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Liu, P.-F.*; Li, X.*; Li, J.*; Zhu, J.*; Tong, Z.*; Kofu, Maiko*; Nirei, Masami; Xu, J.*; Yin, W.*; Wang, F.*; et al.
National Science Review, 11(12), p.nwae216_1 - nwae216_10, 2024/12
Times Cited Count：12 Percentile：91.22(Multidisciplinary Sciences)
-
transitionsYang, Q.*; Yang, X.*; Wang, Y.*; Fei, Y.*; Li, F.*; Zheng, H.*; Li, K.*; Han, Y.*; Hattori, Takanori; Zhu, P.*; et al.
Nature Communications (Internet), 15, p.7778_1 - 7778_9, 2024/09
Times Cited Count：9 Percentile：88.46(Multidisciplinary Sciences)Luminescent materials that simultaneously embody bright singlet and triplet excitons hold great potential in optoelectronics, signage, and information encryption. However, achieving high-performance white-light emission is severely hampered by their inherent unbalanced contribution of fluorescence and phosphorescence. Herein, we address this challenge by pressure treatment engineering via hydrogen bonding cooperativity effect to realize the mixture of n-- transitions, where the triplet state emission was boosted from 7% to 40% in isophthalic acid (IPA). A superior white-light emission based on hybrid fluorescence and phosphorescence was harvested in pressure-treated IPA, and the photoluminescence quantum yield was increased to 75% from the initial 19% (blue-light emission). In-situ high-pressure IR spectra, X ray diffraction, and neutron diffraction reveal continuous strengthening of the hydrogen bonds with the increase of pressure. Furthermore, this enhanced hydrogen bond is retained down to the ambient conditions after pressure treatment, awarding the targeted IPA efficient intersystem crossing for balanced singlet/triplet excitons population and resulting in efficient white-light emission. This work not only proposes a route for brightening triplet states in organic small molecule, but also regulates the ratio of singlet and triplet excitons to construct high-performance white-light emission.
Zhu, L.*; He, H.*; Naeem, M.*; Sun, X.*; Qi, J.*; Liu, P.*; Harjo, S.; Nakajima, Kenji; Li, B.*; Wang, X.-L.*
Physical Review Letters, 133(12), p.126701_1 - 126701_6, 2024/09
Times Cited Count：1 Percentile：48.32(Physics, Multidisciplinary)
Cl via 
and 
decayTripathi, V.*; Bhattacharya, S.*; Rubino, E.*; Benetti, C.*; Perello, J. F.*; Tabor, S. L.*; Liddick, S. N.*; Bender, P. C.*; Carpenter, M. P.*; Carroll, J. J.*; et al.
Physical Review C, 109(4), p.044320_1 - 044320_15, 2024/04
Times Cited Count：0 Percentile：0.00(Physics, Nuclear)no abstracts in English
-MgAgSbLi, J.*; Li, X.*; Zhang, Y.*; Zhu, J.*; Zhao, E.*; Kofu, Maiko; Nakajima, Kenji; Avdeev, M.*; Liu, P.-F.*; Sui, J.*; et al.
Applied Physics Reviews (Internet), 11(1), p.011406_1 - 011406_8, 2024/03
Times Cited Count：7 Percentile：91.57(Physics, Applied) decay of exotic P and S isotopes with neutron number near 28Tripathi, V.*; Bhattacharya, S.*; Rubino, E.*; Benetti, C.*; Perello, J. F.*; Tabor, S. L.*; Liddick, S. N.*; Bender, P. C.*; Carpenter, M. P.*; Carroll, J. J.*; et al.
Physical Review C, 106(6), p.064314_1 - 064314_14, 2022/12
Times Cited Count：4 Percentile：53.47(Physics, Nuclear)no abstracts in English
BiDoherty, D. T.*; Andreyev, A. N.; Seweryniak, D.*; Woods, P. J.*; Carpenter, M. P.*; Auranen, K.*; Ayangeakaa, A. D.*; Back, B. B.*; Bottoni, S.*; Canete, L.*; et al.
Physical Review Letters, 127(20), p.202501_1 - 202501_6, 2021/11
Times Cited Count：10 Percentile：64.86(Physics, Multidisciplinary)
; 
In NQR/NMR and 
Co NMR studySakai, Hironori; Tokunaga, Yo; Kambe, Shinsaku; Zhu, J.-X.*; Ronning, F.*; Thompson, J. D.*; Ramakrishna, S. K.*; Reyes, A. P.*; Suzuki, Kohei*; Oshima, Yoshiki*; et al.
