $$^{3}$$He spin filters for epi-thermal neutron was made using the system. The current status of the development of the $$^{3}$$He spin filter will be talked.

JAEA Reports

Automation technique of analytical pre-treatment for radioactive sample measurement using the program written by visual basic for applications

Yamamoto, Masahiko; Karo, Yoshinori*; Kodaka, Noriyasu; Kuno, Takehiko

JAEA-Technology 2019-014, 68 Pages, 2019/10


Analytical devices like syringe pump, electric burette, fraction collector, and electric valve have been controlled by the program written with Visual Basic for Applications (VBA Macro) to automate the column separation of radioactive sample measurement. It is found that VBA Macro can control each device. Therefore, automatic conditioning and separation equipment were made by combining each device and sequentially controlling with the program. The automation conditioning equipment can repeatedly perform conditioning operation with maximum of 8 columns. The automation separation equipment can separate and recover Sr in simulated highly active liquid waste by using Eichrom Technologies Sr resin. It is found that the developed automation method, using commercially available VBA Macro, is effective to reduce labor work, operator's radiation exposure, and to prevent operational error of analysis, together with reducing the cost of automation.

Journal Articles

Novel universality class for the ferromagnetic transition in the low carrier concentration systems UTeS and USeS exhibiting large negative magnetoresistance

Tateiwa, Naoyuki; Haga, Yoshinori; Sakai, Hironori; Yamamoto, Etsuji

Physical Review B, 100(6), p.064413_1 - 064413_7, 2019/08

 Times Cited Count:1 Percentile:10.83(Materials Science, Multidisciplinary)

We report the novel critical behavior of magnetization in low carrier concentration systems UTeS and USeS that exhibit the large negative magnetoresistance around the ferromagnetic transition temperatures $$T_{rm C}$$ $$sim$$ 85 and 23 K, respectively. We determine the critical exponents, $$beta$$ for the spontaneous magnetization $$M_{rm s}$$, $$gamma$$ for the magnetic susceptibility $$chi$$, and $$delta$$ for the magnetization isotherm at $$T_{rm C}$$ with several analytical methods. The ferromagnetic states in UTeS and USeS have strong uniaxial magnetic anisotropy. However, the critical exponents in the two compounds are different from those in the three-dimensional Ising system. Similar exponents have been reported for the uranium ferromagnetic superconductors UGe$$_2$$ and URhGe. An important finding is that the novel critical phenomenon appears regardless of the charge carrier density or the degree of the itinerancy of the $$5f$$ electrons.

Journal Articles

Observation of a $$Xi$$ bound state in the $$^{12}$$C$$(K^-, K^+)$$ reaction at 1.8 GeV/$$c$$

Nagae, Tomofumi*; Ekawa, Hiroyuki; Hasegawa, Shoichi; Hayakawa, Shuhei; Hosomi, Kenji; Ichikawa, Yudai; Imai, Kenichi; Kimbara, Shinji; Nanamura, Takuya*; Naruki, Megumi; et al.

AIP Conference Proceedings 2130, p.020015_1 - 020015_9, 2019/07

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