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Journal Articles

Rational physical protection design of transuranium fuel cycle site with accelerator-driven system by using material attractiveness

Oizumi, Akito; Sagara, Hiroshi*

Annals of Nuclear Energy, 223, p.111677_1 - 111677_12, 2025/12

This study aims to provide a new rational physical protection (PP) design method by using ${it Material Attractiveness}$ (${it Attractiveness}$) and to design a rational PP system for a site of the transuranium fuel cycle with accelerator-drive systems (ADSs cycle) using the new method. First, the new rational PP design method with different PP design requirements for each ${it Attractiveness}$ was generalized based on the definitions of a national standard method defined by the US Department of Energy, the joint US-Japan study, and the International Atomic Energy Agency. A new PP categorization of Uranium (U), including U-234, which is abundant in the ADS cycle, was also developed based on ${it Attractiveness}$. Second, a PP design was conducted for a general BWR site with MOX fuel and the ADS cycle site by using the new rational method. It was clarified that the highest overall ${it Attractiveness}$ of the items within the ADS cycle site was lower than that of the MOX fuel assembly within the BWR site. The BWR site was determined to be Category I requiring the inner area. The PP design requirement level of the ADS cycle site was determined to be Category II, which does not require an inner area, while the ADS cycle site would have been classified as Category I if the PP design had been conducted using the conventional method.

Journal Articles

Nuclear hydrogen demonstration project using the HTTR; Demarcation of nuclear-industrial laws and design standards

Aoki, Takeshi; Shimizu, Atsushi; Ishii, Katsunori; Morita, Keisuke; Mizuta, Naoki; Kurahayashi, Kaoru; Yasuda, Takanori; Noguchi, Hiroki; Nomoto, Yasunobu; Iigaki, Kazuhiko; et al.

Annals of Nuclear Energy, 220, p.111503_1 - 111503_7, 2025/09

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

Aiming to establish coupling technologies between a high temperature gas cooled reactor and a hydrogen production plant, JAEA has initiated the HTTR Heat Application Test Project and is conducting the safety design and the safety analysis for the licensing of the HTTR Heat Application Test Facility. The present study proposed a relative evaluation methodology for the demarcation of applicable laws and design standards for the nuclear hydrogen production system and applied it to the HTTR Heat Application Test Facility. The evaluation results showed that a candidate applying the High Pressure Gas Safety Act to the Heat Application Test Facility (hydrogen production plant) and design standards established under the High Pressure Gas Safety Act to the steam reformer did not show the lowest category in any of the metrics, and was proposed as the most superior demarcation option for the HTTR Heat Application Test Facility.

Journal Articles

Experimental study on light gas transport during containment venting by using the large-scale test facility CIGMA

Soma, Shu; Ishigaki, Masahiro*; Shibamoto, Yasuteru

Annals of Nuclear Energy, 219, p.111455_1 - 111455_12, 2025/09

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

Journal Articles

Impact of molybdenum on iodine chemistry during fission product transport phenomenology

Rizaal, M.; Nakajima, Kunihisa; Suzuki, Eriko; Miwa, Shuhei

Annals of Nuclear Energy, 218, p.111433_1 - 111433_10, 2025/08

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

Journal Articles

Integrated thermal power measurement in the modified STACY for the performance inspections

Araki, Shohei; Aizawa, Eiju; Murakami, Takahiko; Arakaki, Yu; Tada, Yuta; Kamikawa, Yutaka; Hasegawa, Kenta; Yoshikawa, Tomoki; Sumiya, Masato; Seki, Masakazu; et al.

Annals of Nuclear Energy, 217, p.111323_1 - 111323_8, 2025/07

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

JAEA has modified the STACY from a homogeneous system using solution fuel to a heterogeneous system using fuel rods in order to obtain criticality characteristics of fuel debris. The modification of the STACY was completed in December 2023. A series of performance inspections were conducted for the start of experimental operations. A new thermal power calibration is required for the performance inspections in order to operate at less than 200 W, which is the permitted thermal power. However, the thermal power measurement method and calibration data used in the former STACY is no longer available due to the modification of the modified STACY. We measured the thermal power of the STACY using the activation method that was improved to adapt to the measurement condition and calibrated the power meter system. Since the positions where activation foils could be installed were very limited, the thermal power was evaluated using numerical calculations supplemented by experimental data. Neutron flux data at the positions of the activation foil was measured by the activation method. Neutron distribution in the core was calculated by the Monte Carlo code MVP. A response function of the activation foil was calculated using the PHITS. The uncertainty of the thermal power measurement was conservatively estimated to be about 15%. Four operations were conducted for the thermal power measurement. The power meter was calibrated by using three operational data and tested with the one operational data. It was found that the indicated value of the meter adjusted by the STACY before the modification work would tend to overestimate the actual output by about 40%. In addition, the current calibration was able to calibrate the meter to within 3% accuracy.

