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Journal Articles

Discrimination of disposal-restricted materials in waste containers by nondestructive testing and image analysis with high-energy X-ray computed tomography

Murakami, Masashi; Yoshida, Yukihiko; Nango, Nobuhito*; Kubota, Shogo*; Kurosawa, Takuya*; Sasaki, Toshiki

Journal of Nuclear Science and Technology, 62(7), p.650 - 661, 2025/07

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

Journal Articles

Numerical analysis of natural convective heat transfer with porous medium using JUPITER

Uesawa, Shinichiro; Yamashita, Susumu; Sano, Yoshihiko*; Yoshida, Hiroyuki

Journal of Nuclear Science and Technology, 62(6), p.523 - 541, 2025/06

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

Japan Atomic Energy Agency (JAEA) has developed a numerical method with the JUPITER code with a porous medium model to calculate the thermal behavior in PCVs of 1F. In this study, we performed an experiment and numerical simulation of the natural convective heat transfer with the porous medium to validate JUPITER with the porous medium model. In comparison of the temperature and velocity distributions between the experiment and simulation, the temperature distribution in the simulation was in good agreement with the distribution in the experiment except the temperature near the top surface of the porous medium. The velocity distribution also agreed qualitatively with the experimental result. In addition, we also performed the numerical simulations with various effective thermal conductivity models to discuss the effect of the conductivity based on the internal structure of porous media on the natural convective heat transfer. The result indicated that the temperature distribution in the porous medium and the velocity distribution of the natural convection were significantly different for each model, and thus the conductivity of the fuel debris was one of the key parameters of in the thermal behavior analysis in 1F.

Journal Articles

Numerical investigation of the accuracy of a conductance-type wire-mesh sensor for a single spherical bubble and bubbly flow

Uesawa, Shinichiro; Ono, Ayako; Nagatake, Taku; Yamashita, Susumu; Yoshida, Hiroyuki

Journal of Nuclear Science and Technology, 62(5), p.432 - 456, 2025/05

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

We performed electrostatic simulations of a wire-mesh sensor (WMS) for a single spherical bubble and bubbly flow to clarify the accuracy of the WMS. The electrostatic simulation for the single bubble showed the electric current density distribution and the electric current path from the excited transmitter to receivers for various bubble locations. It indicated systematic errors based on the nonuniform current density distribution around the WMS. The electrostatic simulation for the bubbly flow calculated by the computational fluid dynamics code, JAEA Utility Program for Interdisciplinary Thermal-hydraulics Engineering and Research (JUPITER), indicated that the WMS had difficulty in quantitatively measuring the intermediate values of the instantaneous void fraction between 0 and 1 because they cannot be estimated by previous transformation methods from the WMS signal to the void fraction, such as linear approximation or Maxwell's equation, and have a significant deviation of the void fraction of $$pm$$0.2 for the WMS signal. However, the electrostatic simulation indicated that the time-averaged void fractions around the center of the flow channel can be estimated using linear approximation, and the time-averaged void fraction near the wall of the flow channel can be estimated using Maxwell's equation.

Journal Articles

Achievements and status of the STRAD project for radioactive liquid waste management

Arai, Yoichi; Watanabe, So; Nakahara, Masaumi; Funakoshi, Tomomasa; Hoshino, Takanori; Takahatake, Yoko; Sakamoto, Atsushi; Aihara, Haruka; Hasegawa, Kenta; Yoshida, Toshiki; et al.

Progress in Nuclear Science and Technology (Internet), 7, p.168 - 174, 2025/05

The Japan Atomic Energy Agency (JAEA) has been conducting a project named "Systematic Treatment of RAdioactive liquid waste for Decommissioning (STRAD)" project since 2018 for fundamental and practical studies for treating radioactive liquid wastes with complicated compositions. Fundamental studies have been conducted using genuine liquid wastes accumulated in a hot laboratory of the JAEA called the Chemical Processing Facility (CPF), and treatment procedures for all liquid wastes in CPF were successfully designed on the results obtained. As the next phase of the project, new fundamental and practical studies on primarily organic liquid wastes accumulated in different facilities of JAEA are in progress. This paper reviews the representative achievements of the STRAD project and introduces an overview of ongoing studies.

