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Journal Articles

Two-dimensional Dresselhaus-type spin texture and nonreciprocal magnetoresistance in magnetic semiconductor EuIr$$_4$$In$$_2$$Ge$$_4$$

Yokoyama, Akira*; Nakachi, Ryu*; Homma, Yoshiya*; Nakamura, Ai*; Shimizu, Yusei*; Li, D.*; Miyake, Atsushi*; Honda, Fuminori*; Aoki, Dai*; Onuki, Yoshichika*; et al.

Journal of the Physical Society of Japan, 94(2), p.023701_1 - 023701_4, 2025/02

Journal Articles

Weyl-Kondo semimetal behavior in the chiral structure phase of Ce$$_{3}$$Rh$$_{4}$$Sn$$_{13}$$

Iwasa, Kazuaki*; Suyama, Kazuya*; Kawamura, Seiko; Nakajima, Kenji; Raymond, S.*; Steffens, P.*; Yamada, Akira*; Matsuda, Tatsuma*; Aoki, Yuji*; Kawasaki, Ikuto; et al.

Physical Review Materials (Internet), 7(1), p.014201_1 - 014201_11, 2023/01

 Times Cited Count:5 Percentile:44.41(Materials Science, Multidisciplinary)

Journal Articles

Depth profile analysis of multi-layer laminated thin film interface by spatiotemporal angle-resolved APXPS method

Toyoda, Satoshi*; Yoshimura, Masashi*; Sumida, Hirosuke*; Mineoi, Susumu*; Machida, Masatake*; Yoshigoe, Akitaka; Yoshikawa, Akira*; Suzuki, Satoru*; Yokoyama, Kazushi*

Hoshako, 35(3), p.200 - 206, 2022/05

The present status of spatiotemporal depth profiling analysis of the multilayer stacked film interface based on Ambient Pressure X-ray Photoelectron Spectroscopy (APXPS) is presented. To begin with, depth profiles of the multilayer stacked film interfaces have been achieved by time-division Near Ambient Pressure Hard X-ray Angle-Resolved PhotoEmission Spectroscopy data. We then have promoted our methods to quickly perform peak fittings and depth profiling from time-division angle resolved AP-XPS data including spatial resolution, which enables us to realize spatiotemporal depth profiles of the interfaces under reaction conditions such as oxidation and reduction. In addition, it is found that the traditional maximum entropy method (MEM) combined with Jackknife averaging of sparse modeling is effective to perform dynamic measurement of depth profiles with high precision.

JAEA Reports

Annual report for research on geosphere stability for long-term isolation of radioactive waste in fiscal year 2020

Ishimaru, Tsuneari; Ogata, Nobuhisa; Kokubu, Yoko; Shimada, Koji; Niwa, Masakazu; Shimada, Akiomi; Watanabe, Takahiro; Sueoka, Shigeru; Yokoyama, Tatsunori; Fujita, Natsuko; et al.

JAEA-Research 2021-007, 65 Pages, 2021/10

JAEA-Research-2021-007.pdf:4.21MB

This annual report documents the progress of research and development (R&D) in the 6th fiscal year during the JAEA 3rd Mid- and Long-term Plan (fiscal years 2015-2021) to provide the scientific base for assessing geosphere stability for long-term isolation of the high-level radioactive waste. The planned framework is structured into the following categories: (1) Development and systematization of investigation techniques, (2) Development of models for long-term estimation and effective assessment, (3) Development of dating techniques. The current status of R&D activities with previous scientific and technological progress is summarized.

JAEA Reports

Research plan on geosphere stability for long-term isolation of radioactive waste (Scientific program for fiscal year 2021)

Ishimaru, Tsuneari; Kokubu, Yoko; Shimada, Koji; Shimada, Akiomi; Niwa, Masakazu; Watanabe, Takahiro; Sueoka, Shigeru; Yokoyama, Tatsunori; Fujita, Natsuko; Ogita, Yasuhiro; et al.

