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Journal Articles

Unveiling the effects of Mn, Cr, Al, and Si on the low-temperature tempering behaviors of high-carbon martensite

Zhang, Y.*; Marusawa, Kenji*; Kudo, Kohei*; Morooka, Satoshi; Gong, W.; Harjo, S.; Miyamoto, Goro*; Furuhara, Tadashi*

Journal of Materials Science & Technology, 275, p.250 - 259, 2026/12

Journal Articles

Applicability of instrumented indentation for assessing allowable flaw sizes of circumferentially flawed stainless steel piping

Ha, Yoosung; Negyesi, M.*; Hasegawa, Kunio; Lacroix, V.*

Journal of Nondestructive Evaluation, Diagnostics and Prognostics of Engineering Systems, 9(3), p.031001_1 - 031001_6, 2026/08

Journal Articles

Fundamental consideration of maximum allowable flaw lengths for limit load evaluation based on flat plates for the ASME Code Section XI

Negyesi, M.*; Hasegawa, Kunio

Journal of Pressure Vessel Technology, 148(4), p.044501_1 - 044501_4, 2026/08

Journal Articles

Cold sintering of whitlockite-based phosphate ceramics for ALPS carbonate slurry waste immobilization

Gubarevich, A.*; Kubo, Ryotaro*; Arisaka, Makoto; Osugi, Takeshi; Yoshida, Katsumi*; Takeshita, Kenji*

Journal of Nuclear Science and Technology, 63(6), p.667 - 676, 2026/06

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

To immobilize and solidify carbonate-based Advanced Liquid Processing System (ALPS) sediment wastes, this study introduces a chemical transformation process that converts these wastes into calcium and magnesium phosphate phases, followed by densification using a novel cold sintering press (CSP) technique. Simulated calcium-magnesium carbonate slurries were treated with phosphoric acid to synthesize calcium and magnesium phosphates, which were then sintered at 300-500$$^{circ}$$C using CSP. The effects of the calcium-to-magnesium ratio, strontium incorporation, and sodium chloride addition on phase composition and CSP densification were investigated. Dense bulk samples were successfully fabricated and characterized using X-ray diffraction, scanning electron microscopy, energy-dispersive X-ray spectroscopy, and the Archimedes method. The results showed that the chemical transformation process led to the formation of whitlockite and newberyite, with the calcium-to-magnesium ratio determining the relative proportions of these phases. Strontium was effectively incorporated into the whitlockite crystal structure, while newberyite enhanced densification through a dehydration-driven process. Sodium chloride had no effect on chemical transformation and was not found in the final solid product. These results show that direct conversion of calcium-magnesium carbonate slurries to whitlockite-based phosphate ceramics, followed by CSP, enables stable solidification, making this method promising for ALPS sediment waste management.

Journal Articles

Water-leaching behavior for cesium chemisorbed on stainless steel at room temperature

Nakajima, Kunihisa; Imoto, Jumpei*; Nishioka, Shunichiro*; Osaka, Masahiko; Miwa, Shuhei

Journal of Nuclear Science and Technology, 63(6), p.727 - 736, 2026/06

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

Water-leaching tests at 303 K were performed on cesium (Cs) chemisorbed on stainless steels to investigate its long-term dissolution behavior. The findings showed that Cs continued to dissolve into water even after 1200 hours and that Cs was found to coexist with silicon as ring-shaped particles. This indicates that even water-insoluble Cs, which is defined in the Cs-chemisorption models incorporated into existing SA analysis codes, can dissolve in water over extended periods, with the dissolution attributed to the ring-shaped Cs silicate particles. Additionally, these water-leaching behaviors were accurately described by the Noyes-Whitney equation, suggesting the potential development of a water-dissolution model for the water-insoluble Cs in the chemisorption models. These insights imply that long-term redistributions of chemisorbed Cs could occur within the reactor pressure vessels in Fukushima Daiichi Nuclear Power Station, necessitating a water-dissolution model to predict redistributions through the aqueous phase.