Journal Articles

Redox control in arsenic accumulation with organic matter derived from a varved lacustrine deposit in the Jurassic accretionary complexes

Masuki, Yuma*; Katsuta, Nagayoshi*; Naito, Sayuri*; Murakami, Takuma*; Umemura, Ayako*; Fujita, Natsuko; Matsubara, Akihiro*; Minami, Masayo*; Niwa, Masakazu; Yoshida, Hidekazu*; et al.

Journal of Hazardous Materials, 485, p.136843_1 - 136843_10, 2025/03

 Times Cited Count:0 Percentile:0.00(Engineering, Environmental)

Lacustrine deposits have 30-fold higher As abundance than the average crustal deposit. Arsenic is mostly concentrated as discrete horizons deposited in spring and autumn. As-rich layers contain FeAsS, AsS, and As$$_{2}$$S$$_{3}$$ but As-rich hotspots mostly contain FeAsS. As accumulation to sediment is controlled by redox potential with organic matter.

Journal Articles

3D visualization in rod bundle flow channel using deep learning-based bubble detection

Uesawa, Shinichiro; Ono, Ayako; Yoshida, Hiroyuki

Konsoryu, 39(1), p.61 - 71, 2025/03

Bubble visualization using a high-speed video-camera has been used as a measurement technique of bubble diameters and velocities. However, the bubble detection was difficult under the condition of the high void fraction because the overlapping bubbles for the sight direction of the camera increased with the void fraction. Additionally, the visualization for a system with objects, such as rod bundle flow channels, becomes more difficult. In this study, we applied a deep learning-based bubble detection technique with Shifted Window Transformer to bubble images shoot from two directions to identify the bubble size, three-dimensional (3D) positions of bubbles, 3D bubble trajectories in the rod bundle flow channel. Furthermore, we used perfluoroalkoxy alkane tubes with almost the same reflection as water in the channel to visualize the bubbly flow in the whole of the flow channel. We confirmed that the detection technique can segment individual bubbles in overlapping bubbles and bubbles behind the rod. By using the detection results, we estimated the diameter and velocity of each bubble and cross-sectional void fraction.

Journal Articles

Combustion properties of glove-box panel resins under fire accidents

Tashiro, Shinsuke; Uchiyama, Gunzo; Ono, Takuya; Amano, Yuki; Yoshida, Ryoichiro; Watanabe, Koji*; Abe, Hitoshi; Yamane, Yuichi

Nuclear Technology, 211(3), p.429 - 438, 2025/03

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

Contributing to the confinement safety evaluation of glove-box (GB) connected with high efficiency particle air (HEPA) filters for radioactive materials under fire accidents, combustion tests of a flammable polymer, Polymethyl methacrylate (PMMA), and a flame retardant polymer, Polycarbonate (PC), as typical GB panel resins have been conducted with an engineering-scale combustion apparatus. The combustion properties such as the mass loss rate (MLR) and the heat release rate (HRR) of PMMA and PC were investigated in the combustion tests. In the tests with the same shapes, it was found the followings; MLRs and HRRs of PMMA were larger than those of PC under the same supply flow rate into the combustion cell (Fv); MLRs and HRRs of PMMA and PC were constant under different Fv. Moreover, in the tests of PMMA with different cross section areas (S), MLRs and HRRs were found to be proportional to S. Using these results, the relationships of MLR and HRR to S of PMMA and PC were deduced.