JAEA-Review 2021-012, 48 Pages, 2021/08

JAEA-Review-2021-012.pdf:1.64MB

This report is a plan of research and development (R&D) on geosphere stability for long-term isolation of high-level radioactive waste (HLW) in Japan Atomic Energy Agency (JAEA), in fiscal year 2021. The objectives and contents in fiscal year 2021 are described in detail based on the JAEA 3rd Medium- and Long-term Plan (fiscal years 2015-2021). In addition, the background of this research is described from the necessity and the significance for site investigation and safety assessment, and the past progress. The plan framework is structured into the following categories: (1) Development and systematization of investigation techniques, (2) Development of models for long-term estimation and effective assessment, (3) Development of dating techniques.

Journal Articles

Development of ${it spatiotemporal}$ measurement and analysis techniques in X-ray photoelectron spectroscopy; From NAP-HARPES to 4D-XPS

Toyoda, Satoshi*; Yamamoto, Tomoki*; Yoshimura, Masashi*; Sumida, Hirosuke*; Mineoi, Susumu*; Machida, Masatake*; Yoshigoe, Akitaka; Suzuki, Satoru*; Yokoyama, Kazushi*; Ohashi, Yuji*; et al.

Vacuum and Surface Science, 64(2), p.86 - 91, 2021/02

We have developed ${it spatiotemporal}$ measurement and analysis techniques in X-ray photoelectron spectroscopy. To begin with, time-division depth profiles of gate stacked film interfaces have been achieved by NAP-HARPES (Near Ambient Pressure Hard X-ray Angle-Resolved Photo Emission Spectroscopy) data. We then have promoted our methods to quickly perform peak fittings and depth profiling from time-division ARPES data, which enables us to realize 4D-XPS analysis. It is found that the traditional maximum entropy method (MEM) combined with Jackknife averaging of sparse modeling in NAP-HARPES data is effective to perform dynamic measurement of depth profiles with high precision.

JAEA Reports

Annual report for research on geosphere stability for long-term isolation of radioactive waste in fiscal year 2019

Ishimaru, Tsuneari; Ogata, Nobuhisa; Kokubu, Yoko; Shimada, Koji; Hanamuro, Takahiro; Shimada, Akiomi; Niwa, Masakazu; Asamori, Koichi; Watanabe, Takahiro; Sueoka, Shigeru; et al.

JAEA-Research 2020-011, 67 Pages, 2020/10

JAEA-Research-2020-011.pdf:3.87MB

This annual report documents the progress of research and development (R&D) in the 5th fiscal year during the JAEA 3rd Mid- and Long-term Plan (fiscal years 2015-2021) to provide the scientific base for assessing geosphere stability for long-term isolation of the high-level radioactive waste. The planned framework is structured into the following categories: (1) Development and systematization of investigation techniques, (2) Development of models for long-term estimation and effective assessment, (3) Development of dating techniques. The current status of R&D activities with previous scientific and technological progress is summarized.

JAEA Reports

Research plan on geosphere stability for long-term isolation of radioactive waste (Scientific program for fiscal year 2020)

Ishimaru, Tsuneari; Ogata, Nobuhisa; Shimada, Koji; Kokubu, Yoko; Niwa, Masakazu; Asamori, Koichi; Watanabe, Takahiro; Sueoka, Shigeru; Komatsu, Tetsuya; Yokoyama, Tatsunori; et al.

JAEA-Review 2020-010, 46 Pages, 2020/07

JAEA-Review-2020-010.pdf:1.89MB

This report is a plan of research and development (R&D) on geosphere stability for long-term isolation of high-level radioactive waste (HLW) in Japan Atomic Energy Agency (JAEA), in fiscal year 2020. The objectives and contents in fiscal year 2020 are described in detail based on the JAEA 3rd Medium- and Long-term Plan (fiscal years 2015-2021). In addition, the background of this research is described from the necessity and the significance for site investigation and safety assessment, and the past progress. The plan framework is structured into the following categories: (1) Development and systematization of investigation techniques, (2) Development of models for long-term estimation and effective assessment, (3) Development of dating techniques.