Journal Articles

Non-condensable gas accumulation and distribution due to condensation in the CIGMA Facility; Implications for Fukushima Daiichi Unit 3 (1F3)

Hamdani, A.; Soma, Shu; Abe, Satoshi; Shibamoto, Yasuteru

Progress in Nuclear Energy, 185, p.105771_1 - 105771_13, 2025/07

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

Journal Articles

Prediction of composite neutron source spectra by combination of JENDL-5 and PHITS

Ogawa, Tatsuhiko

Annals of Nuclear Energy, 216, p.111256_1 - 111256_12, 2025/06

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

A novel robust method has been developed to simulate the performance of composite neutron sources composed of an alpha-emitting actinide and a light nucleus with low neutron separation energy. This method is based on the JENDL-5 cross-section data library and the Monte-Carlo radiation transport code PHITS. In contrast to previously devised methods, this approach can predict various quantities of the sources, such as actinide grain size dependence, absolute neutron emission intensity, energy spectra of neutrons and parasitic photons, neutron multiplicity, and time structure, with little approximation. The accurate calculation of stopping power of alpha rays in actinide grains and light elements, as well as the use of ($$alpha$$,n) reaction evaluated cross sections, which is one of the unique features of PHITS Ver.3.34 and its later versions, are the essences of the method. This method allows for the calculation of quantities important for practical applications, such as detection signal frequency, coincidence event rate, and the impact of parasitic gamma-rays.

Journal Articles

Numerical simulation of coupled THM behaviour of full-scale EBS in backfilled experimental gallery in the Horonobe URL

Sugita, Yutaka; Ono, Hirokazu; Beese, S.*; Pan, P.*; Kim, M.*; Lee, C.*; Jove-Colon, C.*; Lopez, C. M.*; Liang, S.-Y.*

Geomechanics for Energy and the Environment, 42, p.100668_1 - 100668_21, 2025/06

 Times Cited Count:1 Percentile:0.00(Energy & Fuels)

The international cooperative project DECOVALEX 2023 focused on the Horonobe EBS experiment in the Task D, which was undertaken to study, using numerical analyses, the thermo-hydro-mechanical (or thermo-hydro) interactions in bentonite based engineered barriers. One full-scale in-situ experiment and four laboratory experiments, largely complementary, were selected for modelling. The Horonobe EBS experiment is a temperature-controlled non-isothermal experiment combined with artificial groundwater injection. The Horonobe EBS experiment consists of the heating and cooling phases. Six research teams performed the THM or TH (depended on research team approach) numerical analyses using a variety of computer codes, formulations and constitutive laws.

Journal Articles

DECOVALEX-2023: An International collaboration for advancing the understanding and modeling of coupled thermo-hydro-mechanical-chemical (THMC) processes in geological systems

Birkholzer, J. T.*; Graupner, B. J.*; Harrington, J.*; Jayne, R.*; Kolditz, O.*; Kuhlman, K. L.*; LaForce, T.*; Leone, R. C.*; Mariner, P. E.*; McDermott, C.*; et al.

Geomechanics for Energy and the Environment, 42, p.100685_1 - 100685_17, 2025/06

 Times Cited Count:0

Journal Articles

Numerical verification for the effect of suppressing hydrogen embrittlement by Sn doping in the Al-Zn-Mg alloy

Ebihara, Kenichi; Fujihara, Hiro*; Shimizu, Kazuyuki*; Yamaguchi, Masatake; Toda, Hiroyuki*

International Journal of Hydrogen Energy, 136, p.751 - 756, 2025/06

 Times Cited Count:0

It has been experimentally reported that adding tin (Sn) to high-strength aluminum-zinc-magnesium (Al-Zn-Mg) alloys effectively suppresses hydrogen (H) embrittlement, which may be attributed to H absorption by the second-phase particles of Sn. To verify this fact, a simulation of H entry into the Sn phase in Al was performed using a model based on the reaction-diffusion equation that incorporates the solid solution energy of H evaluated by first-principles calculations. The results showed that the H solid solution site concentration of the second-phase particles must be at least five times higher than that of the Al phase for H absorption by the Sn second-phase particles to suppress H embrittlement. Therefore, the actual H embrittlement suppression effect of Sn second-phase particles is limited, and other factors may influence the suppression of H embrittlement in the experiment.

