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Tc separation/concentration technology from
Mo by (n,
) method, 4末松 久幸*; Yang, Y.*; 伊藤 陽登*; Le, A. V.*; Su, Y.*; 加藤 涼那*; Do, T. M. D.*; 鈴木 達也*; 大沢 直樹*; 藤田 善貴; et al.
KURNS Progress Report 2025, P. 118, 2026/06
これまでの研究で、中性子照射した
-MoO
ターゲットからホットアトムの反跳効果により水中への
Mo抽出率が時間とともに増加することを示した。本研究では、水抽出後ターゲットを再照射するためのリサイクル性評価を目的に、水浸漬後の
-MoO
粉末を乾燥した試料の
Mo生成量及び構造安定性を確認した。また、比較試料として、
-MoO
、MoO
、Mo
O
及び水浸漬させた水和
-MoO
を用意した。これらの試料を京都大学研究用原子炉(KUR)で20分間照射後、粉末を蒸留水中において室温で5.5時間攪拌させ、水への
Mo抽出率を調べた。その結果、乾燥後の
-MoO
が最も高い抽出率を示し、対照的に水和
-MoO
は通常の
-MoO
相と比較して抽出率が著しく低下した。また、MoO
の抽出率は低く、Mo
O
ではほとんど
Moが抽出されなかった。これらの結果から、ホットアトムによる反跳効果及び水への
Mo抽出率がモリブデン酸化物の結晶構造及び酸化状態に依存することを明らかにした。
三浦 博己*; 渡邊 千尋*; 青柳 吉輝*; 大場 洋次郎; 小林 正和*; 吉永 直樹*
Materials Science & Engineering A, 833, p.142531_1 - 142531_12, 2022/01
被引用回数:11 パーセンタイル:46.42(Nanoscience & Nanotechnology)The nanostructure produced by heavy cold rolling provides tensile strength of 1.9 GPa in SUS316LN austenitic stainless steel, which is further raised up to 2.2 GPa by peak aging at 748 K. Nanostructural observations using electron microscopes, small-angle scattering, and atom probe tomography revealed segregation of solute elements of Mo, Si, and so on at twin and low-angle lamellar boundaries. Finite element calculation demonstrates that this grain-boundary segregation can increase the mechanical strength.
seniority isomers of
SnSimpson, G. S.*; Gey, G.*; Jungclaus, A.*; Taprogge, J.*; 西村 俊二*; Sieja, K.*; Doornenbal, P.*; Lorusso, G.*; S
derstr
m, P.-A.*; 炭竃 聡之*; et al.
Physical Review Letters, 113(13), p.132502_1 - 132502_6, 2014/09
被引用回数:74 パーセンタイル:91.02(Physics, Multidisciplinary)Delayed
-ray cascades, originating from the decay of 6
isomeric states, in the very neutron-rich, semimagic isotopes
Sn were observed following the projectile fission of a
U beam at RIBF, RIKEN. The wave functions of these isomeric states are proposed to be predominantly a fully aligned pair of f
neutrons. Shell-model calculations, performed using a realistic effective interaction, reproduce well the energies of the excited states of these nuclei and the measured transition rates, with the exception of the
2;6
) rate of
Sn, which deviates from a simple seniority scheme. Empirically reducing the 
orbit matrix elements produces a 4+1 state with almost equal seniority 2 and 4 components, correctly reproducing the experimental
2;6
) rate of
Sn. These data provide a key benchmark for shell-model interactions far from stability.
Sn explored with the long-lived isomer in
PdWatanabe, H.*; Lorusso, G.*; 西村 俊二*; Otsuka, T.*; Ogawa, K.*; Xu, Z. Y.*; 炭竃 聡之*; S
derstr
m, P.-A.*; Doornenbal, P.*; Li, Z.*; et al.
Physical Review Letters, 113(4), p.042502_1 - 042502_6, 2014/07
被引用回数:30 パーセンタイル:78.15(Physics, Multidisciplinary)A new isomer with a half-life of 23.0(8) ms has been identified in
Pd at 2406 keV excitation. The proposed spin and parity configuration is 10
, with maximally aligned configuration of two 
neutron hole.
-decay from the long-lived isomer was also observed to populated excited states at high spins in
Ag. The small energy difference between the 10
and 7
isomers in
Pd was interpreted in the frame of the monopole shift of the 1
neutron orbit. The effects of the monopole interaction on the evolution of single-neutron energies below
Sn are discussed in terms of central and tensor forces.
proton-hole state in
Sn and the shell structure along
=82Taprogge, J.*; Jungclaus, A.*; Grawe, H.*; 西村 俊二*; Doornenbal, P.*; Lorusso, G.*; Simpson, G.*; S
derstr
m, P.-A.*; 炭竃 聡之*; Xu, Z. Y.*; et al.
Physical Review Letters, 112(13), p.132501_1 - 132501_6, 2014/04
被引用回数:61 パーセンタイル:88.79(Physics, Multidisciplinary)A low-lying state in
In, the one-proton hole nucleus with respect to double magic
Sn, was observed by its
decay to the beta emitting isomer. The new state, which was populated both in the beta decay of
Cd and after beta-delayed neutron emission from
Cd, was identified, at an excitation energy of 1353 keV, as the previously unknown single-hole state with respect to the
Sn core. Exploiting this crucial new experimental information, shell-model calculations were performed to study the structure of experimentally inaccessible
=82 isotones below
Sn. The results evidence a surprising absence of proton subshell closures along the chain of
=82 isotones. This finding bears consequences on the evolution of the
=82 shell gap along the r-process path.