Physical Review B, 104(8), p.085106_1 - 085106_12, 2021/08
Times Cited Count：5 Percentile：30.79(Materials Science, Multidisciplinary)Antiferromagnetism in a prototypical quantum critical metal CeCoIn is known to be induced by slight substitutions of non-magnetic Zn atoms for In. In nominally 7% Zn substituted CeCoIn, an antiferromagnetic (AFM) state coexists with heavy fermion superconductivity. Heterogeneity of the electronic states is investigated in Zn doped CeCoIn by means of nuclear quadrupole and magnetic resonances (NQR and NMR). Site-dependent NQR relaxation rates 
indicate that the AFM state is locally nucleated around Zn substituents in the matrix of a heavy fermion state, and percolates through the bulk at the AFM transition temperature 
. At lower temperatures, an anisotropic superconducting (SC) gap below the SC transition temperature 
, and the SC state permeates through the AFM regions via a SC proximity effect. Applying an external magnetic field induces a spin-flop transition near 5 T, reducing the volume of the AFM regions. Consequently, a short ranged inhomogeneous AFM state survives and coexists with a paramagnetic Fermi liquid state at high fields.
Pu nuclear magnetic resonance in the candidate topological insulator PuB
Dioguardi, A. P.*; Yasuoka, Hiroshi*; Thomas, S. M.*; Sakai, Hironori; Cary, S. K.*; Kozimor, S. A.*; Albrecht-Schmitt, T. E.*; Choi, H. C.*; Zhu, J.-X.*; Thompson, J. D.*; et al.
Physical Review B, 99(3), p.035104_1 - 035104_6, 2019/01
Times Cited Count：10 Percentile：42.76(Materials Science, Multidisciplinary)We present a detailed nuclear magnetic resonance (NMR) study of Pu in bulk and powdered single-crystal plutonium tetraboride (PuB), which has recently been investigated as a potential correlated topological insulator. The Pu NMR spectra are consistent with axial symmetry of the shift tensor showing for the first time that Pu NMR can be observed in an anisotropic environment and up to room temperature. The temperature dependence of the Pu shift, combined with a relatively long spin-lattice relaxation time (
), indicate that PuB adopts a nonmagnetic state with gaplike behavior consistent with our density functional theory calculations. The temperature dependencies of the NMR Knight shift and 
imply bulk gaplike behavior confirming that PuB is a good candidate topological insulator.
NoLopez-Martens, A.*; Henning, G.*; Khoo, T. L.*; Seweryniak, D.*; Alcorta, M.*; Asai, Masato; Back, B. B.*; Bertone, P. F.*; Boilley, D.*; Carpenter, M. P.*; et al.
EPJ Web of Conferences, 131, p.03001_1 - 03001_6, 2016/12
Times Cited Count：1 Percentile：42.06(Chemistry, Inorganic & Nuclear)Fission barrier height and its angular-momentum dependence have been measured for the first time in the nucleus with the atomic number greater than 100. The entry distribution method, which can determine the excitation energy at which fission starts to dominate the decay process, was applied to No. The fission barrier of No was found to be 6.6 MeV at zero spin, indicating that the No is strongly stabilized by the nuclear shell effects.
= 8
two-quasineutron isomer in 
PuHota, S.*; Tandel, S.*; Chowdhury, P.*; Ahmad, I.*; Carpenter, M. P.*; Chiara, C. J.*; Greene, J. P.*; Hoffman, C. R.*; Jackson, E. G.*; Janssens, R. V. F.*; et al.
Physical Review C, 94(2), p.021303_1 - 021303_5, 2016/08
Times Cited Count：9 Percentile：54.19(Physics, Nuclear)The decay of a = 8 isomer in Pu and the collective band structure populating the isomer are studied using deep inelastic excitations with 
Ti and 
Pb beams, respectively. Precise measurements of 
branching ratios in the band confirm a clean 9/2
[734]
7/2
[624] for the isomer, validating the systematics of K
= 8 two-quasineutron isomers observed in even-
, 
= 150 isotones. These isomers around the deformed shell gap at = 152 provide critical benchmarks for theoretical predictions of single-particle energies in this gateway region to superheavy nuclei.
