Refine your search:     
Report No.
 - 
Search Results: Records 1-20 displayed on this page of 35

Presentation/Publication Type

Initialising ...

Refine

Journal/Book Title

Initialising ...

Meeting title

Initialising ...

First Author

Initialising ...

Keyword

Initialising ...

Language

Initialising ...

Publication Year

Initialising ...

Held year of conference

Initialising ...

Save select records

Journal Articles

Ordered graphane nanoribbons synthesized via high-pressure diels-alder polymerization of 2,2'-bipyrazine

Li, F.*; Tang, X.*; Fei, Y.*; Zhang, J.*; Liu, J.*; Lang, P.*; Che, G.*; Zhao, Z.*; Zheng, Y.*; Fang, Y.*; et al.

Journal of the American Chemical Society, 147(17), p.14054 - 14059, 2025/04

We synthesized a crystalline graphane nanoribbon (GANR) via pressure-induced polymerization of 2,2'-bipyrazine (BPZ). By performing Rietveld refinement of in situ neutron diffraction data, nuclear magnetic resonance spectroscopy, infrared spectra, and theoretical calculation, we found that BPZ experienced Diels-Alder polymerization between the $$pi$$ $$cdots$$ $$pi$$ stacked aromatic rings, and formed extended boat-GANR structures with exceptional long-range order. The unreacted -C=N- groups bridge the two ends of the boat, and ready for further functionalization. The GANR has a bandgap of 2.25 eV, with booming photoelectric response ($$I_{rm on}$$/$$I_{rm off}$$ =18.8). Our work highlights that the high-pressure topochemical polymerization is a promising method for the precise synthesis of graphane with specific structure and desired properties.

Journal Articles

Pressure-induced polymerization of 1,4-difluorobenzene towards fluorinated diamond nanothreads

Che, G.*; Fei, Y.*; Tang, X.*; Zhao, Z.*; Hattori, Takanori; Abe, Jun*; Wang, X.*; Ju, J.*; Dong, X.*; Wang, Y.*; et al.

Physical Chemistry Chemical Physics, 27(2), p.1112 - 1118, 2025/01

 Times Cited Count:2 Percentile:47.21(Chemistry, Physical)

Pressure-induced polymerization (PIP) of aromatic molecules has emerged as an effective method for synthesizing various carbon-based materials. In this work, PIP of 1,4-difluorobenzene (1,4-DFB) was investigated. ${it In situ}$ high-pressure investigations of 1,4-DFB reveal a phase transition at approximately 12.0 GPa and an irreversible chemical reaction at 18.7 GPa. Structural analysis of the product and the kinetics of the reaction uncovered the formation of pseudohexagonal stacked fluoro-diamond nanothreads with linear growth. Compared to the crystal structures of benzene under high pressure, 1,4-DFB exhibits higher compression along the [001] axis. The anisotropic compression is attributed to the stronger H$$cdot cdot cdot pi$$ interaction along the [01$$overline{1}$$] axis and the potential compression-inhibiting H$$cdot cdot cdot$$F interactions along the [100] and [010] axes, and it facilitates a possible reaction pathway along the [01$$overline{1}$$] axis. This work emphasizes the crucial role of functionalization in modulating molecular stacking and influencing the reaction pathway.

Journal Articles

Brightening triplet excitons enable high-performance white-light emission in organic small molecules via integrating n-$$pi^*/pi$$-$$pi^*$$ transitions

Yang, Q.*; Yang, X.*; Wang, Y.*; Fei, Y.*; Li, F.*; Zheng, H.*; Li, K.*; Han, Y.*; Hattori, Takanori; Zhu, P.*; et al.

