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兼田 加珠子*; 白神 宜史*; 角永 悠一郎*; 渡部 直史*; 大江 一弘*; Yin, X.*; 羽場 宏光*; 白崎 謙次*; 菊永 英寿*; 塚田 和明; et al.
International Journal of Molecular Sciences (Internet), 25(2), p.933_1 - 933_14, 2024/01
被引用回数：1 パーセンタイル：0.01(Biochemistry & Molecular Biology)Currently, targeted alpha therapy (TAT) is a new therapy involving the administration of a therapeutic drug that combines a substance of 
-emitting nuclides that kill cancer cells and a drug that selectively accumulates in cancer cells. We labeled the compounds targeting prostate specific membrane antigen (PSMA) with 
At and 
Ac. PSMA is a molecule that has attracted attention as a theranostic target for prostate cancer, and several targeted radioligands have already shown therapeutic effects in patients. The results showed that At, which has a much shorter half-life, is no less cytotoxic than Ac. In At labeling, our group has also developed an original method (Shirakami Reaction). We have succeeded in obtaining a highly purified labeled product in a short timeframe using this method.
He, H.*; Naeem, M.*; Zhang, F.*; Zhao, Y.*; Harjo, S.; 川崎 卓郎; Wang, B.*; Wu, X.*; Lan, S.*; Wu, Z.*; et al.
Nano Letters, 21(3), p.1419 - 1426, 2021/02
被引用回数：41 パーセンタイル：95.34(Chemistry, Multidisciplinary)In CrCoNi, a so-called medium-entropy alloy, an fcc-to-hcp phase transformation has long been anticipated. Here, we report an in situ loading study with neutron diffraction, which revealed a bulk fcc-to-hcp phase transformation in CrCoNi at 15 K under tensile loading. By correlating deformation characteristics of the fcc phase with the development of the hcp phase, it is shown that the nucleation of the hcp phase was triggered by intrinsic stacking faults. The confirmation of a bulk phase transformation adds to the myriads of deformation mechanisms available in CrCoNi, which together underpin the unusually large ductility at low temperatures.
GeWo, H.*; Wang, Q.*; Shen, Y.*; Zhang, X.*; Hao, Y.*; Feng, Y.*; Shen, S.*; He, Z.*; Pan, B.*; Wang, W.*; et al.
Physical Review Letters, 122(21), p.217003_1 - 217003_5, 2019/05
被引用回数：5 パーセンタイル：42.69(Physics, Multidisciplinary)We report neutron scattering measurements of single-crystalline YFeGe in the normal state, which has the same crystal structure as the 122 family of iron pnictide superconductors. YFeGe does not exhibit long-range magnetic order but exhibits strong spin fluctuations. Like the iron pnictides, YFeGe displays anisotropic stripe-type antiferromagnetic spin fluctuations at (
). More interesting, however, is the observation of strong spin fluctuations at the in-plane ferromagnetic wave vector (
). These ferromagnetic spin fluctuations are isotropic in the (
) plane, whose intensity exceeds that of stripe spin fluctuations. Both the ferromagnetic and stripe spin fluctuations remain gapless down to the lowest measured energies. Our results naturally explain the absence of magnetic order in YFeGe and also imply that the ferromagnetic correlations may be a key ingredient for iron-based materials.
and search for 
at 
= 10.96 - 11.05 GeVYin, J. H.*; 谷田 聖; Belle Collaboration*; 他189名*
Physical Review D, 98(9), p.091102_1 - 091102_9, 2018/11
被引用回数：4 パーセンタイル：23.83(Astronomy & Astrophysics)We report searches for the processes 
and 
(J=1,2) in the vicinity of the 
resonance using energy scan data collected by the Belle experiment at the KEKB collider. We observe 
and find evidence for 
processes for data with center-of-mass energies from 10.96 to 11.05~GeV for the first time. The statistical significance for 
and 
are 
and 
, respectively. We investigate energy dependence of the cross section and find that it is consistent with production of 
and resonances without significant non-resonant contribution. Assuming 
proceeds via and , the branching fraction 
is measured for the first time, where the first error is statistical, the second is systematic, and the third from the branching fraction of 
. The signals for 
are not significant, and the upper limits of the Born cross sections at the 90% confidence level are 
and 
~pb for 
and 
, respectively, for center-of-mass energies from 10.96 to 11.05 GeV.