NiChiara, C. J.*; Weisshaar, D.*; Janssens, R. V. F.*; Tsunoda, Yusuke*; Otsuka, Takaharu*; Harker, J. L.*; Walters, W. B.*; Recchia, F.*; Albers, M.*; Alcorta, M.*; et al.
Physical Review C, 91(4), p.044309_1 - 044309_10, 2015/04
Times Cited Count：40 Percentile：90.80(Physics, Nuclear)The neutron-rich isotope Ni was produced by multi-nucleon transfer reactions of Zn in the Argonne National Laboratory, and an in-beam 
-ray experiment were performed using the GRETINA array. The 
and 
levels of Ni were observed for the first time. Those levels are regarded as large deformed states associated with proton excitation from the 
orbit because they cannot be reproduced by a shell-model calculation assuming a small valence space without . A theoretical analysis based on the Monte Carlo shell model published in 2014 indicates that those levels corresponds to a prolate deformed band. The present result demonstrates the occurrence of shape coexistence in neutron-rich Ni isotopes other than a known case of 
Ni, and confirms the predictive power of the Monte Carlo shell-model calculation.
No and 
ThHenning, G.*; Khoo, T. L.*; Lopez-Martens, A.*; Seweryniak, D.*; Alcorta, M.*; Asai, Masato; Back, B. B.*; Bertone, P. F.*; Boilley, D.*; Carpenter, M. P.*; et al.
Physical Review Letters, 113(26), p.262505_1 - 262505_6, 2014/12
Times Cited Count：34 Percentile：81.81(Physics, Multidisciplinary)Fission barrier heights of a shell-stabilized superheavy nucleus No have been determined as a function of spin up to 19
through the measured distribution of entry points of deexcitations in the excitation energy vs. spin plane. The fission barrier height of No was determined to be 6.0 MeV at spin 15, and 6.6 MeV at spin 0 by extrapolation. This demonstrates that the shell effect actually enlarges the fission barrier in such heavy nuclei and keeps the barrier high even at high spin.
NoHenning, G.*; Lopez-Martens, A.*; Khoo, T. L.*; Seweryniak, D.*; Alcorta, M.*; Asai, Masato; Back, B. B.*; Bertone, P. F.*; Boilley, D.*; Carpenter, M. P.*; et al.
EPJ Web of Conferences, 66, p.02046_1 - 02046_8, 2014/03
Times Cited Count：3 Percentile：68.16(Physics, Nuclear)Fission barrier heights of No have been determined through the entry distribution method. The entry distribution is the initial distribution of excitation energy and spin from which the deexcitation starts in the fusion-evaporation reaction. The initial distribution is extracted from measured -ray multiplicity and total -ray energy. This paper describes the details of the entry distribution method, and reports the first determination of the fission barrier heights of No, which is the heaviest nucleus whose fission barrier has been measured.
GeToh, Yosuke; Chiara, C. J.*; McCutchan, E. A.*; Walters, W. B.*; Janssens, R. V. F.*; Carpenter, M. P.*; Zhu, S.*; Broda, R.*; Fornal, B.*; Kay, B. P.*; et al.
Physical Review C, 87(4), p.041304_1 - 041304_5, 2013/04
Times Cited Count：92 Percentile：97.13(Physics, Nuclear)Excited states of Ge have been investigated via the Ge + 
U reaction with 
Ge
MeV by use of in-beam -ray spectroscopy using the sphere array. The band was extended considerably and one new band was identified. Comparisons of the band with collective- and shell-model calculations suggest that Ge may be a rare example of a nucleus exhibiting rigid triaxial deformation in the low-lying states.
PBender, P. C.*; Tabor, S. L.*; Tripathi, V.*; Hoffman, C. R.*; Hamilton, L.*; Volya, A.*; Clark, R. M.*; Fallon, P.*; Macchiavelli, A. O.*; Paschalis, S.*; et al.
