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Journal Articles

Provenance of uranium particulate contained within Fukushima Daiichi Nuclear Power Plant Unit 1 ejecta material

Martin, P. G.*; Louvel, M.*; Cipiccia, S.*; Jones, C. P.*; Batey, D. J.*; Hallam, K. R.*; Yang, I. A. X.*; Satou, Yukihiko; Rau, C.*; Mosselmans, J. F. W.*; et al.

Nature Communications (Internet), 10(1), p.2801_1 - 2801_7, 2019/06

 Times Cited Count:0 Percentile:100(Multidisciplinary Sciences)

Synchrotron radiation (SR) analysis techniques alongside secondary ion mass spectrometry (SIMS) measurements have been made on sub-mm particulate material derived from reactor Unit 1 of the Fukushima Daiichi Nuclear Power Plant (FDNPP). Using these methods, it has been possible to investigate the distribution, state and isotopic composition of micron-scale U particulate contained within the larger Si-based ejecta material. Through combined SR micro-focused X-ray fluorescence (SR-micro-XRF) and absorption contrast SR micro-focused X-ray tomography (SR-micro-XRT), the U particulate was found to be located around the exterior circumference of the highly-porous particle. Synchrotron radiation micro-focused X-ray absorption near edge structure (SR-micro-XANES) analysis of a number of these entrapped particles revealed them to exist within the U(IV) oxidation state, as UO$$_{2}$$, and identical in structure to reactor fuel. Confirmation that this U was of nuclear origin ($$^{235}$$U-enriched) was provided through secondary ion mass spectrometry (SIMS) analysis with an isotopic enrichment ratio characteristic of a provenance from reactor Unit 1 at the FDNPP. These results provide clear evidence of the event scenario (that a degree of core fragmentation and release occurred from reactor Unit 1), with such spent fuel ejecta existing; (i) within the stable U(IV) oxidation state; and (ii) contained within a bulk Si-based particle. While this U is unlikely to represent an environmental or health hazard, such assertions would likely change, however, should break-up of the Si-containing bulk particle occur. However, more important to the long-term decommissioning of the reactors (and clean-up) on the FDNPP, is the knowledge that core integrity of reactor Unit 1 was compromised with nuclear material existing outside of the reactors primary containment.

Journal Articles

Spin Seebeck mechanical force

Harii, Kazuya; Seo, Y.-J.*; Tsutsumi, Yasumasa*; Chudo, Hiroyuki; Oyanagi, Koichi*; Matsuo, Mamoru; Shiomi, Yuki*; Ono, Takahito*; Maekawa, Sadamichi; Saito, Eiji

Nature Communications (Internet), 10(1), p.2616_1 - 2616_5, 2019/06

 Times Cited Count:0 Percentile:100(Multidisciplinary Sciences)

Journal Articles

Evidence for singular-phonon-induced nematic superconductivity in a topological superconductor candidate Sr$$_{0.1}$$Bi$$_{2}$$Se$$_{3}$$

Wang, J.*; Ran, K.*; Li, S.*; Ma, Z.*; Bao, S.*; Cai, Z.*; Zhang, Y.*; Nakajima, Kenji; Kawamura, Seiko; $v{C}$erm$'a$k, P.*; et al.

Nature Communications (Internet), 10, p.2802_1 - 2802_6, 2019/06

 Times Cited Count:0 Percentile:100(Multidisciplinary Sciences)

Journal Articles

Triplon band splitting and topologically protected edge states in the dimerized antiferromagnet

Nawa, Kazuhiro*; Tanaka, Kimihito*; Kurita, Nubuyuki*; Sato, Taku*; Sugiyama, Haruki*; Uekusa, Hidehiro*; Kawamura, Seiko; Nakajima, Kenji; Tanaka, Hidekazu*

Nature Communications (Internet), 10, p.2096_1 - 2096_8, 2019/05

 Times Cited Count:0 Percentile:100(Multidisciplinary Sciences)