Nature Communications (Internet), 15, p.7778_1 - 7778_9, 2024/09

 Times Cited Count:7 Percentile:85.13(Multidisciplinary Sciences)

Luminescent materials that simultaneously embody bright singlet and triplet excitons hold great potential in optoelectronics, signage, and information encryption. However, achieving high-performance white-light emission is severely hampered by their inherent unbalanced contribution of fluorescence and phosphorescence. Herein, we address this challenge by pressure treatment engineering via hydrogen bonding cooperativity effect to realize the mixture of n-$$pi^*/pi$$-$$pi^*$$ transitions, where the triplet state emission was boosted from 7% to 40% in isophthalic acid (IPA). A superior white-light emission based on hybrid fluorescence and phosphorescence was harvested in pressure-treated IPA, and the photoluminescence quantum yield was increased to 75% from the initial 19% (blue-light emission). In-situ high-pressure IR spectra, X ray diffraction, and neutron diffraction reveal continuous strengthening of the hydrogen bonds with the increase of pressure. Furthermore, this enhanced hydrogen bond is retained down to the ambient conditions after pressure treatment, awarding the targeted IPA efficient intersystem crossing for balanced singlet/triplet excitons population and resulting in efficient white-light emission. This work not only proposes a route for brightening triplet states in organic small molecule, but also regulates the ratio of singlet and triplet excitons to construct high-performance white-light emission.

Journal Articles

Crystal-liquid duality driven ultralow two-channel thermal conductivity in $$alpha$$-MgAgSb

Li, J.*; Li, X.*; Zhang, Y.*; Zhu, J.*; Zhao, E.*; Kofu, Maiko; Nakajima, Kenji; Avdeev, M.*; Liu, P.-F.*; Sui, J.*; et al.

Applied Physics Reviews (Internet), 11(1), p.011406_1 - 011406_8, 2024/03

 Times Cited Count:7 Percentile:92.96(Physics, Applied)

Journal Articles

Probing deformation behavior of a refractory high-entropy alloy using ${it in situ}$ neutron diffraction

Zhou, Y.*; Song, W.*; Zhang, F.*; Wu, Y.*; Lei, Z.*; Jiao, M.*; Zhang, X.*; Dong, J.*; Zhang, Y.*; Yang, M.*; et al.

Journal of Alloys and Compounds, 971, p.172635_1 - 172635_7, 2024/01

 Times Cited Count:1 Percentile:13.75(Chemistry, Physical)

Journal Articles

Direct observation of topological magnon polarons in a multiferroic material

Bao, S.*; Gu, Z.-L.*; Shangguan, Y.*; Huang, Z.*; Liao, J.*; Zhao, X.*; Zhang, B.*; Dong, Z.-Y.*; Wang, W.*; Kajimoto, Ryoichi; et al.

Nature Communications (Internet), 14, p.6093_1 - 6093_9, 2023/09

 Times Cited Count:17 Percentile:93.61(Multidisciplinary Sciences)

Journal Articles

A One-third magnetization plateau phase as evidence for the Kitaev interaction in a honeycomb-lattice antiferromagnet

Shangguan, Y.*; Bao, S.*; Dong, Z.-Y.*; Xi, N.*; Gao, Y.-P.*; Ma, Z.*; Wang, W.*; Qi, Z.*; Zhang, S.*; Huang, Z.*; et al.

Nature Physics, 19(12), p.1883 - 1889, 2023/09

 Times Cited Count:19 Percentile:94.23(Physics, Multidisciplinary)

Journal Articles

Pore connectivity influences mass transport in natural rocks; Pore structure, gas diffusion and batch sorption studies

Yuan, X.*; Hu, Q.*; Lin, X.*; Zhao, C.*; Wang, Q.*; Tachi, Yukio; Fukatsu, Yuta; Hamamoto, Shoichiro*; Siitari-Kauppi, M.*; Li, X.*

Journal of Hydrology, 618, p.129172_1 - 129172_15, 2023/03

 Times Cited Count:5 Percentile:54.59(Engineering, Civil)

Journal Articles

Two-dimensional quantum universality in the spin-1/2 triangular-lattice quantum antiferromagnet Na$$_{2}$$BaCo(PO$$_{4}$$)$$_{2}$$

Sheng, J.*; Wang, L.*; Candini, A.*; Jiang, W.*; Huang, L.*; Xi, B.*; Zhao, J.*; Ge, H.*; Zhao, N.*; Fu, Y.*; et al.