Journal Articles

Uncertainty analysis of the inverse LASSO estimation scheme on radioactive source distributions inside reactor building rooms from air does rate measurements

Shi, W.*; Machida, Masahiko; Yamada, Susumu; Okamoto, Koji

Progress in Nuclear Energy, 184, p.105710_1 - 105710_10, 2025/06

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

Very recently, Least Absolute Shrinkage and Selection Operator (LASSO) has been proposed as a scheme capable to inversely estimate radioactive source distributions inside reactor building rooms from air dose rate measurements together with the predicted lower bound of the measurement numbers for successful reconstructions. However, no one has ever analyzed how the uncertainty of input data including the measurement errors influences the accuracy of the inverse estimation results. In this paper, we therefore perform uncertainty analysis of the LASSO scheme and suggest an uncertainty estimation function derived based on the theory of Candes. We actually demonstrate in two types of numerical tests with different input uncertainties obtained by using Monte Carlo code, Particle and Heavy Ion Transport code System (PHITS) that the calculated errors obey the proposed uncertainty estimation function. Thus, the LASSO scheme allows to successfully estimate radioactive distributions within the predicted uncertainty.

Journal Articles

Analysis of dissolved radionuclides trapped into corrosion products formed on carbon steel and the corresponding increase in radioactivity

Aoyama, Takahito; Ueno, Fumiyoshi; Sato, Tomonori; Kato, Chiaki; Sano, Naruto; Yamashita, Naoki; Otani, Kyohei; Igarashi, Takahiro

Annals of Nuclear Energy, 214, p.111229_1 - 111229_6, 2025/05

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

Journal Articles

Numerical analysis of a potential Reactor Pressure Vessel (RPV) boundary failure mechanism in Fukushima Daiichi Nuclear Power Station Unit-2

Li, X.; Yamaji, Akifumi*; Sato, Ikken*; Yamashita, Takuya

Annals of Nuclear Energy, 214, p.111217_1 - 111217_13, 2025/05

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

Journal Articles

Evaluation of uranium-233 neutron capture cross section in keV region

Otsuka, Naohiko*; Tada, Kenichi; Cabellos, O.*; Iwamoto, Osamu

Annals of Nuclear Energy, 212, p.110977_1 - 110977_9, 2025/03

 Times Cited Count:2 Percentile:0.00(Nuclear Science & Technology)

The uranium-233 neutron capture cross section between 3 keV and 1 MeV was evaluated considering the recent new alpha-value measurement performed at the Los Alamos National Laboratory LANCE facility. The obtained capture cross section is systematically lower than the capture cross section in the JENDL-5 library and the reduction is close to 50% around 20 keV. The newly evaluated cross section was validated against 166 criticality experiments chosen from the ICSBEP handbook by performing Monte Carlo neutron transport calculation with the JENDL-5 library, and slight reduction of the chi-square value was achieved by adoption of the newly evaluated capture cross section.

Journal Articles

Built-in physics models and proton-induced nuclear data validation using MCNP, PHITS, and FLUKA; Impact on the shielding design for proton accelerator facilities

$c{C}$elik, Y.*; Stankovskiy, A.*; Iwamoto, Hiroki; Iwamoto, Yosuke; Van den Eynde, G.*

Annals of Nuclear Energy, 212, p.111048_1 - 111048_12, 2025/03

 Times Cited Count:1 Percentile:51.66(Nuclear Science & Technology)

Journal Articles

Comparative analysis of primary variables selection in modeling non-isothermal two-phase flow; Insights from EBS experiment at Horonobe URL

Kim, M.*; Lee, C.*; Sugita, Yutaka; Kim, J.-S.*; Jeon, M.-K.*

Geomechanics for Energy and the Environment, 41, p.100628_1 - 100628_9, 2025/03

 Times Cited Count:1 Percentile:0.00(Energy & Fuels)

This study investigates the impact of primary variables selection on the modeling of non-isothermal two-phase flow, by using the numerical work on the full-scale Engineered Barrier System (EBS) experiment conducted at Horonobe URL as part of the DECOVALEX-2023 project. A validated numerical model is employed to simulate the coupled thermo-hydrological behavior of heterogeneous porous media within the EBS. Two different primary variable schemes are compared in discretizing the governing equations, revealing significant difference in results.

