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Tomita, Ryohei; Tomita, Jumpei; Yomogida, Takumi; Suzuki, Daisuke; Yasuda, Kenichiro; Esaka, Fumitaka; Miyamoto, Yutaka
KEK Proceedings 2022-2, p.108 - 113, 2022/11
Automated Particle Measurement (APM) is the first measurement of environmental sample for safeguard purpose. APM tells us the number of particles in sample, their enrichment and their location. Precision and accuracy of APM is easily affected by particle condition. We have investigated how influential baking temperature in sample preparation are for uranium secondary ion quantity, uranium hydride generation and particle crystallinity. Our experimental results showed that baking temperature of 800
C reduced uranium secondary ion quantity to 33% compared with baking at 350C. Uranium hydride generation ratio of the sample baked at 850C was also 4 times higher than the sample baked at 350C. Baking at 850C raised only crystallinity of uranium particles. Baking sample at too high temperature caused less uranium secondary ion generation and much more uranium hydride generation. It made precision and accuracy of APM worse. In our experiment, baking at 350C is suitable for uranium particles in the safeguards sample.
Tomita, Jumpei; Tomita, Ryohei; Suzuki, Daisuke; Yasuda, Kenichiro; Miyamoto, Yutaka
KEK Proceedings 2022-2, p.154 - 158, 2022/11
Precise determination of minor U isotopes (
U and 
U) of particles from the safeguard environmental samples is powerful method for detecting the undeclared nuclear activities. In this study, preparation method of U particle was examined to utilize for the minor U isotope determination. The porous silica particles were used as the particle matrix and lutetium was mixed to the impregnation solution as U impregnation indicator for the particle picking. The result of the Scanning Electron Microscope indicated that the contacting the solution with Si particles overnight gently could produce the impregnated particles effectively rather than the mixing them with PFA stick.
Tomita, Ryohei; Tomita, Jumpei; Yomogida, Takumi; Suzuki, Daisuke; Yasuda, Kenichiro; Esaka, Fumitaka; Miyamoto, Yutaka
KEK Proceedings 2021-2, p.146 - 150, 2021/12
no abstracts in English
Okutsu, Kenichi*; Yamashita, Takuma*; Kino, Yasushi*; Nakashima, Ryota*; Miyashita, Konan*; Yasuda, Kazuhiro*; Okada, Shinji*; Sato, Motoyasu*; Oka, Toshitaka; Kawamura, Naritoshi*; et al.
Fusion Engineering and Design, 170, p.112712_1 - 112712_4, 2021/09
Times Cited Count：1 Percentile：30.57(Nuclear Science & Technology)A muonic molecule which consists of two hydrogen isotope nuclei (deuteron (d) or tritium (t)) and a muon decays immediately via nuclear fusion and the muon will be released as a recycling muon, and start to find another hydrogen isotope nucleus. The reaction cycle continues until the muon ends up its lifetime of 2.2 
s. Since the muon does not participate in the nuclear reaction, the reaction is so called a muon catalyzed fusion (CF). The recycling muon has a particular kinetic energy (KE) of the muon molecular orbital when the nuclear reaction occurs. Since the KE is based on the unified atom limit where distance between two nuclei is zero. A precise few-body calculation estimating KE distribution (KED) is also in progress, which could be compared with the experimental results. In the present work, we observed recycling muons after CF reaction.
Nishimura, Hayato*; Hojo, Tomohiko*; Ajita, Saya*; Shibayama, Yuki*; Koyama, Motomichi*; Saito, Hiroyuki*; Shiro, Ayumi*; Yasuda, Ryo*; Shobu, Takahisa; Akiyama, Eiji*
Tetsu To Hagane, 107(9), p.760 - 768, 2021/09
Times Cited Count：0 Percentile：0(Metallurgy & Metallurgical Engineering)no abstracts in English
Yamashita, Takuma*; Okutsu, Kenichi*; Kino, Yasushi*; Nakashima, Ryota*; Miyashita, Konan*; Yasuda, Kazuhiro*; Okada, Shinji*; Sato, Motoyasu*; Oka, Toshitaka; Kawamura, Naritoshi*; et al.