Journal Articles

Atomization mechanisms in the vortex-like flow of a wall-impinging jet in a shallow pool

Horiguchi, Naoki; Yoshida, Hiroyuki; Kaneko, Akiko*; Abe, Yutaka*

Physics of Fluids, 37(3), p.033333_1 - 033333_20, 2025/03

 Times Cited Count:0 Percentile:0.00(Mechanics)

In a severe accident, as molten fuel is assumed to behave as a wall-impinging jet in a shallow coolant pool, atomize and accumulate as fuel debris, it is important to reveal the atomization mechanisms of the wall-impinging jet. This study aimed to reveal the atomization mechanisms in the vortex-like flow of a wall-impinging jet in a shallow pool of a liquid-liquid system, focusing on droplet formation as an elementary process of atomization. To quantitatively investigate these mechanisms, we applied quantification methods to three-dimensional interfacial data obtained by a previous experimental study using three-dimensional laser-induced fluorescence with index matching. Detailed observations of the spreading behavior of droplets and vortex-like flow, along with quantitative estimations, found out that the vortex-like flow is the dominant source of droplets on the atomization. Further investigations into the forces acting on the vortex-like flow found out the formation and collapse processes of the vortex-like flow. The accelerations of the normal forces acting on the vortex-like flow can be represented by superficial centrifugal acceleration and gravitational acceleration. Our next analysis focused on investigating droplet formation as the elementary process of atomization. The results showed two droplet formation patterns: liquid-film breaking patterns, wherein droplets directly form from the liquid film, and the surfing pattern, wherein droplets form from interfacial waves on the liquid film. Subsequently, the droplet data were grouped using dimensionless numbers and compared with theoretical lines describing the different droplet formation mechanisms. This comparison revealed the mechanisms of droplet formation within the vortex-like flow.

Journal Articles

Development of a dissolution method for analyzing the elemental composition of fuel debris using sodium peroxide fusion technique

Nakamura, Satoshi; Ishii, Sho*; Kato, Hitoshi*; Ban, Yasutoshi; Hiruta, Kenta; Yoshida, Takuya; Uehara, Hiroyuki; Obata, Hiroki; Kimura, Yasuhiko; Takano, Masahide

Journal of Nuclear Science and Technology, 62(1), p.56 - 64, 2025/01

 Times Cited Count:1 Percentile:57.00(Nuclear Science & Technology)

A dissolution method for analyzing the elemental composition of fuel debris using the sodium peroxide (Na$$_{2}$$O$$_{2}$$) fusion technique has been developed. Herein, two different types of simulated debris materials (such as solid solution of (Zr,RE)O$$_{2}$$ and molten core-concrete interaction products (MCCI)) were taken. At various temperatures, these debris materials were subsequently fused with Na$$_{2}$$O$$_{2}$$ in crucibles, which are made of different materials, such as Ni, Al$$_{2}$$O$$_{3}$$, Fe, and Zr. Then, the fused samples are dissolved in nitric acid. Furthermore, the effects of the experimental conditions on the elemental composition analysis were evaluated using inductively coupled plasma-atomic emission spectroscopy (ICP-AES), which suggested the use of a Ni crucible at 923 K as an optimum testing condition. The optimum testing condition was then applied to the demonstration tests with Three Mile Island unit-2 (TMI-2) debris in a shielded concrete cell, thereby achieving complete dissolution of the debris. The elemental composition of TMI-2 debris revealed by the proposed dissolution method has good reproducibility and has an insignificant contradiction in the mass balance of the sample. Therefore, this newly developed reproducible dissolution method can be effectively utilized in practical applications by dissolving fuel debris and estimating its elemental composition.

Journal Articles

Study on the effect of radiation-resistant resin on water radiolysis

Ito, Tatsuya; Nagaishi, Ryuji; Kuwano, Ryo*; Godo, Masao*; Yoshida, Yoichi*

Radiation Physics and Chemistry, 226, p.112198_1 - 112198_5, 2025/01

 Times Cited Count:0 Percentile:0.00(Chemistry, Physical)

In recent years, the use of radiation-resistant resins of polyimide and polyether ether ketone becomes increasing as vessels for irradiation and unsealed radioisotope experiments. However, in our radiolysis experiments, the possibility of interaction between radiolysis products of water and the resin was found, suggesting concerns that the resin may affect reactions in water in radiation fields. To clarify the interaction, dichromate (Cr$$_{2}$$O$$_{7}$$$$^{2-}$$) reduction and hydrogen peroxide (H$$_{2}$$O$$_{2}$$) formation in $$gamma$$-radiolysis of water were compared with and without the resin. The Cr$$_{2}$$O$$_{7}$$$$^{2-}$$ reduction amount in aqueous solution with the resin became larger than that without the resin at the same dose, indicating the promotion of Cr$$_{2}$$O$$_{7}$$$$^{2-}$$ reduction by the resin. On the other hand, the H$$_{2}$$O$$_{2}$$ formation in pure water with and without an electron scavenger were almost independent of the presence of resin. These suggested the interaction between hydroxyl radical and the resin in contact with water in radiation fields.