Journal Articles

Measurements of neutron capture cross-sections for nuclides of interest in decommissioning (V); $$^{94}$$Zr(n, $$gamma$$)$$^{95}$$Zr and $$^{96}$$Zr(n, $$gamma$$)$$^{97}$$Zr reactions at JRR-3

Nakamura, Shoji; Kimura, Atsushi; Endo, Shunsuke; Rovira Leveroni, G.; Shibahara, Yuji*

Journal of Nuclear Science and Technology, 63(6), p.653 - 666, 2026/06

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

Journal Articles

Hot zone formation in combustion tests simulating solvent fires in reprocessing plants; Concerns on boilover phenomenon

Ono, Takuya; Tashiro, Shinsuke; Amano, Yuki; Yoshida, Naoki; Yoshida, Ryoichiro; Yamane, Yuichi

Journal of Nuclear Science and Technology, 63(6), p.603 - 611, 2026/06

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

This paper reports the first case of hot zone formation in a combustion test simulating an organic solvent fire in a reprocessing plant. Our goal is to add a boilover component to a computational model for quantitatively predicting the accident progression of the fire. Although the scale of boilover combustion increases when hot zones are formed in the solvent, it has not been clarified whether or not a hot zone is formed in the combustion of a 30 percent tributyl phosphate (TBP)/dodecane solvent mixture. To clarify this point, we conducted beaker-scale combustion tests and measured the temperature distribution in the burning solvent with thermocouples to obtain the following results. (1) No hot zone was formed by the combustion of only dodecane. (2) In the combustion of TBP/dodecane, hot zones were not formed as long as dodecane remained in the solvent. (3) A hot zone was formed when only TBP was burned.

Journal Articles

Bayesian approach to model temperature dependence of Charpy absorbed energy and uncertainty evaluation of ductile-to-brittle transition temperature for reactor pressure vessel steel

Takamizawa, Hisashi; Nishiyama, Yutaka

Journal of Pressure Vessel Technology, 148(3), p.031501_1 - 031502_12, 2026/06

Embrittlement of reactor pressure vessel (RPV) steel caused by neutron irradiation has been evaluated using ductile-to-brittle transition temperature (DBTT) derived from surveillance tests (Charpy impact tests) during plant operation. For reliable structural integrity assessment of the RPV, incorporating adequate safety margins which take into account uncertainties inherent in surveillance Charpy impact tests is needed. In this study, a model to evaluate temperature dependence of Charpy absorbed energy variability using approximately 1,900 datasets of unirradiated and irradiated materials manufactured in Japan and United States was developed. Next, probability distribution of Charpy ductile-to-brittle transition temperature at a 41J energy level ($$T$$$$_{rm 41J}$$) was evaluated by estimating the probability distribution of Charpy test data using Monte Carlo sampling and Bayesian inference. From the detailed evaluation of the relationship between the number of specimens and $$T$$$$_{rm 41J}$$ uncertainty, uncertainty of $$T$$$$_{rm 41J}$$ was found to be almost the same in materials manufactured in Japan and U.S., and unchanged with neutron irradiation (no clear change in material inhomogeneity). Regarding product form on the other hand, uncertainty of $$T$$$$_{rm 41J}$$ for base metal and weld metal was almost the same, but the heat affected zone was shown to have large uncertainty.

Journal Articles

JENDL photonuclear data file 2016 revision 1

Iwamoto, Nobuyuki

Journal of Nuclear Science and Technology, 63(5), p.581 - 593, 2026/05

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

Journal Articles

Accurate measurement of the $$^{129}$$I neutron capture cross-section in the keV neutron region

Rovira Leveroni, G.; Kimura, Atsushi; Nakamura, Shoji; Endo, Shunsuke; Iwamoto, Osamu; Iwamoto, Nobuyuki; Katabuchi, Tatsuya*

Journal of Nuclear Science and Technology, 63(4), p.358 - 369, 2026/04

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

Journal Articles

Performance evaluation for rapid-dose estimation of radioactive plume dispersion based on pre-simulation database of wind conditions by large-eddy simulation

Sato, Takuto; Nakayama, Hiromasa; Satoh, Daiki

Journal of Nuclear Science and Technology, 63(4), p.426 - 442, 2026/04

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

We developed a framework for rapid monitoring of radioactive plumes in the vicinity of nuclear facilities based on a quick and practical high-resolution atmospheric dispersion simulation method that combines a large-eddy simulation (LES) model pre-simulation database (pre-sim DB) of wind conditions and onsite meteorological observation results, as proposed by the previous study. However, this framework was not quantitatively demonstrated using measurement data. In this study, we evaluated the performance of the wind condition reproduction and plume dispersion analysis methods. Air dose rates observed at monitoring posts around the stack were compared with the values reproduced by the method using the pre-sim DB, and the reproducibility of both air dose rate and flow field was discussed. The pre-sim DB-based method successfully captured the temporal variation of air dose rates at the monitoring posts, though it tended to overestimate the peak values. Particularly when the vertical wind shear was pronounced, the method using the pre-sim DB could cause significant errors. This is likely because the method relies on wind conditions from a single observation point, which inherently limits its ability to represent vertical wind shear within the pre-sim DB. Despite these limitations, particularly in reproducing complex wind fields, the method utilizing the pre-sim DB offers a valuable and practical tool for rapid dose rate simulation due to its lower computational cost compared to unsteady simulations using an LES model.

