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Journal Articles

All-temperature barocaloric effects at pressure-induced phase transitions

Zhao, X.*; Zhang, Z.*; Hattori, Takanori; Wang, J.*; Li, L.*; Jia, Y.*; Li, W.*; Xue, J.*; Fan, X.*; Song, R.*; et al.

Nature Communications (Internet), 16, p.7713_1 - 7713_8, 2025/08

 Times Cited Count:11 Percentile:84.88(Multidisciplinary Sciences)

Caloric effects usually occur in the vicinity of solid-state phase transitions with a limited refrigeration temperature span. Here, we introduce and realize an unprecedented concept -all temperature barocaloric effect, i.e., a remarkable barocaloric effect in KPF$$_6$$ across an exceptionally wide temperature span, from 77.5 to 300 K and potentially down to 4 K, covering typical room temperature, liquid nitrogen, liquid hydrogen, and liquid helium refrigeration regions. The directly measured barocaloric adiabatic temperature change reaches 12 K at room temperature and 2.5 K at 77.5 K upon the release of a 250 MPa pressure. This effect is attributed to a persistent phase transition to a rhombohedral high pressure phases. We depict the thermodynamic energy landscape to account for the structural instability. This unique all-temperature barocaloric effect presents a novel approach to highly applicable solid-state refrigeration technology, transcending the conventional multi-stage scenario.

Journal Articles

Stabilizing the unstable; Enhancing OER durability with 3$$d$$-orbital transition metal multielemental alloy nanoparticles by atomically dispersed 4$$d$$-orbital Pd for a 100-fold extended lifetime

Zhu, B.*; Huang, S.*; Seo, O.*; Cao, M.*; Matsumura, Daiju; Gu, H.*; Wu, D.*

Journal of the American Chemical Society, 147(13), p.11250 - 11256, 2025/02

 Times Cited Count:81 Percentile:99.62(Chemistry, Multidisciplinary)

Journal Articles

Strong low-energy rattling modes enabled liquid-like ultralow thermal conductivity in a well-ordered solid

Liu, P.-F.*; Li, X.*; Li, J.*; Zhu, J.*; Tong, Z.*; Kofu, Maiko*; Nirei, Masami; Xu, J.*; Yin, W.*; Wang, F.*; et al.

National Science Review, 11(12), p.nwae216_1 - nwae216_10, 2024/12

 Times Cited Count:33 Percentile:91.60(Multidisciplinary Sciences)

Journal Articles

Brightening triplet excitons enable high-performance white-light emission in organic small molecules via integrating n-$$pi^*/pi$$-$$pi^*$$ transitions

Yang, Q.*; Yang, X.*; Wang, Y.*; Fei, Y.*; Li, F.*; Zheng, H.*; Li, K.*; Han, Y.*; Hattori, Takanori; Zhu, P.*; et al.

Nature Communications (Internet), 15, p.7778_1 - 7778_9, 2024/09

 Times Cited Count:50 Percentile:94.52(Multidisciplinary Sciences)

Luminescent materials that simultaneously embody bright singlet and triplet excitons hold great potential in optoelectronics, signage, and information encryption. However, achieving high-performance white-light emission is severely hampered by their inherent unbalanced contribution of fluorescence and phosphorescence. Herein, we address this challenge by pressure treatment engineering via hydrogen bonding cooperativity effect to realize the mixture of n-$$pi^*/pi$$-$$pi^*$$ transitions, where the triplet state emission was boosted from 7% to 40% in isophthalic acid (IPA). A superior white-light emission based on hybrid fluorescence and phosphorescence was harvested in pressure-treated IPA, and the photoluminescence quantum yield was increased to 75% from the initial 19% (blue-light emission). In-situ high-pressure IR spectra, X ray diffraction, and neutron diffraction reveal continuous strengthening of the hydrogen bonds with the increase of pressure. Furthermore, this enhanced hydrogen bond is retained down to the ambient conditions after pressure treatment, awarding the targeted IPA efficient intersystem crossing for balanced singlet/triplet excitons population and resulting in efficient white-light emission. This work not only proposes a route for brightening triplet states in organic small molecule, but also regulates the ratio of singlet and triplet excitons to construct high-performance white-light emission.

