Magnetic and structure transition of MnFeO solid solutions under high-pressure and high-temperature conditions

Yamanaka, Takamitsu*; Hirao, Naohisa*; Nakamoto, Yuki*; Mikouchi, Takashi*; Hattori, Takanori; Komatsu, Kazuki*; Mao, H.-K.*

Physics and Chemistry of Minerals, 49(10), p.41_1 - 41_14, 2022/10

https://doi.org/10.1007/s00269-022-01215-4

Magnetic and crystal structure of MnFeO solid solutions under high-PT conditions are investigated by neutron diffraction and synchrotron Mssbauer spectroscopy. The ferrimagnetic-paramagnetic transition and tetragonal-cubic transition of MnFeO spinel occur at 100C and 180C, respectively, suggesting both the transitions are not coupled. The structure transition temperature decreases with pressure. Mssbauer experiments and neutron diffraction revealed that the Fe occupancy in tetrahedral site increases increase with pressure, suggesting MnFeO phase approaches inverse spinel. Magnetic structure refinement clarified paramagnetic and ferrimagnetic structure of MnFeO and MnFeO. These spinels transform into high-pressure orthorhombic phases at 18.4 and 14.0 GPa, respectively, indicating lower transition pressure with increasing Mn content.

New precise measurements of muonium hyperfine structure at J-PARC MUSE

Strasser, P.*; Abe, Mitsushi*; Aoki, Masaharu*; Choi, S.*; Fukao, Yoshinori*; Higashi, Yoshitaka*; Higuchi, Takashi*; Iinuma, Hiromi*; Ikedo, Yutaka*; Ishida, Katsuhiko*; et al.

EPJ Web of Conferences, 198, p.00003_1 - 00003_8, 2019/01

https://doi.org/10.1051/epjconf/201919800003

Verification of the quantitative method to measure enrichment of uranium-235 in radioactive waste

Yokoyama, Kaoru; Sato, Katsunori*; Yamanaka, Takashi*; Ishimori, Yuu

Radioisotopes, 65(11), p.441 - 450, 2016/11

https://doi.org/10.3769/radioisotopes.65.441

It is important for the processing manufacturers of the uranium fuels to determine the quantity of U-235 and the enrichment. This study shows that the U-235 content evaluated from measurement of 186 keV rays emitted from U-235 can be corrected by a shielding factor, Xgeometry which quantified uneven distribution of U-238. The Xgeometry is evaluated from the direct and the scattered rays from the 1001 keV emitted from the Pa-234m. The Xgeometry was originally introduced for U-238 measurements. Because U-235 coexists with U-238, the Xgeometry is also possible to apply to the U-235 measurements. The experimental study with simulated waste drums demonstrated that the quantification errors of the U-235 content and the enrichment are reduced considering the factor.

Thermophysical properties of americium-containing barium plutonate

Tanaka, Kosuke; Sato, Isamu; Hirosawa, Takashi; Kurosaki, Ken*; Muta, Hiroaki*; Yamanaka, Shinsuke*

Journal of Nuclear Science and Technology, 52(10), p.1285 - 1289, 2015/10

https://doi.org/10.1080/00223131.2015.1029554

Polycrystalline specimens of americium-containing barium plutonate have been prepared by mixing the appropriate amounts of (PuAm)O and BaCO powders followed by reacting and sintering at 1600 K under the flowing gas atmosphere of dry-air. The sintered specimens had a single phase of orthorhombic perovskite structure and were crack-free. The elastic moduli were determined from the longitudinal and shear sound velocities. The Debye temperature was also determined from the sound velocities and lattice parameter measurements. The thermal conductivity was calculated from the measured density at room temperature, literature values of heat capacity, and thermal diffusivity measured by laser flash method in vacuum. The thermal conductivity of americium-containing barium plutonate was roughly independent of the temperature and was almost the same magnitude as that of BaPuO and BaUO.

Long-pulse beam acceleration of MeV-class H ion beams for ITER NB accelerator

Umeda, Naotaka; Kashiwagi, Mieko; Taniguchi, Masaki; Tobari, Hiroyuki; Watanabe, Kazuhiro; Dairaku, Masayuki; Yamanaka, Haruhiko; Inoue, Takashi; Kojima, Atsushi; Hanada, Masaya

Review of Scientific Instruments, 85(2), p.02B304_1 - 02B304_3, 2014/02

https://doi.org/10.1063/1.4825161

In order to realize neutral beam systems in ITER whose target is to produce D ion beam of 1 MeV, 200 A/m during 3600s, the electrostatic five-stages negative ion accelerator has been developed at JAEA. To extend pulse length, heat load of the acceleration grids was reduced by controlling the ion beam trajectory. Namely, the beam deflection due to the residual magnetic filter in the accelerator was suppressed with the newly developed extractor with a 0.5 mm off-set aperture displacement. The use of new extractor improved the deflection angle from 6 mrad to 1 mrad, resulting in the reduction of direct interception of negative ions from 23% to 15% of the total acceleration power, respectively. As a result, the pulse length of 130 A/m, 881 keV H ion beam has been successfully extended from a previous value of 0.4s to 8.7s.

Structural analyses of HV bushing for ITER heating NB system

Tobari, Hiroyuki; Inoue, Takashi; Taniguchi, Masaki; Kashiwagi, Mieko; Umeda, Naotaka; Dairaku, Masayuki; Yamanaka, Haruhiko; Watanabe, Kazuhiro; Sakamoto, Keishi; Kuriyama, Masaaki*; et al.