Search for topological materials has been actively promoted in the field of condensed matter physics for their potential application in energy-efficient information transmission and processing. Recent studies have revealed that topologically invariant states, such as edge states in topological insulators, can emerge not only in a fermionic electron system but also in a bosonic system, enabling nondissipative propagation of quasiparticles. Here we report the topologically nontrivial triplon bands measured by inelastic neutron scattering on the spin-1/2 two-dimensional dimerized antiferromagnet Ba$$_{2}$$CuSi$$_{2}$$O$$_{6}$$Cl$$_{2}$$. The excitation spectrum exhibits two triplon bands that are clearly separated by a band gap due to a small alternation in interdimer exchange interaction, consistent with a refined crystal structure. By analytically modeling the triplon dispersion, we show that Ba$$_{2}$$CuSi$$_{2}$$O$$_{6}$$Cl$$_{2}$$ is the first bosonic realization of the coupled Su-Schrieffer-Heeger model, where the presence of topologically protected edge states is prompted by a bipartite nature of the lattice.

Journal Articles

Divalent EuRh$$_2$$Si$$_2$$ as a reference for the Luttinger theorem and antiferromagnetism in trivalent heavy-fermion YbRh$$_2$$Si$$_2$$

G$"u$ttler, M.*; Generalov, A.*; Fujimori, Shinichi; Kummer, K.*; Chikina, A.*; Seiro, S.*; Danzenb$"a$cher, S.*; Koroteev, Yu. M.*; Chulkov, E. V.*; Radovic, M.*; et al.

Nature Communications (Internet), 10(1), p.796_1 - 796_7, 2019/02

 Times Cited Count:0 Percentile:100(Multidisciplinary Sciences)

Journal Articles

Hydrogen-based metabolism as an ancestral trait in lineages sibling to the Cyanobacteria

Carnevali, P. B. M.*; Schulz, F.*; Castelle, C. J.*; Kantor, R. S.*; Shih, P. M.*; Sharon, I.*; Santini, J.*; Olm, M. R.*; Amano, Yuki; Thomas, B. C.*; et al.

Nature Communications (Internet), 10, p.463_1 - 463_15, 2019/01

 Times Cited Count:3 Percentile:15.2(Multidisciplinary Sciences)

Journal Articles

Vortex rectenna powered by environmental fluctuations

Lustikova, J.*; Shiomi, Yuki*; Yokoi, Naoto*; Kabeya, Noriyuki*; Kimura, Noriaki*; Ienaga, Koichiro*; Kaneko, Shinichi*; Okuma, Satoshi*; Takahashi, Saburo*; Saito, Eiji

Nature Communications (Internet), 9, p.4922_1 - 4922_6, 2018/11

 Times Cited Count:4 Percentile:31.79(Multidisciplinary Sciences)

Journal Articles

Spherical neutron polarimetry under high pressure for a multiferroic delafossite ferrite

Terada, Noriki*; Qureshi, N.*; Chapon, L. C.*; Osakabe, Toyotaka

Nature Communications (Internet), 9, p.4368_1 - 4368_9, 2018/10

 Times Cited Count:0 Percentile:100(Multidisciplinary Sciences)

Journal Articles

Improving atomic displacement and replacement calculations with physically realistic damage models

Nordlund, K.*; Zinkle, S. J.*; Sand, A. E.*; Granberg, F.*; Averback, R. S.*; Stoller, R.*; Suzudo, Tomoaki; Malerba, L.*; Banhart, F.*; Weber, W. J.*; et al.

Nature Communications (Internet), 9, p.1084_1 - 1084_8, 2018/03

 Times Cited Count:35 Percentile:1.42(Multidisciplinary Sciences)

Atomic collision processes are fundamental to numerous advanced materials technologies such as electron microscopy, semiconductor processing and nuclear power generation. Experimental and computer simulation studies over the past several decades provide the physical basis for understanding the atomic-scale processes occurring during primary displacement events. The current international standard for quantifying this particle damage, the Norgett-Robinson-Torrens displacements per atom (NRT-dpa) model, has nowadays several well-known limitations. In particular, the number of radiation defects produced in energetic cascades in metals is only $$sim$$1/3 the NRT-dpa prediction, while the number of atoms involved in atomic mixing is about a factor of 30 larger than the dpa value. Here we propose two new complementary displacement production estimators.