Journal Articles

Isotope-selective dissociation of diatomic molecules by terahertz optical pulses

Ichihara, Akira; Matsuoka, Leo*; Segawa, Etsuo*; Yokoyama, Keiichi

Physical Review A, 91(4), p.043404_1 - 043404_7, 2015/04

 Times Cited Count:13 Percentile:54.51(Optics)

We propose a new method for isotope-selective dissociation of diatomic molecules in the gas phase by using two kinds of terahertz-pulse fields. The first field consists of a train of pulses, which composes a frequency comb, excites the selected isotope into highly-rotationally excited state. The second intense pulse field dissociates the excited molecule by further rotational excitations. We performed wave-packet computations using the lithium chlorides $$^{7}$$Li$$^{35}$$CL and $$^{7}$$Li$$^{37}$$Cl to demonstrate the applicability of our method. Nearly 20% of $$^{7}$$Li$$^{37}$$Cl in the lowest rovibrational state is dissociated in the designed pulse fields, while the dissociation probability is negligible in $$^{7}$$Li$$^{35}$$Cl. This method is expected to be applicable to other diatomic molecules, and to molecular ensembles whose rotational states spread in energy.

Journal Articles

Development of a new continuous dissolution apparatus with a hydrophobic membrane for superheavy element chemistry

Oe, Kazuhiro*; Attallah, M. F.*; Asai, Masato; Goto, Naoya*; Gupta, N. S.*; Haba, Hiromitsu*; Huang, M.*; Kanaya, Jumpei*; Kaneya, Yusuke*; Kasamatsu, Yoshitaka*; et al.

Journal of Radioanalytical and Nuclear Chemistry, 303(2), p.1317 - 1320, 2015/02

 Times Cited Count:10 Percentile:59.08(Chemistry, Analytical)

A new technique for continuous dissolution of nuclear reaction products transported by a gas-jet system was developed for superheavy element (SHE) chemistry. In this technique, a hydrophobic membrane is utilized to separate an aqueous phase from the gas phase. With this technique, the dissolution efficiencies of short-lived radionuclides of $$^{91m,93m}$$Mo and $$^{176}$$W were measured. Yields of more than 80% were observed for short-lived radionuclides at aqueous-phase flow rates of 0.1-0.4 mL/s. The gas flow-rate had no influence on the dissolution efficiency within the studied flow range of 1.0-2.0 L/min. These results show that this technique is applicable for on-line chemical studies of SHEs in the liquid phase.

Journal Articles

Quantum control of isotope-selective rovibrational excitation of diatomic molecules in the thermal distribution

Ichihara, Akira; Matsuoka, Leo*; Kurosaki, Yuzuru; Yokoyama, Keiichi

Optical Review, 22(1), p.153 - 156, 2015/02

 Times Cited Count:6 Percentile:31.52(Optics)

We propose a method to excite the rovibrational states of diatomic molecules in the gas-phase isotope-selectively by optical pulses. In this method, the rotational state of the selected isotope molecule is excited by the terahertz frequency comb, and the vibrational state of high J molecule is excited via the fundamental transitions in the P-branch by using the second pulse. The applicability of the proposed method is demonstrated by computer simulations using the LiCl molecules in the thermal distribution at 70 K.

Journal Articles

Infrared thermography inspection for monoblock divertor target in JT-60SA

Nakamura, Shigetoshi; Sakurai, Shinji; Ozaki, Hidetsugu; Seki, Yohji; Yokoyama, Kenji; Sakasai, Akira; Tsuru, Daigo

Fusion Engineering and Design, 89(7-8), p.1024 - 1028, 2014/10

 Times Cited Count:5 Percentile:33.82(Nuclear Science & Technology)

Carbon Fiber Composite mono-block divertor target is required for power handling in JT-60SA. Heat removal capability of the target is degraded by joint defect which is induced in manufacturing process. For screening heat removal capability, infrared thermography inspection (IR inspection) is improved an accuracy for the target using threaded cooling tube. In IR inspection, the targets heated at 95$$^{circ}$$C by hot water in steady state condition are instantaneously cooled down by cold water flow of 5$$^{circ}$$C in three channels of test section. The heat removal capability of the targets is evaluated with comparing the transient thermal response time between defect-free and tested targets. A construction of a database for a correlation between the known defects, maximum surface temperatures in the heat load test and the IR inspection are successfully completed. Screening criteria is set with finite element methods based on the database.

Journal Articles

High power laser developments with femtosecond to nanosecond pulse durations for laser shock science and engineering

Kiriyama, Hiromitsu; Mori, Michiaki; Suzuki, Masayuki*; Daito, Izuru*; Okada, Hajime; Ochi, Yoshihiro; Tanaka, Momoko; Sato, Masatoshi*; Tamaoki, Yoshinori*; Yoshii, Takehiro*; et al.