Journal Articles

Nanoscale visualization of crack tips inside molten corium-concrete interaction debris using 3D-FIB-SEM with multiphase positional misalignment correction

Miyata, Hokata*; Yoshida, Kenta*; Konashi, Kenji*; Du, Y.*; Kitagaki, Toru; Shobu, Takahisa; Shimada, Yusuke*

Microscopy, p.dfaf005_1 - dfaf005_10, 2025/00

 Times Cited Count:0 Percentile:0.00(Microscopy)

Journal Articles

$$^{149}$$Sm synchrotron-radiation-based M$"{o}$ssbauer and $$mu^+$$SR studies of Sm$$_3$$Ru$$_4$$Ge$$_{13}$$

Tsutsui, Satoshi; Ito, Takashi; Nakamura, Jin*; Yoshida, Mio*; Kobayashi, Yoshio*; Yoda, Yoshitaka*; Nakamura, Jumpei*; Koda, Akihiro*; Higashinaka, Ryuji*; Aoki, Dai*; et al.

Interactions (Internet), 245(1), p.55_1 - 55_9, 2024/12

Journal Articles

Deep learning-based bubble detection with Swin Transformer

Uesawa, Shinichiro; Yoshida, Hiroyuki

Journal of Nuclear Science and Technology, 61(11), p.1438 - 1452, 2024/11

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

We developed a deep learning-based bubble detector with a Shifted window Transformer (Swin Transformer) to detect and segment individual bubbles among overlapping bubbles. To verify the performance of the detector, we calculated its average precision (AP) with different number of training images. The mask AP increased with the increase in the number of training images when there were less than 50 images but remained constant when there were more than 50 images. It was observed that the AP for the Swin Transformer and ResNet were almost the same when there were more than 50 images; however, when few training images were used, the AP of the Swin Transformer were higher than that of the ResNet. Furthermore, with regard to the increase in void fraction, the AP of the Swin Transformer showed a decrease similar to that in the case of the ResNet; however, for few training images, the AP of the Swin Transformer was higher than that of the ResNet in all void fractions. Moreover, we confirmed the detector trained with synthetic bubble images was able to segment overlapping bubbles and deformed bubbles in a bubbly flow experiment. Thus, we verified that the new bubble detector with Swin Transformer provided higher AP than the detector with ResNet for fewer training images.

Journal Articles

Numerical investigation of accuracy of conductance-typed wire-mesh sensor using CFD and electrostatic simulations

Uesawa, Shinichiro; Ono, Ayako; Yamashita, Susumu; Yoshida, Hiroyuki

Proceedings of 13th Korea-Japan Symposium on Nuclear Thermal Hydraulics and Safety (NTHAS13) (Internet), 7 Pages, 2024/11

A conductance-typed wire-mesh sensor (WMS), utilizing the difference in conductivity between gas and liquid phases between the electrodes, is one of the practical measurement techniques of a cross-sectional void fraction distribution in a flow path. In this study, we performed two-phase computational fluid dynamics (CFD) and electrostatic simulations around a WMS for a single spherical bubble and bubbly flow to clarify the systematic error in the WMS. The results for the single bubble indicated that there were systematic errors based on the non-uniform current density distribution around the WMS. The correlation between instantaneous void fractions and WMS signals is not uniquely determined for positions of the single bubble moving across the WMS, even for the same bubble. Moreover, the correlation between the instantaneous void fractions and the WMS signals did not fit in a linear approximation and Maxwell's equation, which traditionally used transformation methods from the WMS signal to the void fraction. The results for the bubbly flow indicated that the WMS had difficulty in quantitative measurements of the instantaneous void fraction because the values had a significant deviation of the void fraction of approximately $$pm$$0.2. On the other hand, time-averaged void fraction values had relatively small deviation. Thus, we concluded that the WMS, using existing transformation methods, can measure time-averaged void fractions, but it is difficult to measure quantitatively instantaneous void fractions.