Fusion Engineering and Design, 88(6-8), p.975 - 979, 2013/10

https://doi.org/10.1016/j.fusengdes.2013.02.020

The HV bushing, one of the ITER NB components, which is to be procured by JADA, is a multi-conductor feed through composed of five-stage double-layered insulator columns with large brazed ceramic ring and fiber reinforced plastic (FRP) ring. The HV bushing is a bulk head between insulation gas at 0.6 MPa and vacuum. The FRP ring is required to sustain the pressure load, seismic load and dead weight. Brazing area of the ceramic ring with Kovar is required to maintain vacuum leak tightness and pressure tightness against the air filled at 0.6 MPa. To design the HV bushing satisfying the safety factor of 3.5, mechanical analyses were carried out. As for the FRP ring, it was confirmed that isotropic fiber cloth FRP rings should be used for sufficient strength against shear stress. Also, shape and fixation area of the Kovar sleeve were modified to lower the stress at the joint area. As a result, a design of the insulator for the HV bushing was established satisfying the requirement.

Vacuum insulation and achievement of 980 keV, 185 A/m H ion beam acceleration at JAEA for the ITER neutral beam injector

Tobari, Hiroyuki; Taniguchi, Masaki; Kashiwagi, Mieko; Dairaku, Masayuki; Umeda, Naotaka; Yamanaka, Haruhiko; Tsuchida, Kazuki; Takemoto, Jumpei; Watanabe, Kazuhiro; Inoue, Takashi; et al.

Plasma Science and Technology, 15(2), p.179 - 183, 2013/02

https://doi.org/10.1088/1009-0630/15/2/21

Vacuum insulation is a common issue for the accelerator and the HV bushing for the ITER NBI. The HV bushing has five-stage structure and each stage consists of double-layered insulators. Hence, several triple points exist around the insulators. To reduce electric field at those points simultaneously, three types of stress ring were developed. In voltage holding test of a full-scale mockup equipped with those stress rings, 120% of rated voltage was sustained and the voltage holding capability required in ITER was verified. In the MeV accelerator, voltage holding capability was not sufficient due to breakdown triggered by electric field concentration at edge and corner on grid components. By extending gap length, 1 MV was sustained in vacuum. Furthermore, with new accelerator grids which compensates beam deflection due to magnetic field and space charge repulsion between beamlets, 980 keV, 185 A/m H ion beam acceleration was demonstrated, which was close to ITER requirement.

Voltage holding study of 1 MeV accelerator for ITER neutral beam injector

Taniguchi, Masaki; Kashiwagi, Mieko; Umeda, Naotaka; Dairaku, Masayuki; Takemoto, Jumpei; Tobari, Hiroyuki; Tsuchida, Kazuki; Yamanaka, Haruhiko; Watanabe, Kazuhiro; Kojima, Atsushi; et al.

Review of Scientific Instruments, 83(2), p.02B121_1 - 02B121_3, 2012/02

https://doi.org/10.1063/1.3675389

JAEA has developed the MeV accelerator to demonstrate 1 MeV, 200 A/m H ion beam acceleration required for ITER NBI. A key to realize such a high power accelerator is improvement of voltage holding capability. Based on detailed investigation of the voltage holding characteristics, MeV accelerator was modified to reduce electric field concentration by extending gaps between the grid supports and increasing curvature radiuses at the support corners. After the modifications, accelerator succeeded in sustaining -1 MV in vacuum without beam acceleration. Moreover, beam deflection due to the magnetic field for electron suppression and space charge repulsion was compensated by aperture displacement technique. As the result, beam deflection was compensated and voltage holding during the beam acceleration was improved. Beam parameter of the MeV accelerator was increased to 980 keV, 185 A/m, which is close to the requirement of ITER accelerator.

Improvement of voltage holding and high current beam acceleration by MeV accelerator for ITER NB

Taniguchi, Masaki; Kashiwagi, Mieko; Inoue, Takashi; Umeda, Naotaka; Watanabe, Kazuhiro; Tobari, Hiroyuki; Dairaku, Masayuki; Yamanaka, Haruhiko; Tsuchida, Kazuki; Kojima, Atsushi; et al.

AIP Conference Proceedings 1390, p.449 - 456, 2011/09

https://doi.org/10.1063/1.3637416

At JAEA, MeV accelerator has been developed as a proof-of-principle accelerator for ITER NBI. To achieve the acceleration of 1 MeV, 200 A/m beam required for ITER, improvement of the voltage holding capability is essential. Review of voltage holding results ever obtained with various geometries of the accelerators showed that voltage holding capability was about a half of that for ideal small electrode. This is due to local electric field concentration in the accelerators, such as edge and corner between grids and its support structures. Based on these results, accelerator was modified to reduce the electric field concentration by reshaping the support structures and expanding the gap length. After the modifications, voltage holding capability in vacuum was increased from 835 kV to 1 MV. Voltage holding progressed the energy and current to 879 keV, 0.36 A (157 A/m).

Development of high voltage power supply system for ITER neutral beam injector

Tsuchida, Kazuki; Watanabe, Kazuhiro; Tobari, Hiroyuki; Takemoto, Jumpei; Yamanaka, Haruhiko; Inoue, Takashi

Denki Gakkai Kenkyukai Shiryo, Genshiryoku Kenkyukai (NE-11-001004 006010), p.17 - 22, 2011/09

A 1 MeV high-energy neutral beam injector is under developing for heating and current drive of ITER plasma in collaboration with EUDA. JADA will provide ultra-high voltage DC power supply components. Design of the 1 MV power supply, R&Ds on a HV bushing and a water choke will be presented. These results satisfy the requirements for the NBI system.