Reza Kenkyu, 42(6), p.441 - 447, 2014/06

We describe three specific high power laser systems that are being developed in our laboratory for many applications in high field science, nonlinear optics and material processing. We report on a femtosecond petawatt-class Ti:sapphire chirped-pulse amplification laser system that can produce a pulse energy of 20 J of 40 fs pulse duration, a picosecond high intensity Yb:YAG chirped-pulse amplification laser system that can generate a pulse energy of 100 mJ of 0.5 ps pulse duration, and a nanosecond high repetition rate Nd:YAG laser system that can provide an average power of 360 W with a pulse duration of 30 ns delivered at a 1 kHz repetition rate. We discuss the basic design aspects and present the results from our experimental investigations of these laser systems.

JAEA Reports

Annual report on the environmental radiation monitoring around the Tokai Reprocessing Plant FY2012

Sumiya, Shuichi; Watanabe, Hitoshi; Miyagawa, Naoto; Nakano, Masanao; Nakada, Akira; Fujita, Hiroki; Takeyasu, Masanori; Isozaki, Tokuju; Morisawa, Masato; Mizutani, Tomoko; et al.

JAEA-Review 2013-056, 181 Pages, 2014/03

JAEA-Review-2013-056.pdf:6.22MB

Environmental radiation monitoring around the Tokai Reprocessing Plant has been performed by the Nuclear Fuel Cycle Engineering Laboratories, based on "Safety Regulations for the Reprocessing Plant of Japan Atomic Energy Agency, Chapter IV - Environmental Monitoring". This annual report presents the results of the environmental monitoring and the dose estimation to the hypothetical inhabitant due to the radioactivity discharged from the plant to the atmosphere and the sea during April 2012 to March 2013. In this report, some data include the influence of the accidental release from the Fukushima Daiichi Nuclear Power Plant of Tokyo Electric Power Co. in March 2011.

Journal Articles

Theoretical study on isotope-selective dissociation of the lithium chloride molecule using a designed terahertz-wave field

Ichihara, Akira; Matsuoka, Leo; Kurosaki, Yuzuru; Yokoyama, Keiichi

JPS Conference Proceedings (Internet), 1, p.013093_1 - 013093_4, 2014/03

Isotope-selective dissociation of the lithium chloride (LiCl) molecule was investigated by quantum mechanical calculations. $$^7$$Li$$^{35}$$Cl in the initial rovibrational state (v=0,J=0) was excited by an optical frequency comb whose spectral frequencies were tuned to the rotational transition frequencies of $$^7$$Li$$^{35}$$Cl. $$^7$$Li$$^{37}$$Cl was not highly excited by the comb because of the difference of the transition frequencies. The time evolution of rovibrational population was evaluated using the close-coupling method during the comb irradiation. The dissociation process in the second pulse was calculated by the wave packet method. The amplitudes of close-coupling were employed as the input of the wave packet computation. The dissociation probability was estimated by absorbing wave packet using a damping function. By the optical pulses adopted, about 60% of $$^7$$Li$$^{35}$$Cl was dissociated. The dissociation probability of $$^7$$Li$$^{37}$$Cl was less than 2%t.

Journal Articles

An Analytic formula for describing the transient rotational dynamics of diatomic molecules in an optical frequency comb

Ichihara, Akira; Matsuoka, Leo*; Kurosaki, Yuzuru; Yokoyama, Keiichi

Chinese Journal of Physics, 51(6), p.1230 - 1240, 2013/12

We derived an analytic expression for evaluating the transient rotational dynamics of diatomic molecules in an optical frequency comb which is tuned to induce a series of pure rotational transitions. The formulation is based on the quantum delta-kicked rotor model, and the orthogonality of delta functions at different time is assumed. The formulation is performed with the matrix decomposition technique. We derived the probability amplitude composed of term corresponding to a Bessel function of the first kind and other oscillating terms. The time dependence of obtained transition probability is shown as a staircase function.

JAEA Reports

Annual report on the environmental radiation monitoring around the Tokai Reprocessing Plant FY2011

Sumiya, Shuichi; Watanabe, Hitoshi; Nakano, Masanao; Takeyasu, Masanori; Nakada, Akira; Fujita, Hiroki; Isozaki, Tokuju; Morisawa, Masato; Mizutani, Tomoko; Nagaoka, Mika; et al.