Journal Articles

Maximizing $$T_c$$ by tuning nematicity and magnetism in FeSe$$_{1-x}$$S$$_x$$ superconductors

Matsuura, Kohei*; Mizukami, Yuta*; Arai, Yuki*; Sugimura, Yuichi*; Maejima, Naoyuki*; Machida, Akihiko*; Watanuki, Tetsu*; Fukuda, Tatsuo; Yajima, Takeshi*; Hiroi, Zenji*; et al.

Nature Communications (Internet), 8, p.1143_1 - 1143_6, 2017/10

 Times Cited Count:22 Percentile:11.22(Multidisciplinary Sciences)

Journal Articles

Structure of the magnetic excitations in the spin-1/2 triangular-lattice Heisenberg antiferromagnet Ba$$_{3}$$CoSb$$_{2}$$O$$_{9}$$

Ito, Saya*; Kurita, Nubuyuki*; Tanaka, Hidekazu*; Kawamura, Seiko; Nakajima, Kenji; Ito, Shinichi*; Kuwahara, Keitaro*; Kakurai, Kazuhisa*

Nature Communications (Internet), 8, p.235_1 - 235_6, 2017/08

 Times Cited Count:20 Percentile:5.7(Multidisciplinary Sciences)

Journal Articles

Non-aqueous selective synthesis of orthosilicic acid and its oligomers

Igarashi, Masayasu*; Matsumoto, Tomohiro*; Yagihashi, Fujio*; Yamashita, Hiroshi*; Ohara, Takashi; Hanashima, Takayasu*; Nakao, Akiko*; Moyoshi, Taketo*; Sato, Kazuhiko*; Shimada, Shigeru*

Nature Communications (Internet), 8, p.140_1 - 140_8, 2017/07

 Times Cited Count:3 Percentile:67.58(Multidisciplinary Sciences)

Journal Articles

Polar rotor scattering as atomic-level origin of low mobility and thermal conductivity of perovskite CH$$_{3}$$NH$$_{3}$$PbI$$_{3}$$

Li, B.; Kawakita, Yukinobu; Liu, Y.*; Wang, M.*; Matsuura, Masato*; Shibata, Kaoru; Kawamura, Seiko; Yamada, Takeshi*; Lin, S.*; Nakajima, Kenji; et al.

Nature Communications (Internet), 8, p.16086_1 - 16086_9, 2017/06

 Times Cited Count:25 Percentile:8.25(Multidisciplinary Sciences)

Journal Articles

Hydrogenation of iron in the early stage of Earth's evolution

Iizuka, Riko*; Yagi, Takehiko*; Goto, Hirotada*; Okuchi, Takuo*; Hattori, Takanori; Sano, Asami

Nature Communications (Internet), 8, p.14096_1 - 14096_7, 2017/01

AA2016-0524.pdf:0.73MB

 Times Cited Count:14 Percentile:9.93(Multidisciplinary Sciences)

Density of the Earth's core is lower than that of pure iron and the light element(s) in the core is a long-standing problem. Hydrogen is the most abundant element in the solar system and thus one of the important candidates. However, the dissolution process of hydrogen into iron remained unclear. Here we carry out high-pressure and high-temperature in situ neutron diffraction experiments and clarify that when the mixture of iron and hydrous minerals are heated, iron is hydrogenized soon after the hydrous mineral is dehydrated. This implies that early in the Earth's evolution, as the accumulated primordial material became hotter, the dissolution of hydrogen into iron occurred before any other materials melted. This suggests that hydrogen is likely the first light element dissolved into iron during the Earth's evolution and it may affect the behaviour of the other light elements in the later processes.