Journal Articles

Simple technique for the preparation of uranium-impregnated porous silica particles and their application as working standard particles for analysis of the safeguards environmental samples

Tomita, Jumpei; Tomita, Ryohei; Suzuki, Daisuke; Yasuda, Kenichiro; Miyamoto, Yutaka

Journal of Nuclear Science and Technology, 63(4), p.443 - 454, 2026/04

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

Journal Articles

Development of Internal Dose Calculation Code (IDCC)

Manabe, Kentaro; Murota, Shuhei; Takahashi, Fumiaki

Journal of Nuclear Science and Technology, 63(4), p.477 - 486, 2026/04

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

We have developed an internal dose assessment code (IDCC) based on the latest dose assessment methods in accordance with the ICRP 2007 Recommendations. This code enables calculation of effective dose coefficients and intake estimation from individual monitoring results for all radioactive nuclides including short-lived nuclides. The validity of the code has been confirmed through comparisons with the dose coefficient database published by the ICRP and multiple literature examples. We plan to enhance the code for evaluating public exposure, and it is expected to contribute to the revision of regulatory standards for radiation protection and serve as a practical dose assessment tool based on new standards.

Journal Articles

Analysis of the effect of crack curvature in Mini-C(T) specimen on fracture toughness evaluation

Shimodaira, Masaki; Ha, Yoosung; Takamizawa, Hisashi; Katsuyama, Jinya; Onizawa, Kunio

Journal of Pressure Vessel Technology, 148(2), p.021504_1 - 021504_10, 2026/04

 Times Cited Count:0 Percentile:0.00

In the current structural integrity assessment of the reactor pressure vessel, the accurate reference temperature (T$$_{o}$$) based on the Master Curve method is necessary. The T$$_{o}$$ can be estimated by using the Mini-C(T) fracture toughness specimen in accordance with ASTM E1921 and JEAC4216, which prescribe the crack straightness criteria. A requirement in ASTM E1921 has been revised in a decade to increase the accuracy and reasonability, and the applicable crack curvature has been varied by applied codes. The crack curvature of the Mini-C(T) specimen might have an impact on the T$$_{o}$$ because of the variation of the plastic constraint. In this work, the effect of the crack curvature on the fracture toughness (K$$_{Jc}$$) evaluation using the Mini-C(T) specimen was quantitatively evaluated by using the finite element analysis (FEA) including the Weibull stress analysis, to discuss the difference in a requirement of the crack straightness in ASTM E1921 and JEAC4216. FEAs showed a possibility that the upper limit curvature would decrease the plastic constraint, and consequently obtain higher K$$_{Jc}$$ in the Mini-C(T) specimen. Furthermore, if the upper limit curvature according to the ASTM E1921-21 was allowed, the T$$_{o}$$ would be estimated as nonconservative based on the Weibull stress analysis. In contrast, the difference in (T$$_{o}$$) between the crack with upper limit curvature according to JEAC4216 and the ideal straight crack was not significant.

Journal Articles

Temperature effect on radiolytically generated hydrogen yield from a plutonium nitric acid aqueous solution

Toigawa, Tomohiro; Hotoku, Shinobu; Kumagai, Yuta; Abe, Yuma*; Oyama, Kanichi*; Fukaya, Hiroyuki; Ban, Yasutoshi; Kida, Takashi; Hasegawa, Satoshi*; Nakano, Masanao*; et al.

Journal of Nuclear Science and Technology, 63(3), p.322 - 327, 2026/03

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

The effect of temperature on hydrogen production generated from radiolysis was investigated to determine the associated implications for nuclear fuel reprocessing safety. The hydrogen yield from radiolysis of plutonium nitric acid solution was measured at temperatures up to the boiling temperature of the solution. The results showed no notable temperature dependence even under boiling conditions. The impact of solution agitation on hydrogen production was also assessed, which revealed minor differences in the hydrogen yield between static and agitated conditions at room temperature. These findings suggest that high temperatures or boiling the solution do not considerably enhance hydrogen generation, and provide crucial information for accurately modeling hydrogen risks under severe accidents.