Fusion Engineering and Design, 169, p.112580_1 - 112580_5, 2021/08
Times Cited Count：2 Percentile：53.86(Nuclear Science & Technology)A muon () having 207 times larger mass of electron and the same charge as the electron has been known to catalyze a nuclear fusion between deuteron (d) and triton (t). These two nuclei are bound by and form a muonic hydrogen molecular ion, dt. Due to the short inter-nuclear distance of dt, the nuclear fusion, d +t
+ n + 17.6 MeV, occurs inside the molecule. This reaction is called muon catalyzed fusion (CF). Recently, the interest on CF is renewed from the viewpoint of applications, such as a source of high-resolution muon beam and mono-energetic neutron beam. In this work, we report a time evolution calculation of CF in a two-layered hydrogen isotope target.
Shibayama, Yuki; Hojo, Tomohiko*; Koyama, Motomichi*; Saito, Hiroyuki*; Shiro, Ayumi*; Yasuda, Ryo*; Shobu, Takahisa; Matsuno, Takashi*; Akiyama, Eiji*
ISIJ International, 61(4), p.1322 - 1329, 2021/04
Times Cited Count：2 Percentile：33.62(Metallurgy & Metallurgical Engineering)Nishimura, Hayato*; Hojo, Tomohiko*; Ajita, Saya*; Shibayama, Yuki*; Koyama, Motomichi*; Saito, Hiroyuki*; Shiro, Ayumi*; Yasuda, Ryo*; Shobu, Takahisa; Akiyama, Eiji*
ISIJ International, 61(4), p.1170 - 1178, 2021/04
Times Cited Count：1 Percentile：17.89(Metallurgy & Metallurgical Engineering)Suzuki, Daisuke; Tomita, Ryohei; Tomita, Jumpei; Esaka, Fumitaka; Yasuda, Kenichiro; Miyamoto, Yutaka
Journal of Radioanalytical and Nuclear Chemistry, 328(1), p.103 - 111, 2021/04
Times Cited Count：2 Percentile：30.57(Chemistry, Analytical)An analytical technique was developed to determine the age of uranium particles for safeguards. After the chemical separation of uranium and thorium, the 
Th/
U ratio was measured using single-collector inductively coupled plasma mass spectrometry and a U-based reference material comprising a certain amount of 
Th as a progeny nuclide of U. The results allowed us to determine the purification age of two certified materials, i.e., U-850 and U-100, which was in good agreement with the reference purification age (61 y). Moreover, the age of a single U-850 particle was determined with a difference of -28 to 2 years from the reference date.
Hojo, Tomohiko*; Akiyama, Eiji*; Saito, Hiroyuki*; Shiro, Ayumi*; Yasuda, Ryo*; Shobu, Takahisa; Kinugasa, Junichiro*; Yuse, Fumio*
Corrosion Science, 177, p.108957_1 - 108957_9, 2020/12
Times Cited Count：14 Percentile：80.72(Materials Science, Multidisciplinary)Hydrogen assisted cracking on hemispherically-stretch-formed specimens of transformation induced plasticity-aided martensitic steel was investigated. Hydrogen charging induced cracking around the foot of the impression formed on the steel sheet, and the cracks propagated along the radial direction toward the hillside and the plains. Distributions of stress, plastic strain and volume fraction of retained austenite were analyzed employing the energy-dispersive X-ray diffraction method utilizing the synchrotron X-ray radiation at SPring-8. It was notable that the crack initiation took place in the region where the measured tensile stress was the highest. Influences of plastic strain and resulted martensitic transformation were also suggested.
Hojo, Tomohiko*; Kumai, B.*; Koyama, Motomichi*; Akiyama, Eiji*; Waki, Hiroyuki*; Saito, Hiroyuki*; Shiro, Ayumi*; Yasuda, Ryo*; Shobu, Takahisa; Nagasawa, Akihiko*
International Journal of Fracture, 224(2), p.253 - 260, 2020/08
Times Cited Count：10 Percentile：68.63(Materials Science, Multidisciplinary)In the study, the pre-strain effect on hydrogen embrittlement property of the ultra-high-strength transformation-induced plasticity -aided bainitic ferrite steel was investigated towards application for automobile frame parts. 3-10% tensile pre-strain suppressed hydrogen-induced mechanical degradation relative to total elongation while 12-15% pre-strained specimen did not exhibit elongation after hydrogen charging. The advantageous effect of the 3-10% pre-strain was attributed to the suppression of crack initiation related to retained austenite. The TRIP by pre-straining decreased the volume fraction of retained austenite before hydrogen charging, thereby reducing existing probabilities of preferential crack initiation sites and propagation paths. Conversely, high pre-strain such as 12-15% does not effectively work due to work hardening resulting in increases in hydrogen embrittlement susceptibility and a significant increase in hydrogen content due to the multiplication of dislocations.