Journal Articles

Thermal imaging of spin Peltier effect

Daimon, Shunsuke*; Iguchi, Ryo*; Hioki, Tomosato*; Saito, Eiji; Uchida, Kenichi*

Nature Communications (Internet), 7, p.13754_1 - 13754_7, 2016/12

 Times Cited Count:31 Percentile:8.18(Multidisciplinary Sciences)

Journal Articles

Spontaneous decays of magneto-elastic excitations in non-collinear antiferromagnet (Y,Lu)MnO$$_{3}$$

Oh, J.*; Le, M. D.*; Nahm, H.-H.*; Sim, H.*; Jeong, J.*; Perring, T. G.*; Woo, H.*; Nakajima, Kenji; Kawamura, Seiko; Yamani, Z.*; et al.

Nature Communications (Internet), 7, p.13146_1 - 13146_6, 2016/10

 Times Cited Count:21 Percentile:10.14(Multidisciplinary Sciences)

Magnons and phonons are fundamental quasiparticles in a solid and can be coupled together to form a hybrid quasi-particle. However, detailed experimental studies on the underlying Hamiltonian of this particle are rare for actual materials. Moreover, the anharmonicity of such magnetoelastic excitations remains largely unexplored, although it is essential for a proper understanding of their diverse thermodynamic behaviour and intrinsic zero-temperature decay. Here we show that in non-collinear antiferromagnets, a strong magnon phonon coupling can significantly enhance the anharmonicity, resulting in the creation of magnetoelastic excitations and their spontaneous decay. By measuring the spin waves over the full Brillouin zone and carrying out anharmonic spin wave calculations using a Hamiltonian with an explicit magnon phonon coupling, we have identified a hybrid magnetoelastic mode in (Y,Lu)MnO$$_{3}$$ and quantified its decay rate and the exchange-striction coupling termrequired to produce it.

Journal Articles

Volume-wise destruction of the antiferromagnetic Mott insulating state through quantum tuning

Frandsen, B. A.*; Liu, L.*; Cheung, S. C.*; Guguchia, Z.*; Khasanov, R.*; Morenzoni, E.*; Munsie, T. J. S.*; Hallas, A. M.*; Wilson, M. N.*; Cai, Y.*; et al.

Nature Communications (Internet), 7, p.12519_1 - 12519_8, 2016/08

 Times Cited Count:8 Percentile:40.55(Multidisciplinary Sciences)

Journal Articles

Spin-current probe for phase transition in an insulator

Qiu, Z.*; Li, J.*; Hou, D.*; Arenholz, E.*; N'Diaye, A. T.*; Tan, A.*; Uchida, Kenichi*; Sato, Koji*; Okamoto, Satoshi*; Tserkovnyak, Y.*; et al.

Nature Communications (Internet), 7, p.12670_1 - 12670_6, 2016/08

 Times Cited Count:59 Percentile:2.88(Multidisciplinary Sciences)

Journal Articles

Observation of temperature-gradient-induced magnetization

Hou, D.*; Qiu, Z.*; Iguchi, Ryo*; Sato, Koji*; Vehstedt, E. K.*; Uchida, Kenichi*; Bauer, G. E. W.*; Saito, Eiji

Nature Communications (Internet), 7, p.12265_1 - 12265_6, 2016/07

 Times Cited Count:9 Percentile:29.49(Multidisciplinary Sciences)

Journal Articles

Origin of the spin Seebeck effect in compensated ferrimagnets

Gepr$"a$gs, S.*; Kehlberger, A.*; Coletta, F.*; Qiu, Z.*; Guo, E.-J.*; Schulz, T.*; Mix, C.*; Meyer, S.*; Kamra, A.*; Althammer, M.*; et al.

Nature Communications (Internet), 7, p.10452_1 - 10452_6, 2016/02

 Times Cited Count:58 Percentile:3.43(Multidisciplinary Sciences)

39 (Records 1-20 displayed on this page)