Proceedings of the National Academy of Sciences of the United States of America, 119(51), p.e2211193119_1 - e2211193119_9, 2022/12

 Times Cited Count:28 Percentile:91.32(Multidisciplinary Sciences)

Journal Articles

Micro- to nano-scale areal heterogeneity in pore structure and mineral compositions of a sub-decimeter-sized Eagle Ford Shale

Wang, Q.*; Hu, Q.*; Zhao, C.*; Yang, X.*; Zhang, T.*; Ilavsky, J.*; Kuzmenko, I.*; Ma, B.*; Tachi, Yukio

International Journal of Coal Geology, 261, p.104093_1 - 104093_15, 2022/09

 Times Cited Count:11 Percentile:72.62(Energy & Fuels)

Journal Articles

Mictomagnetism and suppressed thermal conduction of the prototype high-entropy alloy CrMnFeCoNi

Yang, J.*; Ren, W.*; Zhao, X.*; Kikuchi, Tatsuya*; Miao, P.*; Nakajima, Kenji; Li, B.*; Zhang, Z.*

Journal of Materials Science & Technology, 99, p.55 - 60, 2022/02

 Times Cited Count:11 Percentile:54.87(Materials Science, Multidisciplinary)

High-entropy alloys are characteristic of extensive atomic occupational disorder on high-symmetric lattices, differing from traditional alloys. Here, we investigate magnetic and thermal transport properties of the prototype face-centered-cubic high-entropy alloy CrMnFeCoNi by combining physical properties measurements and neutron scattering. Direct-current (dc) and alternating-current (ac) magnetizations measurements indicate a mictomagnetic behavior with coexisting antiferromagnetic and ferromagnetic interactions in the entire temperature region and three anomalies are found at about 80, 50, and 20 K, which are related to the paramagnetic to antiferromagnetic transition, the antiferromagnetic to ferromagnetic transition, and the spin freezing, respectively. The electrical and thermal conductivities are significantly reduced compared to Ni and the temperature dependence of lattice thermal conductivity exhibits a glass-like plateau. Inelastic neutron scattering measurements suggest weak anharmonicity so that the thermal transport is expected to be dominated by the defect scattering.

Journal Articles

Evidence for strong correlations at finite temperatures in the dimerized magnet Na$$_{2}$$Cu$$_{2}$$TeO$$_{6}$$

Shangguan, Y.*; Bao, S.*; Dong, Z.-Y.*; Cai, Z.*; Wang, W.*; Huang, Z.*; Ma, Z.*; Liao, J.*; Zhao, X.*; Kajimoto, Ryoichi; et al.

Physical Review B, 104(22), p.224430_1 - 224430_8, 2021/12

 Times Cited Count:2 Percentile:11.10(Materials Science, Multidisciplinary)

Journal Articles

Field-tuned magnetic structure and phase diagram of the honeycomb magnet YbCl$$_3$$

Hao, Y. Q.*; Wo, H. L.*; Gu, Y. M.*; Zhang, X. W.*; Gu, Y. Q.*; Zheng, S. Y.*; Zhao, Y.*; Xu, G. Y.*; Lynn, J. W.*; Nakajima, Kenji; et al.

Science China; Physics, Mechanics & Astronomy, 64(3), p.237411_1 - 237411_6, 2021/03

 Times Cited Count:11 Percentile:67.90(Physics, Multidisciplinary)

Journal Articles

Coordination number regulation of molybdenum single-atom nanozyme peroxidase-like specificity

Wang, Y.*; Jia, G.*; Cui, X.*; Zhao, X.*; Zhang, Q.*; Gu, L.*; Zheng, L.*; Li, L. H.*; Wu, Q.*; Singh, D. J.*; et al.

Chem, 7(2), p.436 - 449, 2021/02

 Times Cited Count:277 Percentile:99.77(Chemistry, Multidisciplinary)

Journal Articles

Stacking fault driven phase transformation in CrCoNi medium entropy alloy

He, H.*; Naeem, M.*; Zhang, F.*; Zhao, Y.*; Harjo, S.; Kawasaki, Takuro; Wang, B.*; Wu, X.*; Lan, S.*; Wu, Z.*; et al.