Journal Articles

Neutronics/thermal-hydraulics coupling simulation using JAMPAN in a single BWR fuel assembly

Kamiya, Tomohiro; Nagatake, Taku; Ono, Ayako; Tada, Kenichi; Kondo, Ryoichi; Nagaya, Yasunobu; Yoshida, Hiroyuki

Proceedings of 31st International Conference on Nuclear Engineering (ICONE31) (Internet), 7 Pages, 2024/11

We have developed the JAEA Advances Multi-Physics Analysis platform for Nuclear systems (JAMPAN) to realize high-fidelity neutronics/thermal-hydraulics coupling simulations. We will perform MVP/JUPITER coupling simulation for a single BWR fuel assembly in order to confirm that the neutronics/thermal-hydraulics coupling through JAMPAN is feasible. This presentation explains how to send and receive data between MVP and JUPITER through JAMPAN and simulation results.

Journal Articles

Droplet evaporation characteristics on high-temperature porous surfaces for cooling fuel debris

Yuki, Kohei*; Horiguchi, Naoki; Yoshida, Hiroyuki; Yuki, Kazuhisa*

Proceedings of 31st International Conference on Nuclear Engineering (ICONE31) (Internet), 4 Pages, 2024/11

Fuel debris in the Fukushima Nuclear Power Station is cooled under immersion condition. However, in the event of an unexpected decrease in water level, coolant contacts high-temperature fuel debris having porous structure. In this event, although fuel debris needs to be cooled rapidly, thermal behavior at liquid-solid contact, such as capillary phenomenon, remains unclear. In this paper, as basic research, we evaluate droplet evaporation characteristics after contact with metal porous media with small pores less than 1 mm. In experiment, to obtain life time curve of a droplet, bronze or stainless steel porous media having 1, 40, or 100 $$mu$$m pore diameter are utilized. Experimental results show that Leidenfrost phenomenon is suppressed on the porous surfaces because generated vapor can be discharged from the pores. Further, for bronze porous media, capillary phenomenon is observed as the temperature of the porous media increase because of generation of oxide film having fine structure. On the other hand, due to low wettability of stainless steel porous media, capillary phenomenon does not occur, and the droplet was not sucked and spread into pore. This indicates that rapid cooling by the capillary phenomenon can not be expected if fuel debris has the same characteristics as the stainless steel porous media.

Journal Articles

Activation level of the concrete building and pressure vessel in JAEA-Tokai tandem accelerator

Yoshida, Go*; Matsumura, Hiroshi*; Nakamura, Hajime*; Miura, Taichi*; Toyoda, Akihiro*; Masumoto, Kazuyoshi*; Nakabayashi, Takayuki*; Matsuda, Makoto

Journal of Nuclear Science and Technology, 61(10), p.1298 - 1307, 2024/10

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

Journal Articles

Release behavior of gaseous ruthenium tetroxide during heating of high-level liquid waste simulant during simulated accident conditions

Yoshida, Naoki; Ono, Takuya; Amano, Yuki; Yoshida, Ryoichiro; Abe, Hitoshi; Yamane, Yuichi

