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Yuguchi, Takashi*; Sasao, Eiji; Hibara, Ryoko*; Murakami, Hiroaki; Ozaki, Yusuke
Heliyon (Internet), 10(17), p.e37417_1 - e37417_17, 2024/09
Times Cited Count:0 Percentile:0.00(Multidisciplinary Sciences)Understanding the mass transfer characteristics of matrix diffusion and sorption is important in geological disposal of high-level radioactive waste in crystalline rock. We present a comparative discussion of the effective diffusion coefficient (De), porosity, and petrological data for rock samples collected from the Toki Granite in central Japan, to evaluate the role of micropores within minerals in retardation by matrix diffusion and sorption in granitic rocks. De was derived from the through-diffusion experiments. Petrological data consist of the fracture frequency, the extent of hydrothermal alteration in the minerals, the micropore volume in the minerals, and the three-dimensional modal mineralogy for the target rock samples. The relationship between the De, porosity, and petrological data has the following implications: 1) Micropores act as storage pores that contribute to retardation; 2) Once the uranine, cations, and anion penetrate the micropores in the minerals through matrix diffusion, the cations are sorbed on the micropore surfaces; 3) Regions with a high fracture frequency are associated with not only active advection-dispersion through fractures, but also retardation due to matrix diffusion and sorption.
Yuguchi, Takashi*; Yagi, Koshi*; Sasao, Eiji; Nishiyama, Tadao*
Heliyon (Internet), 7(4), p.e06750_1 - e06750_9, 2021/04
Times Cited Count:2 Percentile:16.21(Multidisciplinary Sciences)Our methodology and interpretations provide new insight for K-Ar geochronology in hydrothermal microcline within altered plagioclase in a granitic pluton. Our methodology employs a two-step separation process consisting of (1) plagioclase extraction from the rock sample and (2) separation of the hydrothermal microcline from the plagioclase, giving precise determination of microcline powders in K-Ar geochronology. This tighter constraint should provide the ability to better unravel thermal and age histories in granite subject to multi-step alteration processes and complex thermal histories.
Yuguchi, Takashi*; Usami, Akane*; Ishibashi, Masayuki
Heliyon (Internet), 6(8), p.e04815_1 - e04815_6, 2020/08
Times Cited Count:1 Percentile:5.81(Multidisciplinary Sciences)The analysis of the distribution of microfractures and micropores is important to accurately characterise mass transfer within a rock body. In this paper, a new "simultaneous polarization-fluorescence microscopy" method is presented, which can be used to analyse the distribution of microscopic voids, including microfractures and micropores, in granitic rock. In this method, thin sections prepared with fluorescent dye are analysed under a polarizing microscope equipped with a fluorescent reflected light source. Using both the transmitted and the fluorescent light sources, both the distribution of microfractures and micropores, and petrographic characteristics (mineral occurrences) can be determined efficiently and simultaneously. The distribution of microfractures and micropores observed in images of granites obtained using simultaneous polarization-fluorescence microscopy is consistent with the distribution observed in backscattered electron images.
Ohdaira, Naoya*; Saito, Shigeru
Heliyon (Internet), 6(2), p.e03429_1 - e03429_8, 2020/02
Times Cited Count:6 Percentile:40.73(Multidisciplinary Sciences)Lead-bismuth eutectic (LBE) is a candidate liquid metal coolant for a fast reactor, especially accelerator driven system (ADS). Freeze sealed valve is a candidate design to be possible to add passive safety to the reactor. On the other hand, since LBE is known that it causes expansion after its solidification, quantitative evaluation of the stress to the pipe produced by the LBE expansion should be considered. Many researchers produced related data for the expansion, however, evaluations of the strain by LBE expansion was barely reported. Therefore, the strain measurement using a stainless steel cup and the stress evaluation was performed together with visual observation using an optical microscopy. The results indicated keeping above room temperature (RT) was a significantly effective way to reduce the strain to the pipe.