JAEA-Review 2013-009, 195 Pages, 2013/06

JAEA-Review-2013-009.pdf:3.35MB

Environmental radiation monitoring around the Tokai Reprocessing Plant has been performed by the Nuclear Fuel Cycle Engineering Laboratories, based on "Safety Regulations for the Reprocessing Plant of Japan Atomic Energy Agency, Chapter IV - Environmental Monitoring". This annual report presents the results of the environmental monitoring and the dose estimation to the hypothetical inhabitant due to the radioactivity discharged from the plant to the atmosphere and the sea during April 2011 to March 2012. In this report, some data include the influence of the accidental release from the Fukushima Daiichi Nuclear Power Plant on Tokyo Electric Power Co. in March 2011.

Journal Articles

Theoretical study on isotope-selective excitation of diatomic molecules by a terahertz frequency comb

Ichihara, Akira; Matsuoka, Leo; Kurosaki, Yuzuru; Yokoyama, Keiichi

Proceedings of 10th Conference on Lasers and Electro-Optics Pacific Rim and 18th OptoElectronics and Communications Conference and Photonics in Switching 2013 (CLEO-PR & OECC/PS 2013) (USB Flash Drive), 2 Pages, 2013/06

Computer simulations were performed for studying isotope-selective excitation of lithium chloride using a terahertz frequency comb. The time evolution of rovibrational population was calculated by the close-coupling method. The $$^7$$Li$$^{35}$$Cl molecule was excited selectively in gaseous mixture of $$^7$$Li$$^{35}$$Cl and $$^7$$Li$$^{37}$$Cl by adjusting pulse parameters. Moreover, the wave packet calculations were performed to investigate the dissociation process. More than half of $$^7$$Li$$^{35}$$Cl in the rovibrational state (v=0, J=150) were dissociated by the second pulse.

Journal Articles

Manufacturing and development of JT-60SA vacuum vessel and divertor

Sakasai, Akira; Masaki, Kei; Shibama, Yusuke; Sakurai, Shinji; Hayashi, Takao; Nakamura, Shigetoshi; Ozaki, Hidetsugu; Yokoyama, Kenji; Seki, Yohji; Shibanuma, Kiyoshi; et al.

Proceedings of 24th IAEA Fusion Energy Conference (FEC 2012) (CD-ROM), 8 Pages, 2013/03

The JT-60SA vacuum vessel (VV) and divertor are key components for the performance requirements. Therefore the manufacturing and development of VV and divertor are in progress, inclusive of the superconducting magnets. The vacuum vessel has a double wall structure in high rigidity to withstand electromagnetic force at disruption and to keep high toroidal one-turn resistance. In addition, the double wall structure fulfills originally two functions. (1) The remarkable reduction of the nuclear heating in the superconducting magnets is made by boric-acid water circulated in the double wall. (2) The effective baking is enabled by nitrogen gas flow of 200$$^{circ}$$C in the double wall after draining of water. Three welding types were chosen for the manufacturing of the double wall structure VV to minimize deformation by welding. Divertor cassettes with fully water cooled plasma facing components were designed to realize the JT-60SA lower single null closed divertor. The divertor cassettes in the radio-active VV have been developed to ensure compatibility with remote handling (RH) maintenance in order to allow long pulse high performance discharges with high neutron yield. The manufacturing of divertor cassettes with typical accuracy of *1 mm has been successfully completed. Brazed CFC (carbon fiber composite) monoblock targets for a divertor target have been manufactured by precise control of tolerances inside CFC blocks. The infrared thermography test of monoblock targets has been developed as new acceptance inspection.

Journal Articles

The Analysis of boron micro-distribution in 9L gliosarmoma cells and HUVEC cells using PIXE and PIGE

Endo, Kiyoshi*; Shibata, Yasushi*; Yamamoto, Tetsuya*; Nakai, Kei*; Matsumura, Akira*; Sato, Takahiro; Yokoyama, Akihito; Koka, Masashi; Okubo, Takeru; Yamazaki, Akiyoshi; et al.

JAEA-Review 2011-043, JAEA Takasaki Annual Report 2010, P. 86, 2012/01

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