Nuclear Technology, 210(10), p.1999 - 2007, 2024/10

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

A malfunction of the cooling system of high-level liquid waste (HLLW) and failure of countermeasures may lead to the "evaporation to dryness due to the loss of cooling functions" (EDLCF) of HLLW. In the EDLCF, ruthenium (Ru) can be released at a greater fraction to initial amount than other elements in HLLW by forming gaseous Ru. It is important to identify the chemical form of the released gaseous Ru to achieve a comprehensive understanding of the events impacting the source term assessment of Ru in this accident, such as particle formation, gas absorption and deposition on migration pathways. In this study, we observed the ultraviolet/visible spectroscopy of the off-gas generated during the heating of an HLLW simulant. Employing a program that allows the separation and quantification of known components within the spectrum (ruthenium tetroxide (RuO$$_{4}$$), nitrogen dioxide, and nitric acid), we attempted to analyze the composition of gaseous Ru within the generated off-gas. Our findings reveal RuO$$_{4}$$ as the main component of the gaseous Ru in off-gas after comparing the total amount of released Ru and the RuO$$_{4}$$ released amount obtained via spectroscopic analysis.

Journal Articles

Bubble visualization in rod bundle flow channel using deep learning-based bubble detection

Uesawa, Shinichiro; Ono, Ayako; Yoshida, Hiroyuki

Konsoryu Shimpojiumu 2024 Koen Rombunshu (Internet), 2 Pages, 2024/09

Bubble visualization using a high-speed video-camera has been used as measurement techniques of bubble diameters, interfacial area concentrations, and void fractions in dispersed bubbly flow. However, the bubble detection was difficult under the condition of the high void fraction because the overlapping bubbles for the sight direction of the camera increased with the increase in the void fraction. In this study, we developed the deep learning-based bubble detector with Shifted window Transformer (Swin Transformer) to overcome the issue. To verify the performance, we used the synthetic bubble images obtained by Generative Adversarial Networks (GAN) and obtained average precisions (APs) for the number of the training dataset. The result showed that the AP was large enough for 50 datasets, and bubble detection was possible even with a small number of the training data. Additionally, we confirmed that the detector can detect and segment individual bubbles in overlapping bubbles obtained in the visualization experiments of pipe and bundle flows. By using the detection results, we estimated the interfacial area concentrations and void fractions. In comparison with commonly used relations, the results were in good agreement with the relations. Thus, the detector can measure not only bubble diameters but also interfacial area concentrations and void fractions.

Journal Articles

R&D status of digital technology on inverse estimation of radioactive source distributions and related source countermeasures; Fast Digital Twin Tech. in Decommissioning Field: 3D-ADRES-Indoor FrontEnd

Machida, Masahiko; Yamada, Susumu; Kim, M.; Tanaka, Satoshi*; Tobita, Yasuhiro*; Iwata, Ayako*; Aoki, Yuto; Aoki, Kazuhisa; Yanagisawa, Kenichi*; Yamaguchi, Takashi; et al.

RIST News, (70), p.3 - 22, 2024/09

Inside the Fukushima Daiichi Nuclear Power Plant (1F), there are many locations with high radiation levels due to contamination by radioactive materials that leaked from the reactor. These pose a significant obstacle to the smooth progress of decommissioning work. To help solve this issue, the Japan Atomic Energy Agency (JAEA), under a subsidy from the Ministry of Economy, Trade, and Industry's decommissioning and contaminated water management project, is conducting research and development on digital technologies to improve the radiation environment inside the decommissioning site. This project, titled "Development of Technology to Improve the Environment Inside Reactor Buildings (Enhancing Digital Technology for Environment and Source Distribution to Reduce Radiation Exposure)," began in April of FY 2023. In this project, the aim is to develop three interconnected systems: FrontEnd, Pro, and BackEnd. The FrontEnd system, based on the previously developed 3D-ADRES-Indoor (prototype) from FY 2021-2022, will be upgraded to a high-speed digital twin technology usable on-site. The Pro system will carry out detailed analysis in rooms such as the new office building at 1F, while the BackEnd system will serve as a database to centrally manage the collected and analyzed data. This report focuses on the FrontEnd system, which will be used on-site. After point cloud measurement, the system will quickly create a 3D mesh model, estimate the radiation source from dose rate measurements, and refine the position and intensity of the estimated source using recalculation techniques (re-observation instructions and re-estimation). The results of verification tests conducted on Unit 5 are also presented. Furthermore, the report briefly discusses the future research and development plans for this project.

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