Yin, H.*; Chung, B.*; Chen, F.*; 大内 隆成*; Zhao, J.*; 田中 伸幸; Sadoway, D. R.*
Nature Energy (Internet), 3(2), p.127 - 131, 2018/02
被引用回数：55 パーセンタイル：87.54(Energy & Fuels)リチウムイオン選択性を有する多孔質伝導膜を用い、正極と負極の電極金属を分離することで、性能劣化が小さく、高い充放電効率が得られるこれまでにない概念の溶融塩蓄電池の開発を行った。多孔質伝導膜にセラミックスの窒化チタン焼結体を、正・負極材に、それぞれ鉛及びリチウム鉛を使用した蓄電池を作製し、作動温度410
Cにおける100サイクル試験を行った。初期の100サイクル平均の性能で、充放電効率が90%以上と優れた性能を達成するとともに、その間の充放電効率の低下速度は1サイクル当たり0.0017%が得られた。これは10年経過後も充放電効率の劣化は10%以下と高寿命であることを示している。また、多孔質状金属(ステンレス及びチタン)に窒化チタンをコーティングした多孔質伝導膜を使用した場合においても、同様の充放電効率を示すことを明らかにした。このように本開発で導入した金属を基盤とする多孔質伝導膜は、低電気抵抗が可能な薄膜化かつ工業的スケールアップに向けた大型化が期待できるものである。
T
As (
= Co,Ni)Tam, D. M.*; Song, Y.*; Man, H.*; Cheung, S. C.*; Yin, Z.*; Lu, X.*; Wang, W.*; Frandsen, B. A.*; Liu, L.*; Gong, Z.*; et al.
Physical Review B, 95(6), p.060505_1 - 060505_6, 2017/02
被引用回数：23 パーセンタイル：71.49(Materials Science, Multidisciplinary)We use neutron diffraction and muon spin relaxation to study the effect of in-plane uniaxial pressure on the antiferromagnetic (AF) orthorhombic phase in BaFeTAs and its Co- and Ni-substituted members near optimal superconductivity. In the low-temperature AF ordered state, uniaxial pressure necessary to detwin the orthorhombic crystals also increases the magnetic ordered moment, reaching an 11% increase under 40 MPa for BaFe
Co
As
, and a 15% increase for BaFe
Ni
As. We also observe an increase of the AF ordering temperature (
) of about 0.25 K/MPa in all compounds, consistent with density functional theory calculations that reveal better Fermi surface nesting for itinerant electrons under uniaxial pressure. The doping dependence of the magnetic ordered moment is captured by combining dynamical mean field theory with density functional theory, suggesting that the pressure-induced moment increase near optimal superconductivity is closely related to quantum fluctuations and the nearby electronic nematic phase.
徐 平光; Yin, J*; Zhang, S. Y.*
Acta Metallurgica Sinica, 51(11), p.1297 - 1305, 2015/11
The tensile deformation behavior of 1250 MPa ultra-high strength steels with and without hydrogen charging was comparably investigated using neutron diffraction together with the fracture morphology and microstructure observation. Before tensile loading, the (110) lattice spacing of hydrogen charged steel was found larger than that of non-charged sample while the (200) lattice spacing of the former was smaller than that of the latter, suggesting that the hydrogen atoms occupied the tetrahedral center promoted the increment of lattice plane spacing of (110) crystal planes while the balanced internal stress resulted in the proper decrement of (200) lattice plane spacing. In the non-charged sample, the non-linear elastic deformation was observed at 700 MPa in (200) planes, and then at 800 MPa in (110) planes. In the hydrogen charged sample, the non-linear elastic deformation was observed at 300 MPa in (110) planes, and then at 400 MPa in (200) planes. The microstructure observation confirmed the cleavage crack propagation and local crystal rotation in the hydrogen charged sample. Here, a concept about crystallographic orientation dependent micro-yielding was proposed, i.e. the hydrogen charging promoted the (110) preferable micro-yielding rather than (200) preferable micro-yielding, and resulted into a special deformation characteristics.
Hu, P.*; 尹 永根; 石川 覚*; 鈴井 伸郎; 河地 有木; 藤巻 秀; 井倉 将人*; Yuan, C.*; Huang, J.*; Li, Z.*; et al.
Environmental Science and Pollution Research, 20(9), p.6306 - 6316, 2013/09
被引用回数：47 パーセンタイル：77.23(Environmental Sciences), a species in the family Crassulaceae, has been reported to be a Cd hyperaccumulator exhibiting fast growth, large biomass, asexual reproduction and perennial habit and showing remarkable potential in the phytoextraction of Cd from polluted soils. The aims of this study are to investigate whether and how the nitrogen form (nitrate (NO
) versus ammonium (NH
)) influences cadmium (Cd) uptake and translocation and subsequent Cd phytoextraction by the 
. This is the first report of successful visualisation and quantification of Cd uptake and root-to-shoot translocation in intact plants of the hyperaccumulator species supplied with different forms of inorganic N using positron-emitting tracer imaging system (PETIS), a real-time imaging method.