Journal Articles

Modeling of coupled processes in full-scale engineered barrier system performance experiment at Horonobe Underground Research Laboratory, Japan

Ono, Hirokazu; Takayama, Yusuke*

Geomechanics for Energy and the Environment, 41, p.100636_1 - 100636_14, 2025/03

 Times Cited Count:1 Percentile:0.00(Energy & Fuels)

Journal Articles

Hydrogen embrittlement in Al-Zn-Mg alloys; Semispontaneous decohesion of precipitates

Shimizu, Kazuyuki*; Toda, Hiroyuki*; Hirayama, Kyosuke*; Fujihara, Hiro*; Tsuru, Tomohito; Yamaguchi, Masatake; Sasaki, Taisuke*; Uesugi, Masayuki*; Takeuchi, Akihisa*

International Journal of Hydrogen Energy, 109, p.1421 - 1436, 2025/03

 Times Cited Count:2 Percentile:93.94(Chemistry, Physical)

Our preceding investigation revealed that multiple hydrogen traps at coherent interfaces of MgZn$$_{2}$$ precipitates initiated spontaneous interface decohesion, causing hydrogen-induced quasicleavage cracking in Al-Zn-Mg alloys. Herein, we performed a quantitative and systematic investigation to discern the mechanisms by which hydrogen trapped at coherent/semi-coherent interfaces of precipitates could influence macroscopic hydrogen embrittlement by modulating the coherent interface of MgZn$$_{2}$$ through aging. To explore this hydrogen embrittlement phenomenon based on hydrogen trapping at the precipitate interface, we determined the hydrogen trapping energy of the semi-coherent MgZn$$_{2}$$ interface via first-principles calculations (0.56 eV/atom). Hydrogen partitioning of all hydrogen trapping sites, including vacancies, grain boundaries, and coherent and semi-coherent MgZn$$_{2}$$ interfaces, revealed that in overaged alloys, over 90% of the hydrogen was sequestered at semi-coherent interfaces. Owing to the inherent characteristics of the MgZn$$_{2}$$ interface, the hydrogen sequestered at the semi-coherent interface decreased the interfacial cohesive energy, causing semispontaneous decohesion of the interface and quasicleavage fracture in the Al-Zn-Mg alloys. These results implied that intergranular fracture was not directly induced by hydrogen trapped at grain boundaries but rather by the decohesion of precipitate interfaces along grain boundaries.

Journal Articles

Effect of Am addition on oxygen potential in (U$$_{0.55}$$Pu$$_{0.3}$$Am$$_{0.15}$$)O$$_{2-x}$$

Yokoyama, Keisuke; Watanabe, Masashi; Usui, Akane; Seki, Takayuki*; Onishi, Takashi; Kato, Masato

Nuclear Materials and Energy (Internet), 42, p.101908_1 - 101908_6, 2025/03

 Times Cited Count:0 Percentile:0.00(Nuclear Science & Technology)

Oxygen potential of high Am content MOX, (U$$_{0.55}$$Pu$$_{0.3}$$Am$$_{0.15}$$)O$$_{2-x}$$, was measured at 1273 K, 1473 K, 1573 K, and 1623 K. by gas equilibrium method using thermogravimeter. Comparing the measured data with the literature data, it was found that the addition of 15% Am increases the oxygen potential of (U, Pu)O$$_{2.00}$$ by 100-150 kJ/mol for the same Pu content and O/M ratio. The proportion of cations in the stoichiometric composition was determined as (U$$^{4+}_{0.4}$$U$$^{5+}_{0.15}$$Pu$$^{4+}_{0.3}$$Am$$^{3+}_{0.15}$$)O$$_{2.00}$$, assuming the presence of Am$$^{3+}$$ and partial oxidation of U$$^{4+}$$ to U$$^{5+}$$. The relationship between oxygen partial pressure and deviation x from stoichiometry in (U$$_{0.55}$$Pu$$_{0.3}$$Am$$_{0.15}$$)O$$_{2-x}$$ was analyzed by defect chemistry model. The equation to represent the O/M ratio was derived as a function of temperature and oxygen partial pressure. A part of this study includes the results of MEXT Innovative Nuclear Research and Development Program Grant Number JPMXD0219214921.

Journal Articles

Uncertainty quantification for severe-accident reactor modelling; Results and conclusions of the MUSA reactor applications work package

Brumm, S.*; Gabrielli, F.*; Sanchez Espinoza, V.*; Stakhanova, A.*; Groudev, P.*; Petrova, P.*; Vryashkova, P.*; Ou, P.*; Zhang, W.*; Malkhasyan, A.*; et al.

Annals of Nuclear Energy, 211, p.110962_1 - 110962_16, 2025/02

 Times Cited Count:6 Percentile:94.85(Nuclear Science & Technology)

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