113
deformation twinning in metastable 
-type Ti alloy focusing on stress-induced 
martensite phaseCho, K.*; Morioka, Ryota*; Harjo, S.; Kawasaki, Takuro; Yasuda, Hiroyuki*
Scripta Materialia, 177, p.106 - 111, 2020/03
Times Cited Count：26 Percentile：93.66(Nanoscience & Nanotechnology)Nakazawa, Yuga*; Iinuma, Hiromi*; Iwata, Yoshiyuki*; Iwashita, Yoshihisa*; Otani, Masashi*; Kawamura, Naritoshi*; Mibe, Tsutomu*; Yamazaki, Takayuki*; Yoshida, Mitsuhiro*; Kitamura, Ryo; et al.
Journal of Physics; Conference Series, 1350, p.012054_1 - 012054_7, 2019/12
Times Cited Count：4 Percentile：92.52An inter-digital H-mode drift-tube linac (IH-DTL) is developed in a muon linac at the J-PARC E34 experiment. IH-DTL will accelerate muons from 0.34 MeV to 4.5 MeV at a drive frequency of 324 MHz. Since IH-DTL adopts an APF method, with which the beam is focused in the transverse direction using the rf field only, the proper beam matching of the phase-space distribution is required before the injection into the IH-DTL. Thus, an IH-DTL prototype was fabricated to evaluate the performance of the cavity and beam transmission. As a preparation of the high-power test, tuners and coupler are designed and fabricated. In this paper, the development of the tuner and the coupler and the result of the low-power measurement will be presented.
Otani, Masashi*; Fukao, Yoshinori*; Futatsukawa, Kenta*; Kawamura, Naritoshi*; Matoba, Shiro*; Mibe, Tsutomu*; Miyake, Yasuhiro*; Shimomura, Koichiro*; Yamazaki, Takayuki*; Hasegawa, Kazuo; et al.
Journal of Physics; Conference Series, 1350, p.012067_1 - 012067_6, 2019/12
Times Cited Count：1 Percentile：53.97Negative muonium atom (
e
e, Mu) has unique features stimulating potential interesting for several scientific fields. Since its discovery in late 1980's in vacuum, it has been discussed that the production efficiency would be improved using a low-work function material. C12A7 was a well-known insulator as a constituent of alumina cement, but was recently confirmed to exhibit electric conductivity by electron doping. The C12A7 electride has relatively low-work function (2.9 eV). In this paper, the negative muonium production measurement with several materials including a C12A7 electride film will be presented. Measured production rate of the Mu were 10
/s for all the Al, electride, and SUS target. Significant enhancement on electride target was not observed, thus it is presumed that the surface condition should be more carefully treated. There was no material dependence of the Mu averaged energy: it was 0.2
0.1keV.
Nakazawa, Yuga*; Bae, S.*; Choi, H.*; Choi, S.*; Iijima, Toru*; Iinuma, Hiromi*; Kawamura, Naritoshi*; Kitamura, Ryo; Kim, B.*; Ko, H. S.*; et al.
Nuclear Instruments and Methods in Physics Research A, 937, p.164 - 167, 2019/09
Times Cited Count：2 Percentile：27.72(Instruments & Instrumentation)A muon linac is under development for the precise measurement of the muon anomalous magnetic moment (
-2) and electric dipole moment (EDM) with a reaccelerated thermal muon beam. An H source driven by an ultraviolet light has been developed for the muon acceleration experiment. Prior to the acceleration experiment, a beamline commissioning was performed using this H beam, since the accelerated muon intensity is very low. We successfully measured the magnetic rigidity, which is essential for identifying the accelerated muons. This H source is capable of utilizing as a general-purpose beam source for other beamline.