Journal Articles

Burnup calculation using POD-based neutron spectrum reconstruction

Watanabe, Tomoaki; Aizawa, Naoto*; Chiba, Go*; Tada, Kenichi; Fujita, Tatsuya*; Yamamoto, Akio*

Journal of Nuclear Science and Technology, 63(2), p.166 - 186, 2026/02

 Times Cited Count:1 Percentile:59.09(Nuclear Science & Technology)

A fast burnup calculation method based on neutron spectrum reconstruction is proposed. The method employs a reduced-order model (ROM), constructed using proper orthogonal decomposition (POD) and regression models, to estimate neutron spectra experienced by fuel during burnup. The ROM is built from snapshot data generated through detailed burnup and neutron transport simulations under various conditions. During burnup calculations, the ROM is used to rapidly reconstruct neutron spectra at each burnup step. These reconstructed spectra are then used to compute one-group cross sections from multi-group effective cross sections derived using background cross sections. The proposed method significantly reduces computational time by avoiding repeated neutron transport simulations. Its performance is demonstrated using a PWR UO$$_{2}$$ fuel pin model. Results show that, with the 6th-order POD, the method predicts nuclide inventories with an average error within $$pm$$5% compared to reference Monte Carlo calculations. Error analysis indicates that prediction accuracy is primarily limited by the regression models, rather than by the POD truncation or the multi-group cross section calculations.

Journal Articles

Sub-pin level distribution tallies and statistical error estimation with POD tallies in two-dimensional C5G7 benchmark

Kondo, Ryoichi; Yamamoto, Akio*; Endo, Tomohiro*

Journal of Nuclear Science and Technology, 63(2), p.142 - 153, 2026/02

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

The flux distribution tallies using proper orthogonal decomposition, called POD tallies, have been developed to address issues of high-fidelity Monte Carlo simulations. The POD tallies can reduce both dimensionality and statistical error. The present study verifies the applicability of the POD tallies to sub-pin level flux distribution in the two-dimensional C5G7 benchmark. Statistical error estimation is also proposed by applying the circular block bootstrap method to the POD tallies to estimate the statistical error of the flux distribution in a single Monte Carlo calculation. In the verification, the dimensionality of the finely discretized distribution is reduced by more than 90% compared with conventional cell tallies. The statistical error is reduced by more than half as the average value of all tally regions. The proposed approach is confirmed to properly estimate the statistical error of flux distribution considering both the inter-cycle correlation and the correlation between the expansion coefficients of different POD orders.

Journal Articles

Experimental measurements for the first series of the modified STACY critical assembly with simple core configurations and experimental analysis using simplified computational models

Gunji, Satoshi; Araki, Shohei; Yoshikawa, Tomoki

Journal of Nuclear Science and Technology, 63(2), p.207 - 215, 2026/02

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

Journal Articles

Study on criticality uncertainties of MCCI products due to concrete compositions

Gunji, Satoshi; Araki, Shohei

Journal of Nuclear Science and Technology, 63(2), p.187 - 199, 2026/02

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

Journal Articles

Feasibility study on the production of $$^{229}$$Th as a long-life $$^{225}$$Ac generator using the experimental fast reactor Joyo

Sasaki, Yuto; Maeda, Shigetaka; Fukasawa, Tetsuo*; Takaki, Naoyuki*

Journal of Nuclear Science and Technology, 63(2), p.154 - 165, 2026/02

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

In recent years, targeted alpha therapy, which utilizes $$^{225}$$Ac combined with antibodies or peptides that selectively accumulate in cancer cells, has garnered attention in the field of nuclear medicine. To meet the resulting increasing demand for $$^{225}$$Ac, exploring alternative production methods is essential. While several researchers, including the authors, have explored production methods using $$^{226}$$Ra as a raw material, challenges remain, such as the limited availability of $$^{226}$$Ra, difficulties in handling it, and the requirement for regular irradiation. To address these challenges, the authors focused on developing a production strategy for a long-life $$^{225}$$Ac generator using $$^{230}$$Th as a raw material and the experimental fast reactor Joyo. A detailed investigation was conducted, encompassing chemical processing after irradiation, target availability, and production yields, including the most probable values and associated uncertainties. Results revealed that although enrichment of the raw material and long-term irradiation are required, $$^{225}$$Ac can be produced in quantities comparable to its current global supply. Furthermore, this research has shown that the THOREX method, which is already in practical use, be applied to effectively separate by-products such as fission products and radioactive materials from thorium during the chemical processing after irradiation, as revealed by a literature survey.

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