Journal Articles

Antiferromagnetism and phase stability of CrMnFeCoNi high-entropy alloy

Zhu, L.*; He, H.*; Naeem, M.*; Sun, X.*; Qi, J.*; Liu, P.*; Harjo, S.; Nakajima, Kenji; Li, B.*; Wang, X.-L.*

Physical Review Letters, 133(12), p.126701_1 - 126701_6, 2024/09

 Times Cited Count:13 Percentile:83.28(Physics, Multidisciplinary)

Journal Articles

Low spin spectroscopy of neutron-rich $$^{43,44,45}$$Cl via $$beta^-$$ and $$beta n$$ decay

Tripathi, V.*; Bhattacharya, S.*; Rubino, E.*; Benetti, C.*; Perello, J. F.*; Tabor, S. L.*; Liddick, S. N.*; Bender, P. C.*; Carpenter, M. P.*; Carroll, J. J.*; et al.

Physical Review C, 109(4), p.044320_1 - 044320_15, 2024/04

 Times Cited Count:5 Percentile:67.88(Physics, Nuclear)

no abstracts in English

Journal Articles

Phase transformation and equation of state in Ti-45Al alloy under high pressure

Li, X.*; Zhu, R.*; Xin, J.*; Luo, M.*; Shang, S.-L.*; Liu, Z.-K.*; Yin, C.*; Funakoshi, Kenichi*; Dippenaar, R. J.*; Higo, Yuji*; et al.

CALPHAD; Computer Coupling of Phase Diagrams and Thermochemistry, 84, p.102641_1 - 102641_6, 2024/03

 Times Cited Count:0 Percentile:0.00(Thermodynamics)

Journal Articles

Chiral perturbation theory for heavy hadrons and chiral effective field theory for heavy hadronic molecules

Meng, L.*; Wang, B.*; Wang, G.-J.*; Zhu, S.-L.*

Physics Reports; A Review Section of Physics Letters, 1019, p.1 - 149, 2023/05

 Times Cited Count:243 Percentile:97.43(Physics, Multidisciplinary)

Journal Articles

$$beta^-$$ decay of exotic P and S isotopes with neutron number near 28

Tripathi, V.*; Bhattacharya, S.*; Rubino, E.*; Benetti, C.*; Perello, J. F.*; Tabor, S. L.*; Liddick, S. N.*; Bender, P. C.*; Carpenter, M. P.*; Carroll, J. J.*; et al.

Physical Review C, 106(6), p.064314_1 - 064314_14, 2022/12

 Times Cited Count:6 Percentile:53.58(Physics, Nuclear)

no abstracts in English

Journal Articles

Revisit the isospin violating decays of $$X$$(3872)

Meng, L.*; Wang, G.-J.*; Wang, B.*; Zhu, S.-L.*

Physical Review D, 104(9), p.094003_1 - 094003_8, 2021/11

 Times Cited Count:33 Percentile:83.22(Astronomy & Astrophysics)

The isospin violating decays of $$X(3872)$$ are revisited in a coupled-channel effective field theory. In a cutoff-independent formalism, we relate the coupling constants of $$X(3872)$$ with the two channels to the molecular wave function. The isospin violating decays of $$X(3872)$$ are obtained by two equivalent approaches, which amend some deficiencies about this issue in literature. In the quantum field theory approach, the isospin violating decays arise from the coupling constants of $$X(3872)$$ to two di-meson channels. In the quantum mechanics approach, the isospin violating is attributed to wave functions at the origin. We bridge the isospin violating decays of $$X(3872)$$ to its inner structure. Our results show that the proportion of the neutral channel in $$X(3872)$$ is over 80%. As a by-product, we find that the strong decay width and radiative decay width are about 30 keV and 10 keV, respectively, for the binding energy from -300 keV to -50 keV.

Journal Articles

Solving the puzzles of the decay of the heaviest known proton-emitting nucleus $$^{185}$$Bi

Doherty, D. T.*; Andreyev, A. N.; Seweryniak, D.*; Woods, P. J.*; Carpenter, M. P.*; Auranen, K.*; Ayangeakaa, A. D.*; Back, B. B.*; Bottoni, S.*; Canete, L.*; et al.