Wang, H.*; Otsu, Hideaki*; Chiga, Nobuyuki*; Kawase, Shoichiro*; Takeuchi, Satoshi*; Sumikama, Toshiyuki*; Koyama, Shumpei*; Sakurai, Hiroyoshi*; Watanabe, Yukinobu*; Nakayama, Shinsuke; et al.
Communications Physics (Internet), 2(1), p.78_1 - 78_6, 2019/07
Times Cited Count：7 Percentile：59.11(Physics, Multidisciplinary)Searching for effective pathways for the production of proton- and neutron-rich isotopes through an optimal combination of reaction mechanism and energy is one of the main driving forces behind experimental and theoretical nuclear reaction studies as well as for practical applications in nuclear transmutation of radioactive waste. We report on a study on incomplete fusion induced by deuteron, which contains one proton and one neutron with a weak binding energy and is easily broken up. This reaction study was achieved by measuring directly the cross sections for both proton and deuteron for 
Pd at 50 MeV/u via inverse kinematics technique. The results provide direct experimental evidence for the onset of a cross-section enhancement at high energy, indicating the potential of incomplete fusion induced by loosely-bound nuclei for creating proton-rich isotopes and nuclear transmutation of radioactive waste.
Strasser, P.*; Abe, Mitsushi*; Aoki, Masaharu*; Choi, S.*; Fukao, Yoshinori*; Higashi, Yoshitaka*; Higuchi, Takashi*; Iinuma, Hiromi*; Ikedo, Yutaka*; Ishida, Katsuhiko*; et al.
EPJ Web of Conferences, 198, p.00003_1 - 00003_8, 2019/01
Times Cited Count：12 Percentile：99.51Nakazawa, Yuga*; Iinuma, Hiromi*; Iwata, Yoshiyuki*; Iwashita, Yoshihisa*; Otani, Masashi*; Kawamura, Naritoshi*; Mibe, Tsutomu*; Yamazaki, Takayuki*; Yoshida, Mitsuhiro*; Kitamura, Ryo*; et al.
Proceedings of 29th International Linear Accelerator Conference (LINAC 2018) (Internet), p.180 - 183, 2019/01
We have developed an Interdigital H-mode (IH) Drift-Tube Linac (DTL) design with an alternative phase focusing (APF) scheme for a muon linac, in order to measure the anomalous magnetic moment and electric dipole moment (EDM) of muons at the Japan Proton Accelerator Research Complex (J-PARC). The IH-DTL accelerates muons from beta 0.08 to 0.28 at an operational frequency of 324 MHz. The output beam emittances are calculated as 0.315 
and 0.195 mm mrad in the horizontal and vertical directions, respectively, which satisfies the experimental requirement.
superstructure of monolayer MoS
and MoSe on Au(111)Yasuda, Satoshi; Takahashi, Ryosuke*; Osaka, Ryo*; Kumagai, Ryota*; Miyata, Yasumitsu*; Okada, Susumu*; Hayamizu, Yuhei*; Murakoshi, kei*
Small, 13(31), p.1700748_1 - 1700748_8, 2017/08
Times Cited Count：16 Percentile：62.92(Chemistry, Multidisciplinary)MoS and MoSe monolayers are grown on Au surface by chemical vapor deposition and it is demonstrated that the contact with a crystalline Au(111) surface gives rise to only out-of-plane strain in both MoS and MoSe layers, whereas no strain generation is observed on polycrystalline Au or SiO/Si surfaces. Scanning tunneling microscopy analysis provides information regarding consequent specific adsorption sites between lower S (Se) atoms in the S-Mo-S (Se-Mo-Se) structure and Au atoms via unique moir superstructure formation for MoS and MoSe layers on Au(111). This observation indicates that the specific adsorption sites give rise to out-of-plane strain in the TMDC layers. Furthermore, it also leads to effective modulation of the electronic structure of the MoS or MoSe layer.
Sakai, Takuro; Yasuda, Ryo; Iikura, Hiroshi; Matsubayashi, Masahito
JPS Conference Proceedings (Internet), 11, p.020005_1 - 020005_6, 2016/11