Nano Letters, 21(3), p.1419 - 1426, 2021/02

 Times Cited Count:68 Percentile:96.32(Chemistry, Multidisciplinary)

Journal Articles

Magnetic-field and composition tuned antiferromagnetic instability in the quantum spin-liquid candidate NaYbO$$_2$$

Guo, J.*; Zhao, X.*; Kawamura, Seiko; Ling, L.*; Wang, J.*; He, L.*; Nakajima, Kenji; Li, B.*; Zhang, Z.*

Physical Review Materials (Internet), 4(6), p.064410_1 - 064410_7, 2020/06

 Times Cited Count:22 Percentile:66.11(Materials Science, Multidisciplinary)

Journal Articles

Ultralow thermal conductivity from transverse acoustic phonon suppression in distorted crystalline $$alpha$$-MgAgSb

Li, X.*; Liu, P.-F.*; Zhao, E.*; Zhang, Z.*; Guide, T.*; Le, M. D.*; Avdeev, M.*; Ikeda, Kazutaka*; Otomo, Toshiya*; Kofu, Maiko; et al.

Nature Communications (Internet), 11, p.942_1 - 942_9, 2020/02

 Times Cited Count:62 Percentile:92.99(Multidisciplinary Sciences)

In high-performance thermoelectric materials, there are two main low thermal conductivity mechanisms: the phonon anharmonic and phonon scattering resulting from the dynamic disorder, which have been successfully revealed by inelastic neutron scattering. Using neutron scattering and ab initio calculations, we report here a mechanism of static local structure distortion combined with phonon-anharmonic-induced ultralow lattice thermal conductivity in $$alpha$$-MgAgSb. Since the transverse acoustic phonons are almost fully scattered by the intrinsic distorted rocksalt sublattice in this compound, the heat is mainly transported by the longitudinal acoustic phonons. The ultralow thermal conductivity in $$alpha$$-MgAgSb is attributed to its atomic dynamics being altered by the structure distortion, which presents a possible microscopic route to enhance the performance of similar thermoelectric materials.

Journal Articles

Coexistence of ferromagnetic and stripe-type antiferromagnetic spin fluctuations in YFe$$_{2}$$Ge$$_{2}$$

Wo, H.*; Wang, Q.*; Shen, Y.*; Zhang, X.*; Hao, Y.*; Feng, Y.*; Shen, S.*; He, Z.*; Pan, B.*; Wang, W.*; et al.

Physical Review Letters, 122(21), p.217003_1 - 217003_5, 2019/05

 Times Cited Count:7 Percentile:47.46(Physics, Multidisciplinary)

Journal Articles

Uniaxial pressure effect on the magnetic ordered moment and transition temperatures in BaFe$$_{2-x}$$T$$_{x}$$As$$_{2}$$ ($$T$$ = Co,Ni)

Tam, D. M.*; Song, Y.*; Man, H.*; Cheung, S. C.*; Yin, Z.*; Lu, X.*; Wang, W.*; Frandsen, B. A.*; Liu, L.*; Gong, Z.*; et al.

Physical Review B, 95(6), p.060505_1 - 060505_6, 2017/02

 Times Cited Count:24 Percentile:68.89(Materials Science, Multidisciplinary)

Journal Articles

Searching for observable effects induced by anomalous triangle singularities

Liu, X.-H.*; Oka, Makoto; Zhao, Q.*

Physics Letters B, 753, p.297 - 302, 2016/02

 Times Cited Count:101 Percentile:98.63(Astronomy & Astrophysics)

We investigate the anomalous triangle singularity (ATS) and its possible manifestations in various processes. We show that the ATS should have important impact on our understanding of the nature of some newly observed threshold states. Discussions on how to distinguish the ATS phenomena from genuine dynamic pole structures are presented.

35 (Records 1-20 displayed on this page)