Physical Review Letters, 127(20), p.202501_1 - 202501_6, 2021/11

 Times Cited Count:17 Percentile:71.32(Physics, Multidisciplinary)

Journal Articles

Implications of the $$Z_{cs}$$(3985) and $$Z_{cs}$$(4000) as two different states

Meng, L.*; Wang, B.*; Wang, G.-J.*; Zhu, S.-L.*

Science Bulletin, 66(20), p.2065 - 2071, 2021/10

 Times Cited Count:33 Percentile:81.47(Multidisciplinary Sciences)

Two recently found tetraquark resonances $$Z_{cs}$$(3985) and $$Z_{cs}$$(4000) are studied in a solvable nonrelativistic effective field theory. We include the possible violations of heavy quark spin symmetry and SU(3) flavor symmetry in a comprehensive approach. Our results show that the decay rates can be used to judge whether these resonances can be different states or not.

Journal Articles

Probing the long-range structure of the $$T^{+}_{cc}$$ with the strong and electromagnetic decays

Meng, L.*; Wang, G.-J.*; Wang, B.*; Zhu, S.-L.*

Physical Review D, 104(5), p.L051502_1 - L051502_8, 2021/09

 Times Cited Count:109 Percentile:98.33(Astronomy & Astrophysics)

We investigate the kinetically allowed strong and electromagnetic decays of the recently observed $$T^+_{cc}$$. Our results show that the decay width of $$T_{cc}to D^0D^0pi^+$$ is the largest one, which is just the experimental observation channel. Our theoretical total strong and radiative widths are in favor of the $$T_{cc}$$ as a $$D^{*+}D^0$$ dominated bound state. Our calculation is cutoff-independent and without prior isospin assignment. The absolute partial widths and ratios of the different decay channels can be used to test the structure of $$T_{cc}$$ state when the updated experimental results are available.

Journal Articles

Ultra-fine CeO$$_{2}$$ particles triggered strong interaction with LaFeO$$_{3}$$ framework for total and preferential CO oxidation

Zheng, Y.*; Xiao, H.*; Li, K.*; Wang, Y.*; Li, Y.*; Wei, Y.*; Zhu, X.*; Li, H.-W.*; Matsumura, Daiju; Guo, B.*; et al.

ACS Applied Materials & Interfaces, 12(37), p.42274 - 42284, 2020/09

 Times Cited Count:34 Percentile:72.44(Nanoscience & Nanotechnology)

Journal Articles

Stability and synthesis of superheavy elements; Fighting the battle against fission - Example of $$^{254}$$No

Lopez-Martens, A.*; Henning, G.*; Khoo, T. L.*; Seweryniak, D.*; Alcorta, M.*; Asai, Masato; Back, B. B.*; Bertone, P. F.*; Boilley, D.*; Carpenter, M. P.*; et al.

EPJ Web of Conferences, 131, p.03001_1 - 03001_6, 2016/12

 Times Cited Count:1 Percentile:39.96(Chemistry, Inorganic & Nuclear)

Fission barrier height and its angular-momentum dependence have been measured for the first time in the nucleus with the atomic number greater than 100. The entry distribution method, which can determine the excitation energy at which fission starts to dominate the decay process, was applied to $$^{254}$$No. The fission barrier of $$^{254}$$No was found to be 6.6 MeV at zero spin, indicating that the $$^{254}$$No is strongly stabilized by the nuclear shell effects.

Journal Articles

Population and decay of a $$K^{pi}$$ = 8$$^{-}$$ two-quasineutron isomer in $$^{244}$$Pu

Hota, S.*; Tandel, S.*; Chowdhury, P.*; Ahmad, I.*; Carpenter, M. P.*; Chiara, C. J.*; Greene, J. P.*; Hoffman, C. R.*; Jackson, E. G.*; Janssens, R. V. F.*; et al.

Physical Review C, 94(2), p.021303_1 - 021303_5, 2016/08

 Times Cited Count:10 Percentile:54.33(Physics, Nuclear)

The decay of a $$K^{pi}$$ = 8$$^{-}$$ isomer in $$^{244}$$Pu and the collective band structure populating the isomer are studied using deep inelastic excitations with $$^{47}$$Ti and $$^{208}$$Pb beams, respectively. Precise measurements of $$M1/E2$$ branching ratios in the band confirm a clean 9/2$$^-$$[734]$$_{nu}$$$$otimes$$7/2$$^+$$[624]$$_{nu}$$ for the isomer, validating the systematics of K$$^{pi}$$ = 8$$^{-}$$ two-quasineutron isomers observed in even-$$Z$$, $$N$$ = 150 isotones. These isomers around the deformed shell gap at $$N$$ = 152 provide critical benchmarks for theoretical predictions of single-particle energies in this gateway region to superheavy nuclei.