Physical Review C, 85(4), p.044305_1 - 044305_10, 2012/04
Times Cited Count：12 Percentile：54.66(Physics, Nuclear)The available experimental information on P has been greatly increased through the analysis of decays in coincidence with protons from the interaction of an 
O beam at 24 MeV with an O target. Light charged particles from the reaction were detected with Microball, and multiple ray coincidences with Gammasphere. Many newly observed transitions have been identified and placed in the level scheme. Additionally, for most states, spins have been assigned based on measured ray angular distributions while parities were inferred from lifetimes determined through Doppler-broadened line-shape analysis. Most of the states observed have been interpreted in terms of shell-model calculations using the WBP-a and SDPF-NR interactions having one particle in the 0
or 1
orbital. The two calculations agree almost equally well with the data resulting in root-mean-square differences of about 200 keV. However, two of a few high-lying states may be associated with stretched 
states, but the calculations over-predict their energies by 2-3 MeV. Furthermore, a newly observed long-lived 7919-keV state is established for which no explanation is available at present.
Schaffer, M. J.*; Snipes, J. A.*; Gohil, P.*; de Vries, P.*; Evans, T. E.*; Fenstermacher, M. E.*; Gao, X.*; Garofalo, A. M.*; Gates, D. A.*; Greenfield, C. M.*; et al.
Nuclear Fusion, 51(10), p.103028_1 - 103028_11, 2011/10
Times Cited Count：42 Percentile：81.84(Physics, Fluids & Plasmas)Experiments at DIII-D investigated the effects of ferromagnetic error fields similar to those expected from proposed ITER Test Blanket Modules (TBMs). Studied were effects on: plasma rotation and locking; confinement; L-H transition; edge localized mode (ELM) suppression by resonant magnetic perturbations; ELMs and the H-mode pedestal; energetic particle losses; and more. The experiments used a 3-coil mock-up of 2 magnetized ITER TBMs in one ITER equatorial port. The experiments did not reveal any effect likely to preclude ITER operations with a TBM-like error field. The largest effect was slowed plasma toroidal rotation v across the entire radial profile by as much as 
via non-resonant braking. Changes to global 
, 
and 
were 
3 times smaller. These effects are stronger at higher 
and lower 
. Other effects were smaller.
isomer in 
RfRobinson, A. P.*; Khoo, T. L.*; Seweryniak, D.*; Ahmad, I.*; Asai, Masato; Back, B. B.*; Carpenter, M. P.*; Chowdhury, P.*; Davids, C. N.*; Greene, J.*; et al.
Physical Review C, 83(6), p.064311_1 - 064311_7, 2011/06
Times Cited Count：35 Percentile：85.00(Physics, Nuclear)We have identified an isomer with a half-life of 17 
s in Rf through a calorimetric conversion electron measurement tagged with implanted Rf nuclei using the fragment mass analyzer at Argonne National Laboratory. The low population yield for this isomer suggests that this isomer should not be a 2-quasiparticle high- isomer which is typically observed in the N = 152 isotones, but should be a 4-quasiparticle one. Possible reasons of the non-observation of a 2-quasiparticle isomer are this isomer decays by fission with a half-life similar to that of the ground state of Rf. Another possibility, that there is no 2-quasiparticle isomer at all, would imply an abrupt termination of axially symmetric deformed shape at Z=104.
MgDaecon, A. N.*; Smith, J. F.*; Freeman, S. J.*; Janssens, R. V. F.*; Carpenter, M. P.*; Hadinia, B.*; Hoffman, C. R.*; Kay, B. P.*; Lauritsen, T.*; Lister, C. J.*; et al.
Physical Review C, 82(3), p.034305_1 - 034305_7, 2010/09
Times Cited Count：24 Percentile：77.04(Physics, Nuclear)no abstracts in English
Seweryniak, D.*; Khoo, T. L.*; Ahmad, I.*; Kondev, F. G.*; Robinson, A.*; Tandel, S. K.*; Asai, Masato; Back, B. B.*; Carpenter, M. P.*; Chowdhury, P.*; et al.
Nuclear Physics A, 834(1-4), p.357c - 361c, 2010/03
Times Cited Count：8 Percentile：46.62(Physics, Nuclear)Experimental data on single-particle energies in nuclei around Z=100 and N=152 play an important role to test validity of theoretical predictions for shell structure of superheavy nuclei. We found high-K two-quasiparticle isomers in 
No and No, and evaluated energies of proton single-particle orbitals around Z=100. We also found a new high-K three quasiparticle isomer in 
Rf. Energies of neutron single-particle orbitals were also evaluated from experimental data of the decay of Rf. Comparisons between the present experimental data and various theoretical calculations for the proton single-particle orbitals indicate that the calculation by using the Woods-Saxon potential gives the best agreement with the data.