Journal Articles

Identification of deformed intruder states in semi-magic $$^{70}$$Ni

Chiara, C. J.*; Weisshaar, D.*; Janssens, R. V. F.*; Tsunoda, Yusuke*; Otsuka, Takaharu*; Harker, J. L.*; Walters, W. B.*; Recchia, F.*; Albers, M.*; Alcorta, M.*; et al.

Physical Review C, 91(4), p.044309_1 - 044309_10, 2015/04

 Times Cited Count:42 Percentile:89.64(Physics, Nuclear)

The neutron-rich isotope $$^{70}$$Ni was produced by multi-nucleon transfer reactions of $$^{70}$$Zn in the Argonne National Laboratory, and an in-beam $$gamma$$-ray experiment were performed using the GRETINA array. The $$2^+_2$$ and $$4^+_2$$ levels of $$^{70}$$Ni were observed for the first time. Those levels are regarded as large deformed states associated with proton excitation from the $$f_{7/2}$$ orbit because they cannot be reproduced by a shell-model calculation assuming a small valence space without $$f_{7/2}$$. A theoretical analysis based on the Monte Carlo shell model published in 2014 indicates that those levels corresponds to a prolate deformed band. The present result demonstrates the occurrence of shape coexistence in neutron-rich Ni isotopes other than a known case of $$^{68}$$Ni, and confirms the predictive power of the Monte Carlo shell-model calculation.

Journal Articles

Fission barrier of superheavy nuclei and persistence of shell effects at high spin; Cases of $$^{254}$$No and $$^{220}$$Th

Henning, G.*; Khoo, T. L.*; Lopez-Martens, A.*; Seweryniak, D.*; Alcorta, M.*; Asai, Masato; Back, B. B.*; Bertone, P. F.*; Boilley, D.*; Carpenter, M. P.*; et al.

Physical Review Letters, 113(26), p.262505_1 - 262505_6, 2014/12

 Times Cited Count:35 Percentile:80.95(Physics, Multidisciplinary)

Fission barrier heights of a shell-stabilized superheavy nucleus $$^{254}$$No have been determined as a function of spin up to 19$$hbar$$ through the measured distribution of entry points of $$gamma$$ deexcitations in the excitation energy vs. spin plane. The fission barrier height of $$^{254}$$No was determined to be 6.0 MeV at spin 15$$hbar$$, and 6.6 MeV at spin 0$$hbar$$ by extrapolation. This demonstrates that the shell effect actually enlarges the fission barrier in such heavy nuclei and keeps the barrier high even at high spin.

Journal Articles

Exploring the stability of super heavy elements; First measurement of the fission barrier of $$^{254}$$No

Henning, G.*; Lopez-Martens, A.*; Khoo, T. L.*; Seweryniak, D.*; Alcorta, M.*; Asai, Masato; Back, B. B.*; Bertone, P. F.*; Boilley, D.*; Carpenter, M. P.*; et al.

EPJ Web of Conferences, 66, p.02046_1 - 02046_8, 2014/03

 Times Cited Count:3 Percentile:66.32(Physics, Nuclear)

Fission barrier heights of $$^{254}$$No have been determined through the entry distribution method. The entry distribution is the initial distribution of excitation energy and spin from which the $$gamma$$ deexcitation starts in the fusion-evaporation reaction. The initial distribution is extracted from measured $$gamma$$-ray multiplicity and total $$gamma$$-ray energy. This paper describes the details of the entry distribution method, and reports the first determination of the fission barrier heights of $$^{254}$$No, which is the heaviest nucleus whose fission barrier has been measured.

Journal Articles

Diluted ferromagnetic semiconductor Li(Zn,Mn)P with decoupled charge and spin doping

Deng, Z.*; Zhao, K.*; Gu, B.; Han, W.*; Zhu, J. L.*; Wang, X. C.*; Li, X.*; Liu, Q. Q.*; Yu, R. C.*; Goko, Tatsuo*; et al.

Physical Review B, 88(8), p.081203_1 - 081203_5, 2013/08

 Times Cited Count:82 Percentile:91.78(Materials Science, Multidisciplinary)

36 (Records 1-20 displayed on this page)